arXiv subjects

Eddy P. Rugeramigabo

Publications and source records attributed to Eddy P. Rugeramigabo.

8 recordsLinked to original sources

arXiv2026

Calibration of systematic distortions in quantum emitter localization microscopy for deterministic nanophotonic fabrication

Quantum photonic technologies greatly benefit from quantum light emitters with high brightness, indistinguishability, and reliable polarization characteristics. Achieving optimal performance relies on the accurate localization of emitters and their deterministic integration into tailored photonic structures with nanometer-scale accuracy. Although marker-based photoluminescence imaging techniques can achieve statistical fitting uncertainties below 10 nm, the ultimate integration yield is often limited by uncorrected systematic distortions in custom cryo-optical setups that compromise metrological accuracy. Here, we present an in situ calibration protocol that uses lithographically defined gold nanodisk arrays as references to calibrate optical distortions with a Zernike vector-field model. On held-out validation patterns beyond the calibration dataset, this correction reduces the residual systematic bias to 5.3 nm with a 2D scatter of 24.6 nm across the analyzed field of view. Furthermore, we demonstrate that applying this correction to the deterministic fabrication of circular mesa structures around semiconductor quantum dots reduces the variance in emission polarization by 49%, indicating improved registration accuracy. This calibration strategy offers a practical route to high-yield deterministic integration of quantum emitters into scalable quantum photonic circuits.

physics.optics↗

arXiv2025

Deterministic Integration of CsPbBr3 Quantum Dots with Plasmonic Ring Microcavities

Perovskite quantum dots hold great promise for quantum information processing as wavelength-tunable single photon sources operable over a broad temperature range. However, their deterministic integration into nanophotonic structures remains a major challenge, limited by their random spatial distribution and non-directional emission. In this work, we employ a two-step electron beam lithography process to deterministically place CsPbBr3 quantum dots within the mode volume of plasmonic ring microcavities. Simulations predict strong field enhancement within the cavity, boosting photon emission rates via the Purcell effect and improving the quantum efficiency of the emitters. Experimentally, coupling ensembles of CsPbBr3 quantum dots to the cavities results in a four-fold enhancement in photoluminescence intensity and a three-fold reduction in fluorescence lifetime at room temperature. Single-emitter coupling is further investigated at cryogenic temperatures, leading to a two-fold reduction in radiative lifetime. These results demonstrate a scalable approach for the integration of perovskite quantum dots into nanophotonic cavities and quantum photonic circuits.

physics.optics↗

arXiv2025

Real-Time Detection and Control of Correlated Charge Tunneling in a Quantum Dot

We experimentally demonstrate the real-time detection and control of correlated charge tunneling in a dynamically driven quantum dot. Specifically, we measure the joint distribution of waiting times between tunneling charges and show that the waiting times for holes may be strongly correlated due to the periodic drive and the Coulomb interactions on the dot, although the electron waiting times are not. Our measurements are in excellent agreement with a theoretical model that allows us to develop a detailed understanding of the correlated tunneling events. We also demonstrate that the degree of correlations can be controlled by the drive. Our experiment paves the way for systematic real-time investigations of correlated electron transport in low-dimensional nanostructures.

cond-mat.mes-hall↗

arXiv2024

Sub-meV Linewidths in Polarized Low-Temperature Photoluminescence of 2D PbS Nanoplatelets

Colloidal semiconductor nanocrystals are promising materials for classical and quantum light sources due to their versatile chemistry and efficient photoluminescence (PL) properties. While visible emitters are well-established, the pursuit of excellent (near-)infrared sources continues. One notable candidate in this regard are photoluminescent two-dimensional (2D) PbS nanoplatelets (NPLs) exhibiting excitonic emission at 720 nm (1.7 eV) directly tying to the typical emission range limit of CdSe NPLs. Here, we present the first comprehensive analysis of low-temperature PL from this material class. Ultrathin 2D PbS NPLs exhibit high crystallinity confirmed by scanning transmission electron microscopy, and revealing Moire patterns in overlapping structures. At 4K, we observe unique PL features in single PbS NPLs, including narrow zero-phonon lines with line widths down to 0.6 meV and a linear degree of polarization up to 90%. Time-resolved measurements identify trions as the dominant emission source with a 2.3 ns decay time. Sub-meV spectral diffusion and no immanent blinking over minutes is observed, as well as discrete spectral jumps without memory effects. These findings advance the understanding and underpin the potential of colloidal PbS NPLs for optical and quantum technologies.

