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Edwin Barnes

Publications and source records attributed to Edwin Barnes.

At least 109 records · Page 6Linked to original sources

A solvable quantum model of dynamic nuclear polarization in quantum dots

We present a quantum mechanical theory of optically induced dynamic nuclear polarization applicable to quantum dots and other interacting spin systems. The exact steady state of the optically driven coupled electron-nuclear system is calculated under the assumption of uniform hyperfine coupling strengths (box model) for an arbitrary number of nuclear spins. This steady state is given by a tractable expression that allows for an intuitive interpretation in terms of spin-flip rates. Based on this result, we investigate the nuclear spin behaviour for different experimental parameter regimes and find that our model reproduces the flat-top and triangular absorption line shapes seen in various experiments (line dragging) under the assumption of fast electron spin dephasing due to phonons and co-tunneling. The mechanism responsible for line dragging has been a matter of controversy so far; in contrast with previous works, we show that the effect can be explained solely in terms of the contact hyperfine interaction, without the need to introduce non-collinear terms or other types of electron-nuclear interactions. Furthermore we predict a novel nuclear spin polarization effect: under particular, experimentally realistic conditions, the nuclear spin system tends to become sharply polarized in such a way as to cancel the effect of the external magnetic field. This effect can therefore suppress electron spin dephasing due to inhomogeneous broadening, which could have important repercussions for quantum technological applications.

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Stabilization and manipulation of multispin states in quantum-dot time crystals with Heisenberg interactions

A discrete time crystal is a recently discovered non-equilibrium phase of matter that has been shown to exist in disordered, periodically driven Ising spin chains. In this phase, if the system is initially prepared in one of a certain class of pure multispin product states, it periodically returns to this state over very long time scales despite the presence of interactions, disorder, and pulse imperfections. Here, we show that this phase occurs in GaAs quantum dot spin arrays containing as few as three quantum dots, each confining one electron spin, for naturally occurring levels of nuclear spin noise and charge noise. Although the physical interaction in these arrays is a nearest-neighbor Heisenberg exchange interaction, we show that this can be effectively converted into an Ising interaction by applying additional pulses during each drive period. We show that by changing the rotation axis of these pulses, we can select the direction of the Ising interaction and, consequently, the quantization axis of the stabilized multispin states. Moreover, we demonstrate that it is possible to perform coherent rotations of the stabilized states while remaining in the time crystal phase. These findings open up the intriguing possibility of using time crystal phases to extend the lifetime of quantum states for information applications.

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Dynamic Nuclear Polarization from Topological Insulator Helical Edge States

Topological insulators are promising for spintronics and related technologies due to their spin-momentum-locked edge states, which are protected by time-reversal symmetry. In addition to the unique fundamental physics that arises in these systems, the potential technological applications of these protected states has also been driving TI research over the past decade. However, most known topological insulator materials naturally contain spinful nuclei, and their hyperfine coupling to helical edge states intrinsically breaks time-reversal symmetry, removing the topological protection and enabling the buildup of dynamic nuclear spin polarization through hyperfine-assisted backscattering. Here, we calculate scattering probabilities and nuclear polarization for edge channels containing up to $34$ nuclear spins using a numerically exact analysis that exploits the symmetries of the problem to drastically reduce the computational complexity. We then show the emergence of universal scaling properties that allow us to extrapolate our findings to vastly larger and experimentally relevant system sizes. We find that significant nuclear polarization can result from relatively weak helical edge currents, suggesting that it may be an important factor affecting spin transport in topological insulator devices.

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Photonic graph state generation from quantum dots and color centers for quantum communications

Highly entangled graph states of photons have applications in universal quantum computing and in quantum communications. In the latter context, they have been proposed as the key ingredient in the establishment of long-distance entanglement across quantum repeater networks. Recently, a general deterministic approach to generate repeater graph states from quantum emitters was given. However, a detailed protocol for the generation of such states from realistic systems is still needed in order to guide experiments. Here, we provide such explicit protocols for the generation of repeater graph states from two types of quantum emitters: NV centers in diamond and self-assembled quantum dots. A crucial element of our designs is an efficient controlled-Z gate between the emitter and a nuclear spin, used as an ancilla qubit. Additionally, a fast protocol for using pairs of exchange-coupled quantum dots to produce repeater graph states is described. Our focus is on near-term experiments feasible with existing experimental capabilities.

