arXiv subjects

Edgar Bonet

Publications and source records attributed to Edgar Bonet.

12 recordsLinked to original sources

arXiv2025

Gain compression in Josephson Traveling-Wave Parametric Amplifiers

Superconducting traveling-wave parametric amplifiers (TWPAs) are increasingly used in various applications, including quantum computing, quantum sensing, and dark matter detection. However, one important characteristic of these amplifiers, gain compression, has not received much attention. As a result, there is a lack of comprehensive experimental exploration of this phenomenon in the existing literature. In this study, we present an experimental investigation of gain compression in a Josephson traveling-wave parametric amplifier based on a four-wave mixing process. We have implemented a novel setup to monitor the complex transmission of both the pump and signal tones, which allows us to simultaneously track pump depletion and signal amplification as functions of signal power and frequency across the entire bandwidth of the device. Our findings indicate that, while pump depletion occurs during gain compression, it is not the only mechanism involved in the saturation of a TWPA. Power-induced phase-matching processes also take place within the device. This study provides valuable insights for optimizing TWPAs for applications that require high total input power, such as multiplexed qubit readout or broadband photon emission.

quant-ph↗

arXiv2024

A Traveling Wave Parametric Amplifier Isolator

Superconducting traveling-wave parametric amplifiers have emerged as highly promising devices for near-quantum-limited broadband amplification of microwave signals and are essential for high quantum-efficiency microwave readout lines. Built-in isolation, as well as gain, would address their primary limitation: lack of true directionality due to potential backward travel of electromagnetic radiation to their input port. Here, we demonstrate a Josephson-junction-based traveling-wave parametric amplifier isolator. It utilizes third-order nonlinearity for amplification and second-order nonlinearity for frequency upconversion of backward propagating modes to provide reverse isolation. These parametric processes, enhanced by a novel phase matching mechanism, exhibit gain of up to 20~dB and reverse isolation of up to 30~dB over a static 3~dB bandwidth greater than 500~MHz, while keeping near-quantum limited added noise. This demonstration of a broadband truly directional amplifier ultimately paves the way towards broadband quantum-limited microwave amplification lines without bulky magnetic isolators and with inhibited back-action.

quant-ph↗

arXiv2021

Thermalization of nuclear spins in lanthanide molecular magnets

Single molecule magnets distinguish themselves in the field of quantum magnetism through the ability to combine fundamental research with promising applications, the evolution of quantum spintronics in the last decade exemplifying the potential held by molecular based quantum devices. Notably, the read-out and manipulation of the embedded nuclear spin states was used in proof of principle studies of quantum computation at the single molecule level. In this paper we study the relaxation dynamics of the $^{159}$Tb nuclear spins in a diluted molecular crystal by using recently acquired understanding of the nonadiabatic dynamics of TbPc$_2$ molecules. We find that phonon modulated hyperfine interaction opens a direct relaxation channel between the nuclear spins and the phonon bath. We highlight the potential importance of the discovered mechanism for the theory of spin bath and the relaxation dynamics of the molecular spins at crossover temperatures.

cond-mat.mes-hall↗

arXiv2021

Kerr reversal in Josephson meta-material and traveling wave parametric amplification

Josephson meta-materials have recently emerged as very promising platform for superconducting quantum science and technologies. Their distinguishing potential resides in ability to engineer them at sub-wavelength scales, which allows complete control over wave dispersion and nonlinear interaction. In this article we report a versatile Josephson transmission line with strong third order nonlinearity which can be tuned from positive to negative values, and suppressed second order non linearity. As an initial implementation of this multipurpose meta-material, we operate it to demonstrate reversed Kerr phase-matching mechanism in traveling wave parametric amplification. Compared to previous state of the art phase matching approaches, this reversed Kerr phase matching avoids the presence of gaps in transmission, can reduce gain ripples, and allows in situ tunability of the amplification band over an unprecedented wide range. Besides such notable advancements in the amplification performance with direct applications to superconducting quantum computing and generation of broadband squeezing, the in-situ tunability with sign reversal of the nonlinearity in traveling wave structures, with no counterpart in optics to the best of our knowledge, opens exciting experimental possibilities in the general framework of microwave quantum optics, single-photon detection and quantum limited amplification.

quant-ph↗

arXiv2020

The role of the quadrupolar interaction in the tunneling dynamics of lanthanide molecular magnets

Quantum tunneling dominates the low temperature magnetization dynamics in molecular magnets and presents features that are strongly system dependent. The current discussion is focused on the terbium(III) bis(phtalocyanine) ([TbPc$_2$]$^{-1}$) complex, that should serve as a prototypical case for lanthanide molecular magnets. We analyze numerically the effect of non-axial interactions on the magnitude of the intrinsic tunnel splitting and show that usual suspects like the transverse ligand field and Zeeman interaction fail to explain the experimentally observed dynamics. We then propose through the nuclear quadrupolar interaction a viable mechanism that mixes, otherwise \textit{almost} degenerate hyperfine states.

cond-mat.mes-hall↗

arXiv2020

Decoherence measurements in crystals of molecular magnets

Decoherence processes in crystals of molecular magnets are prototypical for interacting electronic spin systems. We analyze the Landau-Zener dynamics of the archetypical TbPc$_2$ complex diluted in a diamagnetic monocrystal. The dependence of the tunneling probability on the field sweep rate is evaluated in the framework of the recently proposed master equation in which the decoherence processes are described through a phenomenological Lindblad operator. Thus, we showcase low temperature magnetic measurements that complement resonant techniques in determining small tunnel splittings and dephasing times.

