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E. Schneider

Publications and source records attributed to E. Schneider.

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Efficient formation and identification of single emitters in 4H-SiC following maskless heavy ion implantation

Single photon emitters in silicon carbide (SiC) are a leading platform for scalable quantum technologies. Recent interest has focused on oxygen-vacancy-related emitters, which show exceptionally high optical brightness and strong spin readout contrast. One barrier to scalable quantum devices based on these emitters is the challenge of maskless formation and rapid identification. Here, we demonstrate the formation of isolated bright single emitters in 4H-SiC, using low-energy maskless implantation of heavy ions bismuth and tin. Following annealing, up to 18% of implanted sites host a single emitter, with optimal yields achieved at annealing temperatures of 900-1000 degrees C. Occupancy statistics are modelled to estimate the implantation dose that maximises single-emitter yield. We introduce a tiered characterisation scheme, where a simple intensity threshold isolates single-emitter candidates, confirmed through photon correlation measurements, after which correlations between polarisation, saturation count rate and magnetic resonance frequency assign emitter type. It is shown that time-consuming low-temperature spectroscopy is not necessary to distinguish emitter types. Together, maskless heavy-ion implantation and selective screening offer an efficient route to forming and rapidly identifying near-surface single emitters for room-temperature quantum technologies such as quantum sensing.

quant-ph

Quantum Propagation of Electronic Excitations in Macromolecules: A Computationally Efficient Multi-Scale Approach

We introduce a theoretical approach to study the quantum-dissipative dynamics of electronic excitations in macromolecules, which enables to perform calculations in large systems and cover long time intervals. All the parameters of the underlying microscopic Hamiltonian are obtained from \emph{ab-initio} electronic structure calculations, ensuring chemical detail. In the short-time regime, the theory is solvable using a diagrammatic perturbation theory, enabling analytic insight. To compute the time evolution of the density matrix at intermediate times, typically $\lesssim$~ps, we develop a Monte Carlo algorithm free from any sign or phase problem, hence computationally efficient. Finally, the dynamics in the long-time and large-distance limit can be studied combining the microscopic calculations with renormalization group techniques to define a rigorous low-resolution effective theory. We benchmark our Monte Carlo algorithm against the results obtained in perturbation theory and using a semi-classical non-perturbative scheme. Then we apply it to compute the intra-chain charge mobility in a realistic conjugate polymer.

cond-mat.mes-hall

Long-Distance Quantum Transport Dynamics in Macromolecules

Using renormalization group methods, we develop a rigorous coarse-grained representation of the dissipative dynamics of quantum excitations propagating inside open macromolecular systems. We show that, at very low spatial resolution, this quantum transport theory reduces to a modified Brownian process, in which quantum delocalization effects are accounted for by means of an effective term in the Onsager-Machlup functional. Using this formulation, we derive a simple analytic solution for the time-dependent probability of observing the quantum excitation at a given point in the macromolecule. This formula can be used to predict the migration of natural or charged quantum excitations in a variety of molecular systems including biological and organic polymers, organic crystalline transistors or photosynthetic complexes. For illustration purpose, we apply this method to investigate intelastic electornic hole transport in a long homo-DNA chain.

cond-mat.mes-hall

The UV continua and inferred stellar populations of galaxies at z ~ 7 - 9 revealed by the Hubble Ultra Deep Field 2012 campaign

We use the new ultra-deep, near-infrared imaging of the Hubble Ultra-Deep Field (HUDF) provided by our UDF12 HST WFC3/IR campaign to explore the rest-frame UV properties of galaxies at redshifts z > 6.5. We present the first unbiased measurement of the average UV power-law index, beta, for faint galaxies at z ~ 7, the first meaningful measurements of beta at z ~ 8, and tentative estimates for a new sample of galaxies at z ~ 9. Utilising galaxy selection in the new F140W imaging to minimize colour bias, and applying both colour and power-law estimators of beta, we find beta = -2.1 (+/-0.2) at z ~ 7 for galaxies with M_UV ~ -18. This means that the faintest galaxies uncovered at this epoch have, on average, UV colours no more extreme than those displayed by the bluest star-forming galaxies at low redshift. At z ~ 8 we find a similar value, beta = -1.9 (+/-0.3). At z ~ 9, we find beta = -1.8 (+/-0.6), essentially unchanged from z ~ 6 - 7 (albeit highly uncertain). Finally, we show that there is as yet no evidence for a significant intrinsic scatter in beta within our new, robust z ~ 7 galaxy sample. Our results are most easily explained by a population of steadily star-forming galaxies with either ~ solar metallicity and zero dust, or moderately sub-solar (~ 10-20%) metallicity with modest dust obscuration (A_V ~ 0.1-0.2). This latter interpretation is consistent with the predictions of a state-of-the-art galaxy-formation simulation, which also suggests that a significant population of very-low metallicity, dust-free galaxies with beta ~ -2.5 may not emerge until M_UV > -16, a regime likely to remain inaccessible until the James Webb Space Telescope.

