arXiv subjects

Edan Lerner

Publications and source records attributed to Edan Lerner.

At least 91 records · Page 5Linked to original sources

arXiv2016

The micromechanics of nonlinear plastic modes

Nonlinear plastic modes (NPMs) are collective displacements that are indicative of imminent plastic instabilities in elastic solids. In this work we formulate the atomistic theory that describes the reversible evolution of NPMs and their associated stiffnesses under external deformations. The deformation-dynamics of NPMs is compared to those of the analogous observables derived from atomistic linear elastic theory, namely destabilizing eigenmodes of the dynamical matrix and their associated eigenvalues. The key result we present and explain is that the dynamics of NPMs and of destabilizing eigenmodes under external deformations follow different scaling laws with respect to the proximity to imminent instabilities. In particular, destabilizing modes vary with a singular rate, whereas NPMs' exhibit no such singularity. As a result, NPMs converge much earlier than destabilizing eigenmodes to their common final form at plastic instabilities. This dynamical difference between NPMs and linear destabilizing eigenmodes underlines the usefulness of NPMs for predicting the locus and geometry of plastic instabilities, compared to their linear-elastic counterparts.

cond-mat.soft↗

arXiv2016

Effect of particle collisions in dense suspension flows

We study non-local effects associated with particle collisions in dense suspension flows, in the context of the affine solvent model known to capture various aspects of the jamming transition. We show that an individual collision changes significantly the velocity field on a characteristic volume $Ω_c\sim 1/δz$ that diverges as jamming is approached, where $δz$ is the deficit in coordination number required to jam the system. Such an event also affects the contact forces between particles on that same volume $Ω_c$, but this change is modest in relative terms, of order $f_{coll}\sim \bar{f}^{0.8}$, where $\bar{f}$ is the typical contact force scale. We then show that the requirement that coordination is stationary (such that a collision has a finite probability to open one contact elsewhere in the system) yields the scaling of the viscosity (or equivalently the viscous number) with coordination deficit $δz$. The same scaling result was derived in [E.~DeGiuli, G.~Düring, E.~Lerner, and M.~Wyart, Phys.~Rev.~E {\bf 91}, 062206 (2015)] via different arguments making an additional assumption. The present approach gives a mechanistic justification as to why the correct finite size scaling volume behaves as $1/δz$, and can be used to recover a marginality condition known to characterize the distributions of contact forces and gaps in jammed packings.

cond-mat.stat-mech↗

arXiv2015

Nonlinear plastic modes in disordered solids

We propose a framework within which a robust mechanical definition of precursors to plastic instabilities, often termed `soft-spots', naturally emerges. They are shown to be collective displacements (modes) $\hat{z}_0$ that correspond to local minima of the `barrier function' $b(\hat{z})$. The latter is derived from the cubic approximation of the variation $δU_{\hat{z}}(s)$ of the potential energy upon displacing particles a distance $s$ along $\hat{z}$. We show that modes $\hat{z}_0$ corresponding to low-lying minima of $b(\hat{z})$ lead to transitions over energy barriers in the glass, and are therefore associated with highly asymmetric variations $δU_{\hat{z}}(s)$ with $s$. We further demonstrate how a heuristic search for local minima of $b(\hat{z})$ can a-priori detect the locus and geometry of imminent plastic instabilities with remarkable accuracy, at strains as large as $γ_c-γ\sim 10^{-2}$ away from the instability strain $γ_c$, where the non-affine displacements under shear are still largely delocalized. Our findings suggest that the a-priori detection of plastic instabilities can be effectively carried out by the investigation of the landscape of $b(\hat{z})$.

cond-mat.soft↗

arXiv2014

Scaling description of the yielding transition in soft amorphous solids at zero temperature

Yield stress materials flow if a sufficiently large shear stress is ap- plied. Although such materials are ubiquitous and relevant for indus- try, there is no accepted microscopic description of how they yield, even in the simplest situations where temperature is negligible and where flow inhomogeneities such as shear bands or fractures are ab- sent. Here we propose a scaling description of the yielding transition in amorphous solids made of soft particles at zero temperature. Our description makes a connection between the Herschel-Bulkley expo- nent characterizing the singularity of the flow curve near the yield stress Σc, the extension and duration of the avalanches of plasticity observed at threshold, and the density P(x) of soft spots, or shear transformation zones, as a function of the stress increment x be- yond which they yield. We argue that the critical exponents of the yielding transition can be expressed in terms of three independent exponents θ, df and z, characterizing respectively the density of soft spots, the fractal dimension of the avalanches, and their duration. Our description shares some similarity with the depinning transition that occurs when an elastic manifold is driven through a random potential, but also presents some striking differences. We test our arguments in an elasto-plastic model, an automaton model similar to those used in depinning, but with a different interaction kernel, and find satisfying agreement with our predictions both in two and three dimensions.

