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Elyas Mattivi

Publications and source records attributed to Elyas Mattivi.

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Strategies for implementing quantum error correction in molecular rotation

The rotation of trapped molecules offers a promising platform for quantum technologies and quantum information processing. In parallel, quantum error correction codes that can protect quantum information encoded in rotational states of a single molecule have been developed. These codes are currently an abstract concept, as no implementation strategy is yet known. Here, we present a step towards experimental implementation of one family of such codes, namely absorption-emission codes. We first construct architecture-agnostic check and correction operators. These operators are then decomposed into elements of the quantum logic spectroscopy toolbox that is available for molecular ions. We then describe and analyze a measurement-based sequential as well as an autonomous implementation strategy in the presence of thermal background radiation, a major noise source for rotation in polar molecules. The presented strategies and methods might enable robust sensing or even fault-tolerant quantum computing using the rotation of individual molecules.

quant-ph

Photodissociation spectra of single trapped CaOH+ molecular ions

Molecular ions that are generated by chemical reactions with trapped atomic ions can serve as an accessible testbed for developing molecular quantum technologies. On the other hand, they are also a hindrance to scaling up quantum computers based on atomic ions as unavoidable reactions with background gas destroy the information carriers. Here, we investigate the single- and two-photon dissociation processes of single $\text{CaOH}^+$ molecular ions co-trapped in $\text{Ca}^+$ ion crystals using a femtosecond laser system. We report the photodissociation cross section spectra of $\text{CaOH}^+$ for single-photon processes at $λ=$245 - 275$\,$nm and for two-photon processes at $λ=$500 - 540$\,$nm. Measurements are interpreted with quantum-chemical calculations, which predict the photodissociation threshold for $\text{CaOH}^+\to \text{Ca}^++\text{OH}$ at 265$\,$nm. This result can serve as a basis for dissociation-based spectroscopy for studying the internal structure of $\text{CaOH}^+$. The result also gives a prescription for recycling $\text{Ca}^+$ ions in large-scale trapped $\text{Ca}^+$ quantum experiments from undesired $\text{CaOH}^+$ ions formed in the presence of background water vapor.

physics.atom-ph