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Ennio Arimondo

Publications and source records attributed to Ennio Arimondo.

At least 19 recordsLinked to original sources

Dark state role in time-reversal symmetry breaking

We investigate the role of the global driving phase $Φ$ in the dynamics of driven few-level quantum systems, a central setting in coherent control of atomic, molecular, and solid-state platforms. In particular, we focus on systems with closed-loop couplings, where external driving fields induce interference effects that strongly influence population transfer and symmetry properties of time-evolution. While full time-reversal symmetry requires $Φ=0,π$, leading to a real Hamiltonian, we focus on a less restrictive transformation, the phase inversion (or complex conjugation of the Hamiltonian), under which population dynamics can remain symmetric even though coherences generally do not. We show that the presence of a dark (spectator) state is a sufficient condition for this population phase symmetry (P$Φ$S), as it constrains the dynamics to reduced subspaces characterized by SU(2) or open-loop SU(3) evolution. We analyze this mechanism in three- and four-level systems and derive general conditions for P$Φ$S that extend to generic $n$-level configurations, with $n$ even. These findings provide practical guidelines for achieving robust control in quantum systems, with potential applications in quantum information processing and quantum computing.

quant-ph↗

Shortcut-to-Adiabatic Controlled-Phase Gate in Rydberg Atoms

A shortcut-to-adiabatic protocol for the realization of a fast and high-fidelity controlled-phase gate in Rydberg atoms is developed. The adiabatic state transfer, driven in the high-blockade limit, is sped up by compensating nonadiabatic transitions via oscillating fields that mimic a counterdiabatic Hamiltonian. High fidelities are obtained in wide parameter regions. The implementation of the bare effective counterdiabatic field, without original adiabatic pulses, enables to bypass gate errors produced by the accumulation of blockade-dependent dynamical phases, making the protocol efficient also at low blockade values. As an application toward quantum algorithms, how the fidelity of the gate impacts the efficiency of a minimal quantum-error correction circuit is analyzed.

quant-ph↗

Multipassage Landau-Zener tunneling oscillations in transverse/longitudinal dual dressing of atomic qubits

We investigate the time evolution of a non-resonant dressed-atom qubit in an XZ original configuration. It is composed of two electromagnetic fields, one oscillating parallel and the other orthogonal to the quantisation magnetic static field. The experiments are performed in rubidium and caesium atomic magnetometers, confined in a magneto-optical trap and in a vapour cell, respectively. Static fields in the $μ$T range and kHz oscillating fields with large Rabi frequencies are applied. This dual-dressing configuration is an extension of the Landau-Zener multipassage interferometry in the presence of an additional dressing field controlling the tunneling process by its amplitude and phase. Our measurement of the qubit coherence introduces additional features to the transition probability readout of standard interferometry. The coherence time evolution is characterized by oscillations at several frequencies, each of them produced by a different quantum contribution. Such frequency description introduces a new picture of the qubit multipassage evolution. Because the present low-frequency dressing operation does not fall within the standard Floquet engineering paradigm based on the high-frequency expansion, we develop an ad-hoc dressing perturbation treatment. Numerical simulations support the adiabatic and non-adiabatic qubit evolution.

quant-ph↗

High-fidelity quantum control via Autler-Townes splitting

We propose quantum control protocols for the high-fidelity preparation of target states in systems with Autler-Townes splitting. We investigate an approximated three-level system obtained from a four-level one by adiabatically eliminating a state that does not participate in the evolution. In our work we use linear, arctan, and Roland-Cerf functions for transferring population between two eigenstates of the system obtaining a high fidelity for long evolution times. Additionally, in order to overcome the restriction given by the lifetimes of the experimental setup, we propose an accelerated adiabatic evolution with a shortcut to adiabaticity protocol, which allows us to reach fidelities close to one but much faster.

quant-ph↗

Bright and dark Autler-Townes states in the atomic Rydberg multilevel spectroscopy

We investigated the Autler-Townes splitting produced by microwave transitions between atomic Rydberg states explored by optical spectroscopy from the ground electronic state. The laser-atom Hamiltonian describing the double irradiation of such a multilevel system is analysed on the basis of the Morris-Shore transformation. The application of this transformation to the microwave-dressed atomic system allows the identification of bright, dark, and spectator states associated with different configurations of atomic states and microwave polarisation. We derived synthetic spectra that show the main features of Rydberg spectroscopy. Complex Autler-Townes spectra are obtained in a regime of strong microwave dressing, where a hybridisation of the Rydberg fine structure states is produced by the driving.