physics.optics↗

arXiv2024

Unveiling the 3D Morphology of Epitaxial GaAs/AlGaAs Quantum Dots

Strain-free GaAs/AlGaAs semiconductor quantum dots (QDs) grown by droplet etching and nanohole infilling (DENI) are highly promising candidates for the on-demand generation of indistinguishable and entangled photon sources. The spectroscopic fingerprint and quantum optical properties of QDs are significantly influenced by their morphology. The effects of nanohole geometry and infilled material on the exciton binding energies and fine structure splitting are well understood. However, a comprehensive understanding of GaAs/AlGaAs QD morphology remains elusive. To address this, we employ high-resolution scanning transmission electron microscopy (STEM) and reverse engineering through selective chemical etching and atomic force microscopy (AFM). Cross-sectional STEM of uncapped QDs reveals an inverted conical nanohole with Al-rich sidewalls and defect-free interfaces. Subsequent selective chemical etching and AFM measurements further reveal asymmetries in element distribution. This study enhances the understanding of DENI QD morphology and provides a fundamental three-dimensional structural model for simulating and optimizing their optoelectronic properties.

quant-ph↗

arXiv2024

Circular photonic crystal grating design for charge-tunable quantum light sources in the telecom C-band

Efficient generation of entangled photon pairs at telecom wavelengths is a key ingredient for long-range quantum networks. While embedding semiconductor quantum dots into hybrid circular Bragg gratings has proven effective, it conflicts with $p$-$i$-$n$ diode heterostructures which offer superior coherence. We propose and analyze hybrid circular photonic crystal gratings, incorporating air holes to facilitate charge carrier transport without compromising optical properties. Through numerical simulations, a broad cavity mode with a Purcell factor of 23 enhancing both exciton and biexciton transitions, and exceptional collection efficiency of 92.4% into an objective with numerical aperture of 0.7 are achieved. Furthermore, our design demonstrates direct coupling efficiency over 90% into a single-mode fiber over the entire telecom C-band. The hybrid circular photonic crystal grating thereby emerges as a promising solution for the efficient generation of highly coherent, polarization-entangled photon pairs.

quant-ph↗

arXiv2023

Surface quantum dots with pure, coherent, and blinking-free single photon emission

The surface of semiconductor nanostructures has a major impact on their electronic and optical properties. Disorder and defects in the surface layer typically cause degradation of charge carrier transport and radiative recombination dynamics. However, surface vicinity is inevitable for many scalable nano-optical applications. Epitaxially grown quantum dots are the best candidate for high-performance single photon emission and show great potential for quantum technologies. Yet, these emitters only reveal their excellent properties if they are deeply embedded in a semiconductor host. Until today, quantum dots close to surfaces yield weak, broad, and unstable emissions. Here, we show the complete restoration of optical properties from quantum dots grown directly on a semiconductor surface. The vanishing luminescence from the as-grown sample turns into bright, ultra-stable, coherent and blinking-free single photon emission after sulphur passivation. Under quasi-resonant excitation, single photons are generated with 98.8% purity, 77% indistinguishability, linewidths down to 4 $μ$eV and 99.69% persistency across 11 orders of magnitude in time. The emission is stable even after two years and when being subjected to nanomanufacturing processes. Some long-standing stumbling blocks for surface-dominated quantum dots are thereby removed, unveiling new possibilities for hybrid nano-devices and applications in quantum communication or sensing.

cond-mat.mes-hall↗

arXiv2023

A solid-state source of single and entangled photons at diamond SiV$^-$-center transitions operating at 80K

Large-scale quantum networks require the implementation of long-lived quantum memories as stationary nodes interacting with qubits of light. Epitaxially grown quantum dots hold great potential for the on-demand generation of single and entangled photons with high purity and indistinguishability. Coupling these emitters to memories with long coherence times enables the development of hybrid nanophotonic devices incorporating the advantages of both systems. Here we report the first GaAs/AlGaAs quantum dots grown by droplet etching and nanohole infilling method, emitting single photons with a narrow wavelength distribution (736.2 $\pm$ 1.7 nm) close to the zero-phonon line of Silicon-vacancy centers. Polarization entangled photons are generated via the biexciton-exciton cascade with a fidelity of (0.73 $\pm$ 0.09). High single photon purity is maintained from 4 K (g$^($$^2$$^)$(0) = 0.07 $\pm$ 0.02) up to 80 K (g$^($$^2$$^)$(0) = 0.11 $\pm$ 0.01), therefore making this hybrid system technologically attractive for real-world quantum photonic applications.

quant-ph↗