arXiv subjects

Eliezer Estrecho

Publications and source records attributed to Eliezer Estrecho.

At least 19 recordsLinked to original sources

arXiv2026

Dynamical development of long-range spatial coherence in non-equilibrium bosonic condensation

Development of spontaneous coherence is one of the hallmarks of bosonic condensation in a variety of physical systems, such as cold atoms, confined photons, and hybrid light-matter quasiparticles like exciton polaritons in semiconductors. While spatial coherence is well understood once a steady-state condensate has been established, its temporal evolution as the condensate forms is largely unexplored. Here, we explore the dynamical formation of a non-equilibrium, driven-dissipative exciton-polariton condensate through both time-resolved experiments and numerical modeling. Our study reveals that the spatial coherence is established through two distinct stages. The early-time stage is interaction-driven and features transient oscillations in spatial coherence. This stage is followed by a steady-state regime characterized by a spatially-uniform high degree of coherence that extends over the entire size of the system and persists over time. These stages of spatial coherence development occur in both free flowing and confined exciton-polariton systems that undergo a quench - rapid growth of the condensate starting from two different initial settings. Our study offers a deep insight into the process by which long-range spatial coherence is established in a non-equilibrium bosonic condensate.

cond-mat.quant-gas↗

arXiv2025

Momentum-space non-Hermitian skin effect in an exciton-polariton system

Localization of a macroscopic number of eigenstates on a real-space boundary, known as the non-Hermitian skin effect, is one of the striking topological features emerging from non-Hermiticity. Realizing this effect typically requires periodic (lattice) systems with asymmetry of intersite coupling, which is not readily available in many physical platforms. Instead, it is meticulously engineered, e.g., in photonics, which results in complex structures requiring precise fabrication steps. Here, we propose a simpler mechanism: introducing an asymmetric, purely imaginary potential in a topologically trivial system induces momentum-space localization akin to the skin effect. We experimentally demonstrate this localization using exciton polaritons, hybrid light-matter quasi-particles in a simple engineered `round box' trap, pumped by a laser pump offset from the trap center. The effect disappears if the pump is concentric with the trap. The localization persists and becomes stronger at higher densities of polaritons, when a non-equilibrium Bose-Einstein condensate is formed and the system becomes nonlinear. Our approach offers a new route to realizing skin effects in continuous, non-periodic systems and exploring the interplay of non-Hermiticity, topology, and nonlinearity in macroscopic quantum states.

physics.optics↗

arXiv2025

Intrinsically chiral exciton polaritons in an atomically-thin semiconductor

Photonic bound states in the continuum (BICs) have emerged as a versatile tool for enhancing light-matter interactions by strongly confining light fields. Chiral BICs are photonic resonances with a high degree of circular polarisation, which hold great promise for spin-selective applications in quantum optics and nanophotonics. Here, we demonstrate a novel application of a chiral BIC for inducing strong coupling between the circularly polarised photons and spin-polarised (valley) excitons (bound electron-hole pairs) in atomically-thin transition metal dichalcogenide crystals (TMDCs). By placing monolayer WS$_2$ onto the BIC-hosting metasurface, we observe the formation of intrinsically chiral, valley-selective exciton polaritons, evidenced by circularly polarised photoluminescence (PL) at two distinct energy levels. The PL intensity and degree of circular polarisation of polaritons exceed those of uncoupled excitons in our structure by an order of magnitude. Our microscopic model shows that this enhancement is due to folding of the Brillouin zone creating a direct emission path for high-momenta polaritonic states far outside the light cone, thereby providing a shortcut to thermalisation (energy relaxation) and suppressing depolarisation. Moreover, while the polarisation of the upper polariton is determined by the valley excitons, the lower polariton behaves like an intrinsic chiral emitter with its polarisation fixed by the BIC. Therefore, the spin alignment of the upper and lower polaritons ($\uparrow\downarrow$ and $\uparrow \uparrow$) can be controlled by $σ^+$ and $σ^-$ polarised optical excitation, respectively. Our work introduces a new type of chiral light-matter quasi-particles in atomically-thin semiconductors and provides an insight into their energy relaxation dynamics.

cond-mat.mes-hall↗

arXiv2025

Zitterbewegung Effect and Quantum Geometry in Non-Hermitian Exciton-Polariton Systems

