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Edwin W. Huang

Publications and source records attributed to Edwin W. Huang.

At least 19 recordsLinked to original sources

Probing the pseudogap and beyond: Examining single-particle properties of the hole- and electron-doped Hubbard model

We compute high-resolution angle-resolved photoemission spectroscopy of the Hubbard model using the unbiased determinant quantum Monte Carlo algorithm, revealing an asymmetry between electron and hole doping. Electron doping exhibits more coherent quasiparticles and stronger antiferromagnetic correlations compared to hole doping. At low doping, a nodal-antinodal dichotomy on the Fermi surface is observed, similar to cuprate experiments. The dichotomy reflects the momentum dependence of the Mott gap, as manifested in both the spectral function and the self-energy. For hole doping, we observe a transition towards the pseudogap, without signature of pocket formation. The simulated nuclear magnetic resonance pseudogap temperatures do not necessarily agree with the temperature determined by spectroscopy. These findings collectively suggest the pseudogap is a smooth crossover driven by strong correlations.

cond-mat.str-el

Robust fluctuating intertwined charge stripes in the Emery model

The single-band Hubbard model is one of the most extensively studied models in condensed matter physics, giving rise to intertwined spin and charge stripes that coexist with, or lie in the vicinity of, superconductivity in the phase diagram. However, whether the low energy physics of the single-band Hubbard model is fully equivalent to the multi-band (multi-orbital) Emery model remains an unsettled question. While the intertwined stripes and nematicity have been studied in the single-band Hubbard model, a comprehensive picture in the Emery model is lacking. In this paper, we focus on the less investigated intertwined charge stripes using complementary density matrix renormalization group (DMRG) and determinant quantum Monte Carlo (DQMC) techniques. Our ground state DMRG confirms the presence of the oxygen-centered charge stripes at a reduced amplitude in the Emery model parameter regime widely used in the study of intertwined stripes. Close analysis of the oxygen orbital structure of the static charge correlation function from DQMC reveals the charge stripe pattern in real-space, showcasing stronger charge density modulation on $p$-orbitals pointing along ``the rivers of charge'', consistent with DMRG. For the parameter set with the largest fermion signs, we managed to reach a temperature where the system first demonstrated tendencies to form purely unidirectional spin and charge stripes, and the $B_{1g}$ component becomes dominant in the bond-charge nematic susceptibility. This observation correlates with the doping dependence of the kinetic energy anisotropy, suggesting a close relation between the nematicity and charge stripes in the Emery model.

cond-mat.str-el

Enhanced superconducting correlations in the Emery model and its connections to strange metallic transport and normal state coherence

Numerical evidence for superconductivity in the single-band Hubbard model is elusive or ambiguous despite extensive study, raising the question of whether the single-band Hubbard model is a faithful low energy effective model for cuprates, and whether explicitly including the oxygen ions will recover the properties necessary for a superconducting transition. Here we show, by using numerically exact determinant quantum Monte Carlo (DQMC) simulations of the doped Emery model, that while the single-band model exhibits strikingly T-linear resistivity, the three-band model crosses the resistivity of the single-band model from above, indicating a crossover to a more metallic transport regime. The enhanced conductivity is mainly contributed by a steep increase in the diffusivity of the three-band model at the crossover, suggesting that three-band transport is more coherent than single-band transport at lower temperatures. Below the same crossover temperature in the three-band model, the pair-field susceptibility increases more steeply than at higher temperatures or when compared to the single-band model. This suggests a possible connection between superconductivity and coherent transport, and further implies that coherent transport might be necessary for a model to capture the high-temperature superconductivity observed in hole-doped cuprates.

cond-mat.str-el

A light-induced charge order mode in a metastable cuprate ladder

We report the observation of an emergent charge order mode in the optically-excited cuprate ladder Sr$_{14}$Cu$_{24}$O$_{41}$. Near-infrared light in the ladder plane drives a symmetry-protected electronic metastable state together with a partial melting of the equilibrium charge order. Our time-resolved resonant inelastic x-ray scattering measurements at the upper Hubbard band reveal a gapless collective excitation dispersing from the charge-order wavevector up to 0.8 eV with a slope on the order of the quasiparticle velocity. These findings reveal a regime where correlated carriers acquire itinerant character at finite momentum, and charge order becomes dynamically fluctuating, offering a platform to explore light-induced pairing instabilities.

