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Eirik Holm Fyhn

Publications and source records attributed to Eirik Holm Fyhn.

14 recordsLinked to original sources

Influence of ammonia-water fog formation on ammonia dispersion from a liquid spill

Ammonia is expected to play an important role in the green transition, both as a hydrogen carrier and a zero-emission fuel. The use of refrigerated ammonia is attractive due to its relatively high volumetric energy density and increased safety compared to pressurized solutions. Ammonia is highly toxic, and with new applications and increased global demand come stricter requirements for safe handling. Cold gaseous ammonia following a spill of refrigerated ammonia will in contact with humid air cause fog formation. In an environment rich in ammonia, these droplets will due to ammonia's strong hygroscopicity consist of considerable amounts of liquid ammonia as well as water. Fog formation affects the ammonia-air density and thus influences the dispersion dynamics, with a potentially significant impact on hazardous zones. In this work, we present a CFD model including an ammonia-water fog formation model based on accurate thermodynamics. This includes modeling the vapor-liquid equilibrium and accounting for the exothermic mixing of ammonia and water. We apply this CFD model to relevant cases and demonstrate the significant impact of the fog. We analyze the effect of varying relative humidity, fog visibility, influence of wind, and pool evaporation rate. Finally, we model the experimental Red Squirrel test 1F.

physics.flu-dyn↗

Barrier and finite size effects on the extension of topological surface-states into magnetic insulators

The interplay between magnetic and topological order can give rise to phenomena such as the quantum anomalous Hall effect. The extension of topological surface states into magnetic insulators (MIs) has been proposed as an alternative to using intrinsically magnetic topological insulators (TIs). Here, we theoretically study how this extension of surface states into a magnetic insulator are influenced both by the interface barrier potential separating a topological insulator and a magnetic insulator and by finite size effects in such structures. We find that the the gap in the surface states depends non-monotonically on the barrier strength. A small, but finite, barrier potential turns out to be advantageous as it permits the surface states to penetrate even further into the MI. Moreover, we find that due to finite size effects in thin samples, increasing the spin-splitting in the MI can actually decrease the gap of the surface states, in contrast to the usual expectation that the gap opens as the spin-splitting increases.

cond-mat.mes-hall↗

Superconducting proximity effect and long-ranged triplets in dirty metallic antiferromagnets

Antiferromagnets have no net spin-splitting on the scale of the superconducting coherence length. Despite this, antiferromagnets have been observed to suppress superconductivity in a similar way as ferromagnets, a phenomenon that still lacks a clear understanding. We find that this effect can be explained by the role of impurities in antiferromagnets. Using quasiclassical Green's functions, we study the proximity effect and critical temperature in diffusive superconductor-metallic antiferromagnet bilayers. The non-magnetic impurities acquire an effective magnetic component in the antiferromagnet. This not only reduces the critical temperature but also separates the superconducting correlations into short-ranged and long-ranged components, similar to ferromagnetic proximity systems.

cond-mat.supr-con↗

Quasiclassical theory for antiferromagnetic metals

Unlike ferromagnetism, antiferromagnetism cannot readily be included in the quasiclassical Keldysh theory because of the rapid spatial variation in the directions of the magnetic moments. The quasiclassical framework is useful because it separates the quantum effects occurring at length scales comparable to the Fermi wavelength from other length scales, and has successfully been used to study a wide range of phenomena involving both superconductivity and ferromagnetism. Starting from a tight-binding Hamiltonian, we develop general quasiclassical equations of motion and boundary conditions, which can be used to describe two-sublattice metallic antiferromagnets in the dirty limit. The boundary conditions are applicable also for spin-active boundaries that can be either compensated or uncompensated. Additionally, we show how nonuniform or dynamic magnetic textures influence the equations and we derive a general expression for observables within this framework.

cond-mat.supr-con↗

Threefold enhancement of superconductivity and the role of field-induced odd-frequency pairing in epitaxial aluminum films near the 2D limit

BCS theory has been widely successful at describing elemental bulk superconductors. Yet, as the length scales of such superconductors approach the atomic limit, dimensionality as well as the environment of the superconductor can lead to drastically different and unpredictable superconducting behavior. Here, we report a threefold enhancement of the superconducting critical temperature and gap size in ultrathin epitaxial Al films on Si(111), when approaching the 2D limit, based on high-resolution scanning tunneling microscopy/spectroscopy (STM/STS) measurements. In magnetic field, the Al films show type II behavior and the Meservey-Tedrow-Fulde (MTF) effect for in-plane magnetic fields. Using spatially resolved spectroscopy, we characterize the vortex structure in the MTF regime and find strong deviations from the typical Abrikosov vortex. We corroborate these findings with calculations that unveil the role of odd-frequency pairing and a paramagnetic Meissner effect. These results illustrate two striking influences of reduced dimensionality on a BCS superconductor and present a new platform to study BCS superconductivity in large magnetic fields.

