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Emmanuel Jacquet

Publications and source records attributed to Emmanuel Jacquet.

At least 19 recordsLinked to original sources
arXiv2026

Alkali recondensation into chondrules

While sub-mm melt droplets should rapidly lose alkali elements in a vacuum at liquidus temperatures, chondrules are only modestly depleted in them (by less than one order of magnitude). The detection of sodium in olivine cores has previously suggested very high saturating partial pressures of gaseous sodium, but we show that alkalis were lost during heating and recondensed at lower temperatures, essentially in the present-day chondrule mesostases. This recondensation was accompanied by mass-dependent enrichment in light isotopes (for multi-isotope alkalis such as K and Rb), but its limited extent indicates a cooling acceleration (or "quenching"). The isotopic fractionation also constrains the ratio of the chondrule density and the cooling rate prior to the quench around $10^{-6}\:\mathrm{kg.m^{-3}.K^{-1}.h}$ suggesting densities above $\sim 10^{-6}\:\mathrm{kg/m^3}$. In a nebular context, this is achievable by radial and vertical concentrations near pressure bumps.

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arXiv2024

The secondary classification of unequilibrated chondrites

The multiplication of decimal petrologic schemes for different or the same chondrite groups evinces a lack of unified guiding principle in the secondary classification of type 1-3 chondrites. We show that the current OC, R and CO classifications can be a posteriori unified, with only minor reclassifications, if the decimal part of the subtype is defined as the ratio $m=Fa_I/Fa_{II}$ of the mean fayalite contents of type I and type II chondrules rounded to the nearest tenth (with adaptations from Cr systematics for the lowest subtypes). This parameter is more efficiently evaluable than the oft-used relative standard deviations of fayalite contents and defines a general metamorphic scale from M0.0 to M1 (where the suffixed number is the rounded $m$). Type 3 chondrites thus span the range M0.0-M0.9 and M1 designates type 4. Corresponding applications are then proposed for other chondrite groups. Known type 1 and 2 chondrites are at M0.0 (i.e. the metamorphic grade of type 3.0 chondrites). Independently, we define an aqueous alteration scale from A0.0 to A1.0, where the suffixed number is the (rounded) phyllosilicate fraction (PSF). For CM and CR chondrites, the subtypes can be characterized in terms of the thin-section-based criteria of previous schemes which are thus incorporated in the present framework. The rounding of the PSF to the (in principle) nearest tenth makes the proposed taxonomy somewhat coarser than those schemes, but hereby more robust and more likely to be generalized in future meteorite declarations. We propose the corresponding petrologic subtype to be 3-PSF, rounded to the nearest tenth (so that type 1 would correspond to subtypes 2.0 and 2.1). At the level of precision chosen, nonzero alteration and metamorphic degrees remain mutually exclusive, so that a single petrologic subtype $\approx$ 3+$m$-PSF indeed remains a good descriptor of secondary processes.

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arXiv2024

The early Solar System and its meteoritical witnesses

Meteorites, and in particular primitive meteorites (chondrites), are irreplaceable probes of the solar protoplanetary disk. We review their essential properties and endeavour to place them in astrophysical context. The earliest solar system solids, refractory inclusions, may have formed over the innermost au of the disk and have been transported outward by its expansion or turbulent diffusion. The age spread of chondrite components may be reconciled with the tendency of drag-induced radial drift if they were captured in pressure maxima, which may account for the non-carbonaceous/carbonaceous meteorite isotopic dichotomy. The solid/gas ratio around unity witnessed by chondrules, if interpreted as nebular (non-impact) products, suggests efficient radial concentration and settling at such locations, conducive to planetesimal formation by the streaming instability. The cause of the pressure bumps, e.g. Jupiter or condensation lines, remains to be ascertained.

