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Eikichi Kimura

Publications and source records attributed to Eikichi Kimura.

4 recordsLinked to original sources

Universal scaling of electrochemical information transfer at solid-liquid interfaces

Electrochemical potentials at solid-liquid interfaces govern diverse chemical and energy conversion processes; however, the extent to which their electrochemical influence extends into the solid remains unclear. Here, we show that the maximum accessible electrochemical information is governed by a single dimensionless screening parameter $u$, defined as the ratio of the effective electrostatic separation between the interface and probe to the electrostatic propagation length in the solid. The maximum Fisher information follows a universal inverse-square scaling with this parameter. This relation identifies electrostatic screening as a fundamental constraint on information transfer across solid-liquid interfaces and provides quantitative design principles for interfacial electrochemical sensing.

physics.app-ph↗

Current-dipole detection of microscale metal defects

An effective electric current dipole provides a compact description of localized current disturbances and has been employed across a broad range of physical systems and length scales. Despite its extensive use in macroscopic systems, its applicability to microscale material diagnostics remains unexplored. In this study, we demonstrate that the current-dipole representation provides an effective physical framework for the detection and characterization of microscopic defects in conductive materials. When an external current is applied to a metal, defects locally perturb the current distribution, thus generating an effective in-plane current dipole that yields a characteristic magnetic-field pattern. By measuring the magnetic-field distribution above the metal and fitting it with a dipole model, we reconstruct the position and effective strength of the dipole, thereby enabling the inference of the defect location and an effective defect-volume metric. Using wide-field magnetic imaging as a measurement platform, we observe a defect-associated magnetic signal from a 38-um-long defect on the front surface of copper samples and identify a defect on the back surface using a 0.5-mm-thick copper plate. We further examine the applicability of this approach to magnetic materials, where permeability contrasts modify the field distribution. Our results establish current-dipole imaging as a general physical framework for magnetic detection of defects and highlight its potential for nondestructive inspection across a wide range of length scales.

physics.app-ph↗

Wide-field NV magnetometry under simultaneous high-pressure and high-temperature conditions

We demonstrate wide-field optically detected magnetic resonance (ODMR) under simultaneous high-pressure and high-temperature conditions using nitrogen-vacancy (NV) centers. Although NV-center magnetometry has been widely used for spatially resolved magnetic-field imaging, its application to extreme environments combining pressure and temperature remains challenging. In this work, we show that ODMR can be observed at 5 GPa and 500 K, demonstrating the feasibility of NV spin readout under such combined extreme conditions. We further perform wide-field ODMR of iron at 7 GPa and 500 K, where the stray magnetic field from the sample is spatially visualized through the pressure cell. These results establish NV-center magnetometry as a promising platform for imaging magnetic phenomena in materials under high-pressure and high-temperature environments.

physics.app-ph↗

Coherent control of solid-state defect spins via patterned boron-doped diamond circuit

Monolithic integration, which refers to the incorporation of all device functionalities within a single material, shows significant potential for creating scalable solid-state quantum devices. This study demonstrated the coherent control of nitrogen-vacancy (NV) spins using an electronic circuit monolithically integrated within diamond: a patterned, conductive boron-doped diamond (BDD) microwave waveguide. First, we validated the high-frequency performance of the circuit by characterizing its impedance up to the microwave range, confirming its capability for efficient microwave transmission. Then, using this monolithically integrated BDD--NV hybrid system, we performed optically detected magnetic resonance and observed noticeable Rabi oscillations driven by the metallic BDD circuit. Importantly, we verified that the BDD antenna has a minimal detrimental impact on the NV spins; microwave-induced heating is negligible under both pulsed and continuous driving, and the spin relaxation time ($T_1$) remains unperturbed. This approach paves the way for a new class of compact, robust, and versatile quantum platforms suitable for sensing and information processing in various environments.

physics.app-ph↗