cond-mat.str-el

Charge Susceptibility and Kubo Response in Hatsugai-Kohmoto-related Models

We study in depth the charge susceptibility for the band Hatsugai-Kohmoto (HK) and orbital (OHK) models. As either of these models describes a Mott insulator, the charge susceptibility takes on the form of a modified density response function with lower and upper Hubbard bands, thereby giving rise to a multi-pole structure. The particle-hole continuum consists of hot spots along the $ω$ vs $q$ axis arising from inter-band transitions. Such transitions, which are strongly suppressed in non-interacting systems, obtain here because of the non-rigidity of the Hubbard bands. This modified density response function gives rise to a plasmon dispersion that is inversely dependent on the momentum, resulting in an additional contribution to the conventional f-sum rule. This extra contribution originates from a long-range diamagnetic contribution to the current. This results in a non-commutativity of the long-wavelength ($q\rightarrow 0$) and thermodynamic ($L\rightarrow\infty$) limits. When the correct limits are taken, we find that the Kubo response computed with either open or periodic boundary conditions yields identical results that are consistent with the continuity equation contrary to recent claims. We also show that the long wavelength pathology of the current noted previously also plagues the Anderson impurity model interpretation of dynamical mean-field theory (DMFT).

cond-mat.str-el

Direct Observation of the Lindhard Continuum using Resonant Inelastic X-ray Scattering

Understanding the excitations of quantum materials is essential for unraveling how their microscopic constituents interact. Among these, particle-hole excitations form a particularly important class, as they govern fundamental processes such as screening, dissipation, and transport. In metals, the continuum of electron-hole excitations is described by the Lindhard function. Although central to the theory of Fermi liquids, the corresponding Lindhard continuum has remained experimentally elusive. Here, we report its direct observation in the weakly correlated metal MgB$_{2}$ using ultra-soft resonant inelastic X-ray scattering (RIXS). We resolve a linearly dispersing excitation with velocity comparable to the Fermi velocity and find quantitative agreement with simulations of the non-interacting charge susceptibility. A detailed analysis and decomposition of the simulations reveal the intra-band origin of this low-energy excitation, confirming it as the Lindhard continuum. Our results establish ultra-soft RIXS as a momentum-resolved probe of the fermiology in metals and call for deeper investigations of continuum features in RIXS and related spectroscopy of other materials beyond MgB$_{2}$.

cond-mat.str-el

The Future of the Correlated Electron Problem

A central problem in modern condensed matter physics is the understanding of materials with strong electron correlations. Despite extensive work, the essential physics of many of these systems is not understood and there is very little ability to make predictions in this class of materials. In this manuscript we share our personal views on the major open problems in the field of correlated electron systems. We discuss some possible routes to make progress in this rich and fascinating field. This manuscript is the result of the vigorous discussions and deliberations that took place at Johns Hopkins University during a three-day workshop January 27, 28, and 29, 2020 that brought together six senior scientists and 46 more junior scientists. Our hope, is that the topics we have presented will provide inspiration for others working in this field and motivation for the idea that significant progress can be made on very hard problems if we focus our collective energies.

cond-mat.str-el

Enhanced pair-density-wave vertices in a bilayer Hubbard model at half-filling

Motivated by the pair-density-wave (PDW) state found in the one-dimensional Kondo-Heisenberg chain, we report on a determinant quantum Monte Carlo DQMC study of pair-fields for a two-dimensional half-filled Hubbard layer coupled to an itinerant, non-interacting layer with one electron per site. In a specific range of interlayer hopping, the pairing vertex associated with PDW order becomes more attractive than that for uniform d-wave pairing, although both remain subdominant to the leading antiferromagnetic correlations at half-filling. Our result sheds light on where one potentially may find a PDW state in such a model.

cond-mat.str-el

The emergence of antiferromagnetic correlations and Kondo-like features in a two-band model for infinite-layer nickelates

We report a determinant quantum Monte Carlo study of a two-band model, inspired by infinite-layer nickelates, focusing on the influence of interlayer hybridization between $3d_{x^2-y^2}$ orbitals derived from Ni (or Ni and O) in one layer and rare-earth ($R$) 5d orbitals in the other layer, hereafter the NI and $R$ layers, respectively. For a filling with one electron shared between the two layers on average, interlayer hybridization leads to "self-doped" holes in the Ni layer and the absence of antiferromagnetic ordering, but rather the appearance of spin-density and charge-density stripe-like states. As the interlayer hybridization increases, both the Ni and $R$ layers develop antiferromagnetic correlations, even though either layer individually remains away from half-filling. For hybridization within an intermediate range, roughly comparable to the intralayer nearest-neighbor hopping $t_{\text{Ni}}$, the model develops signatures of Kondo-like physics.

cond-mat.str-el

Particle-hole asymmetric ferromagnetism and spin textures in the triangular Hubbard-Hofstadter model

