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E. Pomjakushina

Publications and source records attributed to E. Pomjakushina.

At least 127 records · Page 7Linked to original sources
arXiv2011

Ferroelectric charge order stabilized by antiferromagnetism in multiferroic LuFe2O4

Neutron diffraction measurements on multiferroic LuFe2O4 show changes in the antiferromagnetic (AFM) structure characterized by wavevector q = (1/3 1/3 1/2) as a function of electric field cooling procedures. The increase of intensity from all magnetic domains and the decrease in the 2D magnetic order observed below the Neel temperature are indicative of increased ferroelectric charge order. The AFM order changes the dynamics of the CO state, and stabilizes it. It is determined that the increase in electric polarization observed at the magnetic ordering temperature is due to a transition from paramagnetic 2D charge order to AFM 3D charge order.

cond-mat.str-el↗
arXiv2011

Double-k phase of the Dzyaloshinskii-Moriya helimagnet Ba2CuGe2O7

Neutron diffraction is used to re-investigate the magnetic phase diagram of the noncentrosymmetric tetragonal antiferromagnet Ba2CuGe2O7. A novel incommensurate double-k magnetic phase is detected near the commensurate-incommensurate phase transition. This phase is stable only for magnetic field closely aligned with the 4-fold symmetry axis. The results emphasize the inadequacy of existing theoretical models for this unique material, and points to additional terms in the Hamiltonian or lattice effects.

cond-mat.str-el↗
arXiv2011

Muon spin rotation investigation of the pressure effect on the magnetic penetration depth in YBa2Cu3Ox

The pressure dependence of the magnetic penetration depth in polycrystalline samples of YBa2Cu3Ox with different oxygen concentrations x = 6.45, 6.6, 6.8, and 6.98 was studied by muon spin rotation (muSR). The pressure dependence of the superfluid density (p_s) as a function of the superconducting transition temperature Tc is found to deviate from the usual Uemura line. The ratio (dTc/dP)/(dp_s/dP) is factor of 2 smaller than that of the Uemura relation. In underdoped samples, the zero temperature superconducting gap and the BCS ratio both increase with increasing external hydrostatic pressure, implying an increase of the coupling strength with pressure. The relation between the pressure effect and the oxygen isotope effect on the magnetic penetration depth is also discussed. In order to analyze reliably the muSR spectra of samples with strong magnetic moments in a pressure cell, a special model was developed and applied.

cond-mat.supr-con↗
arXiv2011

Correlation of conductivity and angle integrated valence band photoemission characteristics in single crystal iron perovskites for 300 K < T < 800 K: Comparison of surface and bulk sensitive methods

A single crystal monolith of La0.9Sr0.1FeO3 and thin pulsed laser deposited film of La0.8Sr0.2Fe0.8Ni0.2O3 were subject to angle integrated valence band photoemission spectroscopy in ultra high vacuum and conductivity experiments in ambient air at temperatures from 300 K to 800 K. Except for several sputtering and annealing cycles, the specimen were not prepared in-situ.. Peculiar changes in the temperature dependent, bulk representative conductivity profile as a result of reversible phase transitions, and irreversible chemical changes are semi-quantitatively reflected by the intensity variation in the more surface representative valence band spectra near the Fermi energy. X-ray photoelectron diffraction images reflect the symmetry as expected from bulk iron perovskites. The correlation of spectral details in the valence band photoemission spectra (VB PES) and details of the conductivity during temperature variation suggest that valuable information on electronic structure and transport properties of complex materials may be obtained without in-situ preparation.

cond-mat.str-el↗
arXiv2011

Electron hole - phonon interaction and structural changes in La0.9Sr0.1FeO3 by temperature dependent conductivity and valence band photoemission spectros-copy

