SearcharxivSearch

arXiv subjects

Elizabeth Krenkel

Publications and source records attributed to Elizabeth Krenkel.

3 recordsLinked to original sources

Resistive Switching and Neuromorphic Computing in Metal/Nb:SrTiO$_3$: Mechanisms, Interface Physics, and Charge Transport

Resistive switching (RS) in Nb-doped SrTiO$_3$ (Nb:STO) based memristive devices has attracted sustained interest in information processing and novel computing because of its forming-free operation, large on/off ratio, and gradual conductance modulation. Metal/Nb:STO Schottky junctions have emerged as a prototypical system for understanding RS mechanisms. Despite more than two decades of research, the physical origin of RS remains controversial, with proposed mechanisms including charge trapping and detrapping, oxygen vacancy migration, tunneling, interfacial redox reactions, and conductive filament formation. In this review, we examine these seemingly competing mechanisms and show that many experimental observations can be understood within a unified framework centered on the formation and evolution of an extrinsic interfacial layer at the metal/Nb:STO interface. We discuss how interface quality and defect-mediated processes, including proton incorporation, oxygen vacancy dynamics, and tunneling, govern Schottky barrier modulation and RS behavior. We further summarize how fabrication conditions, measurement protocols, and aging influence the interface formation and switching characteristics. This review establishes an integrated picture of M/Nb:STO heterojunctions and provides design principles for reliable oxide memristive devices through interface and defect engineering in M/Nb:STO and M/oxide/Nb:STO systems.

cond-mat.mtrl-sci

High-field-stabilized reentrant superconductivity in infinite-layer nickelate thin films

Magnetic fields typically suppress superconductivity through Pauli and orbital limiting effects. However, there are rare instances of magnetic-field-induced superconductivity, as seen in Chevrel phase compounds [1], organic conductors [2], uranium-based heavy-fermion systems [3, 4], and moire graphene [5], though these materials possess inherently low superconducting transition temperatures (Tc). Here, we demonstrate high field-stabilized superconductivity in a class of materials with a significantly higher Tc (up to 40 K): the infinite-layer nickelates [6]. Both low-field and high-field superconducting states can be plausibly explained by a compensation mechanism akin to the Jaccarino-Peter effect. These findings demonstrate the possibility of achieving substantially enhanced upper critical fields in high-temperature superconductors.

cond-mat.supr-con

Magnetic properties of double perovskite $Ln_2$CoIrO$_6$ ($Ln$ = Eu, Tb, Ho): hetero-tri-spin $3d$-$5d$-$4f$ systems

The field of double perovskites is now advancing to three magnetic elements on the A, B and B$'$ sites. A series of iridium-based double perovskite compounds, $Ln_2$CoIrO$_6$ ($Ln$ = Eu, Tb, Ho) with three magnetic elements were synthesized as polycrystalline samples. The compounds crystalize in monoclinic structures with the space group $P2_1/n$. Magnetic properties of these hetero-tri-spin $3d$-$5d$-$4f$ systems were studied by magnetic susceptibility and field dependent magnetization in both DC and pulsed magnetic fields. All these compounds show ferrimagnetic transitions at temperatures $T_C$ above 100 K, which are attributable to antiferromagnetic coupling between Co$^{2+}$ and Ir$^{4+}$ spins. For Eu$_2$CoIrO$_6$, the magnetic properties are similar to those of La$_2$CoIrO$_6$. The Eu$^{3+}$ spins show Van Vleck paramagnetism that don't significantly interact with transition-metal cations. By contrast, Tb$_2$CoIrO$_6$ and Ho$_2$CoIrO$_6$ reveal a second transition to antiferromagnetic order below a lower temperature $T_N$. The temperature-induced ferrimagnetic-to-antiferromagnetic phase transition might be explained by a spin-reorientation transition. Moreover, a magnetic-field-induced spin-flop transition with a small hysteresis was observed below $T_N$ in these two compounds. The magnetic moment of all three compounds do not saturate up to 60 T at low temperatures. Moderate magnetocaloric effect was also observed in all three compounds. Our results should motivate further investigation of the spin configuration on single crystals of these iridium-based double perovskites.

cond-mat.mtrl-sci