In this work, we analytically derive a semi-classical equation of motion describing the zitterbewegung effects arising in the dynamics of wavepackets in non-Hermitian systems. In Hermitian non-relativistic quantum systems, the zitterbewegung effects can arise due to the spin precession and spin-orbit coupling. Interestingly, the spin dynamics in non-Hermitian systems are qualitatively different because of the effective nonlinear terms induced by the non-Hermitian part of the Hamiltonian. In this work, we show the effects from the non-Hermitian spin dynamics by generalising the description of zitterbewegung effects to non-Hermitian systems. We also uncover novel non-Hermitian correction to the group velocity, which can be expressed in terms of the non-Hermitian quantum metric tensor in the absence of out-of-plane effective field.

quant-ph↗

arXiv2025

Emergent momentum-space topological pseudospin defects in non-Hermitian systems

Topological defects are central to modern physics, from spintronics to photonics, due to their robustness and potential application in information processing. In this work, we discuss topological point defects that spontaneously emerge at the imaginary Fermi arcs (degeneracy lines) in momentum space of two-dimensional systems described by non-Hermitian effective Hamiltonians. In particular, we consider a generic non-Hermitian Dirac model and a phenomenological model describing hybrid light-matter quasiparticles - exciton polaritons hosted in an optical microcavity. In both cases, the eigenenergies of the system have both real and imaginary parts and form two distinct bands corresponding to two (pseudo-)spin states. We describe the trajectories of the point defects characterized by integer-valued topological winding (vorticity) analytically and show that the defects with opposite vorticity annihilate with each other in the fully gapped phases, but are protected from annihilation by the non-Hermitian spectral degeneracies (exceptional and hybrid points) in the gapless phases. We also suggest that the signatures of these defects can be experimentally measured in an exciton-polariton system.

cond-mat.mes-hall↗

arXiv2025

Quantum geometric tensor and wavepacket dynamics in two-dimensional non-Hermitian systems

The quantum geometric tensor (QGT) characterizes the local geometry of quantum states, and its components directly account for the dynamical effects observed, e.g., in condensed matter systems. In this work, we address the problem of extending the QGT formalism to non-Hermitian systems with gain and loss. In particular, we investigate a wave-packet dynamics in two-band non-Hermitian systems to elucidate how non-Hermiticity affects the definition of QGT. We employ first-order perturbation theory to account for non-adiabatic corrections due to interband mixing. Our results suggest that two different generalizations of the QGT, one defined using only the right eigenstates and the other one using both the left and right eigenstates, both play a significant role in wave-packet dynamics. We then determine the accuracy of the perturbative approach by simulating a wave-packet dynamics in a well studied physical non-Hermitian system -- exciton polaritons in a semiconductor microcavity. Our work aids deeper understanding of quantum geometry and dynamical behaviour in non-Hermitian systems.

cond-mat.mes-hall↗

arXiv2024

Robust Room-Temperature Polariton Condensation and Lasing in Scalable FAPbBr$_3$ Perovskite Microcavities

Exciton-polariton condensation in direct bandgap semiconductors strongly coupled to light enables a broad range of fundamental studies and applications like low-threshold and electrically driven lasing. Yet, materials hosting exciton-polariton condensation in ambient conditions are rare, with fabrication protocols that are often inefficient and non-scalable. Here, room-temperature exciton-polariton condensation and lasing is observed in a microcavity with embedded formamidiniumlead bromide (FAPbBr$_3$) perovskite film. This optically active material is spin-coated onto the microcavity mirror, which makes the whole device scalable up to large lateral sizes. The sub-$μ$m granulation of the polycrystalline FAPbBr$_3$ film allows for observation of polariton lasing in a single quantum-confined mode of a polaritonic 'quantum dot'. Compared to random photon lasing, observed in bare FAPbBr$_3$ films, polariton lasing exhibits a lower threshold, narrower linewidth, and an order of magnitude longer coherence time. Both polariton and random photon lasing are observed under the conditions of pulsed optical pumping, and persist without significant degradation for up to 6 and 17 hours of a continuous experimental run, respectively. This study demonstrates the excellent potential of the FAPbBr$_3$ perovskite as a new material for room-temperature polaritonics, with the added value of efficient and scalable fabrication offered by the solution-based spin-coating process.