Electric conductivity and structural details of the hole-doped polaron conductor La0.9Sr0.1FeO3 (LSF10) are reported. The conductivity of a single crystal shows an exponential increase with temperature with a maxi-mum of 100 S/cm at 700 K and with activation energy of about 375 meV, and a decrease for higher temperatures that follows a power law. The exponential increase of the electric conductivity for 300 K {\leg} T {\leg} 700 is accompanied by a shift of spectral weight in the photoemission valence band towards the Fermi level, indicative of a strong electron-phonon interaction. The subsequent decrease of the conductivity for T > 700 K is accompanied by a reversible phase transformation from orthorhombic to rhombohedral symmetry. The decreasing conductivity for T > 700 K is likely due to the reduction of the iron due to oxygen loss causing a decreasing hole concentration, as evidenced by a substantial chemical shift in the Fe K-shell x-ray absorption spectra. Two additional fine structures in the conductivity data at 357 K, this is, a small temperature reversible jump in the conductivity, and at 573 K, a slight reversible increase of the polaron activation energy, are correlated with an exceptionally strong decrease in spectral valence band intensity near the Fermi level, and with the onset of a corresponding structural transition.

cond-mat.str-el↗
arXiv2011

Ferromagnetic and antiferromagnetic dimer splittings in LaMn0.1Ga0.9O3

Inelastic neutron scattering was employed to study the magnetic excitations of Mn3+ dimers in LaMn0.1Ga0.9O3. The nearest-neighbor interaction of Mn3+ ions is ferromagnetic in the basal (a,b)-plane, but antiferromagnetic along the c-direction, thus two different types of dimer excitations are simultaneously present in the experiments. From the observed energy spectra we derive Heisenberg-type exchange interactions Jab=0.210(4) meV and Jc=-0.285(5) meV as well as an axial anisotropy parameter D=0.036(6) meV. These parameters considerably differ from those derived for the isostructural parent compound LaMnO3 due to structural effects.

cond-mat.str-el↗
arXiv2011

Temperature and pressure evolution of the crystal structure of Ax(Fe1-ySe)2 (A = Cs, Rb, K) studied by synchrotron powder diffraction

Temperature-dependent synchrotron powder diffraction on Cs0.83(Fe0.86Se)2 revealed first order I4/m to I4/mmm structural transformation around 216°C associated with the disorder of the Fe vacancies. Irreversibility observed during the transition is likely associated with a mobility of intercalated Alkali atoms. Pressure-dependent synchrotron powder diffraction on Cs0.83(Fe1-ySe)2, Rb0.85(Fe1-ySe)2 and K0.8(Fe1-ySe)2 (y ~ 0.14) indicated that the I4/m superstructure reflections are present up to pressures of 120 kbar. This may indicate that the ordering of the Fe vacancies is present in both superconducting and non-superconductive states.

cond-mat.mtrl-sci↗
arXiv2011

Spin anisotropy of the resonance in superconducting FeSe0.5Te0.5

We have used polarized-neutron inelastic scattering to resolve the spin fluctuations in superconducting FeSe0.5Te0.5 into components parallel and perpendicular to the layers. A spin resonance at an energy of 6.5 meV is observed to develop below T_c in both fluctuation components. The resonance peak is anisotropic, with the in-plane component slightly larger than the out-of-plane component. Away from the resonance peak the magnetic fluctuations are isotropic in the energy range studied. The results are consistent with a dominant singlet pairing state with s^{\pm} symmetry, with a possible minority component of different symmetry.

cond-mat.supr-con↗
arXiv2011

Pressure cycle of superconducting Cs0.8Fe2Se2: a transport study

We report measurements of the temperature and pressure dependence of the electrical resistivity of single crystalline iron-based chalcogenide Cs0.8Fe2Se2. In this material superconductivity Tc~30K develops from a normal state with extremely large resistivity. At ambient pressure a large "hump" in the resistivity is observed around 200K. Under pressure, the resistivity decreases by two orders of magnitude, concomitant with a sudden Tc suppression around p~8GPa. Even at 9GPa a metallic resistivity state is not recovered, and the ρ(T) "hump" is still detected. A comparison of the data measured upon increasing and decreasing the external pressure leads us to suggest that superconductivity is not related to this hump.