astro-ph.CO

Dissipative Quantum Transport in Macromolecules: An Effective Field Theory Approach

We introduce an atomistic approach to the dissipative quantum dynamics of charged or neutral excitations propagating through macromolecular systems. Using the Feynman-Vernon path integral formalism, we analytically trace out from the density matrix the atomic coordinates and the heat bath degrees of freedom. This way we obtain an effective field theory which describes the real-time evolution of the quantum excitation and is fully consistent with the fluctuation-dissipation relation. The main advantage of the field-theoretic approach is that it allows to avoid using the Keldysh contour formulation. This simplification makes it straightforward to derive Feynman diagrams to analytically compute the effects of the interaction of the propagating quantum excitation with the heat bath and with the molecular atomic vibrations. For illustration purposes, we apply this formalism to investigate the loss of quantum coherence of holes propagating through a poly(3-alkylthiophene) polymer

cond-mat.soft

Energy Spectra, Altitude Profiles and Charge Ratios of Atmospheric Muons

We present a new measurement of air shower muons made during atmospheric ascent of the High Energy Antimatter Telescope balloon experiment. The muon charge ratio mu+ / mu- is presented as a function of atmospheric depth in the momentum interval 0.3-0.9 GeV/c. The differential mu- momentum spectra are presented between 0.3 and about 50 GeV/c at atmospheric depths between 13 and 960 g/cm^2. We compare our measurements with other recent data and with Monte Carlo calculations of the same type as those used in predicting atmospheric neutrino fluxes. We find that our measured mu- fluxes are smaller than the predictions by as much as 70% at shallow atmospheric depths, by about 20% at the depth of shower maximum, and are in good agreement with the predictions at greater depths. We explore the consequences of this on the question of atmospheric neutrino production.

hep-ex

The Energy Spectra and Relative Abundances of Electrons and Positrons in the Galactic Cosmic Radiation

Observations of cosmic-ray electrons and positrons have been made with a new balloon-borne detector, HEAT (the "High-Energy Antimatter Telescope"), first flown in 1994 May from Fort Sumner, NM. We describe the instrumental approach and the data analysis procedures, and we present results from this flight. The measurement has provided a new determination of the individual energy spectra of electrons and positrons from 5 GeV to about 50 GeV, and of the combined "all-electron" intensity (e+ + e-) up to about 100 GeV. The single power-law spectral indices for electrons and positrons are alpha = 3.09 +/- 0.08 and 3.3 +/- 0.2, respectively. We find that a contribution from primary sources to the positron intensity in this energy region, if it exists, must be quite small.

astro-ph

Measurements of the Cosmic-Ray Positron Fraction From 1 to 50 GeV

Two measurements of the cosmic-ray positron fraction as a function of energy have been made using the High Energy Antimatter Telescope (HEAT) balloon-borne instrument. The first flight took place from Ft. Sumner, New Mexico in 1994, and yielded results above the geomagnetic cutoff energy of 4.5 GeV. The second flight from Lynn Lake, Manitoba in 1995 permitted measurements over a larger energy interval, from 1 GeV to 50 GeV. In this letter we present results on the positron fraction based on data from the Lynn Lake flight, and compare these with the previously published results from the Ft. Sumner flight. The results confirm that the positron fraction does not increase with energy above ~10 GeV, although a small excess above purely secondary production cannot be ruled out. At low energies the positron fraction is slightly larger than that reported from measurements made in the 1960's. This effect could possibly be a consequence of charge dependence in the level of solar modulation.

astro-ph