cond-mat.mes-hall↗

arXiv2024

Narrow-linewidth exciton-polariton laser

Exciton-polariton laser is a promising source of coherent light for low-energy applications due to its low-threshold operation. However, a detailed experimental study of its spectral purity, which directly affects its coherence properties is still missing. Here}, we present a high-resolution spectroscopic investigation of the energy and linewidth of an exciton-polariton laser in the single-mode regime, which derives its coherent emission from an optically pumped and confined exciton-polariton condensate. We report an ultra-narrow linewidth of 56~MHz or 0.24~$μ$eV, corresponding to a coherence time of 5.7~ns. The narrow linewidth is consistently achieved by using an exciton-polariton condensate with a high photonic content confined in an optically induced trap. Contrary to previous studies, we show that the excitonic reservoir created by the pump and responsible for creating the trap does not strongly affect the emission linewidth as long as the condensate is trapped and the pump power is well above the condensation (lasing) threshold. \red{The long coherence time of the exciton-polariton system uncovered here opens up opportunities for manipulating its macroscopic quantum state, which is essential for applications in classical and quantum computing.

physics.optics↗

arXiv2024

Generalized Quantum Geometric Tensor in a Non-Hermitian Exciton-Polariton System

In this work, we review different generalizations of the quantum geometric tensor (QGT) in two-band non-Hermitian systems and propose a protocol for measuring them in experiments. We present the generalized QGT components, i.e. the quantum metric and Berry curvature, for a non-Hermitian hybrid photonic (exciton-polariton) system and show that the generalized non-Hermitian QGT can be constructed from experimental observables. In particular, we extend the existing method of measuring the QGT that uses the pseudospins in photonic and exciton-polariton systems by suggesting a method to construct the left eigenstates from experiments. We also show that the QGT components have clear signatures in wave-packet dynamics, where the anomalous Hall drift arises from both the non-Hermitian Berry curvature and Berry connection, suggesting that both left and right eigenstates are necessary for defining non-Hermitian band geometries and topologies.

cond-mat.mes-hall↗

arXiv2022

Wave packet dynamics in a non-Hermitian exciton-polariton system

We theoretically investigate the dynamics of wave packets in a generic, non-Hermitian, optically anisotropic exciton-polariton system that exhibits degeneracies of its complex-valued eigenenergies in the form of pairs of exceptional points in momentum space. We observe the self-acceleration and reshaping of the wave packets governed by their eigenenergies. We further find that the exciton-polariton wave packets tend to self-organize into the eigenstate with the smaller decay rate, then propagate towards the minima of the decay rates in momentum space, resulting in directional transport in real space. We also describe the formation of pseudospin topological defects on the imaginary Fermi arc, where the decay rates of the two eigenstate coincide in momentum space. These effects of non-Hermiticity on the dynamics of exciton polaritons can be observed experimentally in a microcavity with optically anisotropic cavity spacer or exciton-hosting materials.

cond-mat.mes-hall↗

arXiv2022

Fabrication of high-quality PMMA/SiO$_x$ spaced planar microcavities for strong coupling of light with monolayer WS$_2$ excitons

Exciton polaritons in atomically-thin transition metal dichalcogenide crystals (monolayer TMDCs) have emerged as a promising candidate to enable topological transport, ultra-efficient laser technologies, and collective quantum phenomena such as polariton condensation and superfluidity at room temperature. However, integrating monolayer TMDCs into high-quality planar microcavities to achieve the required strong coupling between the cavity photons and the TMDC excitons (bound electron-hole pairs) has proven challenging. Previous approaches to integration had to compromise between various adverse effects on the strength of light-matter interactions in the monolayer, the cavity photon lifetime, and the lateral size of the microcavity. Here, we demonstrate a scalable approach to fabricating high-quality planar microcavities with an integrated monolayer WS$_2$ layer-by-layer by using polymethyl methacrylate/silicon oxide (PMMA/SiO$_x$) as a cavity spacer. Because the exciton oscillator strength is well protected against the required processing steps by the PMMA layer, the microcavities investigated in this work, which have quality factors of above $10^3$, can operate in the strong light-matter coupling regime at room temperature. This is an important step towards fabricating wafer-scale and patterned microcavities for engineering the exciton-polariton potential landscape, which is essential for enabling many proposed technologies.

cond-mat.mtrl-sci↗

arXiv2022

Bogoliubov excitations of a polariton condensate in dynamical equilibrium with an incoherent reservoir

