arXiv subjects

Edwin Herrera

Publications and source records attributed to Edwin Herrera.

At least 19 recordsLinked to original sources

arXiv2026

Scanning Tunneling Microscopy in high vectorial magnetic fields

The Scanning Tunneling Microscope (STM) is a powerful instrument to study electronic density of states at surfaces down to atomic scale. Many interesting samples require studying variations as a function of the magnetic field, which is most often applied perpendicular to the surface. Conventional STM designs make it challenging to perform measurements when the magnetic field must be applied in other directions. Here we present a new STM setup installed on a rotatable platform. We have designed and built a new STM, which is small enough to allow for full rotation on a space with a diameter of 37 mm, well below the available space within many magnets. We show that the new rotatable STM setup preserves the performance of state-of-the-art STMs in terms of noise and accuracy. Our new approach significantly enhances control over the direction of the applied magnetic field and opens exciting new possibilities to study quantum materials.

cond-mat.supr-con↗

arXiv2026

Direct observation of vortex liquid droplets in the iron pnictide superconductor CaKAs$_4$Fe$_4$ at $0.5T$_c$

Type-II superconductors under magnetic fields are in a quantum coherent non-dissipative state as long as vortices remain pinned. Dissipation appears when vortices depin, eventually driven by thermal fluctuations. This can be associated to a melting transition between a vortex solid and a vortex liquid. This transition is almost always observed very close to T$_c$ when probed by macroscopic experiments. However, it remains unclear how the vortex solid responds to thermal fluctuations at the scale of individual vortices far from the melting transition. Here we use scanning tunneling microscopy (STM) to visualize vortices in CaKAs$_4$Fe$_4$ (T$_c \approx$ 35 K). We find vortex liquid droplets-localized regions in space where vortices strongly fluctuate due to thermal exctiation-at temperatures as low as 0.5\,T$_c$. Our results show that the onset of dissipation at the local scale occurs at temperatures considerably below T$_c$ in type-II superconductors.

cond-mat.supr-con↗

arXiv2026

Superconducting density of states and vortex lattice of LaRu$_2$P$_2$ observed by Scanning Tunneling Spectroscopy

We provide the superconducting density of states of the iron based superconductor LaRu2P2 (Tc= 4.1 K), measured using millikelvin Scanning Tunneling Microscopy. From the tunneling conductance, we extract a density of states which shows the opening of a s-wave single superconducting gap. The temperature dependence of the gap also follows BCS theory. Under magnetic fields, vortices present Caroli de Gennes Matricon states, although these are strongly broadened by defect scattering. From the vortex core size we obtain a superconducting coherence length of {\xi} = 50 nm, compatible with the value extracted from macroscopic Hc2 measurements. We discuss the comparison between s-wave LaRu2P2 and pnictide unconventional multiple gap and strongly correlated Fe based superconductors.

cond-mat.supr-con↗

arXiv2025

Robust two-dimensional surface superconductivity and vortex lattice in the Weyl semimetal $\gamma$-PtBi$_2$

The layered compound $\gamma$-PtBi$_2$ is a topological semimetal with Fermi arcs at the surface joining bulk Weyl points. Recent work has found signatures of surface superconductivity consisting of gap openings compatible with a critical temperature orders of magnitude larger than the bulk value. However, no superconducting vortices have been identified, raising questions about the robustness of the phase coherence. Here we use very low temperature Scanning Tunneling Microscopy (STM) and find robust superconductivity with T$_C=$2.9 K and H$_{C2}\approx$1.8 T linked to the Fermi arcs. We observe quantized superconducting vortices and the Josephson effect, demonstrating two-dimensional macroscopic quantum phase coherence.

cond-mat.supr-con↗

arXiv2025

Gapless superconductivity from extremely dilute magnetic disorder in 2H-NbSe2-xSx