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Negative exchange interactions in coupled few-electron quantum dots

It has been experimentally shown that negative exchange interactions can arise in a linear three-dot system when a two-electron double quantum dot is exchange coupled to a larger quantum dot containing on the order of one hundred electrons. The origin of this negative exchange can be traced to the larger quantum dot exhibiting a spin triplet-like rather than singlet-like ground state. Here, we show using a microscopic model based on the configuration interaction (CI) method that both triplet-like and singlet-like ground states are realized depending on the number of electrons. In the case of only four electrons, a full CI calculation reveals that triplet-like ground states occur for sufficiently large dots. These results hold for symmetric and asymmetric quantum dots in both Si and GaAs, showing that negative exchange interactions are robust in few-electron double quantum dots and do not require large numbers of electrons.

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The fastest pulses that implement dynamically corrected gates

Dynamically correcting for unwanted interactions between a quantum system and its environment is vital to achieving the high-fidelity quantum control necessary for a broad range of quantum information technologies. In recent work, we uncovered the complete solution space of all possible driving fields that suppress transverse quasistatic noise errors while performing single-qubit operations. This solution space lives within a simple geometrical framework that makes it possible to obtain globally optimal pulses subject to a set of experimental constraints by solving certain geometrical optimization problems. In this work, we solve such a geometrical optimization problem to find the fastest possible pulses that implement single-qubit gates while cancelling transverse quasistatic noise to second order. Because the time-optimized pulses are not smooth, we provide a method based on our geometrical approach to obtain experimentally feasible smooth pulses that approximate the time-optimal ones with minimal loss in gate speed. We show that in the presence of realistic constraints on pulse rise times, our smooth pulses significantly outperform sequences based on ideal pulse shapes, highlighting the benefits of building experimental waveform constraints directly into dynamically corrected gate designs.

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General solution to inhomogeneous dephasing and smooth pulse dynamical decoupling

In order to achieve the high-fidelity quantum control needed for a broad range of quantum information technologies, reducing the effects of noise and system inhomogeneities is an essential task. It is well known that a system can be decoupled from noise or made insensitive to inhomogeneous dephasing dynamically by using carefully designed pulse sequences based on square or delta-function waveforms such as Hahn spin echo or CPMG. However, such ideal pulses are often challenging to implement experimentally with high fidelity. Here, we uncover a new geometrical framework for visualizing all possible driving fields, which enables one to generate an unlimited number of smooth, experimentally feasible pulses that perform dynamical decoupling or dynamically corrected gates to arbitrarily high order. We demonstrate that this scheme can significantly enhance the fidelity of single-qubit operations in the presence of noise and when realistic limitations on pulse rise times and amplitudes are taken into account.

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Topological insulator ring with magnetic impurities

Topological insulators exhibit gapless edge or surface states that are topologically protected by time-reversal symmetry. However, several promising candidates for topologically insulating materials (such as Bi$_2$Se$_3$ and HgTe) contain spinful nuclei or other types of magnetic impurities that break time-reversal symmetry. We investigate the consequences of such impurities coupled to electronic edge states in a topological insulator quantum ring threaded by a magnetic flux. We use spin conservation and additional symmetry arguments to derive a universal formula for the spectrum of propagating edge modes in terms of the amplitude of transmission through the impurity. Our results apply for impurities of arbitrary spin. We show that there exists an energy regime in which the spectrum becomes nearly independent of the flux and significant spectral gaps form. We further analyze the electron-impurity entanglement entropy, finding that maximal entanglement occurs near the gaps in the spectrum. Our predictions can be investigated with quantum ring transport interference experiments or through spin-resolved STM measurements, providing a new approach to understand the role of impurities in topological insulator edge transport.

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Deterministic generation of all-photonic quantum repeaters from solid-state emitters

Quantum repeaters are nodes in a quantum communication network that allow reliable transmission of entanglement over large distances. It was recently shown that highly entangled photons in so-called graph states can be used for all-photonic quantum repeaters, which require substantially fewer resources compared to atomic-memory based repeaters. However, standard approaches to building multi-photon entangled states through pairwise probabilistic entanglement generation severely limit the size of the state that can be created. Here, we present a protocol for the deterministic generation of large photonic repeater states using quantum emitters such as semiconductor quantum dots and defect centers in solids. We show that arbitrarily large repeater states can be generated using only two coupled emitters, reducing the necessary number of photon sources by six orders of magnitude. Our protocol includes a built-in redundancy which makes it resilient to photon loss.