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arXiv2022

Meteorite petrology versus genetics: Toward a unified binominal classification

The current meteorite taxonomy, a result of two centuries of meteorite research and tradition, entangles textural and genetic terms in a less than consistent fashion, with some taxa (like shergottites) representing varied lithologies from a single putative parent body while others (like pallasites) subsume texturally similar objects of multifarious solar system origins. The familiar concept of group as representative of one primary parent body is also difficult to define empirically. It is proposed that the classification becomes explicitly binominal throughout the meteorite spectrum, with classes referring to petrographically defined primary rock types, whereas groups retain a genetic meaning, but no longer tied to any assumption on the number of represented parent bodies. The classification of a meteorite would thus involve both a class and a group, in a two-dimensional fashion analogous to the way Van Schmus and Wood decoupled primary and secondary properties in chondrites. Since groups would not substantially differ, at first, from those in current use de facto, the taxonomic treatment of normal meteorites, whose class would bring no new information, would hardly change. Yet classes combined with high- or low-level groups would provide a standardized grid to characterize petrographically and/or isotopically unusual or anomalous meteorites (which make up the majority of represented meteorite parent bodies) for example, in relation to the carbonaceous/noncarbonaceous dichotomy. In the longer term, the mergers of genetically related groups, a more systematic treatment of lithology mixtures, and the chondrite/achondrite transition can further simplify the nomenclature.

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arXiv2021

Collisions and compositional variability in chondrule-forming events

Compound chondrules, i.e. chondrules fused together, make a powerful probe of the density and compositional diversity in chondrule-forming environments, but their abundance among the dominating porphyritic textures may have been drastically underestimated. I report herein microscopic observations and LA-ICP-MS analyses of lobate chondrules in the CO3 chondrites Miller Range 07193 and 07342. Lobes in a given chondrule show correlated volatile and moderately volatile element abundances but refractory element concentrations are essentially independent. This indicates that they formed by the collision of preexisting droplets whose refractory elements behaved in closed system, while their more volatile elements were buffered by the same gaseous medium. The presence of lobes would otherwise be difficult to explain, as surface tension should have rapidly imposed a spherical shape at the temperature peak. In fact, since most chondrules across chondrite groups are nonspherical, a majority are probably compounds variously relaxed toward sphericity. The lack of correlation of refractory elements between conjoined compound chondrule components is inconsistent with derivation of chondrules from the disruption of homogenized melt bodies as in impact scenarios and evokes rather the melting of independent mm-size nebular aggregates. Yet a "nebular" setting for chondrule formation would need to involve not only increased solid concentration, e.g. by settling to the midplane, but also a boost in relative velocities between droplets during chondrule-forming events to account for observed compound chondrule frequencies .

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arXiv2021

Origin of isolated olivine grains in carbonaceous chondrites

We report microscopic, cathodoluminescence, chemical and O isotopic measurements of FeO-poor isolated olivine grains (IOG) in the carbonaceous chondrites Allende (CV3), Northwest Africa 5958 (C2-ung), Northwest Africa 11086 (CM2-an), Allan Hills 77307 (CO3.0). The general petrographic, chemical and isotopic similarity with bona fide type I chondrules confirms that the IOG derived from them. The concentric CL zoning, reflecting a decrease in refractory elements toward the margins, and frequent rimming by enstatite are taken as evidence of interaction of the IOG with the gas as stand-alone objects. This indicates that they were splashed out of chondrules when these were still partially molten. CaO-rich refractory forsterites, which are restricted to $Δ^{17}O < -4\permil$ likely escaped equilibration at lower temperatures because of their large size and possibly quicker quenching. The IOG thus bear witness to frequent collisions in the chondrule-forming regions.

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arXiv2019

Fingerprints of the protosolar cloud collapse in the Solar System II: Nucleosynthetic anomalies in meteorites

The isotopic heterogeneity of the Solar System shown by meteorite analyses is more pronounced for its earliest objects, the Calcium-Aluminum-rich Inclusions (CAIs). This suggests that it was inherited from spatial variations in different stardust populations in the protosolar cloud. We model the formation of the solar protoplanetary disk following its collapse and find that the solid-weighted standard deviation of different nucleosynthetic contributions in the disk is reduced by one order of magnitude compared to the protosolar cloud, whose successive isotopic signatures are fossilized by CAIs. The enrichment of carbonaceous chondrites in r-process components, whose proportions are inferred to have diminished near the end of infall, is consistent with their formation at large heliocentric distances, where the early signatures would have been preferentially preserved after outward advection. We also argue that thermal processing had little effect on the (mass-independent) isotopic composition of bulk meteorites for refractory elements.

