arXiv subjects

Emmanuel Paspalakis

Publications and source records attributed to Emmanuel Paspalakis.

At least 19 recordsLinked to original sources

arXiv2025

Fast chiral resolution with optimal control

In this work, we formulate the problem of achieving in minimum-time perfect chiral resolution with bounded control fields, as an optimal control problem on two non-interacting spins-$1/2$. We assume the same control bound for the two Raman fields (pump and Stokes) and a different bound for the field connecting directly the two lower-energy states. Using control theory, we show that the optimal fields can only take the boundary values or be zero, the latter corresponding to singular control. Subsequently, using numerical optimal control and intuitive arguments, we identify some three-stage symmetric optimal pulse-sequences, for relatively larger values of the ratio between the two control bounds, and analytically calculate the corresponding pulse timings as functions of this ratio. For smaller values of the bounds ratio, numerical optimal control indicates that the optimal pulse-sequence loses its symmetry and the number of stages increases in general. In all cases, the analytical or numerical optimal protocol achieves a faster perfect chiral resolution than other pulsed protocols, mainly because of the simultaneous action of the control fields. The present work is expected to be useful in the wide spectrum of applications across the natural sciences where enantiomer separation is a crucial task.

quant-ph↗

arXiv2025

Efficient population transfer in a quantum dot exciton under phonon-induced decoherence via shortcuts to adiabaticity

In the present study, we apply shortcut to adiabaticity pulses (time-dependent Rabi frequency and detuning) for the efficient population transfer from the ground to the exciton state in a GaAs/InGaAs quantum dot with phonon-induced dephasing. We use the time-evolving matrix product operator (TEMPO) method to propagate system in time and find that, for temperatures below $ 20 \ \text{K} $ and pulse duration up to $ 10 \ \text{ps} $, a very good transfer efficiency is obtained in general. We explain these results using a Bloch-like equation derived from a generalized Lindblad equation, which adequately describes system dynamics at lower temperatures. For higher temperatures, the transfer efficiency is significantly reduced except for subpicosecond pulses, where the shortcut Rabi frequency reduces to a delta pulse attaining a fast population inversion. The present work is expected to find application in quantum technologies which exploit quantum dots for single-photon generation on demand.

cond-mat.mes-hall↗

arXiv2024

Fast generation of entanglement between coupled spins using optimization and deep learning methods

Coupled spins form composite quantum systems which play an important role in many quantum technology applications, with an essential task often being the efficient generation of entanglement between two constituent qubits. The simplest such system is a pair of spins-$1/2$ coupled with Ising interaction, and in previous works various quantum control methods such as adiabatic processes, shortcuts to adiabaticity and optimal control have been employed to quickly generate there one of the maximally entangled Bell states. In this study, we use machine learning and optimization methods to produce maximally entangled states in minimum time, with the Rabi frequency and the detuning used as bounded control functions. We do not target a specific maximally entangled state, like the preceding studies, but rather find the controls which maximize the concurrence, leading thus automatically the system to the closest such state in shorter time. By increasing the bounds of the control functions we observe that the corresponding optimally selected maximally entangled state also changes and the necessary time to reach it is reduced. The present work demonstrates also that machine learning and optimization offer efficient and flexible techniques for the fast generation of entanglement in coupled spin systems, and we plan to extent it to systems involving more spins, for example spin chains.

quant-ph↗

arXiv2024

Fast charging of an Ising spin pair quantum battery using optimal control

We consider the problem of maximizing the stored energy for a given charging duration in a quantum battery composed of a pair of spins-$1/2$ with Ising coupling starting from the spin-down state, using bounded transverse field control. We map this problem to an optimal control problem on a single qubit and using optimal control theory we show that, although a single bang pulse can quickly achieve considerable charging levels for relatively large upper control bounds, higher levels of stored energy including complete charging are accomplished by a bang-singular-bang pulse-sequence, where the intermediate singular pulse is an Off pulse. If the control is restricted between zero and a maximum value, the initial and final bang pulses attain the maximum bound but have different durations, while if it is restricted between symmetric negative and positive boundaries, the bang pulses have the same duration but opposite boundary values. For both cases we provide transcendental equations from which the durations of the individual pulses in the optimal pulse-sequence can be calculated. For the case of full charging we surprisingly find that the three ``switching" functions for the equivalent qubit problem become zero while the adjoint ket does not, in consistency with optimal control theory.

quant-ph↗

arXiv2024

TorchQC -- A framework for efficiently integrating machine and deep learning methods in quantum dynamics and control