Most superconducting materials exhibit a vanishing density of states at the Fermi level and Anderson's theorem posits that the superconducting gap is robust against nonmagnetic disorder. Although dilute magnetic impurities lead to localized in-gap states, these states typically have no bearing on the material's bulk superconducting properties. However, numerous experiments reveal a finite density of states at the Fermi level in systems with an apparently negligible number of magnetic impurities. Here, using scanning tunneling microscopy and self-consistent Bogoliubov-de Gennes calculations, we find that gapless superconductivity emerges in 2H-NbSe2-xSx at remarkably low magnetic impurity concentrations. Furthermore, our density functional theory calculations and in-gap quasiparticle interference measurements demonstrate that the Se-S substitution significantly modifies the band structure. This modification favours nesting and dictates the in-gap scattering for x>0, in stark contrast to the dominant charge density wave interactions in pure 2H-NbSe2. Our findings reveal an unusual superconducting response to disorder and highlight the importance of incorporating material-specific band structures in the understanding of a superconductor's response to even very low concentrations of magnetic impurities.

cond-mat.supr-con↗

arXiv2025

Superconducting density of states of PtPb4

PtPb$_4$ is a type II superconductor with a bulk critical temperature $T_{c}\approx 3 $K and an upper critical field of $H_{c2}=0.36 $T. PtPb$_4$ is related to non-superconducting PtSn$_4$, which presents nodal arc states at the surface. Here we measure the superconducting density of states of PtPb$_4$ using millikelvin Scanning Tunneling Microscopy (STM). We observe a fully opened superconducting gap of $\Delta=0.48$\ meV similar to expectations from Bardeen Cooper and Schrieffer (BCS) theory ($\Delta_0=1.76k_BT_{c}=0.49 $meV). Measurements under magnetic fields applied perpendicular to the surface show a spatially inhomogeneous gap structure, presenting superconducting signatures at fields as high as 1.5 T, significantly above $H_{c2}=0.36 $T. On some locations we find that the superconducting density of states does not vanish above $T_{c}$. We can find signatures of a superconducting gap up to 5K. We discuss possible reasons for the observation of superconducting properties above $T_{c}$ and $H_{c2}$, emphasizing the role played by structural defects.

cond-mat.supr-con↗

arXiv2025

Surface charge density wave in UTe2

The spatially uniform electronic density characteristic of a metal can become unstable at low temperatures, leading to the formation of charge density waves (CDWs). These CDWs, observed in dichalcogenides, cuprates and pnictides, arise from the interplay between the crystal lattice and the electronic structure, which can facilitate charge ordering. However, CDWs are rarely observed in the presence of Kondo screening and heavy fermion quasiparticles. The heavy fermion topological superconductor candidate UTe$_2$ presents a notable exception, exhibiting a CDW whose origin remains elusive. Here we report high resolution scanning tunneling microscopy (STM) experiments that reveal the primitive wavevectors of the CDW in UTe$_2$. This allows us to identify hot spots in the electronic band structure that are connected to the CDW. Although the corresponding wavevectors have apparently no specific influence on some bulk properties, for example on antiferromagnetic fluctuations, we find that they lead to a spatial modulation of the heavy fermion hybridization pattern. We propose that surface induced modifications in the U 5f electron valence enable a novel form of purely electron-driven charge ordering.

cond-mat.str-el↗

arXiv2025

Revealing inter-band electron pairing in a superconductor with spin-orbit coupling

