arXiv subjects

E. Saitoh

Publications and source records attributed to E. Saitoh.

53 records · Page 3Linked to original sources

arXiv2014

Paramagnetic spin pumping

We have demonstrated spin pumping from a paramagnetic state of an insulator La2NiMnO6 into a Pt film. Single-crystalline films of La2NiMnO6 which exhibit a ferromagnetic order at TC ~ 270 K were grown by pulsed laser deposition. The inverse spin Hall voltage induced by spin-current injection has been observed in the Pt layer not only in the ferromagnetic phase of La2NiMnO6 but also in a wide temperature range above TC. The efficient spin pumping in the paramagnetic phase is ascribable to ferromagnetic correlation, not to ferromagnetic order.

cond-mat.mes-hall↗

arXiv2014

Spin current generation from sputtered Y3Fe5O12 films

Spin current injection from sputtered yttrium iron garnet (YIG) films into an adjacent platinum layer has been investigated by means of the spin pumping and the spin Seebeck effects. Films with a thickness of 83 and 96 nanometers were fabricated by on-axis magnetron rf sputtering at room temperature and subsequent post-annealing. From the frequency dependence of the ferromagnetic resonance linewidth, the damping constant has been estimated to be $(7.0\pm1.0)\times 10^{-4}$. Magnitudes of the spin current generated by the spin pumping and the spin Seebeck effect are of the same order as values for YIG films prepared by liquid phase epitaxy. The efficient spin current injection can be ascribed to a good YIG|Pt interface, which is confirmed by the large spin-mixing conductance $(2.0\pm0.2)\times 10^{18}$ m$^{-2}$.

cond-mat.mes-hall↗

arXiv2014

Influence of interface condition on spin-Seebeck effects

The longitudinal spin-Seebeck effect (LSSE) has been investigated for Pt/yttrium iron garnet (YIG) bilayer systems. The magnitude of the voltage induced by the LSSE is found to be sensitive to the Pt/YIG interface condition. We observed large LSSE voltage in a Pt/YIG system with a better crystalline interface, while the voltage decays steeply when an amorphous layer is introduced at the interface artificially.

cond-mat.mtrl-sci↗

arXiv2014

Interface-dependent magnetotransport properties for thin Pt films on ferrimagnetic Y3Fe5O12

We have studied magnetoresistance and Hall effects for 1.8-nm-thick Pt films grown on a ferrimagnetic insulator Y3Fe5O12 in a wide temperature (0.46-300 K) and magnetic-field (-15-15 T) region. In the low-temperature regime where quantum corrections to conductivity are observed, weak antilocalization behavior observed in Pt films is critically suppressed when the film is attached to Y3Fe5O12. Hall resistance in the Pt film is also affected by Y3Fe5O12, and it exhibits logarithmic temperature dependence in a broad temperature range. The magnetotransport properties in the high-field range are significantly influenced by the interface between Pt and Y3Fe5O12.

cond-mat.mes-hall↗

arXiv2013

Bulk topological insulators as inborn spintronics detectors

Detection and manipulation of electrons' spins are key prerequisites for spin-based electronics or spintronics. This is usually achieved by contacting ferromagnets with metals or semiconductors, in which the relaxation of spins due to spin-orbit coupling limits both the efficiency and the length scale. In topological insulator materials, on the contrary, the spin-orbit coupling is so strong that the spin direction uniquely determines the current direction, which allows us to conceive a whole new scheme for spin detection and manipulation. Nevertheless, even the most basic process, the spin injection into a topological insulator from a ferromagnet, has not yet been demonstrated. Here we report successful spin injection into the surface states of topological insulators by using a spin pumping technique. By measuring the voltage that shows up across the samples as a result of spin pumping, we demonstrate that a spin-electricity conversion effect takes place in the surface states of bulk-insulating topological insulators Bi1.5Sb0.5Te1.7Se1.3 and Sn-doped Bi2Te2Se. In this process, due to the two-dimensional nature of the surface state, there is no spin current along the perpendicular direction. Hence, the mechanism of this phenomenon is different from the inverse spin Hall effect and even predicts perfect conversion between spin and electricity at room temperature. The present results reveal a great advantage of topological insulators as inborn spintronics devices.

cond-mat.mtrl-sci↗

arXiv2013

Observation of Longitudinal Spin Seebeck Effect with Various Transition Metal Films