Machine learning has been revolutionizing our world over the last few years and is also increasingly exploited in several areas of physics, including quantum dynamics and control.The need for a framework that brings together machine learning models and quantum simulation methods has been quite high within the quantum control field, with the ultimate goal of exploiting these powerful computational methods for the efficient implementation of modern quantum technologies. The existing frameworks for quantum system simulations, such as QuTip and QuantumOptics.jl, even though they are very successful in simulating quantum dynamics, cannot be easily incorporated into the platforms used for the development of machine learning models, like for example PyTorch. The TorchQC framework introduced in the present work comes exactly to fill this gap. It is a new library written entirely in Python and based on the PyTorch deep learning library. PyTorch and other deep learning frameworks are based on tensors, a structure that is also used in quantum mechanics. This is the common ground that TorchQC utilizes to combine quantum physics simulations and deep learning models.TorchQC exploits PyTorch and its tensor mechanism to represent quantum states and operators as tensors, while it also incorporates all the tools needed to simulate quantum system dynamics. All necessary operations are internal in the PyTorch library, thus TorchQC programs can be executed in GPUs, substantially reducing the simulation time. We believe that the proposed TorchQC library has the potential to accelerate the development of deep learning models directly incorporating quantum simulations, enabling the easier integration of these powerful techniques in modern quantum technologies.

quant-ph↗

arXiv2024

Spatio-spectral control of spontaneous emission

We propose a scheme aimed at achieving spatio-spectral control over spontaneous emission within a four-level atom-light coupling system interacting with optical vortices carrying orbital angular momentum (OAM). The atom comprises a ground level and two excited states coupled with two laser fields, forming a V subsystem where the upper states exclusively decay to a common fourth state via two channels. By investigating various initial states of the atom and considering the presence or absence of quantum interference in spontaneous emission channels, we analyze how the characteristics of the OAM-carrying vortex beam imprint onto the emission spectrum. The interplay between the optical vortex and the quantum system, including its environment modes, induces a wide variety of spatio-spectral behaviour, including two-dimensional spectral-peak narrowing, spectralpeak enhancement, spectral-peak suppression, and spontaneous emission reduction or quenching in the spatial azimuthal plane. Our findings shed light on the dynamics of atom-vortex beam light interactions and offer insights into the manipulation of emission properties at the quantum level.

quant-ph↗

arXiv2023

Efficient four-wave mixing in four-subband semiconductor quantum wells using spatially modulated control fields with a linearly varying mixing angle

In this article, we use spatially modulated control fields to increase the four-wave mixing efficiency in a four-subband semiconductor asymmetric double quantum well, motivated by similar works in atomic systems. Using a simplified version of the propagation equations, we show analytically that for control fields with constant amplitude and linearly varying mixing angle with the propagation distance, a conversion efficiency close to unity can be achieved even for relatively short propagation distances. Subsequently, we confirm these results by numerically simulating the full set of propagation equations.

physics.optics↗

arXiv2023

Optimal STIRAP shortcuts using the spin to spring mapping

We derive shortcuts to adiabaticity maximizing population transfer in a three-level $\Lambda$ quantum system, using the spin to spring mapping to formulate the corresponding optimal control problem on the simpler system of a classical driven dissipative harmonic oscillator. We solve the spring optimal control problem and obtain analytical expressions for the impulses, the durations of the zero control intervals and the singular control, which are the elements composing the optimal pulse sequence. We also derive suboptimal solutions for the spring problem, one with less impulses than the optimal and others with smoother polynomial controls. We then apply the solutions derived for the spring system to the original system, and compare the population transfer efficiency with that obtained for the original system using numerical optimal control. For all dissipation rates used, the efficiency of the optimal spring control approaches that of the numerical optimal solution for longer durations, with the approach accomplished earlier for smaller decay rates. The efficiency achieved with the suboptimal spring control with less impulses is very close to that of the optimal spring control in all cases, while that obtained with polynomial controls lies below, and this is the price paid for not using impulses, which can quickly build a nonzero population in the intermediate state. The analysis of the optimal solution for the classical driven dissipative oscillator is not restricted to the system at hand but can also be applied in the transport of a coherent state trapped in a moving harmonic potential and the transport of a mesoscopic object in stochastic thermodynamics.

quant-ph↗

arXiv2023

Minimum time generation of a uniform superposition in a qubit with only transverse field control