In a lattice model subject to a perpendicular magnetic field, when the lattice constant is comparable to the magnetic length, one enters the "Hofstadter regime," where continuum Landau levels become fractal magnetic Bloch bands. Strong mixing between bands alters the nature of the resulting quantum phases compared to the continuum limit; lattice potential, magnetic field, and Coulomb interaction must be treated on equal footing. Using determinant quantum Monte Carlo (DQMC) and density matrix renormalization group (DMRG) techniques, we study this regime numerically in the context of the Hubbard-Hofstadter model on a triangular lattice. In the field-filling phase diagram, we find a broad wedge-shaped region of ferromagnetic ground states for filling factor $ν\leq 1$, bounded below by filling factor $ν= 1$ and bounded above by half-filling the lowest Hofstadter subband. We observe signatures of SU(2) quantum Hall ferromagnetism at filling factors $ν=1$ and $ν=3$. The phases near $ν=1$ are particle-hole asymmetric, and we observe a rapid decrease in ground state spin polarization consistent with the formation of skyrmions only on the electron doped side. At large fields, above the ferromagnetic wedge, we observe a low-spin metallic region with spin correlations peaked at small momenta. We argue that the phenomenology of this region likely results from exchange interaction mixing fractal Hofstadter subbands. The phase diagram derived beyond the continuum limit points to a rich landscape to explore interaction effects in magnetic Bloch bands.

cond-mat.str-el

The Wiedemann-Franz law in doped Mott insulators without quasiparticles

Many metallic quantum materials display anomalous transport phenomena that defy a Fermi liquid description. Here, we use numerical methods to calculate thermal and charge transport in the doped Hubbard model and observe a cross-over separating high- and low-temperature behaviors. Distinct from the behavior at high temperatures, the Lorenz number $L$ becomes weakly doping dependent and less sensitive to parameters at low temperatures. At the lowest numerically accessible temperatures, $L$ roughly approaches the Wiedemann-Franz constant $L_0$, even in a doped Mott insulator that lacks well-defined quasiparticles. Decomposing the energy current operator indicates a compensation between kinetic and potential contributions, which may help to clarify the interpretation of transport experiments beyond Boltzmann theory in strongly correlated metals.

cond-mat.str-el

Quantitative assessment of the universal thermopower in the Hubbard model

As primarily an electronic observable, the room-temperature thermopower $S$ in cuprates provides possibilities for a quantitative assessment of the Hubbard model. Using determinant quantum Monte Carlo, we demonstrate agreement between Hubbard model calculations and experimentally measured room-temperature $S$ across multiple cuprate families, both qualitatively in terms of the doping dependence and quantitatively in terms of magnitude. We observe an upturn in $S$ with decreasing temperatures, which possesses a slope comparable to that observed experimentally in cuprates. From our calculations, the doping at which $S$ changes sign occurs in close proximity to a vanishing temperature dependence of the chemical potential at fixed density. Our results emphasize the importance of interaction effects in the systematic assessment of the thermopower $S$ in cuprates.

cond-mat.str-el

Interaction-driven Spontaneous Ferromagnetic Insulating States with Odd Chern Numbers

Motivated by recent experimental work on moiré systems in a strong magnetic field, we compute the compressibility as well as the spin correlations and Hofstadter spectrum of spinful electrons on a honeycomb lattice with Hubbard interactions using the determinantal quantum Monte Carlo method. While the interactions in general preserve quantum and anomalous Hall states, emergent features arise corresponding to an antiferromagnetic insulator at half-filling and other incompressible states following the Chern sequence $\pm (2N+1)$. These odd integer Chern states exhibit strong ferromagnetic correlations and arise spontaneously without any external mechanism for breaking the spin-rotation symmetry. Analogs of these magnetic states should be observable in general interacting quantum Hall systems. In addition, the interacting Hofstadter spectrum is qualitatively similar to the experimental data at intermediate values of the on-site interaction.

cond-mat.str-el

Exact solution for finite center-of-mass momentum Cooper pairing

Pair density waves (PDWs) are superconducting states formed by ``Cooper pairs" of electrons containing a non-zero center-of-mass momentum. They are characterized by a spatially modulated order parameter and may occur in a variety of emerging quantum materials such as cuprates, transition metal dichalcogenides (TMDs) and Kagome metals. Despite extensive theoretical and numerical studies seeking PDWs in a variety of lattices and interacting settings, there is currently no generic and robust mechanism that favors a modulated solution of the superconducting order parameter in the presence of time reversal symmetry. Here, we study the problem of two electrons subject to an anisotropic ($d$-wave) attractive potential. We solve the two-body Schrodinger wave equation exactly to determine the pair binding energy as a function of the center-of-mass momentum. We find that a modulated (finite momentum) pair is favored over a homogeneous (zero momentum) solution above a critical interaction. Using this insight from the exact two-body solution, we construct a BCS-like variational many-body wave function and calculate the free energy and superconducting gap as a function of the center-of-mass momentum. A zero temperature analysis of the energy shows that the conclusions of the two-body problem are robust in the many-body limit. Our results lay the theoretical and microscopic foundation for the existence of PDWs.

