arXiv subjects

Eiji Saitoh

Publications and source records attributed to Eiji Saitoh.

At least 19 recordsLinked to original sources

arXiv2026

Magnetoelastic coupling in stripe-domain states of yttrium iron garnet

We study magnetoelastic coupling in stripe-domain magnetic states of $3\,\mathrm{μm}$-thick YIG thin films grown on a GGG substrate. Broadband ferromagnetic resonance reveals low-frequency stripe-domain magnon branches modulated by a field-independent phonon comb with a frequency spacing of $3.5\,\mathrm{MHz}$, matching the value predicted for confined thickness-shear modes of the GGG substrate. Analytical fitting yields coupling rates that vary between $0.33$--$0.54\,\mathrm{MHz}$ and cooperativities of order $10^{-1}$, indicating that the system is in the weak-coupling regime without resolvable avoided-crossing gaps. Magnon-phonon mode-overlap calculations using finite-element simulations show that the weak coupling arises from phase and domain-sign cancellation: the local magnetoelastic coupling is sizable, but more than $99\%$ of the coherent overlap cancels across the stripe texture. Fully coupled simulations further demonstrate phonon-mediated excitation of a remote YIG layer and show that efficient propagating-phonon generation requires spatially asymmetric magnon modes, establishing magnetic texture as a control parameter for magnon--phonon coupling.

cond-mat.mes-hall↗

arXiv2026

Double anticrossings induced by nonlinear magnon interactions

We observe pump-induced double anticrossings whose gap sizes and center-frequency shifts depend strongly on pump power, indicating a nonlinear mechanism. The anticrossings vanish at high magnetic fields, where energy conservation suppresses three-magnon splitting, thereby identifying the underlying process as three-magnon scattering. We attribute the double anticrossings to nondegenerate three-magnon splitting, which generates two magnon populations at distinct frequencies. Each population forms a standing-wave mode and couples independently to the Kittel mode, giving rise to two effective coupling channels. These results demonstrate that nonlinear magnon interactions can dynamically generate multiple coupling channels within a single system.

cond-mat.mes-hall↗

arXiv2026

Electronic manipulation of polar order in electron crystal

When interaction among atoms or ions is strong enough, they often arrange periodically, forming a crystal. The arrangement patterns of atoms or ions can encode information, a concept that has enabled devices such as ferroelectric memories. It has been found that not only atoms or ions but also electrons in condensed matter can crystallize when Coulomb interaction is strong enough. Typical examples are charge-ordered states in solids, where different valences, or different electron numbers, of an ion spontaneously form a spatial pattern on the lattice. In such electron crystals, information is expected to be encoded into the electron-ordering patterns. Here, we demonstrate electronic manipulation and readout of charge-ordering directions in a paramagnetic semiconductor LuFe$_2$O$_4$. By applying current pulses at room temperature, we observed that the non-reciprocal resistivity of LuFe$_2$O$_4$ is modulated along with a sign reversal, which disappears above the charge-ordering temperature. A numerical calculation incorporating inter-band Berry curvature affected by the charge ordering is consistent with the experimental results. By applying the observed phenomenon, we also demonstrate a non-reciprocal resistance memory operation in the charge-ordered LuFe$_2$O$_4$. This result opens the door to realizing charge-ordering electronics.

cond-mat.mtrl-sci↗

arXiv2026

All optical excitation of spin polarization in d-wave altermagnets

The recently discovered altermagnets exhibit collinear magnetic order with zero net magnetization but with unconventional spin-polarized d/g/i-wave band structures, expanding the known paradigms of ferromagnets and antiferromagnets. In addition to novel current-driven electronic transport effects, the unconventional time-reversal symmetry breaking in these systems also makes it possible to obtain a spin response to \emph{linearly polarized} fields in the optical frequency domain. We show through ab-initio calculations of the prototypical d-wave altermagnet RuO$_2$, with a symmetry combining twofold spin rotation with fourfold lattice rotation, $[C_2\|C_{4z}]$, that there is an optical analogue of a spin splitter effect, as the coupling to a linearly polarized exciting laser field makes the d-wave character of the altermagnet directly visible. By magneto-optical measurements on RuO$_2$ films of different thicknesses ranging from $2$ to $8\,$nanometers, we demonstrate the predicted connection of the linear polarization of an ultrashort pump pulse to the sign and magnitude of the optically excited electronic spin polarization in the ultrathin RuO$_2$ films. The possibility of exciting and controlling an electronic spin polarization by linearly polarized optical pulses in a compensated system is a unique consequence of the altermagnetic material properties. Our experimental results therefore establish an optical pump-probe based protocol for detection of altermagnetic characteristics in ultrathin RuO$_2$ films, but our all-optical approach should apply more generally to materials in this altermagnetic symmetry class.