We evaluated the thermoelectric properties of longitudinal spin Seebeck devices by using ten different transition metals (TMs). Both the intensity and sign of spin Seebeck coefficients were noticeably dependent on the degree of the inverse spin Hall effect and the resistivity of each TM film. Spin dependent behaviors were also observed under ferromagnetic resonance. These results indicate that the output of the spin Seebeck devices originates in the spin current.

cond-mat.mtrl-sci↗

arXiv2013

Spin mixing conductance at a well-controlled platinum/yttrium iron garnet interface

A platinum (Pt)/yttrium iron garnet (YIG) bilayer system with a well-controlled interface has been developed; spin mixing conductance at the Pt/YIG interface has been studied. Crystal perfection at the interface is experimentally demonstrated to contribute to large spin mixing conductance. The spin mixing conductance is obtained to be $1.3\times10^{18} \rm{m^{-2}}$ at the well-controlled Pt/YIG interface, which is close to a theoretical prediction.

cond-mat.mes-hall↗

arXiv2013

Longitudinal Spin Seebeck Effect Free from the Proximity Nernst Effect

This letter provides evidence for intrinsic longitudinal spin Seebeck effects (LSSEs) that are free from the anomalous Nernst effect (ANE) caused by an extrinsic proximity effect. We report the observation of LSSEs in Au/Y3Fe5O12 (YIG) and Pt/Cu/YIG systems, showing that LSSE appears even when the mechanism of the proximity ANE is clearly removed. In the conventional Pt/YIG structure, furthermore, we separate the LSSE from the ANE by comparing the voltages in different magnetization and temperature-gradient configurations; the ANE contamination was found to be negligibly small even in the Pt/YIG structure.

cond-mat.mtrl-sci↗

arXiv2012

Observation of the spin Seebeck effect in epitaxial Fe3O4 thin films

We report the first experimental observation of the spin Seebeck effect in magnetite thin films. The signal observed at temperatures above the Verwey transition is a contribution from both the anomalous Nernst (ANE) and spin Seebeck effects (SSE). The contribution from the ANE of the Fe3O4 layer to the SSE is found to be negligible due to the resistivity difference between Fe3O4 and Pt layers. Below the Verwey transition the SSE is free from the ANE of the ferromagnetic layer and it is also found to dominate over the ANE due to magnetic proximity effect on the Pt layer.

cond-mat.mtrl-sci↗

arXiv2012

Heat-induced damping modification in YIG/Pt hetero-structures

We experimentally demonstrate the manipulation of magnetization relaxation utilizing a temperature difference across the thickness of an yttrium iron garnet/platinum (YIG/Pt) hetero-structure: the damping is either increased or decreased depending on the sign of the temperature gradient. This effect might be explained by a thermally-induced spin torque on the magnetization precession. The heat-induced variation of the damping is detected by microwave techniques as well as by a DC voltage caused by spin pumping into the adjacent Pt layer and the subsequent conversion into a charge current by the inverse spin Hall effect.

cond-mat.mes-hall↗

arXiv2012

Spin Hall Magnetoresistance Induced by a Non-Equilibrium Proximity Effect

We report anisotropic magnetoresistance in Pt|Y3Fe5O12 bilayers. In spite of Y3Fe5O12 being a very good electrical insulator, the resistance of the Pt layer reflects its magnetization direction. The effect persists even when a Cu layer is inserted between Pt and Y3Fe5O12, excluding the contribution of induced equilibrium magnetization at the interface. Instead, we show that the effect originates from concerted actions of the direct and inverse spin Hall effects and therefore call it "spin Hall magnetoresistance."

cond-mat.mtrl-sci↗

arXiv2012

Thermal spin pumping and magnon-phonon-mediated spin-Seebeck effect

The spin-Seebeck effect (SSE) in ferromagnetic metals and insulators has been investigated systematically by means of the inverse spin-Hall effect (ISHE) in paramagnetic metals. The SSE generates a spin voltage as a result of a temperature gradient in a ferromagnet, which injects a spin current into an attached paramagnetic metal. In the paramagnet, this spin current is converted into an electric field due to the ISHE, enabling the electric detection of the SSE. The observation of the SSE is performed in longitudinal and transverse configurations consisting of a ferromagnet/paramagnet hybrid structure, where thermally generated spin currents flowing parallel and perpendicular to the temperature gradient are detected, respectively. Our results explain the SSE in terms of a two-step process: (1) the temperature gradient creates a non-equilibrium state in the ferromagnet governed by both magnon and phonon propagations and (2) the non-equilibrium between magnons in the ferromagnet and electrons in the paramagnet at the contact interface leads to "thermal spin pumping" and the ISHE signal. The non-equilibrium state of metallic magnets (e.g. Ni81Fe19) under a temperature gradient is governed mainly by the phonons in the sample and the substrate, while in insulating magnets (e.g. Y3Fe5O12) both magnon and phonon propagations appear to be important. The phonon-mediated non-equilibrium that drives the thermal spin pumping is confirmed also by temperature-dependent measurements, giving rise to a giant enhancement of the SSE signals at low temperatures.