cond-mat.supr-con↗

Spin-orbit pumping

We study theoretically the effect of a rotating electric field on a diffusive nanowire and find an effect that is analogous to spin pumping, which refers to the generation of spin through a rotating magnetic field. The electron spin couples to the electric field because the particle motion induces an effective magnetic field in its rest frame. In a diffusive system the velocity of the particle, and therefore also its effective magnetic field, rapidly and randomly changes direction. Nevertheless, we demonstrate analytically and via a physical argument why the combination of the two effects described above produces a finite magnetization along the axis of rotation. This manifests as a measurable spin-voltage in the range of tens of microvolts.

cond-mat.mes-hall↗

Planar graphene-NbSe$_2$ Josephson junctions in a parallel magnetic field

Thin transition metal dichalcogenides sustain superconductivity at large in-plane magnetic fields due to Ising spin-orbit protection, which locks their spins in an out-of-plane orientation. Here we use thin NbSe$_2$ as superconducting electrodes laterally coupled to graphene, making a planar, all van der Waals two-dimensional Josephson junction (2DJJ). We map out the behavior of these novel devices with respect to temperature, gate voltage, and both out-of-plane and in-plane magnetic fields. Notably, the 2DJJs sustain supercurrent up to $H_\parallel$ as high as 8.5 T, where the Zeeman energy $E_Z$ rivals the Thouless energy $E_{Th}$, a regime hitherto inaccessible in graphene. As the parallel magnetic field $H_\parallel$ increases, the 2DJJ's critical current is suppressed and in a few cases undergoes suppression and recovery. We explore the behavior in $H_\parallel$ by considering theoretically two effects: a 0-$π$ transition induced by tuning of the Zeeman energy and the unique effect of ripples in an atomically thin layer which create a small spatially varying perpendicular component of the field. The 2DJJs have potential utility as flexible probes for two-dimensional superconductivity in a variety of materials and introduce high $H_\parallel$ as a newly accessible experimental knob.

cond-mat.supr-con↗

Spin-pumping in superconductor-antiferromagnetic insulator bilayers

We study theoretically spin pumping in bilayers consisting of superconductors and antiferromagnetic insulators. We consider both compensated and uncompensated interfaces and include both the regular scattering channel and the Umklapp scattering channel. We find that at temperatures close to the critical temperatures and precession frequencies much lower than the gap, the spin-current is enhanced in superconductors as compared to normal metals. Otherwise, the spin-current is suppressed. The relevant precession frequencies where the spin-current in SC/AFI is enhanced compared to NM/AFI is much lower than the typical resonance frequencies of antiferromagnets, which makes the detection of this effect experimentally challenging. A possible solution lies in the shifting of the resonance frequency by a static magnetic field.

cond-mat.supr-con↗

Temporarily enhanced superconductivity from magnetic fields

Contrary to the expected detrimental influence on superconductivity when applying a magnetic field, we predict that the abrupt onset of such a field can temporarily strongly enhance the superconducting order parameter. Specifically, we find that the supercurrent in a Josephson junction with a normal metal weak link can increase more than twentyfold in this way. The effect can be understood from the interplay between the energy-dependence of Andreev reflection and the abrupt spin-dependent shift in the distribution functions for excitations in the system. The duration of the increase depends on the inelastic scattering rate in the system and is estimated to be in the range of nanoseconds. We demonstrate this by developing a method which solves the Usadel equation for an arbitrary time-dependence. This enables the study of ultrafast time-dependent physics in heterostructures combining superconductors with different types of materials.

cond-mat.supr-con↗

A combined fluid-dynamic and thermodynamic model to predict the onset of rapid phase transitions in LNG spills

Transport of liquefied natural gas (LNG) by ship occurs globally on a massive scale. The large temperature difference between LNG and water means LNG will boil violently if spilled onto water. This may cause a physical explosion known as rapid phase transition (RPT). Since RPT results from a complex interplay between physical phenomena on several scales, the risk of its occurrence is difficult to estimate. In this work, we present a combined fluid-dynamic and thermodynamic model to predict the onset of delayed RPT. On the basis of the full coupled model, we derive analytical solutions for the location and time of delayed RPT in an axisymmetric steady-state spill of LNG onto water. These equations are shown to be accurate when compared to simulation results for a range of relevant parameters. The relative discrepancy between the analytic solutions and predictions from the full coupled model is within 2% for the RPT position and within 8% for the time of RPT. This provides a simple procedure to quantify the risk of occurrence for delayed RPT for LNG on water. Due to its modular formulation, the full coupled model can straightforwardly be extended to study RPT in other systems.