cond-mat.mtrl-sci↗

arXiv2026

Giant orbital magnetoresistance in the antiferromagnet CoO driven by dynamic orbital angular momentum interaction

Recent predictions of orders of magnitude larger orbital current effects compared to spin currents have attracted significant interest. However, the full potential of giant orbital currents remains to be fully harnessed, since so far, the orbital currents need to be converted into spin currents before they can interact with the static magnetization that is dominated by spin angular momentum in conventional magnets. By using a magnet dominated by orbital angular momentum, we demonstrate a more than fifty-fold enhancement in orbital Hall magnetoresistance in CoO/Cu*, compared to conventional CoO/Pt. This is found to be driven by a unique interaction between dynamic orbital angular momentum from surface oxidized Cu* (i.e., the orbital current) and the static orbital angular momentum which constitutes the magnetic moments in the antiferromagnetic insulator CoO. A distinctive scattering mechanism for orbital currents at the CoO interface leads to a sign reversal in orbital magnetoresistance in CoO/Cu* compared to CoO/Pt. Our results show how by using orbital angular momentum-dominated materials such as CoO, we can harness the benefits of giant orbital currents that have not been possible using conventional spin-dominated magnets, for orbitronics-based devices, offering unprecedented energy efficiency for operations of antiferromagnets that combine ultimate stability with THz dynamics.

cond-mat.mtrl-sci↗

arXiv2025

Shift of quantum critical point of discrete time crystal on a noisy quantum simulator

Recent advances in quantum technology have enabled the simulation of quantum many-body systems on real quantum devices. However, such quantum simulators are inherently subject to decoherence, and its impact on system dynamics - particularly near quantum phase transitions - remains insufficiently understood. In this work, we experimentally investigate how decoherence in quantum devices affects the dynamics of quantum time crystals, using a 156-qubit IBM Quantum system. We find that decoherence shifts the location of critical behavior associated with the phase transition, suggesting that noisy simulations can lead to inaccurate identification of phase boundaries. Our results underscore the importance of understanding and mitigating decoherence to reliably simulate quantum many-body systems on near-term quantum hardware.

quant-ph↗

arXiv2025

Observing Differential Spin Currents by Resonant Inelastic X-ray Scattering

Controlling spin currents, i.e., the flow of spin angular momentum, in small magnetic devices is the principal objective of spin electronics, a main contender for future energy efficient information technologies. Surprisingly, a pure spin current has never been measured directly since the associated electric stray fields and/or shifts in the non-equilibrium spin-dependent distribution functions are too small for conventional experimental detection methods optimized for charge transport. Here we report that resonant inelastic x-ray scattering (RIXS) can bridge this gap by measuring the spin current carried by magnons -- the quanta of the spin wave excitations of the magnetic order -- in the presence of temperature gradients across a magnetic insulator. This is possible due to the sensitivity of the momentum- and energy-resolved RIXS intensity to minute changes in the magnon distribution under non-equilibrium conditions. We use the Boltzmann equation in the relaxation time approximation to extract transport parameters, such as the magnon lifetime at finite momentum, essential for the realization of magnon spintronics.

cond-mat.mes-hall↗

arXiv2025

Spin wave resonance in yttrium iron garnet stripe domains

We study a thin film yttrium iron garnet sample that exhibits magnetic stripe domains due to a small perpendicular magnetic anisotropy. Using wide-field magneto-optic Kerr effect measurements we reveal the domain pattern evolution as a function of applied field and discuss the role of the cubic anisotropy in the domain formation. Rich magnon spectra are observed in the stripe domain states, with a range of excitation conditions providing distinct spectra. The measurements are interpreted using micromagnetic simulations to provide the spatial profiles of each resonance mode. We further simulate domain patterns and resonance spectra accounting for the cubic anisotropy,with good correlation to experiment. This study highlights how non-collinear magnetic domain structures can host complex resonant behaviour in a low-damping magnetic material, with potential use in future magnonic applications.

