arXiv subjects

Emre Ozan Polat

Publications and source records attributed to Emre Ozan Polat.

8 recordsLinked to original sources

arXiv2026

Spacer-Mediated Gold Nanocube Arrays for Edge-Localized Excitonic Enhancement in Monolayer MoS2

Plasmonic nanostructures offer an effective route for enhancing light-matter interaction in atomically thin semiconductors, whose optical response is intrinsically limited by their sub-nanometer active thickness. Here, we numerically investigate excitonic enhancement in monolayer (ML) Molybdenum Disulfide (MoS2) coupled to size-tuned gold (Au) nanocube arrays separated by thin aluminum oxide (Al2O3) and hexagonal boron nitride (h-BN) spacer layers. By varying the nanocube side length, the localized surface plasmon resonance is tuned across the visible spectral range to modulate the A- and B-excitonic transitions of monolayer MoS2. We show that the nanocube-size-dependent spectral redshift can be further controlled through the spacer material and thickness, enabling systematic tuning of the near-field distribution, carrier generation rate, quantum yield, and radiative decay enhancement. Localized plasmonic confinement yields excitation-rate enhancements of up to 4.35 at B-excitonic transition (605 nm) and 3.66 at A-excitonic transition (650 nm), while the radiative decay-rate enhancement exceeds 80, leading to 350-fold photoluminescence enhancement. Although both A- and B-excitonic channels are enhanced simultaneously, their relative contributions depend on nanocube size, spacer material, and spacer thickness, indicating wavelength-dependent excitonic modulation rather than strict exciton-selective switching. These findings establish Au nanocube arrays as a simple, scalable, and tunable plasmonic platform for enhancing excitonic carrier generation and emission in ML MoS2.

physics.optics↗

arXiv2026

Geometry-Controlled Exciton Selectivity in Monolayer MoS2 Using Plasmonic Hollow Nanocavities

Spectral control of closely spaced excitonic transitions is central to valleytronic photonics, nanoscale light sources, and wavelength-encoded sensing. In monolayer molybdenum disulfide (MoS2), the A and B excitons are separated by only tens of meV, making selective excitonic emission control both fundamentally important and technologically challenging. Here, we numerically investigate plasmon-enhanced excitonic emission from monolayer MoS2 coupled to vertically oriented hollow gold nanocylindrical cavities through a dielectric spacer. Finite-difference time-domain simulations combined with a photoluminescence-rate framework enable separate evaluation of excitation enhancement, radiative decay modification, nonradiative quenching, and excitonic charge generation. By tuning the cavity aspect ratio, the localized surface plasmon resonance is selectively aligned with either the A- or B-exciton transition, while the spacer thickness and refractive index regulate near-field coupling and the local density of optical states. Under optimized conditions, the excitation rate is enhanced by up to 4.34-fold and the radiative decay rate by more than 40-fold, yielding photoluminescence enhancements of 143.85 and 87.27 for the A and B excitons, respectively. The cavity also redistributes the relative excitonic peak intensities, producing exciton-selective peak ratios up to 2.4 times higher than those of bare MoS2. These results establish hollow plasmonic nanocavities as geometry-tunable platforms for exciton-selective emission and charge-generation control in atomically thin semiconductors.

physics.optics↗

arXiv2026

Programmable Quantum Mode Switches via Plasmonic Toroidal Nanoantennae

The ability to switch and program the spectral response of quantum modes via deterministically located plasmonic nanoantennae presents opportunities for wide spectrum of applications from biosensors to quantum computing. Due to its topology, toroidal nanoantenna (TNA) focuses immense amount of three-dimensional (3D) local electric field by toroidal moment while allowing pre and post positioning around quantum emitters (QEs). Here, within local-response finite difference time domain (FDTD) simulations, we demonstrate high-contrast spectral switching of the radiative decay channel of a dipolar QE coupled to a TNA by introducing effective Lorentzian quantum objects (QOs). At optimized TNA geometries, Fano interference between the broadband plasmonic continuum and narrow quantum transitions of QOs suppresses both radiative and non-radiative decay channels near 850 nm, yielding an observable full switching that traps energy within the hybrid mode instead of re-emitting it. To show the promises of the concept, we further demonstrate systems with multiple QOs where spectral degeneracy enhances the transparency bandwidth, while detuning generates distinct minima, enabling individually addressable spectral responses. These results establish plasmonic TNAs as promising architectures for spectral detection and individual mode switching of single- or multi-QO configurations and empowers the user for the implementation of photonic processing of continuous photon sources.

physics.optics↗

arXiv2026

Toroidal Plasmonic Nanodimers for Enhanced Near-Infrared Emission in Heterostructured InP Quantum Dots