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Fast pulse sequences for dynamically corrected gates in single-triplet qubits

We present a set of experimentally feasible pulse sequences that implement any single-qubit gate on a singlet-triplet spin qubit and demonstrate that these new sequences are up to three times faster than existing sequences in the literature. We show that these sequences can be extended to incorporate built-in dynamical error correction, yielding gates that are robust to both charge and magnetic field noise and up to twice as fast as previous dynamically corrected gate schemes. We present a thorough comparison of the performance of our new sequences with that of several existing ones using randomized benchmarking, considering both quasistatic and $1/f^α$ noise models. We provide our results both as a function of evolution time and as a function of the number of gates, which respectively yield both an effective coherence time and an estimate of the number of gates that can be performed within this coherence time. We determine which set of pulse sequences gives the best results for a wide range of noise strengths and power spectra. Overall, we find that the traditional, slower sequences perform best when there is no field noise or when the noise contains significant high-frequency components; otherwise, our new, fast sequences exhibit the best performance.

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Interplay of valley polarization and dynamic nuclear polarization in 2D transition metal dichalcogenides

The interplay of Ising spin-orbit coupling and non-trivial band topology in transition metal dichalcogenides (TMDs) produces anomalous transport and optical properties that are very different from a regular 2D electron gas. The spin-momentum locking of optically excited carriers near a valley point can give rise to an anomalous spin-valley Hall current under the application of an in-plane electric field. TMDs also exhibit strong electron-nuclear hyperfine interactions, but their effect on spin-valley-locked currents remains unknown. Here, we show that hyperfine interactions can create a feedback mechanism in which spin-valley currents generate significant dynamical nuclear polarization which in turn Zeeman shifts excitonic transitions out of resonance with an optical driving field, saturating the production of spin-valley polarization. We propose an experimental signature of dynamic nuclear polarization which can be detected via measurements of the anomalous Hall current. Our results help to elucidate the interplay of valley polarization and nuclear spin dynamics in TMDs.

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Robustness of error-suppressing entangling gates in cavity-coupled transmon qubits

Superconducting transmon qubits comprise one of the most promising platforms for quantum information processing due to their long coherence times and to their scalability into larger qubit networks. However, their weakly anharmonic spectrum leads to spectral crowding in multiqubit systems, making it challenging to implement fast, high-fidelity gates while avoiding leakage errors. To address this challenge, we use a protocol known as SWIPHT [Phys. Rev. B 91, 161405(R) (2015)], which yields smooth, simple microwave pulses designed to suppress leakage without sacrificing gate speed through spectral selectivity. Here, we determine the parameter regimes in which SWIPHT is effective and demonstrate that in these regimes it systematically produces two-qubit gate fidelities for cavity-coupled transmons in the range 99.6%-99.9% with gate times as fast as 23 ns. Our results are obtained from full numerical simulations that include current experimental levels of relaxation and dephasing. These high fidelities persist over a wide range of system parameters that encompass many current experimental setups and are insensitive to small parameter variations and pulse imperfections.

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Randomized benchmarking of barrier versus tilt control of a singlet-triplet qubit

Decoherence due to charge noise is one of the central challenges in using spin qubits in semiconductor quantum dots as a platform for quantum information processing. Recently, it has been experimentally demonstrated in both Si and GaAs singlet-triplet qubits that the effects of charge noise can be suppressed if qubit operations are implemented using symmetric barrier control instead of the standard tilt control. Here, we investigate the key issue of whether the benefits of barrier control persist over the entire set of single-qubit gates by performing randomized benchmarking simulations. We find the surprising result that the improvement afforded by barrier control depends sensitively on the amount of spin noise: for the minimal nuclear spin noise levels present in Si, the coherence time improves by more than two orders of magnitude whereas in GaAs, by contrast the coherence time is essentially the same for barrier and tilt control. However, we establish that barrier control becomes beneficial if qubit operations are performed using a new family of composite pulses that reduce gate times by up to 90%. With these optimized pulses, barrier control is the best way to achieve high-fidelity quantum gates in singlet-triplet qubits.