We consider a two-level system with a fixed energy spacing (detuning) between the two levels and a single transverse control field which can take values between zero and a maximum amplitude. Using Pontryagin's maximum principle, we completely solve the problem of generating in minimum time a uniform superposition of the two quantum states when starting from one of them, for all the values of the ratio between the maximum control amplitude and the detuning. For each value of this ratio we find the optimal pulse sequence to have the bang-bang form, and calculate the durations of the pulses composing it. The suggested framework is not only restricted to the problem at hand, but it can be also exploited in the problem of fast charging a quantum battery based on a two-level system, as well as for the optimization of pulse-sequences used for the controlled preparation of the excited state in a quantum emitter, which is a prerequisite for its usage as a single-photon source.

quant-ph↗

arXiv2022

On the optimality of optical pumping for a closed $Λ$-system with large decay rates of the intermediate excited state

We use optimal control theory to show that for a closed $Λ$-system where the excited intermediate level decays to the lower levels with a common large rate, the optimal scheme for population transfer between the lower levels is actually optical pumping. In order to obtain this result we exploit the large decay rate to eliminate adiabatically the weakly coupled excited state, then perform a transformation to the basis comprised of the dark and bright states, and finally apply optimal control to this transformed system. Subsequently, we confirm the optimality of the optical pumping scheme for the original closed $Λ$-system using numerical optimal control. We also demonstrate numerically that optical pumping remains optimal when the decay rate to the target state is larger than that to the initial state or the two rates are not very different from each other. The present work is expected to find application in various tasks of quantum information processing, where such systems are encountered.

quant-ph↗

arXiv2022

Optimal shortcuts of Stimulated Raman Adiabatic Passage in the presence of dissipation

We use optimal control theory to obtain shortcuts to adiabaticity which maximize population transfer in a three-level STIRAP system, for a given finite duration of the process and specified dissipation rate at the intermediate state. We fix the sum of the intensities of the pump and Stokes pulses and use the mixing angle as the sole control variable. We determine the optimal variation of this angle and reveal the role of singular arc in the optimal trajectory, in order to minimize the effect of dissipation.

quant-ph↗

arXiv2022

Efficient exciton generation in a semiconductor quantum dot-metal nanoparticle composite structure using conventional chirped pulses

We consider a nanostructure consisting of a semiconductor quantum dot coupled to a metal nanoparticle, and show with numerical simulations that the exciton state of the quantum dot can be robustly generated from the ground state even for small interparticle distances, using conventional chirped pulses with Gaussian and hyperbolic secant envelopes. The asymmetry observed in the final exciton population with respect to the chirp sign of the applied pulses is explained using the nonlinear density matrix equations describing the system, and is attributed to the real part of the parameter emerging from the interaction between excitons in the quantum dot and plasmons in the metal nanoparticle. The simplicity of the conventional chirped pulses, which can also be easily implemented in the laboratory, make the proposed robust quantum control scheme potentially useful for the implementation of ultrafast nanoswitches and quantum information processing tasks with semiconductor quantum dots.

cond-mat.mes-hall↗

arXiv2021

Optimal shape of STIRAP pulses for large dissipation at the intermediate level

We study the problem of maximizing population transfer efficiency in the STIRAP system for the case where the dissipation rate of the intermediate state is much higher than the maximum amplitude of the control fields. Under this assumption, the original three-level system can be reduced to a couple of equations involving the initial and target states only. We find the control fields which maximize the population transfer to the target state for a given duration $T$, without using any penalty involving the population of the lossy intermediate state, but under the constraint that the sum of the intensities of the pump and Stokes pulses is constant, so the total field has constant amplitude and the only control parameter is the mixing angle of the two fields. In the optimal solution the mixing angle changes in the bang-singular-bang manner, where the initial and final bangs correspond to equal instantaneous rotations, while the intermediate singular arc to a linear change with time. We show that the optimal angle of the initial and final rotations is the unique solution of a transcendental equation where duration $T$ appears as a parameter, while the optimal slope of the intermediate linear change as well as the optimal transfer efficiency are expressed as functions of this optimal angle. The corresponding optimal solution recovers the counterintuitive pulse-sequence, with nonzero pump and Stokes fields at the boundaries. We also show with numerical simulations that, transfer efficiency values close to the optimal derived using the approximate system, can also be obtained with the original STIRAP system using dissipation rates comparable to the maximum control amplitude.

quant-ph↗

arXiv2021

Coherent preparation of the biexciton state in a semiconductor quantum dot coupled to a metallic nanoparticle