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arXiv2019

Fingerprints of the protosolar cloud collapse in the Solar System I: Distribution of presolar short-lived $^{26}$Al

The short-lived radionuclide $^{26}$Al is widely used to determine the relative ages of chondrite components and timescales of physical and thermal events that attended the formation of the Solar System. However, an important assumption for using $^{26}$Al as a chronometer is its homogeneous distribution in the disk. Yet, the oldest components in chondrites, the Ca-Al-rich inclusions (CAIs), which are usually considered as time anchors for this chronometer, show evidence of $^{26}$Al/$^{27}$Al variations independent of radioactive decay. Since their formation epoch may have been contemporaneous with the collapse of the parent cloud that formed the disk, this suggests that $^{26}$Al was heteregeneously distributed in the cloud. We model the collapse of such an heterogeneous cloud, using two different $^{26}$Al distributions (monotonic and non-monotonic), and follow its re-distribution in the first condensates and bulk dust that populate the forming disk. We find that CAIs inherit the $^{26}$Al/$^{27}$Al ratio of the matter infalling at the time of their formation, so that variations of $^{26}$Al/$^{27}$Al among primordial CAIs can be accounted for, independently of radioactive decay. The prevalence of a canonical ratio among them and its necessity for the differentiation of the first planetesimals suggest a (monotonic) scenario where $^{26}$Al sharply rose relatively close to the center of the protosolar cloud and essentially remained at a high level outward (rather than decreased since). As the $ ^{26}$Al abundance would be relatively homogeneous after cessation of infall, this would warrant the use of the Al-Mg chronometer from the formation of "regular" CAIs onward, to chondrules and chondrite accretion.

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arXiv2019

On beryllium-10 production in gaseous protoplanetary disks and implications on the astrophysical setting of refractory inclusions

Calcium-Aluminum-rich Inclusions (CAIs), the oldest known solids of the solar system, show evidence for the past presence of short-lived radionuclide beryllium-10, which was likely produced by spallation during protosolar flares. While such $^{10}$Be production has hitherto been modeled at the inner edge of the protoplanetary disk, I calculate here that spallation at the disk surface may reproduce the measured $^{10}$Be/$^9$Be ratios at larger heliocentric distances. Beryllium-10 production in the gas prior to CAI formation would dominate that in the solid. Interestingly, provided the Sun's proton to X-ray output ratio does not decrease strongly, $^{10}$Be/$^9$Be at the CAI condensation front would increase with time, explaining the reduced values in a (presumably early) generation of CAIs with nucleosynthetic anomalies. CAIs thus need not have formed very close to the Sun and may have condensed at 0.1-1 AU where sufficiently high temperatures originally prevailed.

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arXiv2018

Chondrule heritage and thermal histories from trace element and oxygen isotope analyses of chondrules and amoeboid olivine aggregates

We report combined oxygen isotope and mineral-scale trace element analyses of amoeboid olivine aggregates (AOA) and chondrules in ungrouped carbonaceous chondrite Northwest Africa 5958. The trace element geochemistry of olivine in AOA, for the first time measured by LA-ICP-MS, is consistent with a condensation origin although the shallow slope of its rare earth element (REE) pattern has yet to be physically explained. Ferromagnesian silicates in type I chondrules resemble those in other carbonaceous chondrites both geochemically and isotopically, and we find a correlation between 16O enrichment and many incompatible elements in olivine. The variation in incompatible element concentrations may relate to varying amounts of olivine crystallization during a sub-isothermal stage of chondrule-forming events, the duration of which may be anticorrelated with the local solid/gas ratio if this was the determinant of oxygen isotopic ratios as recently proposed. While aqueous alteration has depleted many chondrule mesostases in REE, some chondrules show recognizable subdued group II-like patterns supporting the idea that the immediate precursors of chondrules were nebular condensates.