cond-mat.soft↗

arXiv2014

Density scaling and quasiuniversality of flow-event statistics for athermal plastic flows

Athermal plastic flows were simulated for the Kob-Andersen binary Lennard-Jones system and its repulsive version in which the sign of the attractive terms is changed to a plus. Properties evaluated from simulations at different densities include the distributions of energy drops, stress drops, and strain intervals between the flow events. By reference to hidden scale invariance we show that simulations at a single density in conjunction with an equilibrium-liquid simulation at the same density allows one to predict the plastic flow-event properties at other densities. We furthermore demonstrate quasiuniversality of the flow-event statistics.

cond-mat.soft↗

arXiv2014

Phonon gap and localization lengths in floppy materials

Gels of semi-flexible polymers, network glasses made of low valence elements, softly compressed ellipses and dense suspensions under flow are examples of floppy materials. These systems present collective motions with almost no restoring force. We study theoretically and numerically the frequency-dependence of the response of these materials, and the length scales that characterize their elasticity. We show that isotropic floppy elastic networks present a phonon gap for frequencies smaller than a frequency $ω^*$ governed by coordination, and that the elastic response is localized on a length scale $l_c\sim 1/\sqrt{ω^*}$ that diverges as the phonon gap vanishes (with a logarithmic correction in the two dimensional case). $l_c$ also characterizes velocity correlations under shear, whereas another length scale $l^*\sim 1/ω^*$ characterizes the effect of pinning boundaries on elasticity. We discuss the implications of our findings for suspensions flows, and the correspondence between floppy materials and amorphous solids near unjamming, where $l_c$ and $l^*$ have also been identified but where their roles are not fully understood.

cond-mat.stat-mech↗

arXiv2014

Length scales and self-organization in dense suspension flows

Dense non-Brownian suspension flows of hard particles display mystifying properties: as the jamming threshold is approached, the viscosity diverges, as well as a length scale that can be identified from velocity correlations. To unravel the microscopic mechanism governing dissipation and its connection to the observed long-range correlations, we develop an analogy between suspension flows and the rigidity transition occurring when floppy networks are pulled -- a transition believed to be associated to the stress-stiffening of certain gels. After deriving the critical properties near the rigidity transition, we show numerically that suspensions flows lie close to it. We find that this proximity causes a decoupling between viscosity and the correlation length of velocities ξ, which scales as the length l_c characterizing the response of the velocity in flow to a local perturbation, previously predicted to follow l_c\sim 1/\sqrt{z_c-z}\sim p^{0.18} where p is the dimensionless particle pressure, z the coordination of the contact network made by the particles and z_c is twice the spatial dimension. We confirm these predictions numerically, predict the existence of a larger length scale l_r\sim 1/\sqrt{p} with mild effects on velocity correlation and the existence of a vanishing strain δγ\sim 1/p that characterizes de-correlation in flow.

cond-mat.stat-mech↗

arXiv2014

Effects of coordination and pressure on sound attenuation, boson peak and elasticity in amorphous solids

Connectedness and applied stress strongly affect elasticity in solids. In various amorphous solids, mechanical stability can be lost either by reducing connectedness or by increasing pressure. We present an effective medium theory of elasticity that extends previous approaches by incorporating the effect of compression, of amplitude $e$, allowing one to describe quantitative features of sound propagation, transport, the boson peak, and elastic moduli near the elastic instability occurring at a compression $e_c$. The theory disentangles several frequencies characterizing the vibrational spectrum: the onset frequency $ω_0\sim \sqrt{e_c-e}$ where strongly-scattered modes appear in the vibrational spectrum, the pressure-independent frequency $ω_*$ where the density of states displays a plateau, the boson peak frequency $ω_{BP}$, and the Ioffe-Regel frequency $ω_{IR}$ where scattering length and wavelength become equal. We predict that sound attenuation crosses over from $ω^4$ to $ω^2$ behaviour at $ω_0$. We predict that a frequency-dependent length scale $l_s(ω)$ and speed of sound $ν(ω)$ characterize vibrational modes, and could be extracted from scattering data. One key result is the prediction of a flat diffusivity above $ω_0$, in agreement with previously unexplained observations. We find that the shear modulus does not vanish at the elastic instability, but drops by a factor of 2. We check our predictions in packings of soft particles and study the case of covalent networks and silica. Overall, our approach unifies sound attenuation, transport and length scales entering elasticity in a single framework where disorder is not the main parameter controlling the boson peak, in agreement with observations. This framework leads to a phase diagram where various glasses can be placed, connecting microscopic structure to vibrational properties.