cond-mat.mes-hall↗

arXiv2018

Generalized Ramsey Interferometry Explored with a Single Nuclear Spin Qudit

Qudits, with their state space of dimension d > 2, open fascinating experimental prospects. The quantum properties of their states provide new potentialities for quantum information, quantum contextuality, expressions of geometric phases, facets of quantum entanglement and many other foundational aspects of the quantum world, which are unapproachable with qubits. We here experimentally investigate the quantum dynamics of a qudit (d = 4) that consists of a single 3/2 nuclear spin embedded in a molecular magnet transistor geometry, coherently driven by a microwave electric field. We propose and implement three protocols based on a generalization of the Ramsey interferometry to a multilevel system. First, the standard Ramsey interference is used to measure the accumulation of geometric phases. Then, two distinct transitions of the nuclear spin are addressed to measure the phase of an iSWAP quantum gate. Finally, through a succession of two Hadamard gates, the coherence time of a 3-state superposition is measured.

cond-mat.mes-hall↗

arXiv2011

First order $0/π$ quantum phase transition in the Kondo regime of a superconducting carbon nanotube quantum dot

We study a carbon nanotube quantum dot embedded into a SQUID loop in order to investigate the competition of strong electron correlations with proximity effect. Depending whether local pairing or local magnetism prevails, a superconducting quantum dot will respectively exhibit positive or negative supercurrent, referred to as a 0 or $π$ Josephson junction. In the regime of strong Coulomb blockade, the 0 to $π$ transition is typically controlled by a change in the discrete charge state of the dot, from even to odd. In contrast, at larger tunneling amplitude the Kondo effect develops for an odd charge (magnetic) dot in the normal state, and quenches magnetism. In this situation, we find that a first order 0 to $π$ quantum phase transition can be triggered at fixed valence when superconductivity is brought in, due to the competition of the superconducting gap and the Kondo temperature. The SQUID geometry together with the tunability of our device allows the exploration of the associated phase diagram predicted by recent theories. We also report on the observation of anharmonic behavior of the current-phase relation in the transition regime, that we associate with the two different accessible superconducting states. Our results ultimately reveal the spin singlet nature of the Kondo ground state, which is the key process in allowing the stability of the 0-phase far from the mixed valence regime.

cond-mat.mes-hall↗

arXiv2009

High domain wall velocity at zero magnetic field induced by low current densities in spin-valve nanostripes

Current-induced magnetic domain wall motion at zero magnetic field is observed in the permalloy layer of a spin-valve-based nanostripe using photoemission electron microscopy. The domain wall movement is hampered by pinning sites, but in between them high domain wall velocities (exceeding 150 m/s) are obtained for current densities well below $10^{12} \unit{A/m^2}$, suggesting that these trilayer systems are promising for applications in domain wall devices in case of well controlled pinning positions. Vertical spin currents in these structures provide a potential explanation for the increase in domain wall velocity at low current densities.

cond-mat.mtrl-sci↗

arXiv2006

Magnetic anisotropy of $Co_x Pt_{1-x}$ clusters embedded in matrix: Influences of the cluster chemical composition and the matrix nature

We report on the magnetic properties of Co$\_x$Pt$\_{1-x}$ clusters embedded in various matrices. Using a careful analysis of magnetization curves and ZFC susceptibility measurements, we determine the clusters magnetic anisotropy energy (MAE) and separate the surface and volume contributions. By comparing different chemical compositions, we show that a small amount of Pt (15%) induces an important increase in the volume anisotropy with respect to pure Co clusters, even in chemically disordered fcc clusters. Comparing the measurements of clusters embedded in Nb and MgO matrices, we show that the oxide matrix induces an important increase of the surface MAE attributed to the formation of an antiferromagnetic CoO shell around the clusters.

cond-mat.mtrl-sci↗

arXiv2001

Solving rate equations for electron tunneling via discrete quantum states

We consider the form of the current-voltage curves generated when tunneling spectroscopy is used to measure the energies of individual electronic energy levels in nanometer-scale systems. We point out that the voltage positions of the tunneling resonances can undergo temperature-dependent shifts, leading to errors in spectroscopic measurements that are proportional to temperature. We do this by solving the set of rate equations that can be used to describe electron tunneling via discrete quantum states, for a number of cases important for comparison to experiments, including (1) when just one spin-degenerate level is accessible for transport, (2) when 2 spin-degenerate levels are accessible, with no variation in electron-electron interactions between eigenstates, and (3) when 2 spin-degenerate levels are accessible, but with variations in electron-electron interactions. We also comment on the general case with an arbitrary number of accessible levels. In each case we analyze the voltage-positions, amplitudes, and widths of the current steps due to the quantum states.

cond-mat.mes-hall↗

arXiv2001

Equilibrium and non-equilibrium electron tunneling via discrete quantum states

Tunneling is measured via the quantum levels of a metal nanoparticle. We analyze quantitatively the resonance energies, widths, and amplitudes, both in the regime where only one state is accessible for tunneling and in the non-equilibrium regime when additional states are made accessible one-by-one. For tunneling through one state, our results agree with expectations for sequential tunneling, but in the non-equilibrium regime the resonances are broadened and shifted in ways that require taking into account electron interactions and relaxation.

cond-mat.mes-hall↗