Most superconducting mechanisms pair electrons within the same band, forming spin singlets. However, the discovery of multi-band superconductivity has opened new scenarios for pairing, particularly in systems with strong spin-orbit coupling. Here, we reveal inter-band pairing in the superconductor \bipd\ by mapping the amplitude of sub-gap Yu-Shiba-Rusinov (YSR) states around Vanadium adatoms deposited on its surface. The surface of \bipd\ is characterized by spin-helical-like bands near the Fermi level. Scanning tunneling spectroscopy reveals anisotropic YSR amplitude oscillations around the impurity, driven by spin-conserving Bogoliubov quasiparticle interference (BQPI). Analysis of the BQPI patterns at the YSR energy exposes inter-band pairing in this material. Interestingly, only a small subset of all possible inter-band scattering processes observed in the normal state contribute to the BQPI patterns. Combining experimental data and theory, we demonstrate that the observed band selectivity results from the hybridization of the band coupled with the impurity with other bands. Our findings reveal unconventional pairing mechanisms in \bipd\ and highlight the crucial role of spin-orbit interactions in their formation.

cond-mat.mes-hall↗

arXiv2024

Field-induced antiferromagnetic correlations in a nanopatterned van der Waals ferromagnet: a potential artificial spin ice

Nano-patterned magnetic materials have opened new venues on the investigation of strongly correlated phenomena including artificial spin-ice systems, geometric frustration, magnetic monopoles, for technologically important applications such as reconfigurable ferromagnetism. With the advent of atomically thin two-dimensional (2D) van der Waals (vdW) magnets a pertinent question is whether such compounds could make their way into this realm where interactions can be tailored so that unconventional states of matter could be assessed. Here we show that square islands of CrGeTe3 vdW ferromagnets distributed in a grid manifest antiferromagnetic correlations, essential to enable frustration resulting in an artificial spin-ice. By using a combination of SQUID-on-tip microscopy, focused ion beam lithography, and atomistic spin dynamic simulations, we show that pristine, isolated CGT flakes as small as 150*150*60 nm3 have tunable dipole-dipole interactions, which can be precisely controlled by their lateral spacing. There is a crossover between non-interacting islands and significant inter-island anticorrelation depending how they are spatially distributed allowing the creation of complex magnetic patterns not observable at the isolated flakes. Our findings suggest that the cross-talk between the nano-patterned magnets can be explored in the generation of even more complex spin configurations where exotic interactions may be manipulated in an unprecedent way.

cond-mat.mtrl-sci↗

arXiv2024

Anomalous size dependence of the coercivity of nanopatterned CrGeTe3

The coercivity of single-domain magnetic nanoparticles typically decreases with the nanoparticle size and reaches zero when thermal fluctuations overcome the magnetic anisotropy. Here, we used SQUID-on-tip microscopy to investigate the coercivity of square-shaped CrGeTe3 nanoislands with a wide range of sizes and width-to-thickness aspect ratios. The results reveal an anomalous size-dependent coercivity, with smaller islands exhibiting higher coercivity. The nonconventional scaling of the coercivity in CrGeTe3 nanoislands was found to be inversely proportional to the island width and thickness (1 over wd). This scaling implies that the nanoisland magnetic anisotropy is proportional to the perimeter rather than the volume, suggesting a magnetic edge state. In addition, we observe that 1600 nm wide islands display multi-domain structures with zero net remnant field, corresponding to the magnetic properties of pristine CrGeTe3 flakes. Our findings highlight the significant influence of edge states on the magnetic properties of CrGeTe3 and deepen our understanding of low-dimensional magnetic systems.

cond-mat.mtrl-sci↗

arXiv2024

Diluted Yu-Shiba-Rusinov arrays on the $\beta$-Bi$_2$Pd anisotropic superconductor

Magnetic adatoms on s-wave superconductors induce bound states inside the superconducting gap, called Yu-Shiba-Rusinov states (YSR). The anisotropy of the Fermi surface determines the spatial extension of bound states in a quasi-two-dimensional superconductor. This is especially important in the diluted impurity limit since the orbital overlap determines the coupling of YSR states of neighboring atoms and the formation of the collective YSR system. Here, we build diluted arrays of Mn atoms with different dimensionalities on the surface of $\beta$-Bi$_2$Pd, and we measure the evolution of their YSR spectra with the structure. We detect the coupling as a split of YSR peaks in subgap spectra and find that the split size increases with the number of atoms. The orientation of the structures along different directions of the \bipd substrate modulates the split and particle-hole asymmetry of the YSR states due to the anisotropic character of the Fermi surface, captured by the Green function model. With the aid of the model, we found multiple YSR excitations in an extended 2D array of 25 Mn atoms, and we identified that their spatial distribution reflects a chiral LDOS.

