arXiv subjects

Emanuel Chimanski

Publications and source records attributed to Emanuel Chimanski.

8 recordsLinked to original sources

arXiv2026

Fast-reactor neutron sources in evaluated nuclear data library validation

Two different neutron sources, based on $^{235}$U-fission neutrons with different average energies, provide integral benchmark data for validation of $\gamma$-ray production data in the evaluated nuclear data libraries corresponding to fast-neutron-induced inelastic-neutron scattering reactions. Firstly, we consider the IRT-M Research Reactor, formerly located at the Nuclear Research Institute just outside of Baghdad, Iraq, to demonstrate the validation methodology using the associated $\gamma$-ray data in the Evaluated Nuclear Data File, version VIII.0 (ENDF/B-VIII.0), for several $\gamma$-ray transitions over a wide range of nuclides including $^{28}$Si, $^{32}$S, $^{56}$Fe, and $^{186}$W. Using the characterized neutron flux of the Baghdad IRT-M Reactor, we find flux-weighted cross-sections deduced using the ENDF/B-VIII.0 $\gamma$-ray data to be in good agreement with the integral measurements performed at the Baghdad Research Reactor in addition to the corresponding results of different reaction-model calculations, {\tt CoH$_{3}$} and {\tt EMPIRE}. Given the excitation thresholds for the $\gamma$-ray transitions involved in this investigation, these observations lend further support to the characterization of the IRT-M flux in the fast-neutron energy region $0.862 \leq E_{n} \leq 5.0$ MeV. The additional detail devoted to the IRT-M source reflects the broader scope of the validation work carried out at that facility. A second neutron source considered for this validation work is the Forschungsreaktor M{\"u}nich (FRM-II), Garching, Germany. Again, the flux-weighted $\gamma$-ray data from ENDF/B-VIII.0 for $^{56}$Fe compare well to the integral FRM-II measurement and reaction-model calculations.

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arXiv2026

Precision cross section measurements of neutron-induced non-elastic gamma production reactions at 14 MeV

We present a technique for high-precision absolute measurements of gamma-ray production cross sections (n,xg) induced by 14 MeV neutrons. The technique is based on the Associated Particle Imaging (API) method, which tags individual neutrons emitted from a deuterium-tritium source with their associated alpha-particles, enabling coincidence-based suppression of lower-energy neutrons and room background signals, while also providing neutron flux measurements with uncertainties on the order of 1%. This compact, laboratory-scale technique has the potential to address gaps and discrepancies in existing cross section libraries at a fraction of the cost of large-scale dedicated facilities, with direct applications in active neutron interrogation, detector calibration, nuclear fusion science, and Monte Carlo simulations, among others. We demonstrate the technique through proof-of-concept experiments on thin and thick samples of natural Fe (1 mm, 8 mm) and natural C (2 mm, 10 mm). For Fe, gamma-ray production cross sections were measured for the 846.78 and 1238.33 keV transitions from the first and second excited states of 56Fe. For C, the (n,n'g) cross section was measured for the 4438.91 keV transition from the first excited state of 12C. Measurements were performed at 110 and 48 degrees relative to the neutron beam to characterize gamma-ray anisotropy. For the thin samples, the measured cross sections are 723 +/- 70 mb (56Fe, 846.78 keV, 110 deg), 303 +/- 42 mb (56Fe, 1238.33 keV, 110 deg), 755 +/- 106 mb (56Fe, 846.78 keV, 48 deg), 321 +/- 149 mb (56Fe, 1238.33 keV, 48 deg), 141 +/- 16 mb (12C, 4438.91 keV, 110 deg), and 279 +/- 105 mb (12C, 4438.91 keV, 48 deg). Uncertainties are dominated by counting statistics and detector efficiency calibration, both of which can be reduced in future experiments to achieve overall uncertainties of 5% or better.

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arXiv2026

Nuclear Reaction Data for Fission Products Off Stability

Neutron cross sections on fission products are relevant to a wide range of applications, including nuclear nonproliferation and forensics, spent-fuel assay, reactor burnup and design, as well as astrophysics. Evaluated nuclear data libraries generally fulfill application needs for isotopes on or near stability, however, for unstable fission products, theoretical descriptions of neutron-induced reactions often constitute the only available source of information. These models often make use of simplified assumptions, leading to unquantified impacts on predicted cross sections. In this work, we discuss possible approaches to addressing these issues, particularly by leveraging machine-learning methods, improved predictive reaction modeling, and experimental data to better constrain model parameters. Our goal is to eventually produce evaluated files for the most-produced nuclei off stability in the fission process of $^{235}$U and submit them to the ENDF/B for consideration in the future ENDF/B-IX.0 release. Here we present the methodology and discuss preliminary results comparing usual simplified approaches with a more realistic one accounting for nuclear deformation.