cond-mat.supr-con

Thermodynamics of correlated electrons in a magnetic field

The Hofstadter-Hubbard model captures the physics of strongly correlated electrons in an applied magnetic field, which is relevant to many recent experiments on Moiré materials. Few large-scale, numerically exact simulations exists for this model. In this work, we simulate the Hubbard-Hofstadter model using the determinant quantum Monte Carlo (DQMC) algorithm. We report the field and Hubbard interaction strength dependence of charge compressibility, fermion sign, local moment, magnetic structure factor, and specific heat. The gross structure of magnetic Bloch bands and band gaps determined by the non-interacting Hofstadter spectrum is preserved in the presence of $U$. Incompressible regions of the phase diagram have improved fermion sign. At half filling and intermediate and larger couplings, a strong orbital magnetic field delocalizes electrons and reduces the effect of Hubbard $U$ on thermodynamic properties of the system.

cond-mat.str-el

Magnon heat transport in a two-dimensional Mott insulator

Whether or not anomalies in the thermal conductivity in insulating cuprates can be attributed to antiferromagnetic order and magnons in a 2D Mott insulator remains an intriguing open question. To shed light on this issue, we investigate the thermal conductivity $κ$ and its relationship with the specific heat $c_v$ in the half-filled 2D single-band Hubbard model, using the numerically exact determinant quantum Monte Carlo algorithm and maximum entropy analytic continuation. At low temperatures where the charge degrees of freedom are gapped-out and $c_v$ exhibits a clear magnon peak, we observe that thermal conductivity $κ$ also tends to form a peak at similar temperatures. Reducing temperature further produces a sharp upturn in $κ$, associated with an increasing mean-free path. We identify this as the high-temperature side of the anomalous peak in insulating cuprates, where the mean-free path eventually is cut-off by other scattering effects, including phonons, disorder, and physical size. Different scattering effects in our model are identified and analyzed in the thermal diffusivity.

cond-mat.str-el

Doped Mott Insulators Break $\mathbb Z_2$ Symmetry of a Fermi Liquid: Stability of Strongly Coupled Fixed Points

Because Fermi liquids are inherently non-interacting states of matter, all electronic levels below the chemical potential are doubly occupied. Consequently, the simplest way of breaking Fermi liquid theory is to engineer a model in which some of those states are singly occupied keeping time-reversal invariance intact. We show that breaking an overlooked local-in-momentum space $\mathbb Z_2$ symmetry of a Fermi liquid does precisely this. As a result, while the Mott transition from a Fermi liquid is correctly believed to obtain without the breaking of any continuous symmetry, a discrete symmetry is broken. This symmetry breaking serves as an organizing principle for Mott physics whether it arises from the tractable Hatsugai-Kohmoto (HK) model or the intractable Hubbard model. That both are controlled by the same fixed point we establish through a renormalization group analysis. An experimental manifestation of this fixed point is the onset of particle-hole asymmetry, a widely observed phenomenon in strongly correlated systems. Theoretically, the singly-occupied region of the spectrum gives rise to a surface of zeros of the single-particle Green function, denoted as the Luttinger surface. Using K-homology, we show that the Bott topological invariant guarantees the stability of this surface to local perturbations. Our proof demonstrates that the strongly coupled fixed point only corresponds to those Luttinger surfaces with co-dimension $p+1$ with $p$ odd. We conclude that the Hubbard and HK models both lie in the same high temperature universality class and are controlled by the broken $\mathbb Z_2$ symmetry quartic fixed point.

cond-mat.str-el

Fluctuating intertwined stripes in the strange metal regime of the Hubbard model

Strongly correlated electron systems host a variety of poorly understood correlations in their high temperature normal state. Unlike ordered phases defined by order parameters, these normal state phases are often defined through unconventional properties such as strange metallic transport or spectroscopic pseudogaps. Characterizing the microscopic correlations in the normal state is necessary to elucidate mechanisms that lead to these properties and their connection to ground state orders. Here we establish the presence of intertwined charge and spin stripes in the strange metal normal state of the Hubbard model using determinant quantum Monte Carlo calculations. The charge and spin density waves constituting the stripes are fluctuating and short-ranged, yet they obey a mutual commensurability relation and remain microscopically interlocked, as evidenced through measurements of three-point spin-spin-hole correlation functions. Our findings demonstrate the ability of many-body numerical simulations to unravel the microscopic correlations that define quantum states of matter.

cond-mat.str-el