cond-mat.supr-con↗

arXiv2024

Conductance of atomic size contacts of Ag and Au at high magnetic fields

Electronic conduction at the atomic scale can be described by Landauer's formalism. In single atom point contacts of noble metals like Au and Ag, there is just one channel open between both electrodes and the conductance is very close to the quantum of conductance $G \approx G_0=\frac{2e^2}{h}$, with the factor of two coming from spin degeneracy. The magnetoconductivity of atomic size contacts has been studied for numerous systems, unveiling local Kondo screening, magnetic order and spin-polarized currents. However, these have been mostly performed in elements with multiple open conduction channels where $G$ differs from $G_0$. The realization of a magnetically active conductor with a single open channel remains difficult to achieve. Here we present measurements of the electronic conductance of single channel Au and Ag atomic-size contacts in magnetic fields up to 20 Tesla. We observe a decrease in $G$ which goes up to about 15% in many Au contacts at 20 T. We perform calculations and find that pure Ag and Au do not present a strong field dependence of $G$, in agreement with previous results at smaller magnetic fields. We also find, however, that residual O$_2$ molecules attached close to the contact produce an an induced spin-polarized current, which leads to a decrease in $G$. We discuss the role of the magnetic response of the electrodes in the jump to contact. Our results suggest that single channel atomic size conductors with a sizeable response to a magnetic field can be built by combining noble metals and magnetically active molecular systems.

cond-mat.mes-hall↗

arXiv2024

Anti-hyperuniform diluted vortex matter induced by correlated disorder

Disordered hyperuniform materials are very promising for applications but the successful route for synthesizing them requires to understand the interactions induced by the host media that can switch off this hidden order. With this aim we study the model system of vortices in the $\beta$-Bi$_2$Pd superconductor where correlated defects seem to play a determinant role for the nucleation of a gel vortex phase at low densities. We directly image vortices in extended fields-of-view and show that the disordered vortex structure in this material is anti-hyperuniform, contrasting with the case of vortex structures nucleated in samples with point-like disorder. Based on numerical simulations, we show that this anti-hyperuniform structure arises both, from the interaction of a diluted vortex structure with a fourfold-symmetric correlated disorder quite likely generated when cleaving the samples and from the out of equilibrium nature of the quenched configuration.

cond-mat.supr-con↗

arXiv2024

Electronic band structure from quasiparticle interference and Landau quantization in WTe$_2$

WTe$_2$ stands out as a semimetal presenting Fermi level quantum oscillations in most measured quantities under magnetic fields. However, the electronic band structure above and below the Fermi level has not been explored completely. Here we study the electronic band structure of WTe$_2$ by quasiparticle interference with Scanning Tunneling Microscopy (STM) and observe, with the support of Density Functional Theory (DFT), the electron and hole bands around the Fermi level. We also report on the observation of Landau quantization in atomically resolved measurements and discuss the possible connection with band structure calculations.

cond-mat.mes-hall↗

arXiv2023

The feedback driven atomic scale Josephson microscope

The ultimate spatial limit to establish a Josephson coupling between two superconducting electrodes is an atomic-scale junction. The Josephson effect in such ultrasmall junctions has been used to unveil new switching dynamics, study coupling close to superconducting bound states or reveal non-reciprocal effects. However, the Josephson coupling is weak and the sensitivity to temperature reduces the Cooper pair current magnitude. Here we show that a feedback element induces a time-dependent bistable regime which consists of spontaneous periodic oscillations between two different Cooper pair tunneling states (corresponding to the DC and AC Josephson regimes respectively). The amplitude of the time-averaged current within the bistable regime is almost independent of temperature. By tracing the periodic oscillations in the new bistable regime as a function of the position in a Scanning Tunneling Microscope, we obtain atomic scale maps of the critical current in 2H-NbSe$_2$ and find spatial modulations due to a pair density wave. Our results fundamentally improve our understanding of atomic size Josephson junctions including a feedback element in the circuit and provide a promising new route to study superconducting materials through atomic scale maps of the Josephson coupling.