cond-mat.mtrl-sci↗

arXiv2025

Diffusion model for analyzing quantum fingerprints in conductance fluctuation

A conditional diffusion model has been developed to analyze intricate conductance fluctuations called universal conductance fluctuations or quantum fingerprints appearing in quantum transport phenomena. The model reconstructs impurity arrangements and quantum interference patterns in nanometals by using magnetoconductance data, providing a novel approach to analyze complex data based on machine learning. In addition, we visualize the attention weights in the model, which efficiently extract information on the non-local correlation of the electron wave functions, and the score functions, which represent the force fields in the wave-function space.

cond-mat.mes-hall↗

arXiv2024

Separating terahertz spin and charge contributions from ultrathin antiferromagnetic heterostructures

Femtosecond laser excitation of nanometer thin heterostructures comprising a heavy metal and a magnetically ordered material is known to result in the emission of terahertz radiation. However, the nature of the emitted radiation from heavy metal~/~antiferromagnet heterostructures has sparked debates and controversies in the literature. Here, we unambiguously separate spin and charge contributions from Pt~/~NiO heterostructures by introducing an unprecedented methodology combining high external magnetic fields with a symmetry analysis of the emitted terahertz polarization. We observe two distinct mechanisms of terahertz emission which we identify as optical difference frequency generation and ultrafast laser-induced quenching of the magnetization. We emphasize the absence of spin transport effects and signatures of coherent magnons. Overall, our work provides a general experimental methodology to separate spin and charge contributions to the laser-induced terahertz emission from heterostructures comprising a magnetically ordered material thus holding great potential for advancing terahertz spintronics and establishing terahertz orbitronics.

cond-mat.mes-hall↗

arXiv2024

Inverse magneto-conductance design by automatic differentiation

Magneto-conductance in thin wires often exhibits complicated patterns due to the quantum interference of conduction electrons. These patterns reflect microscopic structures in the wires, such as defects or potential distributions. In this study, we propose an inverse design method to automatically generate a microscopic structure that exhibits desired magneto-conductance patterns. We numerically demonstrate that our method accurately generates defect positions in wires and can be effectively applied to various complicated patterns. We also discuss techniques for designing structures that facilitate experimental investigation.

cond-mat.mtrl-sci↗

arXiv2024

Negative longitudinal resistance of monolayer graphene in the quantum Hall regime

In the quantum Hall regime the charge current is carried by ideal one-dimensional edge channels where the backscattering is prohibited by topology. This results in the constant potential along the edge of the Hall bar leading to zero 4-terminal longitudinal resistance r_xx. Finite scattering between the counter-propagating edge states, when the topological protection is broken, commonly results in r_xx > 0. However, a local disorder, if allowing intersection of the edge states, can result in a counter-intuitive scenario when r_xx<0. In this work we report the observation and a systematic study of such unconventional negative longitudinal resistance seen in an encapsulated monolayer graphene Hall bar device measured in the quantum Hall regime. We supplement our findings with the numerical calculations which allow us to outline the conditions necessary for the appearance of negative r_xx and to exclude the macroscopic disorder (contamination bubble) as the main origin of it.

cond-mat.mes-hall↗

arXiv2024

Field Dispersion and Strong Coupling of Nuclear-Electron Spin Excitation in MnCO$_3$

Hybridized nuclear and electron spin excitation in a MnCO$_3$ crystal, a weakly-anisotropic antiferromagnet, has been investigated. In this material, the hyperfine interaction is strong enough to form a nuclear spin wave. We measure the microwave absorption by a bulk MnCO$_3$ and observe the dispersion representing strong frequency repulsion between electron and nuclear modes due to their hybridization, the signature of nuclear spin wave. Additionally, we observe that the nuclear spin resonance enters a nonlinear regime above a certain excitation power, attributed to the excitation of finite wavenumber nuclear spin waves.