physics.atom-ph↗

Measurements of blackbody radiation-induced transition rates between high-lying S, P and D Rydberg levels

We report experimental measurements of the rates of blackbody radiation-induced transitions between high-lying (n>60) S, P and D Rydberg levels of rubidium atoms in a magneto-optical trap using a hybrid field ionization and state-selective depumping technique. Our results reveal significant deviations of the measured transition rates from theory for well-defined ranges of the principal quantum number. We assume that the most likely cause for those deviations is a modified blackbody spectrum inside the glass cell in which the magneto-optical trap is formed, and we test this assumption by installing electrodes to create an additional microwave cavity around the cell. From the results we conclude that it should be possible to use such external cavities to control and suppress the blackbody radiation-induced transitions.

physics.atom-ph↗

Atomic interactions for qubit-error compensations

Experimental imperfections induce phase and population errors in quantum systems. We present a method to compensate unitary errors affecting also the population of the qubit states. This is achieved through the interaction of the target qubit with an additional control qubit. We show that our approach works well for single-photon and two-photon excitation schemes. In the first case, we study two reduced models (i) a two-level system in which the interaction corresponds to an effective level shift and (ii) a three-level one describing two qubits in the Bell triplet subspace. In the second case, instead, a double-STIRAP process is presented with comparable compensation efficiency with respect to the single-photon case.

quant-ph↗

Harmonic dual dressing of spin one-half systems

Controlled modifications of the quantum magnetic response are produced in dressed systems by a high frequency, strong and not-resonant electromagnetic field. This quantum control is greatly enhanced and enriched by the harmonic, commensurable and orthogonally oriented dual dressing theoretically discussed here. The secondary field enables a fine tuning of the qubit response, with control parameters amplitude, harmonic content, spatial orientation and phase relation. Our analysis is based on a perturbative approach and includes few numerical solutions. The long-time dynamics is described in terms of an anisotropic effective static magnetic field representing the handle for the system full engineering. Through a low-order harmonic mixing the bichromatic driving generates a rectified static field acting on the spin. The Zeeman response becomes anisotropic in a triaxial geometry and includes a quadratic contribution. Our dressing increases the two-level energy splitting, improving the spin detection sensitivity. On the low field direction it compensates the static fields applied in different geometries. A resonant spin exchange between two species having very different magnetic response as electron and nucleus is allowed by the dressing. The spin temporal evolution includes a micromotion at harmonics of the driving frequency whose role in the spin detection is examined and can be exploited in quantum information. The results presented here lay a foundation for additional applications to be harnessed in quantum simulations.

quant-ph↗

Harmonic fine tuning and triaxial spatial anisotropy of dressed atomic spins

The addition of a weak oscillating field modifying strongly dressed spins enhances and enriches the system quantum dynamics. Through low-order harmonic mixing the bichromatic driving generates additional rectified static field acting on the spin system. The secondary field allows for a fine tuning of the atomic response and produces effects not accessible with a single dressing field, such as a spatial triaxial anisotropy of the spin coupling constants and acceleration of the spin dynamics. This tuning-dressed configuration introduces an extra handle for the system full engineering for quantum control applications. Tuning amplitude, harmonic content, spatial orientation and phase relation are control parameters. A theoretical analysis, based on perturbative approach, is experimentally validated by applying a bichromatic radiofrequency field to an optically pumped Cs atomic vapour. We measure the resonance shifts produced by tuning fields up to the third harmonic.

quant-ph↗

Progress and perspectives on composite laser-pulses spectroscopy for high-accuracy optical clocks

Probing an atomic resonance without disturbing it is an ubiquitous issue in physics. This problem is critical in high-accuracy spectroscopy or for the next generation of atomic optical clocks. Ultra-high resolution frequency metrology requires sophisticated interrogation schemes and robust protocols handling pulse length errors and residual frequency detuning offsets . This review reports recent progress and perspective in such schemes, using sequences of composite laser-pulses tailored in pulse duration, frequency and phase, inspired by NMR techniques and quantum information processing. After a short presentation of Rabi technique and NMR-like composite pulses allowing efficient compensation of electromagnetic field perturbations to achieve robust population transfers, composite laser-pulses are investigated within Ramsey's method of separated oscillating fields in order to generate non-linear compensation of probe-induced frequency shifts. Laser-pulses protocols such as Hyper-Ramsey (HR), Modified Hyper-Ramsey (MHR), Generalized Hyper-Ramsey (GHR) and hybrid schemes are reviewed. These techniques provide excellent protection against both probe induced light-shift perturbations and laser intensity variations. More sophisticated schemes generating synthetic frequency-shifts are presented. They allow to reduce or completely eliminate imperfect correction of probe-induced frequency-shifts even in presence of decoherence due to the laser line-width. Finally, two universal protocols are presented which provide complete elimination of probe-induced frequency shifts in the general case where both decoherence and relaxation dissipation effects are present by using exact analytic expressions for phase-shifts and the clock frequency detuning. These techniques might be applied to atomic, molecular and nuclear frequency metrology, mass spectrometry as well as precision spectroscopy.