cond-mat.supr-con↗

arXiv2023

Nano-Patterned Magnetic Edges in CrGeTe3 for Quasi 1-D Spintronic Devices

The synthesis of two-dimensional van der Waals magnets has paved the way for both technological applications and fundamental research on magnetism confined to ultra-small length scales. Edge magnetic moments in ferromagnets are expected to be less magnetized than in the sample interior because of the reduced amount of neighboring ferromagnetic spins at the sample edge. We recently demonstrated that CrGeTe3 (CGT) flakes thinner than 10 nm are hard ferromagnets; i.e., they exhibit an open hysteresis loop. In contrast, thicker flakes exhibit zero net remnant field in the interior, with hard ferromagnetism present only at the cleaved edges. This experimental observation suggests that a nontrivial interaction exists between the sample edge and the interior. Here, we demonstrate that artificial edges fabricated by focus ion beam etching also display hard ferromagnetism. This enables us to write magnetic nanowires in CGT directly and use this method to characterize the magnetic interaction between the interior and edge. The results indicate that the interior saturation and depolarization fields depend on the lateral dimensions of the sample. Most notably, the interior region between the edges of a sample narrower than 300 nm becomes a hard ferromagnet, suggesting an enhancement of the magnetic exchange induced by the proximity of the edges. Last, we find that the CGT regions amorphized by the gallium beam are nonmagnetic, which introduces a novel method to tune the local magnetic properties of CGT films, potentially enabling integration into spintronic devices.

cond-mat.mes-hall↗

arXiv2022

Band structure, superconductivity and polytypism in AuSn$_4$

The orthorhombic compound AuSn4 is compositionally similar to the Dirac node arc semimetal PtSn$_4$. AuSn$_4$ is, contrary to PtSn$_4$, superconducting with a critical temperature of T$_c$ = 2.35 K. Recent measurements present indications for quasi two-dimensional superconducting behavior in AuSn$_4$. Here we present measurements of the superconducting density of states and the band structure of AuSn$_4$ through Scanning Tunneling Microscopy (STM) and Angular Resolved Photoemission Spectroscopy (ARPES). The superconducting gap values in different portions of the Fermi surface are spread around {\Delta}0 = 0.4 meV, which is close to but somewhat larger than $\Delta =$ 1.76kBT$_c$ expected from BCS theory. We observe superconducting features in the tunneling conductance at the surface up to temperatures about 20% larger than bulk Tc. The band structure calculated with Density Functional Theory (DFT) follows well the results of ARPES. The crystal structure presents two possible stackings of Sn layers, giving two nearly degenerate polytypes. This makes AuSn$_4$ a rather unique case with a three dimensional electronic band structure but properties ressembling those of low dimensional layered compounds.

cond-mat.supr-con↗

arXiv2022

Superconducting density of states and bandstructure at the surface of the candidate topological superconductor Au2Pb

The electronic bandstructure of Au$_2$Pb has a Dirac cone which gaps when undergoing a structural transition into a low temperature superconducting phase. This suggests that the superconducting phase ($T_c=1.1$ K) might hold topological properties at the surface. Here we make Scanning Tunneling Microscopy experiments on the surface of superconducting Au$_2$Pb. We measure the superconducting gap and find a sizeable superconducting density of states at the Fermi level. We discuss possible origins for this finding in terms of superconductivity induced into surface states.

cond-mat.supr-con↗