cond-mat.supr-con↗
arXiv2011

Coexistence of Magnetism and Superconductivity in the Iron-based Compound Cs_0.8(FeSe_0.98)_2

We report on muon-spin rotation/relaxation (\muSR), electrical resistivity, magnetization and differential scanning calorimetry measurements performed on a high-quality single crystal of Cs_0.8(FeSe_0.98)_2. Whereas our transport and magnetization data confirm the bulk character of the superconducting state below T_c = 28.5(2)K, the \muSR data indicate that the system is {\it magnetic} below T_N = 478.5(3)K, where a first-order transition occurs. The first-order character of the magnetic transition is confirmed by differential scanning calorimetry data. Taken all together, these data indicate in Cs_0.8(FeSe_0.98)_2 a microscopic coexistence between the superconducting phase and a strong magnetic phase. The observed ratio between T_N and T_c is the highest one reported to date for a magnetic superconductor.

cond-mat.supr-con↗
arXiv2010

Synthesis and crystal growth of Cs0.8(FeSe0.98)2: a new iron-based superconductor with Tc=27K

We report on the synthesis of large single crystals of a new FeSe-layer superconductor Cs0.8(FeSe0.98)2. X-ray powder diffraction, neutron powder-diffraction and magnetization measurements have been used to compare the crystal structure and the magnetic properties of Cs0.8(FeSe0.98)2 with those of the recently discovered potassium intercalated system KxFe2Se2. The new compound Cs0.8(FeSe0.98)2 shows a slightly lower superconducting transition temperature (Tc=27.4 K) in comparison to 29.5 in K0.8(FeSe0.98)2). The volume of the crystal unit cell increases by replacing K by Cs - the c-parameter grows from 14.1353(13) Å to 15.2846(11) Å. For the so far known alkali metal intercalated layered compounds (K0.8Fe2Se2 and Cs0.8(FeSe0.98)2) the Tc dependence on the anion height (distance between Fe-layers and Se-layers) was found to be analogous to those reported for As-containing Fe-superconductors and Fe(Se1-xChx), where Ch=Te, S.

cond-mat.supr-con↗
arXiv2010

Doping and temperature dependence of Mn 3d states in A-site ordered manganites

We present a systematic study of the electronic structure in A-site ordered manganites as function of doping and temperature. The energy dependencies observed with soft x-ray resonant diffraction (SXRD) at the Mn L_{2,3} edges are compared with structural investigations using neutron powder diffraction as well as with cluster calculations. The crystal structures obtained with neutron powder diffraction reflect the various orbital and charge ordered phases and show an increase of the Mn-O-Mn bond angle as function of doping and temperature. Cluster calculations show that the observed spectral changes in SXRD as a function of doping are more pronounced than expected from an increase in bandwitdh due to the increase in Mn-O-Mn bond angle, and are best described by holes that are distributed at the neighbouring oxygen ions. These holes are not directly added to the Mn 3d shell, but centered at the Mn site. In contrast, the spectral changes in SXRD as function of temperature are best described by an increase of magnetic correlations. This demonstrates the strong correlations between orbitals and magnetic moments of the 3d states.

cond-mat.str-el↗
arXiv2010

Tuning the superconducting and magnetic properties in Fe_ySe_0.25Te_0.75 by varying the Fe-content

The superconducting and magnetic properties of Fe$_{y}$Se$_{0.25}$Te$_{0.75}$ single crystals ($0.9\leq y \leq1.1$) were studied by means of x-ray diffraction, SQUID magnetometry, muon spin rotation, and elastic neutron diffraction. The samples with $y<1$ exhibit coexistence of bulk superconductivity and incommensurate magnetism. The magnetic order remains incommensurate for $y\geq 1$, but with increasing Fe content superconductivity is suppressed and the magnetic correlation length increases. The results show that the superconducting and the magnetic properties of the Fe$_{y}$Se$_{1-x}$Te$_{x}$ can be tuned not only by varying the Se/Te ratio but also by changing the Fe content.

