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Elodie Strupiechonski

Publications and source records attributed to Elodie Strupiechonski.

3 recordsLinked to original sources

Terahertz cavity hybridization of collective proteins vibrations

Hybrid light-matter states have transformed photonics, yet their realization with driven collective vibrations in biological systems remains an open challenge. Here we show that optically pumped R-phycoerythrin proteins at room temperature support coherent sub-terahertz vibrational modes consistent with Frohlich condensation, and that these modes hybridize with confined terahertz cavity photons in a microfluidic cavity platform. The resulting spectra exhibit a resolved doublet, power- and concentration-dependent redistribution of spectral weight, and linewidth narrowing indicative of cavity-modified dissipation. Quantitative analysis reveals collective square-root of N-scaling of the coupling strength, with cooperativity and splitting-to-linewidth ratios exceeding unity, consistent with the onset of strong collective coupling driven by the vibrational molecular mode. A microscopic nonequilibrium analysis further indicates that the relaxation timescale toward the Frohlich polariton state is on the order of 1-10 microseconds. These findings identify terahertz cavities as a platform for stabilizing and controlling collective molecular vibration dynamics and open opportunities for cavity-engineered vibrational spectroscopy, label-free biosensing and photonic control of energy transport in complex biomolecular systems.

cond-mat.other

Gate-tunable emission of exciton-plasmon polaritons in hybrid MoS2-gap-mode metasurfaces

The advance in designing arrays of ultrathin two-dimensional optical nano-resonators, known as metasurfaces, is currently enabling a large variety of novel flat optical components. The remarkable control over the electromagnetic fields offered by this technology can be further extended to the active regime in order to manipulate the light characteristics in real-time. In this contribution, we couple the excitonic resonance of atomic thin MoS2 monolayers with gap-surface-plasmon (GSP) metasurfaces, and demonstrate selective enhancement of the exciton-plasmon polariton emissions. We further demonstrate tunable emissions by controlling the charge density at interface through electrically gating in MOS structure. Straddling two very active fields of research, this demonstration of electrically tunable light-emitting metasurfaces enables real-time manipulation of light-matter interactions at the extreme subwavelength dimensions.

physics.optics

Hybrid MoS$_2$-gap-mode metasurfaces photodetectors

Two-dimensional molybdenum disulfide (MoS$_2$) featuring atomically thin thickness and unique electronic structure with favorable bandgap has been widely recognized as an attractive new material for the development of the next generation of ultra-compact, light-weight optoelectronic components. In parallel, the recently emerged metasurfaces have demonstrated exceptional controllability over electromagnetic field within ultra-compact subwavelength dimension offering an unprecedented approach to improve the performance of optoelectronic devices. In this work, we are proposing an integration of metasurfaces with 2D semiconductor materials to achieve polarization sensitive, fast-response photodetectors. The reported devices are among the most compact hybrid MoS2-gap-plasmon metasurface detectors. Relying on the significant electromagnetic field confinement provided by the metasurfaces to enhance light absorption and to reduce the surface states, which generally limit the photo-generated carriers lifetime, we measured enhanced photocurrent and a fast detection speed. Moreover, the strong optical anisotropy introduced by the metasurfaces is used to efficiently control the polarization sensitivity of the photodetector. This work provides a feasible and effective solution to improve the performance of two-dimensional materials based photodetectors.

physics.app-ph