We study the potential for controlled transfer of population to the biexciton state of a semiconductor quantum dot coupled with a metal nanoparticle, under the influence of an electromagnetic pulse with hyperbolic secant shape, and derive analytical solutions of the density matrix equations, for both zero and nonzero biexciton energy shift. These solutions lead to efficient transfer to the biexciton state, for various interparticle distances, including relatively small values. In certain cases, when the distance between the two particles is small, the transfer of population is strongly modified because of the influence of surface plasmons to the excitons, and the effect is more pronounced for shorter pulses. The hybrid snanostructure that we study has been proposed for generating efficiently polarization-entangled photons, thus the successful biexciton state preparation considered here is expected to contribute in this line of research.

cond-mat.mes-hall↗

arXiv2021

Optimized pulses for population transfer via laser induced continuum structures

We use optimal control in order to find the optimal shapes of pulses maximizing the population transfer between two bound states which are coupled via a continuum of states. We find that the optimal bounded controls acquire the bang-interior and interior-bang form, with the bang part corresponding to the maximum allowed control value and the interior part to values between zero and the maximum. Then, we use numerical optimal control to obtain the switching times and the interior control values. We compare our results with those obtained using Gaussian STIRAP pulses, and find that the optimal method performs better, with the extent of improvement depending on the effective two-photon detuning and the size of incoherent losses. When we consider effective two-photon resonance, the improvement is more dramatic for larger incoherent losses, while when we take into account the effective two-photon detuning, the improvement is better for smaller incoherent losses. We also obtain how the transfer efficiency increases with increasing absolute value of the Fano factor. The present work is expected to find application in areas where the population transfer between two bound states through a continuum structure plays an important role, for example coherence effects, like population trapping and electromagnetically induced transparency, optical analogs for light waves propagating in waveguide-based photonic structures, and qubits coupled via a continuum of bosonic or waveguide modes.

quant-ph↗

arXiv2021

Ultimate conversion efficiency bound for the forward double-$Λ$ atom-light coupling scheme

We show that for the two widely used configurations of the double-$Λ$ atom-light coupling scheme, one where the control fields are applied in the same $Λ$-subsystem and another where they applied in different $Λ$-subsystems, the forward propagation of the probe and signal fields is described by the same set of equations. We then use optimal control theory to find the spatially-dependent optimal control fields which maximize the conversion efficiency from the probe to the signal field, for a given optical density. The present work is expected to find application in the implementation of efficient frequency and orbital angular momentum conversion devices for quantum information processing, as well as to be useful to many other applications using the double-$Λ$ atom-light coupling scheme.

quant-ph↗

arXiv2020

Rapid biexciton state preparation in a quantum dot using on-off pulse-sequences

We consider the problem of pulsed biexciton preparation in a quantum dot and show that a pulse-sequence with a simple on-off-on modulation can achieve complete preparation of the target state faster than the commonly used constant and hyperbolic secant pulses. The durations of the pulses composing the sequence are obtained from the solution of a transcendental equation. Furthermore, using numerical optimal control, we demonstrate that for a wide range of values of the maximum pulse amplitude, the proposed pulse-sequence prepares the biexciton state in the numerically obtained minimum time, for the specific system under consideration. We finally show with numerical simulations that, even in the presence of dissipation and dephasing, high levels of biexciton state fidelity can be generated in short times.

quant-ph↗

arXiv2020

Performance of superadiabatic stimulated Raman adiabatic passage in the presence of dissipation and Ornstein-Uhlenbeck dephasing

In this paper we evaluate the performance of two superadiabatic stimulated Raman adiabatic passage (STIRAP) protocols derived from Gaussian and sin-cos pulses, under dissipation and Ornstein-Uhlenbeck noise in the energy levels. We find that for small amplitudes of Stokes and pump pulses, the population transfer is mainly achieved directly through the counterdiabatic pulse, while for large amplitudes the conventional STIRAP path dominates. This kind of "hedging" leads to a remarkable robustness against dissipation in the lossy intermediate state. For small pulse amplitudes and increasing noise correlation time the performance is decreased, since the dominant counterdiabatic pulse is affected more, while for large pulse amplitudes, where the STIRAP path dominates, the efficiency is degraded more for intermediate correlation times (compared to the pulse duration). For the Gaussian superadiabatic STIRAP protocol we also investigate the effect of delay between pump and Stokes pulses and find that under the presence of noise the performance is improved for increasing delay. We conclude that the Gaussian protocol with suitably chosen delay and the sin-cos protocol perform quite well even under severe noise conditions. The present work is expected to have a broad spectrum of applications, since STIRAP has a crucial role in modern quantum technology.

quant-ph↗