cond-mat.supr-con↗
arXiv2010

Direct observation of impurity-induced magnetism in an S = 1/2 antiferromagnetic Heisenberg 2-leg spin ladder

Nuclear magnetic resonance and magnetization measurements were used to probe the magnetic features of single-crystalline Bi(Cu(1-x)Znx)2PO6 with 0 0 and we present clear evidence for a temperature dependent variation of the local magnetization close to the Zn sites. The generic nature of this observation is indicated by results of model calculations on appropriate spin systems of limited size employing QMC methods.

cond-mat.str-el↗
arXiv2010

Iron isotope effect on the superconducting transition temperature and the crystal structure of FeSe_1-x

The Fe isotope effect (Fe-IE) on the transition temperature T_c and the crystal structure was studied in the Fe chalcogenide superconductor FeSe_1-x by means of magnetization and neutron powder diffraction (NPD). The substitution of natural Fe (containing \simeq 92% of ^{56}Fe) by its lighter ^{54}Fe isotope leads to a shift of T_c of 0.22(5)K corresponding to an Fe-IE exponent of α_Fe=0.81(15). Simultaneously, a small structural change with isotope substitution is observed by NDP which may contribute to the total Fe isotope shift of T_c.

cond-mat.supr-con↗
arXiv2010

2D orbital-like magnetic order in ${\rm La_{2-x}Sr_xCuO_4}$

In high temperature copper oxides superconductors, a novel magnetic order associated with the pseudogap phase has been identified in two different cuprate families over a wide region of temperature and doping. We here report the observation below 120 K of a similar magnetic ordering in the archetypal cuprate ${\rm La_{2-x}Sr_xCuO_4}$ (LSCO) system for x=0.085. In contrast to the previous reports, the magnetic ordering in LSCO is {\it\bf only} short range with an in-plane correlation length of $\sim$ 10 Å and is bidimensional (2D). Such a less pronounced order suggests an interaction with other electronic instabilities. In particular, LSCO also exhibits a strong tendency towards stripes ordering at the expense of the superconducting state.

cond-mat.supr-con↗
arXiv2010

Anisotropic superconducting properties of single-crystalline FeSe0.5Te0.5

Iron-chalcogenide single crystals with the nominal composition FeSe$_{0.5}$Te$_{0.5}$ and a transition temperature of $T_{c}\simeq14.6$ K were synthesized by the Bridgman method. The structural and anisotropic superconducting properties of those crystals were investigated by means of single crystal X-ray and neutron powder diffraction, SQUID and torque magnetometry, and muon-spin rotation. Room temperature neutron powder diffraction reveals that 95% of the crystal volume is of the same tetragonal structure as PbO. The structure refinement yields a stoichiometry of Fe_1.045Se_0.406Te_0.594. Additionally, a minor hexagonal Fe_7Se_8 impurity phase was identified. The magnetic penetration depth λat zero temperature was found to be 491(8) nm in the ab-plane and 1320(14) nm along the c-axis. The zero-temperature value of the superfluid density ρ_s(0) λ^-2(0) obeys the empirical Uemura relation observed for various unconventional superconductors, including cuprates and iron-pnictides. The temperature dependences of both λ_ab and λ_c are well described by a two-gap s+s-wave model with the zero-temperature gap values of Δ_S(0)=0.51(3) meV and Δ_L(0)=2.61(9) meV for the small and the large gap, respectively. The magnetic penetration depth anisotropy parameter γ_λ(T)=λ_c(T)/λ_{ab}(T) increases with decreasing temperature, in agreement with γ_λ(T) observed in the iron-pnictide superconductors.

cond-mat.supr-con↗