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arXiv2018

Making the Planetary Material Diversity During the Early Assembling of the Solar System

Chondritic meteorites, the building blocks of terrestrial planets, are made of an out-of-equilibrium assemblage of solids formed at high and low temperatures, either in our Solar system or previous generations of stars. This was considered for decades to result from large scale transport processes in the Sun's isolated accretion disk. However, mounting evidences suggest that refractory inclusions in chondrites formed contemporaneously with the disk building. Here we numerically investigate, using a 1D model and several physical and chemical processes, the formation and transport of rocky materials during the collapse of the Sun's parent cloud and the consequent Solar Nebula assembling. The interplay between the cloud collapse, the dynamics of gas and dust, vaporization, recondensation and thermal processing of different species in the disk, results in a local mixing of solids with different thermal histories. Moreover, our results also explains the overabundance of refractory materials far from the Sun and their short formation timescales, during the first tens of kyr of the Sun, corresponding to class 0-I, opening new windows into the origin of the compositional diversity of chondrites.

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arXiv2017

Chondrules in enstatite chondrites

We review silicate chondrules and metal-sulfide nodules in unequilibrated enstatite chondrites (EH3 and EL3). Their unique mineralogical assemblage, with a wide diversity of opaque phases, nitrides, nearly FeO-free enstatite etc. testify to exceptionally reduced conditions. While those have long been ascribed to a condensation sequence at supersolar C/O ratios, with the oldhamite-rich nodules among the earliest condensates, evidence for relatively oxidized local precursors suggests that their peculiarities may have been acquired during the chondrule-forming process itself. Silicate phases may have been then sulfidized in an O-poor and S-rich environment; metal-sulfide nodules in EH3 chondrites could have originated in the silicate chondrules whereas those in EL3 may be impact products. The astrophysical setting (nebular or planetary) where such conditions were achieved, whether by depletion in water or enrichment in dry organics-silicate mixtures, is uncertain, but was most likely sited inside the snow line, consistent with the Earth-like oxygen isotopic signature of most EC silicates, with little data constraining its epoch yet.

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arXiv2017

Northwest Africa 5958: a weakly altered CM-related ungrouped chondrite, not a CI3

Northwest Africa (NWA) 5958 is a carbonaceous chondrite found in Morocco in 2009. Preliminary chemical and isotopic data leading to its initial classification as C3.0 ungrouped have prompted us to conduct a multi-technique study of this meteorite and present a general description here. The petrography and chemistry of NWA 5958 is most similar to a CM chondrite, with a low degree of aqueous alteration, apparently under oxidizing conditions, and evidence of a second, limited alteration episode manifested by alteration fronts. The oxygen isotopic composition, with $Δ^{17}$O = -4.3 $\permil$, is more 16O-rich than all CM chondrites, indicating, along with other compositional arguments, a separate parent body of origin. We suggest that NWA 5958 be reclassified as an ungrouped carbonaceous chondrite related to the CM group.

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arXiv2016

The formation conditions of enstatite chondrites: Insights from trace element geochemistry of olivine-bearing chondrules in Sahara 97096 (EH3)

We report in situ LA-ICP-MS trace element analyses of silicate phases in olivine-bearing chondrules in the Sahara 97096 (EH3) enstatite chondrite. Most olivine and enstatite present rare earth element (REE) patterns comparable to their counterparts in type I chondrules in ordinary chondrites. They thus likely share a similar igneous origin, likely under similar redox conditions. The mesostasis however frequently shows negative Eu and/or Yb (and more rarely Sm) anomalies, evidently out of equilibrium with olivine and enstatite. We suggest that this reflects crystallization of oldhamite during a sulfidation event, already inferred by others, during which the mesostasis was molten, where the complementary positive Eu and Yb anomalies exhibited by oldhamite would have possibly arisen due to a divalent state of these elements. Much of this igneous oldhamite would have been expelled from the chondrules, presumably by inertial acceleration or surface tension effects, and would have contributed to the high abundance of opaque nodules found outside them in EH chondrites. In two chondrules, olivine and enstatite exhibit negatively sloped REE patterns, which may be an extreme manifestation of a general phenomenon (possibly linked to near-liquidus partitioning) underlying the overabundance of light REE observed in most chondrule silicates relative to equilibrium predictions. The silicate phases in one of these two chondrules show complementary Eu, Yb and Sm anomalies providing direct evidence for the postulated occurrence of the divalent state for these elements at some stage in the formation reservoir of enstatite chondrites. Our work supports the idea that the peculiarities of enstatite chondrites may not require a condensation sequence at high C/O ratios as has long been believed.