cond-mat.mtrl-sci↗

arXiv2012

Spin Pumping Driven by Bistable Exchange Spin Waves

Spin pumping driven by bistable exchange spin waves is demonstrated in a Pt/Y$_3$Fe$_5$O$_{12}$ film under parametric excitation. In the Pt/Y$_3$Fe$_5$O$_{12}$ film, the spin pumping driven by parametric excitation selectively enhances the relaxation of short-wavelength exchange spin waves, indicating strong coupling between the exchange spin waves and spin currents at the interface through efficient spin transfer. The parametric spin pumping, furthermore, allows direct access to nonlinear spin wave dynamics in combination with the inverse spin Hall effect, revealing unconventional bistability of the exchange spin waves.

cond-mat.mtrl-sci↗

arXiv2011

Acoustic spin pumping: Direct generation of spin currents from sound waves in Pt/Y3Fe5O12 hybrid structures

Using a Pt/Y3Fe5O12 (YIG) hybrid structure attached to a piezoelectric actuator, we demonstrate the generation of spin currents from sound waves. This "acoustic spin pumping" (ASP) is caused by the sound wave generated by the piezoelectric actuator, which then modulates the distribution function of magnons in the YIG layer and results in a pure-spin-current injection into the Pt layer across the Pt/YIG interface. In the Pt layer, this injected spin current is converted into an electric voltage due to the inverse spin-Hall effect (ISHE). The ISHE voltage induced by the ASP is detected by measuring voltage in the Pt layer at the piezoelectric resonance frequency of the actuator coupled with the Pt/YIG system. The frequency-dependent measurements enable us to separate the ASP-induced signals from extrinsic heating effects. Our model calculation based on the linear response theory provides us with a qualitative and quantitative understanding of the ASP in the Pt/YIG system.

cond-mat.mtrl-sci↗

arXiv2011

Temporal behavior of the inverse spin Hall voltage in a magnetic insulator-nonmagnetic metal structure

It is demonstrated that upon pulsed microwave excitation, the temporal behavior of a spin-wave induced inverse spin Hall voltage in a magnetic insulator-nonmagnetic metal structure is distinctly different from the temporal evolution of the directly excited spin-wave mode from which it originates. The difference in temporal behavior is attributed to the excitation of long-lived secondary spin-wave modes localized at the insulator-metal interface.

cond-mat.mes-hall↗

arXiv2010

Spin Seebeck insulator

Thermoelectric generation is an essential function of future energy-saving technologies. However, this generation has been an exclusive feature of electric conductors, a situation which inflicts a heavy toll on its application; a conduction electron often becomes a nuisance in thermal design of devices. Here we report electric-voltage generation from heat flowing in an insulator. We reveal that, despite the absence of conduction electrons, a magnetic insulator LaY2Fe5O12 converts a heat flow into spin voltage. Attached Pt films transform this spin voltage into electric voltage by the inverse spin Hall effect. The experimental results require us to introduce thermally activated interface spin exchange between LaY2Fe5O12 and Pt. Our findings extend the range of potential materials for thermoelectric applications and provide a crucial piece of information for understanding the physics of the spin Seebeck effect.

cond-mat.mtrl-sci↗

arXiv2010

Enhancement of the spin pumping efficiency by spin-wave mode selection

The spin pumping efficiency of lateral standing spin wave modes in a rectangular YIG/Pt sample has been investigated by means of the inverse spin-Hall effect (ISHE). The standing spin waves drive spin pumping, the generation of spin currents from magnetization precession, into the Pt layer which is converted into a detectable voltage due to the ISHE. We discovered that the spin pumping efficiency is significantly higher for lateral standing surface spin waves rather than for volume spin wave modes. The results suggest that the use of higher-mode surface spin waves allows for the fabrication of an efficient spin-current injector.

cond-mat.mes-hall↗