cond-mat.soft↗

arXiv2013

Breakdown of continuum elasticity in amorphous solids

We show numerically that the response of simple amorphous solids (elastic networks and particle packings) to a local force dipole is characterized by a lengthscale $\ell_c$ that diverges as unjamming is approached as $\ell_c \sim (z - 2d)^{-1/2}$, where $z \ge 2d$ is the mean coordination, and $d$ is the spatial dimension, at odds with previous numerical claims. We also show how the magnitude of the lengthscale $\ell_c$ is amplified by the presence of internal stresses in the disordered solid. Our data suggests a divergence of $\ell_c\sim (p_c-p)^{-1/4}$ with proximity to a critical internal stress $p_c$ at which soft elastic modes become unstable.

cond-mat.soft↗

arXiv2013

On the density of shear transformation zones in amorphous solids

We study the stability of amorphous solids, focusing on the distribution P(x) of the local stress increase x that would lead to an instability. We argue that this distribution is singular P(x)x^θ, where the exponent θ is non-zero if the elastic interaction between rearranging regions is non-monotonic, and increases with the interaction range. For a class of finite dimensional models we show that stability implies a lower bound on θ, which is found to lie near saturation. For quadrupolar interactions these models yield θ ~ 0.6 for d=2 and θ~ 0.4 in d=3 where d is the spatial dimension, accurately capturing previously unresolved observations in atomistic models, both in quasi-static flow and after a fast quench.

cond-mat.soft↗

arXiv2013

Low-energy non-linear excitations in sphere packings

We study theoretically and numerically how hard frictionless particles in random packings can rearrange. We demonstrate the existence of two distinct unstable non-linear modes of rearrangement, both associated with the opening and the closing of contacts. Mode one, whose density is characterized by some exponent θ', corresponds to motions of particles extending throughout the entire system. Mode two, whose density is characterized by an exponent θ != θ', corresponds to the local buckling of a few particles. Mode one is shown to yield at a much higher rate than mode two when a stress is applied. We show that the distribution of contact forces follows P(f) f^{min(θ',θ)}, and that imposing that the packing cannot be densified further leads to the bounds γ >= 1/(2+θ') and γ >= (1-θ)/2, where γ characterizes the singularity of the pair distribution function g(r) at contact. These results extend the theoretical analysis of [M. Wyart, Phys. Rev. Lett 109, 125502 (2012)] where the existence of mode two was not considered. We perform numerics that support that these bounds are saturated with γ \approx 0.38, θ \approx 0.17 and θ' \approx 0.44. We measure systematically the stability of all such modes in packings, and confirm their marginal stability. The principle of marginal stability thus allows to make clearcut predictions on the ensemble of configurations visited in these out-of-equilibrium systems, and on the contact forces and pair distribution functions. It also reveals the excitations that need to be included in a description of plasticity or flow near jamming, and suggests a new path to study two-level systems and soft spots in simple amorphous solids of repulsive particles.

cond-mat.soft↗

arXiv2013

Simulations of driven overdamped frictionless hard spheres

We introduce an event-driven simulation scheme for overdamped dynamics of frictionless hard spheres subjected to external forces, neglecting hydrodynamic interactions. Our event-driven approach is based on an exact equation of motion which relates the driving force to the resulting velocities through the geometric information characterizing the underlying network of contacts between the hard spheres. Our method allows for a robust extraction of the instantaneous coordination of the particles as well as contact force statistics and dynamics, under any chosen driving force, in addition to shear flow and compression. It can also be used for generating high-precision jammed packings under shear, compression, or both. We present a number of additional applications of our method.

cond-mat.soft↗

arXiv2012

Toward a microscopic description of flow near the jamming threshold

We study the relationship between microscopic structure and viscosity in non-Brownian suspensions. We argue that the formation and opening of contacts between particles in flow effectively leads to a negative selection of the contacts carrying weak forces. We show that an analytically tractable model capturing this negative selection correctly reproduces scaling properties of flows near the jamming transition. In particular, we predict that (i) the viscosity η diverges with the coordination z as η ~ (z_c-z)^{-(3+θ)/(1+θ)}, (ii) the operator that governs flow displays a low-frequency mode that controls the divergence of viscosity, at a frequency ω_min\sim(z_c-z)^{(3+θ)/(2+2θ)}, and (iii) the distribution of forces displays a scale f* that vanishes near jamming as f*/ \sim(z_c-z)^{1/(1+θ)} where θ characterizes the distribution of contact forces P(f)\simf^θ at jamming, and where z_c is the Maxwell threshold for rigidity.