physics.flu-dyn↗

Combined Zeeman and orbital effect on the Josephson effect in rippled graphene

The two-dimensional nature of graphene Josephson junctions offers the possibility of creating effective superconductor-ferromagnet-superconductor junctions with tunable Zeeman splitting caused by an in-plane magnetic field. Such junctions would be able to alternate between a conventional superconducting ground state and a ground state with an intrinsic phase difference, making them controllable $0-π$ Josephson junctions. However, in addition to the Zeeman splitting, an in-plane magnetic field will in general also produce an orbital effect because of height variations in graphene, colloquially known as ripples. Both the Zeeman and orbital effect will thus affect the critical current, so to be able to identify $0-π$ transitions it is necessary to understand their combined effect. From both analytical and numerical solutions of the Usadel equation we find that ripples can in fact produce a current response similar to that which is characteristic of a $0-π$ transition. Hence, additional analysis is required in order to reveal the presence of a $0-π$ transition caused by spin-splitting in graphene with ripples. We provide a closed form analytical expression for the critical current in the presence of exchange field and ripple effects as well as an expression for the scaling of critical current zeroes with junction parameters.

cond-mat.supr-con↗

Controllable Vortex Loops in Superconducting Proximity Systems

Superconducting vortex loops have so far avoided experimental detection despite being the focus of much theoretical work. We here propose a method of creating controllable vortex loops in the superconducting condensate arising in a normal metal through the proximity effect. We demonstrate both analytically and numerically that superconducting vortex loops emerge when the junction is pierced by a current-carrying insulated wire and give an analytical expression for their radii. The vortex loops can readily be tuned big enough to hit the sample surface, making them directly observable through scanning tunneling microscopy.

cond-mat.supr-con↗

Superconducting Vortices in Half-Metals

When the impurity mean free path is short, only spin-polarized Cooper pairs which are non-locally and antisymmetrically correlated in time may exist in a half-metallic ferromagnet. As a consequence, the half-metal acts as an odd-frequency superconducting condensate. We demonstrate both analytically and numerically that quantum vortices can emerge in half-metals despite the complete absence of conventional superconducting correlations. Because these metals are conducting in only one spin band, we show that a circulating spin supercurrent accompanies these vortices. Moreover, we demonstrate that magnetic disorder at the interfaces with the superconductor influences the position at which the vortices nucleate. This insight can be used to help determine the effective interfacial misalignment angles for the magnetization in hybrid structures, since the vortex position is experimentally observable via STM-measurements. We also give a brief discussion regarding which superconducting order parameter to use for odd-frequency triplet Cooper pairs in the quasiclassical theory.

cond-mat.supr-con↗

A consistent reduction of the two-layer shallow-water equations to an accurate one-layer spreading model

The gravity-driven spreading of one fluid in contact with another fluid is of key importance to a range of topics. To describe these phenomena, the two-layer shallow-water equations is commonly employed. When one layer is significantly deeper than the other, it is common to approximate the system with the much simpler one-layer shallow water equations. So far, it has been assumed that this approximation is invalid near shocks, and one has applied additional front conditions for the shock speed. In this paper, we prove mathematically that an effective one-layer model can be derived from the two-layer equations that correctly captures the behaviour of shocks and contact discontinuities without any additional closure relations. The proof yields a novel formulation of an effective one-layer shallow water model. The result shows that simplification to an effective one-layer model is well justified mathematically and can be made without additional knowledge of the shock behaviour. The shock speed in the proposed model is consistent with empirical models and identical to the front conditions that have been found theoretically by e.g. von Kármán and by Benjamin. This suggests that the breakdown of the shallow-water equations in the vicinity of shocks is less severe than previously thought. We further investigate the applicability of the shallow water framework to shocks by studying shocks in one-dimensional lock-exchange/lock-release. We derive expressions for the Froude number that are in good agreement with the widely employed expression by Benjamin. We then solve the equations numerically to illustrate how quickly the proposed model converges to solutions of the full two-layer shallow-water equations. We also compare numerical results using our model with results from dam break experiments. Predictions from the one-layer model are found to be in good agreement with experiments.

physics.flu-dyn↗