The classic Bogoliubov theory of weakly interacting Bose gases rests upon the assumption that nearly all the bosons condense into the lowest quantum state at sufficiently low temperatures. Here we develop a generalized version of Bogoliubov theory for the case of a driven-dissipative exciton-polariton condensate with a large incoherent uncondensed component, or excitonic reservoir. We argue that such a reservoir can consist of both excitonic high-momentum polaritons and optically dark superpositions of excitons across different optically active layers, such as multiple quantum wells in a microcavity. In particular, we predict interconversion between the dark and bright (light-coupled) excitonic states that can lead to a dynamical equilibrium between the condensate and reservoir populations. We show that the presence of the reservoir fundamentally modifies both the energy and the amplitudes of the Bogoliubov quasiparticle excitations due to the non-Galilean-invariant nature of polaritons. Our theoretical findings are supported by our experiment, where we directly detect the Bogoliubov excitation branches of an optically trapped polariton condensate in the high-density regime. By analyzing the measured occupations of the excitation branches, we extract the Bogoliubov amplitudes across a range of momenta and show that they agree with our generalized theory.

cond-mat.quant-gas↗

arXiv2022

Exciton-polaron interactions in monolayer WS$_2$

Interactions between quasiparticles are of fundamental importance and ultimately determine the macroscopic properties of quantum matter. A famous example is the phenomenon of superconductivity, which arises from attractive electron-electron interactions that are mediated by phonons or even other more exotic fluctuations in the material. Here we introduce mobile exciton impurities into a two-dimensional electron gas and investigate the interactions between the resulting Fermi polaron quasiparticles. We employ multi-dimensional coherent spectroscopy on monolayer WS$_2$, which provides an ideal platform for determining the nature of polaron-polaron interactions due to the underlying trion fine structure and the valley specific optical selection rules. At low electron doping densities, we find that the dominant interactions are between polaron states that are dressed by the same Fermi sea. In the absence of bound polaron pairs (bipolarons), we show using a minimal microscopic model that these interactions originate from a phase-space filling effect, where excitons compete for the same electrons. We furthermore reveal the existence of a bipolaron bound state with remarkably large binding energy, involving excitons in different valleys cooperatively bound to the same electron. Our work lays the foundation for probing and understanding strong electron correlation effects in two-dimensional layered structures such as moiré superlattices.

cond-mat.mes-hall↗

arXiv2021

Direct Measurement of a Non-Hermitian Topological Invariant in a Hybrid Light-Matter System

Topology is central to understanding and engineering materials that display robust physical phenomena immune to imperfections. Different topological phases of matter are characterised by topological invariants. In energy-conserving (Hermitian) systems, these invariants are determined by the winding of eigenstates in momentum space. In non-Hermitian systems, a novel topological invariant is predicted to emerge from the winding of the complex eigenenergies. Here, we directly measure the non-Hermitian topological invariant arising from exceptional points in the momentum-resolved spectrum of exciton polaritons. These are hybrid light-matter quasiparticles formed by photons strongly coupled to electron-hole pairs (excitons) in a halide perovskite semiconductor at room temperature. We experimentally map out both the real (energy) and imaginary (linewidth) parts of the spectrum near the exceptional points and extract the novel topological invariant - fractional spectral winding. Our work represents an essential step towards realisation of non-Hermitian topological phases in a condensed matter system.

physics.optics↗

arXiv2021

Influence of direct deposition of dielectric materials on the optical response of monolayer WS$_2$

The integration of two-dimensional transition metal dichalcogenide crystals (TMDCs) into a dielectric environment is critical for optoelectronic and photonic device applications. Here, we investigate the effects of direct deposition of different dielectric materials (Al$_2$O$_3$, SiO$_2$, SiN$_x$) onto atomically thin (monolayer) TMDC WS$_2$ on its optical response. Atomic layer deposition (ALD), electron beam evaporation (EBE), plasma enhanced chemical vapour deposition (PECVD), and magnetron sputtering methods of material deposition are investigated. The photoluminescence (PL) measurements reveal quenching of the excitonic emission after all deposition processes. The reduction in neutral exciton PL is linked to the increased level of charge doping and associated rise of the trion emission, and/or the localized (bound) exciton emission. Furthermore, Raman spectroscopy allows us to clearly correlate the observed changes of excitonic emission with the increased levels of lattice disorder and defects. Overall, the EBE process results in the lowest level of doping and defect densities and preserves the spectral weight of the exciton emission in the PL, as well as the exciton oscillator strength. Encapsulation with ALD appears to cause chemical changes, which makes it distinct from all other techniques. Sputtering is revealed as the most aggressive deposition method for WS$_2$, fully quenching its optical response. Our results demonstrate and quantify the effects of direct deposition of dielectric materials onto monolayer WS$_2$, which can provide a valuable guidance for the efforts to integrate monolayer TMDCs into functional optoelectronic devices.