cond-mat.soft↗

arXiv2012

A unified framework for non-Brownian suspension flows and soft amorphous solids

While the rheology of non-Brownian suspensions in the dilute regime is well-understood, their behavior in the dense limit remains mystifying. As the packing fraction of particles increases, particle motion becomes more collective, leading to a growing length scale and scaling properties in the rheology as the material approaches the jamming transition. There is no accepted microscopic description of this phenomenon. However, in recent years it has been understood that the elasticity of simple amorphous solids is governed by a critical point, the unjamming transition where the pressure vanishes, and where elastic properties display scaling and a diverging length scale. The correspondence between these two transitions is at present unclear. Here we show that for a simple model of dense flow, which we argue captures the essential physics near the jamming threshold, a formal analogy can be made between the rheology of the flow and the elasticity of simple networks. This analogy leads to a new conceptual framework to relate microscopic structure to rheology. It enables us to define and compute numerically normal modes and a density of states. We find striking similarities between the density of states in flow, and that of amorphous solids near unjamming: both display a plateau above some frequency scale ω* ~ |z_c-z|, where z is the coordination of the network of particles in contact, z_c = 2D where D is the spatial dimension. However, a spectacular difference appears: the density of states in flow displays a single mode at another frequency scale ω_{min} << ω* governing the divergence of the viscosity.

cond-mat.soft↗

arXiv2011

Direct Estimate of the Static Length-Scale Accompanying the Glass Transition

Characterizing the glass state remains elusive since its distinction from a liquid state is not obvious. Glasses are liquids whose viscosity has increased so much that they cannot flow. Accordingly there have been many attempts to define a static length-scale associated with the dramatic slowing down of supercooled liquid with decreasing temperature. Here we present a simple method to extract the desired length-scale which is highly accessible both for experiments and for numerical simulations. The fundamental idea is that low lying vibrational frequencies come in two types, those related to elastic response and those determined by plastic instabilities. The minimal observed frequency is determined by one or the other, crossing at a typical length-scale which is growing with the approach of the glass transition. This length-scale characterizes the correlated disorder in the system, where on longer length-scales the details of the disorder become irrelevant, dominated by the Debye model of elastic modes.

cond-mat.stat-mech↗

arXiv2011

Do Athermal Amorphous Solids Exist?

We study the elastic theory of amorphous solids made of particles with finite range interactions in the thermodynamic limit. For the elastic theory to exist one requires all the elastic coefficients, linear and nonlinear, to attain a finite thermodynamic limit. We show that for such systems the existence of non-affine mechanical responses results in anomalous fluctuations of all the nonlinear coefficients of the elastic theory. While the shear modulus exists, the first nonlinear coefficient B_2 has anomalous fluctuations and the second nonlinear coefficient B_3 and all the higher order coefficients (which are non-zero by symmetry) diverge in the thermodynamic limit. These results put a question mark on the existence of elasticity (or solidity) of amorphous solids at finite strains, even at zero temperature. We discuss the physical meaning of these results and propose that in these systems elasticity can never be decoupled from plasticity: the nonlinear response must be very substantially plastic.

cond-mat.stat-mech↗

arXiv2010

What Determines the Yield Stress in Amorphous Solids?

A crucially important material parameter for all amorphous solids is the yield stress, which is the value of the stress for which the material yields to plastic flow when it is strained quasi-statically at zero temperature. It is difficult in laboratory experiments to determine what parameters of the inter-particle potential effect the value of the yield stress. Here we use the versatility of numerical simulations to study the dependence of the yield stress on the parameters of the inter-particle potential. We find a very simple dependence on the fundamental scales which characterize the repulsive and attractive parts of the potential respectively, and offer a scaling theory that collapses the data for widely different potentials and in different space dimensions.

physics.comp-ph↗

arXiv2010

Density Scaling of Avalanche Statistics in Amorphous Solids

Stress vs. strain fluctuations in athermal amorphous solids are an example of `crackling noise' of the type studied extensively in the context of elastic membranes moving through random potentials. Contrary to the latter, we do not have a stochastic equation whose statistics agree with the measured ones. On the other hand we show in this Letter that the statistics of the former exhibit 'density scaling' when the interparticle potential can be well approximated by a power law. The distributions of sizes of dissipative events for a wide range of densities and system sizes follow a single scaling function. We find that both the system-size scaling of energy drops and the entire strain interval statistics are invariant to changes in density. We use this to determine accurately the exponents in the scaling laws, establishing that the present crackling noise belongs to a different universality class.

cond-mat.stat-mech↗