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Qubit gates using hyperbolic secant pulses

It has been known since the early days of quantum mechanics that hyperbolic secant pulses possess the unique property that they can perform cyclic evolution on two-level quantum systems independently of the pulse detuning. More recently, it was realized that they induce detuning- controlled phases without changing state populations. Here, we experimentally demonstrate the properties of hyperbolic secant pulses on superconducting transmon qubits and contrast them with the more commonly used Gaussian and square waves. We further show that these properties can be exploited to implement phase gates, nominally without exiting the computational subspace. This enables us to demonstrate the first microwave-driven Z-gates with a single control parameter, the detuning.

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Environmental noise effects on entanglement fidelity of exchange-coupled semiconductor spin qubits

We investigate the effect of magnetic field and charge noise on the generation of entanglement between two Heisenberg exchange-coupled electron spins in a double quantum dot. We focus on exchange-driven evolution that would ideally take an initial unentangled tensor product state to a maximally-entangled state in the absence of noise. The presence of noise obviously adversely affects the attainment of maximal entanglement, which we study quantitatively and exactly. To quantify the effects of noise, we calculate two-qubit coherence times and entanglement fidelity, both of which can be extracted from simulations or measurements of the return probability as a function of interaction time, i.e., the time period during which the exchange coupling remains effective between the two spins. We perform these calculations for a broad range of noise strengths that includes the regime of recent experiments. We find that the two types of noise reduce the amount of entanglement in qualitatively distinct ways and that, although charge noise generally leads to faster decoherence, the relative importance of the two types of noise in entanglement creation depends sensitively on the strength of the exchange coupling. Our results can be used to determine the level of noise suppression needed to reach quantum error correction thresholds. We provide quantitative guidance for the requisite noise constraints necessary to eventually reach the $>99\%$ fidelity consistent with the quantum error correction threshold.

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Fast microwave-driven three-qubit gates for cavity-coupled superconducting qubits

Although single and two-qubit gates are sufficient for universal quantum computation, single-shot three-qubit gates greatly simplify quantum error correction schemes and algorithms. We design fast, high-fidelity three-qubit entangling gates based on microwave pulses for transmon qubits coupled through a superconducting resonator. We show that when interqubit frequency differences are comparable to single-qubit anharmonicities, errors occur primarily through a single unwanted transition. This feature enables the design of fast three-qubit gates based on simple analytical pulse shapes that are engineered to minimize such errors. We show that a three-qubit ccz gate can be performed in 260 ns with fidelities exceeding $99.38\%$, or $99.99\%$ with numerical optimization.

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Electromagnetic signatures of the chiral anomaly in Weyl semimetals

Weyl semimetals are predicted to realize the three-dimensional axial anomaly first discussed in particle physics. The anomaly leads to unusual transport phenomena such as the chiral magnetic effect in which an applied magnetic field induces a current parallel to the field. Here we investigate diagnostics of the axial anomaly based on the fundamental equations of axion electrodynamics. We find that materials with Weyl nodes of opposite chirality and finite energy separation immersed in a uniform magnetic field exhibit an anomaly-induced oscillatory magnetic field with a period set by the chemical potential difference of the nodes. In the case where a chemical potential imbalance is created by applying parallel electric and magnetic fields, we find a suppression of the magnetic field component parallel to the electric field inside the material for rectangular samples, suggesting that the chiral magnetic current opposes this imbalance. For cylindrical geometries, we instead find an enhancement of this magnetic field component along with an anomaly-induced azimuthal component. We propose experiments to detect such magnetic signatures of the axial anomaly.

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Engineering and probing topological properties of Dirac semimetal films by asymmetric charge transfer

Dirac semimetals (DSMs) have topologically robust three-dimensional Dirac (doubled Weyl) nodes with Fermi-arc states. In heterostructures involving DSMs, charge transfer occurs at the interfaces, which can be used to probe and control their bulk and surface topological properties through surface-bulk connectivity. Here we demonstrate that despite a band gap in DSM films, asymmetric charge transfer at the surface enables one to accurately identify locations of the Dirac-node projections from gapless band crossings and to examine and engineer properties of the topological Fermi-arc surface states connecting the projections, by simulating adatom-adsorbed DSM films using a first-principles method with an effective model. The positions of the Dirac-node projections are insensitive to charge transfer amount or slab thickness except for extremely thin films. By varying the amount of charge transfer, unique spin textures near the projections and a separation between the Fermi-arc states change, which can be observed by gating without adatoms.

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