cond-mat.mtrl-sci↗

arXiv2020

Long-lived populations of momentum- and spin-indirect excitons in monolayer WSe$_2$

Monolayer transition metal dichalcogenides are a promising platform to investigate many-body interactions of excitonic complexes. In monolayer tungsten diselenide, the ground-state exciton is dark (spin-indirect), and the valley degeneracy allows low-energy dark momentum-indirect excitons to form. Interactions between the dark exciton species and the optically accessible bright exciton (X) are likely to play significant roles in determining the optical properties of X at high power, as well as limiting the ultimate exciton densities that can be achieved, yet so far little is known about these interactions. Here, we demonstrate long-lived dense populations of momentum-indirect intervalley ($X_K$) and spin-indirect intravalley (D) dark excitons by time-resolved photoluminescence measurements (Tr-PL). Our results uncover an efficient inter-state conversion between X to D excitons through the spin-flip process and the one between D and $X_K$ excitons mediated by the exchange interaction (D + D to $X_K$ + $X_K$). Moreover, we observe a persistent redshift of the X exciton due to strong excitonic screening by $X_K$ exciton with a response time in the timescale of sub-ns, revealing a non-trivial inter-state exciton-exciton interaction. Our results provide a new insight into the interaction between bright and dark excitons, and point to a possibility to employ dark excitons for investigating exciton condensation and the valleytronics.

cond-mat.mes-hall↗

arXiv2020

Two-dimensional Ga$_2$O$_3$ glass: a large scale passivation and protection material for monolayer WS$_2$

Atomically thin transition metal dichalcogenide crystals (TMDCs) have extraordinary optical properties that make them attractive for future optoelectronic applications. Integration of TMDCs into practical all-dielectric heterostructures hinges on the ability to passivate and protect them against necessary fabrication steps on large scales. Despite its limited scalability, encapsulation of TMDCs in hexagonal boron nitride (hBN) currently has no viable alternative for achieving high performance of the final device. Here, we show that the novel, ultrathin Ga$_2$O$_3$ glass is an ideal centimeter-scale coating material that enhances optical performance of the monolayers and protects them against further material deposition. In particular, Ga$_2$O$_3$ capping of commercial grade WS$_2$ monolayers outperforms hBN in both scalability and optical performance at room temperature. These properties make Ga$_2$O$_3$ highly suitable for large scale passivation and protection of monolayer TMDCs in functional heterostructures.

cond-mat.mtrl-sci↗

arXiv2019

Observation of quantum depletion in a nonequilibrium exciton-polariton condensate

The property of superfluidity, first discovered in liquid 4He, is closely related to Bose-Einstein condensation (BEC) of interacting bosons. However, even at zero temperature, when one would expect the whole bosonic quantum liquid to become condensed, a fraction of it is excited into higher momentum states via interparticle interactions and quantum fluctuations -- the phenomenon of quantum depletion. Quantum depletion of weakly interacting atomic BECs in thermal equilibrium is well understood theoretically but is difficult to measure. This is even more challenging in driven-dissipative systems such as exciton-polariton condensates(photons coupled to electron-hole pairs in a semiconductor), since their nonequilibrium nature is predicted to suppress quantum depletion. Here, we observe quantum depletion of an optically trapped high-density exciton-polariton condensate by directly detecting the spectral branch of elementary excitations populated by this process. Analysis of the population of this branch in momentum space shows that quantum depletion of an exciton-polariton condensate can closely follow or strongly deviate from the equilibrium Bogoliubov theory, depending on the fraction of matter (exciton) in an exciton-polariton. Our results reveal the effects of exciton-polariton interactions beyond the mean-field description and call for a deeper understanding of the relationship between equilibrium and nonequilibrium BECs.

cond-mat.quant-gas↗