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arXiv2025

Constraining capture cross sections using proton inelastic scattering as a surrogate reaction

The surrogate reaction method is an alternative to direct measurements of compound nuclear reaction cross sections. We introduce theory tools for extracting capture cross sections from experiments that use proton inelastic scattering as a surrogate reaction mechanism. This makes it possible to constrain compound nucleus decay models which are typically the largest source of uncertainty in capture cross section calculations. This letter describes the theory developments that were used to simultaneously infer $^{89}$Y$(p,\gamma)$ and $^{89}$Zr$(n,\gamma)$ cross sections from $^{90}$Zr$(p,p'\gamma)$ surrogate measurements.

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arXiv2025

Uncovering the nature of low-lying dipole states with QRPA calculations: is Z=42 the answer?

The pygmy dipole resonance (PDR), marked by enhanced electric dipole strength near particle emission energies, offers a unique perspective on the collective dynamics of nuclear structure. Its precise nature, particularly its degree of collectivity, remains a topic of debate. In this study, we investigate low-energy dipole excitations in spherical Mo isotopes ($^{82}$Mo to $^{98}$Mo) using a fully consistent Hartree-Fock-Bogoliubov (HFB) and quasiparticle random phase approximation (QRPA) framework. We observe that an enhancement in dipole strength near particle emission energies is closely correlated with the development of either neutron or proton skins. To further understand the nature of this enhancement, we examine the behavior of proton and neutron transition densities. Our analysis shows that these (low-lying dipole) states exhibit distinct characteristics involving in-phase oscillations within the nucleus and neutron- or proton-dominated oscillations at the surface, while the primary contributor to this enhancement displays an intricate underlying structure. We also investigate the collectivity of these excitations by analyzing two-quasiparticle fragmentations and relative energy shifts. Our findings reveal that skin oscillation states exhibit moderate collectivity, as indicated by substantial configuration mixing, but limited coherence, whereas the GDR states exhibit strong coherence and large energy shifts characteristic of fully developed collective motion. This study paves the way for future investigations into the collective nature of low-energy dipole states in the enhancement region, particularly in deformed nuclei, where nuclear shape effects may play a crucial role in their excitation dynamics.

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arXiv2025

Electric dipole excitations near the neutron separation energies in $^{96}$Mo

Electric dipole strength near the neutron separation energy significantly impacts nuclear structure properties and astrophysical scenarios. These excitations are complex in nature and may involve the so-called pygmy dipole resonance (PDR). Transition densities play a crucial role in understanding the nature of nuclear excited states, including collective excitations, as well as in constructing transition potentials in DWBA or coupled-channels equations. In this work, we focus on electric dipole excitations in spherical molybdenum isotopes, particularly $^{96}$Mo, employing fully consistent Hartree-Fock-Bogoliubov (HFB) and Quasiparticle Random Phase Approximation (QRPA) methods. We analyze the dipole strength near the neutron separation energy, which represents the threshold for neutron capture processes, and examine the isospin characteristics of PDR states through transition density calculations. Examination of proton and neutron transition densities reveals distinctive features of each dipole state, indicating their isoscalar and isovector nature. We observe that the primary component in the enhanced low-energy region exhibits isovector character. The PDR displays a mixture of isoscalar and isovector nature, distinguishing it from the isovector giant dipole resonance (IVGDR). These findings lay the groundwork for future investigations into the role of transition densities in reaction models and for their application to inelastic scattering calculations.

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arXiv2024

Predicting nucleon-nucleus scattering observables using nuclear structure theory

Developing a predictive capability for inelastic scattering will find applications in multiple areas. Experimental data for neutron-nucleus inelastic scattering is limited and thus one needs a robust theoretical framework to complement it. Charged-particle inelastic scattering can be used as a surrogate for $(n, \gamma)$ reactions to predict capture cross sections for unstable nuclei. Our work uses microscopic nuclear structure calculations for spherical nuclei to obtain nucleon-nucleus scattering potentials and calculate cross sections for these processes. We implement the Jeukenne, Lejeune, Mahaux (JLM) semi-microscopic folding approach, where the medium effects on nuclear interaction are parameterized in nuclear matter to obtain the nucleon-nucleon $(NN)$ interaction in a medium at positive energies. We solve for the nuclear ground state using the Hartree-Fock-Bogliubov (HFB) many-body method, assuming the nucleons within the nucleus interact via the Gogny-D1M potential. The vibrational excited states of the target nucleus are calculated using the quasi-particle random phase approximation (QRPA). We demonstrate our approach for spherical nuclei in the medium-mass region, showing scattering results for the $^{90}$Zr nucleus.

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arXiv2023

Improving nuclear data evaluations with predictive reaction theory and indirect measurements

Nuclear reaction data required for astrophysics and applications is incomplete, as not all nuclear reactions can be measured or reliably predicted. Neutron-induced reactions involving unstable targets are particularly challenging, but often critical for simulations. In response to this need, indirect approaches, such as the surrogate reaction method, have been developed. Nuclear theory is key to extract reliable cross sections from such indirect measurements. We describe ongoing efforts to expand the theoretical capabilities that enable surrogate reaction measurements. We focus on microscopic predictions for charged-particle inelastic scattering, uncertainty-quantified optical nucleon-nucleus models, and neural-network enhanced parameter inference.

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