Near-infrared (NIR) emitters operating in the 650-900 nm range are highly attractive for imaging and sensing in turbid media; however, cadmium-free InP-based quantum dots (QDs) often suffer from limited brightness due to nonradiative pathways and inefficient photon outcoupling. In particular, heterostructured InP QDs can exhibit band alignments that induce partial spatial separation of charge carriers, leading to reduced electron-hole wavefunction overlap. This modifies intrinsic recombination dynamics and enhances the sensitivity of their emission to the surrounding photonic environment. Here, we investigate silver toroidal plasmonic nanoantenna dimers (Ag TPNDs) through finite-difference-time-domain (FDTD) simulations as a geometry-tunable platform for enhancing NIR emission of heterostructured InP-based QDs. The coupled toroidal geometry supports strongly confined bonding modes that generate intense nanogap hotspots, while its resonance can be systematically tuned through the toroid aspect ratio. By spectrally aligning the antenna response with QD emission bands (675-845 nm), we achieve large Purcell enhancements together with high quantum efficiencies, demonstrating efficient conversion of enhanced decay rates into radiative emission. We further show that nanometer-scale variations in emitter-antenna separation strongly modulate the radiative rates and spectral response. These results establish toroidal plasmonic nanodimers as a topology-driven platform for controlling emission in NIR quantum emitters and for advancing NIR nanophotonic applications.

physics.optics↗

arXiv2026

Optically Switchable Fluorescence Enhancement at Critical Interparticle Distances

Plasmonic nanostructures provide electric field localization to be used as a fluorescence enhancement tool for the closely located fluorophores. However, metallic structures exhibit non-radiative energy transfer at close proximity, which suppresses the boost in the photoluminescence spectrum due to inhomogeneous medium. Compensation to non-radiative losses is fundamentally restricted, therefore defining the critical interparticle distances, where the fluorescence enhancement is detectable hold utmost importance for device applications. In this work, we numerically identified the critical interparticle distances of a metal nanoparticle (MNP) and quantum emitters (QEs) with angstrom resolution by analyzing the interplay between quantum yield and non-radiative decay. By engaging a collimated light application on silver nanoparticle (AgNP) placed at a critical distance, we simulated an active fluorescence enhancement switch yielding observable 7-fold increase in fluorescence intensity. The provided free space simulation includes the complete response of AgNP with retardation and higher order multi-polar effects for which the previous analytical works fall short. While the model bridges the absorption and emission spectra via corresponding Stokes shift values and presents a general approach for the interaction of QEs and MNPs in Rayleigh regime, it can be extended to Mie regime for larger QEs and can be modified for dielectric device environment.

physics.optics↗

arXiv2025

Continuous and Reversible Electrical Tuning of Fluorescent Decay Rate via Fano Resonance

We demonstrate that the decay rates of a fluorescent molecule can be controlled by electrically shifting a transparency introduced by a Fano resonance. An auxiliary quantum object (QO), located at the hotspot of a plasmonic nanoparticle, suppresses plasmonic excitation at its level spacing ω_QO. As a result, the local density of states (LDOS) associated with the plasmonic spectrum is also suppressed at ω=ω_QO. By shifting ω_QO via an applied voltage, we continuously tune the radiative and nonradiative decay rates of the fluorescent molecule by up to two orders of magnitude. This mechanism offers a valuable tool for integrated quantum technologies, enabling on-demand entanglement and single-photon sources, voltage-controlled quantum gate operations, and electrical control of superradiant-like phase transitions. The approach also holds promise for applications in super-resolution microscopy and surface-enhanced Raman spectroscopy (SERS).

physics.optics↗

arXiv2022

On-demand continuous-variable quantum entanglement source for integrated circuits

Integration of devices generating nonclassical states~(such as entanglement) into photonic circuits is one of the major goals in achieving integrated quantum circuits~(IQCs). This is demonstrated successfully in recent decades. Controlling the nonclassicality generation in these micron-scale devices is also crucial for the robust operation of the IQCs. Here, we propose a micron-scale quantum entanglement device whose nonlinearity (so the generated nonclassicality) can be tuned by several orders of magnitude via an \textit{applied voltage} without altering the linear response. Quantum emitters~(QEs), whose level-spacing can be tuned by voltage, are embedded into the hotspot of a metal nanostructure~(MNS). QE-MNS coupling introduces a Fano resonance in the ``nonlinear response''. Nonlinearity, already enhanced extremely due to localization, can be controlled by the QEs' level-spacing. Nonlinearity can either be suppressed (also when the probe is on the device) or be further enhanced by several orders. Fano resonance takes place in a relatively narrow frequency window so that $\sim$meV voltage-tunability for QEs becomes sufficient for a \textit{continuous} turning on/off of the nonclassicality. This provides as much as 5 orders of magnitude modulation depths.

physics.optics↗

arXiv2019

Electrically Switchable Metadevices via Graphene

Metamaterials bring sub-wavelength resonating structures together to overcome the limitations of conventional materials. The realization of active metadevices has been an outstanding challenge that requires electrically reconfigurable components operating over a broad spectrum with a wide dynamic range. The existing capability of metamaterials, however, is not sufficient to realize this goal. Here, by integrating passive metamaterials with active graphene devices, we demonstrate a new class of electrically controlled active metadevices working in microwave frequencies. The fabricated active metadevices enable efficient control of both amplitude (> 50 dB) and phase (> 90°) of electromagnetic waves. In this hybrid system, graphene operates as a tunable Drude metal that controls the radiation of the passive metamaterials. Furthermore, by integrating individually addressable arrays of metadevices, we demonstrate a new class of spatially varying digital metasurfaces where the local dielectric constant can be reconfigured with applied bias voltages. Additionally, we reconfigure resonance frequency of split ring resonators without changing its amplitude by damping one of the two coupled metasurfaces via graphene. Our approach is general enough to implement various metamaterial systems that could yield new applications ranging from electrically switchable cloaking devices to adaptive camouflage systems.

physics.optics↗