arXiv subjects

E. Uykur

Publications and source records attributed to E. Uykur.

25 records · Page 2Linked to original sources

arXiv2019

Low-Temperature Dielectric Anomalies at the Mott Insulator-Metal Transition

The correlation-driven Mott transition is commonly characterized by a drop in resistivity across the insulator-metal phase boundary; yet, the complex permittivity provides a deeper insight into the microscopic nature. We investigate the frequency- and temperature-dependent dielectric response of the Mott insulator $κ$-(BEDT-TTF)$_{2}$-Cu$_2$(CN)$_3$ when tuning from a quantum spin liquid into the Fermi-liquid state by applying external pressure and chemical substitution of the donor molecules. At low temperatures the coexistence region at the first-order transition leads to a strong enhancement of the quasi-static dielectric constant $ε_1$ when the effective correlations are tuned through the critical value. Several dynamical regimes are identified around the Mott point and vividly mapped through pronounced permittivity crossovers. All experimental trends are captured by dynamical mean-field theory of the single-band Hubbard model supplemented by percolation theory.

cond-mat.str-el↗

arXiv2019

Hertz-to-terahertz dielectric response of nanoconfined water molecules

Broad-band dielectric spectroscopy, heat capacity measurements and molecular dynamic simulations are applied to study excitations of interacting electric dipoles spatially arranged in a network with an inter-dipole distance of 5-10 A. The dipoles with magnitude of 1.85 Debye are represented by single H2O molecules located in voids (0.5 nm size) formed by ions of the crystal lattice of cordierite. We discover emergence of nontrivial disordered paraelectric phase of dipolar system with signs of phase transition below 3 K.

cond-mat.mtrl-sci↗

arXiv2019

Magneto-optical probe of the fully gapped Dirac band in ZrSiS

We present a far-infrared magneto-optical study of the gapped nodal-line semimetal ZrSiS in magnetic fields $B$ up to 7 T. The observed field-dependent features, which represent intra- (cyclotron resonance) and interband transitions, develop as $\sqrt{B}$ in increasing field and can be consistently explained within a simple 2D Dirac band model with a gap of 26 meV and an averaged Fermi velocity of $3\times10^{5}$ m/s. This indicates a rather narrow distribution of these parameters along the in-plane portions of the nodal line in the Brillouin zone. A field-induced feature with an energy position that does not depend on $B$ is also detected in the spectra. Possible origins of this feature are discussed.

cond-mat.mes-hall↗

arXiv2018

Unique interplay between superconducting and ferromagnetic orders in EuRbFe$_4$As$_4$

Transport, magnetic and optical investigations on EuRbFe$_4$As$_4$ single crystals evidence that the ferromagnetic ordering of the Eu$^{2+}$ magnetic moments at $T_N=15$ K, below the superconducting transition ($T_c=36$ K), affects superconductivity in a weak but intriguing way. Upon cooling below $T_N$, the zero resistance state is preserved and the superconductivity is affected by the in-plane ferromagnetism mainly at domain boundaries; a perfect diamagnetism is recovered at low temperatures. The infrared conductivity is strongly suppressed in the far-infrared region below $T_c$, associated with the opening of a complete superconducting gap at $2Δ= 10$ meV. A gap smaller than the weak coupling limit suggests the strong orbital effects or, within a multiband superconductivity scenario, the existence of a larger yet unrevealed gap.

cond-mat.supr-con↗

arXiv2017

Optical spectroscopy study on pressure-induced phase transitions in the three-dimensional Dirac semimetal Cd$_3$As$_2$

We report a room-temperature optical reflectivity study performed on [112]-oriented Cd$_3$As$_2$ single crystals over a broad energy range under external pressure up to 10 GPa. The abrupt drop of the band dispersion parameter ($z$-parameter) and the interruption of the gradual redshift of the bandgap at $\sim$4~GPa confirms the structural phase transition from a tetragonal to a monoclinic phase in this material. The pressure-induced increase of the overall optical conductivity at low energies and the continuous redshift of the high-energy bands indicate that the system evolves towards a topologically trivial metallic state, although a complete closing of the band gap could not be observed in the studied pressure range. Furthermore, a detailed investigation of the low-pressure regime suggests the possible existence of an intermediate state between 2 and 4~GPa , that might be a precursor of the structural phase transition or due to the lifted degeneracy of the Dirac nodes. Several optical parameters show yet another anomaly at 8~GPa, where low-temperature superconductivity was found in an earlier study.

cond-mat.mtrl-sci↗

arXiv2015

Optical Study of BaFe$_2$As$_2$ under pressure: Coexistence of spin-density-wave gap and superconductivity

Temperature-dependent reflectivity measurements in the frequency range 85 - 7000 cm$^{-1}$ were performed on BaFe$_2$As$_2$ single crystals under pressure up to $\sim$5 GPa. The corresponding pressure- and temperature-dependent optical conductivity was analyzed with the Drude-Lorentz model to extract the coherent and incoherent contributions. The gradual suppression of the spin-density wave (SDW) state with increasing pressure and the appearance of the superconducting phase coexisting with the SDW phase at 3.6~GPa were observed. At 3.6~GPa, the reflectivity reaches unity below $\sim$95~cm$^{-1}$ indicating the opening of the superconducting gap and shows a full gap tendency at 6 K.

cond-mat.supr-con↗

arXiv2012

In-plane optical spectra of Y$_{1-x}$Ca$_{x}$Ba$_{2}$Cu$_{3}$O$_{7-δ}$: Overdoping and disorder effect on residual conductivity

We measured the temperature dependence of the in-plane polarized reflectivity spectra of twin-free Y$_{1-x}$Ca$_{x}$Ba$_{2}$Cu$_{3}$O$_{7-δ}$ single crystals with different Ca-concentrations (x=0,0.11 and 0.16) from optimally doped to heavily overdoped region. Low energy optical conductivity spectra showed a Drude-like residual conductivity at temperatures far below the superconducting transition temperature, which indicates the presence of unpaired-normal carriers in the superconducting state. Comparing the spectra at a fixed Ca-content or at a fixed doping level, we have revealed that the carrier overdoping increases unpaired carriers in addition to those induced by the Ca-disorder. We also found the superconducting behavior of the one-dimensional CuO chains for the Ca-free samples.

cond-mat.supr-con↗