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arXiv2016

Chondrule Transport in Protoplanetary Disks

Chondrule formation remains one of the most elusive early Solar System events. Here, we take the novel approach of employing numerical simulations to investigate chondrule origin beyond purely cosmochemical methods. We model the transport of generically-produced chondrules and dust in a 1D viscous protoplanetary disk model, in order to constrain the chondrule formation events. For a single formation event we are able to match analytical predictions of the memory chondrule and dust populations retain of each other (complementarity), finding that a large mass accretion rate ($\gtrsim 10^{-7}$~M$_\odot$~yr$^{-1}$) allows for delays on the order of the disk's viscous timescale between chondrule formation and chondrite accretion. Further, we find older disks to be severely diminished of chondrules, with accretion rates $\lesssim 10^{-9}$~M$_\odot$~yr$^{-1}$ for nominal parameters. We then characterize the distribution of chondrule origins in both space and time, as functions of disk parameters and chondrule formation rates, in runs with continuous chondrule formation and both static and evolving disks. Our data suggest that these can account for the observed diversity between distinct chondrite classes, if some diversity in accretion time is allowed for.

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arXiv2015

New Paradigms For Asteroid Formation

Asteroids and meteorites provide key evidence on the formation of planetesimals in the Solar System. Asteroids are traditionally thought to form in a bottom-up process by coagulation within a population of initially km-scale planetesimals. However, new models challenge this idea by demonstrating that asteroids of sizes from 100 to 1000 km can form directly from the gravitational collapse of small particles which have organised themselves in dense filaments and clusters in the turbulent gas. Particles concentrate passively between eddies down to the smallest scales of the turbulent gas flow and inside large-scale pressure bumps and vortices. The streaming instability causes particles to take an active role in the concentration, by piling up in dense filaments whose friction on the gas reduces the radial drift compared to that of isolated particles. In this chapter we review new paradigms for asteroid formation and compare critically against the observed properties of asteroids as well as constraints from meteorites. Chondrules of typical sizes from 0.1 to 1 mm are ubiquitous in primitive meteorites and likely represent the primary building blocks of asteroids. Chondrule-sized particles are nevertheless tightly coupled to the gas via friction and are therefore hard to concentrate in large amounts in the turbulent gas. We review recent progress on understanding the incorporation of chondrules into the asteroids, including layered accretion models where chondrules are accreted onto asteroids over millions of years. We highlight in the end ten unsolved questions in asteroid formation where we expect that progress will be made over the next decade.

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arXiv2015

Trace element geochemistry of ordinary chondrite chondrules: the type I/type II chondrule dichotomy

We report trace element concentrations of silicate phases in chondrules from LL3 ordinary chondrites Bishunpur and Semarkona. Results are similar to previously reported data for carbonaceous chondrites, with rare earth element (REE) concentrations increasing in the sequence olivine < pyroxene < mesostasis, and heavy REE (HREE) being enriched by 1-2 orders of magnitude (CI-normalized) relative to light REE (LREE) in ferromagnesian silicates, although no single olivine with very large LREE/HREE fractionation has been found. On average, olivine in type II chondrules is poorer in refractory lithophile incompatible elements (such as REE) than its type I counterpart by a factor of ~2. This suggests that olivine in type I and II chondrules formed by batch and fractional crystallization, respectively, implying that type II chondrules formed under faster cooling rates (> ~ 10 K/h) than type I chondrules. Appreciable Na concentrations (3-221 ppm) are measured in olivine from both chondrule types; type II chondrules seem to have behaved as closed systems, which may require chondrule formation in the vicinity of protoplanets or planetesimals. At any rate, higher solid concentrations in type II chondrule forming regions may explain the higher oxygen fugacities they record compared to type I chondrules. Type I and type II chondrules formed in different environments and the correlation between high solid concentrations and/or oxygen fugacities with rapid cooling rates is a key constraint that chondrule formation models must account for.

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