cond-mat.str-el↗

arXiv2024

Current-induced magnon trapping in spin torque oscillation

Spin torque nano-oscillators realized by magnetization dynamics trapped in a current-induced potential are reported. We fabricated Ni$_{81}$Fe$_{19}$/Pt nanostructures and measured current-induced microwave emission from the structures. The result shows an increase in the magnitude and spectral narrowing of the microwave emission. We demonstrate that the current-induced magnetic field suppresses magnon radiation loss and significantly reduces the linewidth and the threshold current required for the spin torque oscillation.

cond-mat.mes-hall↗

arXiv2024

Dynamics of measurement-induced state transitions in superconducting qubits

We have investigated temporal fluctuation of superconducting qubits via the time-resolved measurement for an IBM Quantum system. We found that the qubit error rate abruptly changes during specific time intervals. Each high error state persists for several tens of seconds, and exhibits an on-off behavior. The observed temporal instability can be attributed to qubit transitions induced by a measurement stimulus. Resonant transition between fluctuating dressed states of the qubits coupled with high-frequency resonators can be responsible for the error-rate change.

quant-ph↗

arXiv2023

Detecting bulk carbon ferromagnetism in graphene multi-edge structure

The emergence of bulk carbon ferromagnetism is long-expected over years. At nanoscale, carbon ferromagnetism was detected by analyzing the magnetic edge states via scanning tunneling microscopy(STM), and its origin can be explained by local redistribution of electron wave function. In larger scale, carbon ferromagnetism can be created by deliberately producing defects in graphite, and detected by macroscopic technical magnetization. Meanwhile, it becomes crucial to determine that the detected magnetization is originated from carbon rather than from magnetic impurities. One solution is X-ray magnetic circular dichroism (XMCD). Nonetheless, a reproducible, full section of XMCD spectrum across C-1s absorption energy has not appeared yet, which should be decisive for assuring the indisputable existence of bulk carbon ferromagnetism. Besides, the lack of direct observation on the atomic structure of the ferromagnetic carbon leaves the structural origin of its ferromagnetism still in mist. In this work, for detecting bulk carbon ferromagnetism, we managed to grow all-carbon film consisting of vertically aligned graphene multi-edge (VGME), which wove into a three-dimensional hyperfine-porous network. Magnetization (M-H) curves and XMCD spectra co-confirmed bulk carbon ferromagnetism of VGME at room temperature, with the average unit magnetic momentum of ~0.0006 miuB/atom. The influence of magnetic impurities on magnetization was excluded by both absorption spectra and inductively coupled plasma mass spectrometry measurements. The spin transfer behavior also verified the long-range and robust feature of the bulk carbon ferromagnetism. Our work provides direct evidence of elementary resolved bulk carbon ferromagnetism at room temperature and clarifies its origin from pi-electrons at graphene edges.

cond-mat.mtrl-sci↗

arXiv2023

Nonlinear enhancement of coherent magnetization dynamics

Magnets are interesting materials for classical and quantum information technologies. However, the short decoherence and dephasing times that determine the scale and speed of information networks, severely limit the appeal of employing the ferromagnetic resonance. Here we show that the lifetime and coherence of the uniform Kittel mode can be enhanced by 3-magnon interaction-induced mixing with the long-lived magnons at the minima of the dispersion relation. Analytical and numerical calculations based on this model explain recent experimental results and predict experimental signatures of quantum coherence.

cond-mat.mes-hall↗

arXiv2023

Fabrication of damage-free and/or contamination-free sub-um electrodes using PMMA masks

Quality of the electrical contacts and interfaces in various metal/semiconductor/insulator heterostructures is one of the pivotal aspects in both applied and fundamental research areas. For instance, non-optimal contact resistance can limit the overall efficiency of a certain developed technology and thus considerably narrow the range or fully block its practical application. On the other hand in fundamental research it is often the case that the manifestation of targeted phenomenon crucially depends on the level of contamination in the fabricated experimental samples. Here we offer a set of recipes that are aimed at contamination-free and damage-free fabrication of the devices, mostly developed for the two dimensional materials, but nevertheless applicable for a wider range of the systems, where the quality of the interfaces and/or non-invasiveness of the fabrication recipes are important. Our recipes are based on the preparation of the flexible PMMA membranes, with the help of which we can prepare residue-free or damage-free electrical connections to the studied material.

cond-mat.mes-hall↗