physics.atom-ph↗

Experimental signatures of an absorbing-state phase transition in an open driven many-body quantum system

Understanding and probing phase transitions in non-equilibrium systems is an ongoing challenge in physics. A particular instance are phase transitions that occur between a non-fluctuating absorbing phase, e.g., an extinct population, and one in which the relevant order parameter, such as the population density, assumes a finite value. Here we report the observation of signatures of such a non-equilibrium phase transition in an open driven quantum system. In our experiment rubidium atoms in a quasi one-dimensional cold disordered gas are laser-excited to Rydberg states under so-called facilitation conditions. This conditional excitation process competes with spontaneous decay and leads to a crossover between a stationary state with no excitations and one with a finite number of excitations. We relate the underlying physics to that of an absorbing state phase transition in the presence of a field (i.e. off-resonant excitation processes) which slightly offsets the system from criticality. We observe a characteristic power-law scaling of the Rydberg excitation density as well as increased fluctuations close to the transition point. Furthermore, we argue that the observed transition relies on the presence of atomic motion which introduces annealed disorder into the system and enables the formation of long-ranged correlations. Our study paves the road for future investigations into the largely unexplored physics of non-equilibrium phase transitions in open many-body quantum systems.

cond-mat.stat-mech↗

Pulsed high magnetic field measurement via a Rubidium vapor sensor

We present a new technique to measure pulsed magnetic fields based on the use of Rubidium in gas phase as a metrological standard. We have therefore developed an instrument based on laser inducing transitions at about 780~nm (D2 line) in a Rubidium gas contained in a mini-cell of 3~mm~x~3~mm cross section. To be able to insert such a cell in a standard high field pulsed magnet we have realized a fibred probe kept at a fixed temperature. Transition frequencies for both the $π$ (light polarization parallel to the magnetic field) and $σ$ (light polarization perpendicular to the magnetic field) configurations are measured by a commercial wavemeter. One innovation of our sensor is that in addition of monitoring the light transmitted by the Rb cell, which is usual, we also monitor the fluorescence emission of the gas sample from a very small volume with the advantage of reducing the impact of the field inhomogeneity on the field measurement. Our sensor has been tested up to about 58~T.

physics.atom-ph↗

Probe light-shift elimination in Generalized Hyper-Ramsey quantum clocks

We present a new interrogation scheme for the next generation of quantum clocks to suppress frequency-shifts induced by laser probing fields themselves based on Generalized Hyper-Ramsey resonances. Sequences of composite laser pulses with specific selection of phases, frequency detunings and durations are combined to generate a very efficient and robust frequency locking signal with almost a perfect elimination of the light-shift from off resonant states and to decouple the unperturbed frequency measurement from the laser's intensity. The frequency lock point generated from synthesized error signals using either $π/4$ or $3π/4$ laser phase-steps during the intermediate pulse is tightly protected against large laser pulse area variations and errors in potentially applied frequency shift compensations. Quantum clocks based on weakly allowed or completely forbidden optical transitions in atoms, ions, molecules and nuclei will benefit from these hyper-stable laser frequency stabilization schemes to reach relative accuracies below the 10$^{-18}$ level.

physics.atom-ph↗

Seeded excitation avalanches in off-resonantly driven Rydberg gases

We report an experimental investigation of the facilitated excitation dynamics in off-resonantly driven Rydberg gases by separating the initial off-resonant excitation phase from the facilitation phase, in which successive facilitation events lead to excitation avalanches. We achieve this by creating a controlled number of initial seed excitations. Greater insight into the avalanche mechanism is obtained from an analysis of the full counting distributions. We also present simple mathematical models and numerical simulations of the excitation avalanches that agree well with our experimental results.

physics.atom-ph↗

Quasi-forbidden 2-body Förster resonances in cold Cs Rydberg gas

Cold Rydberg atoms are known to display dipole-dipole interaction allowed resonances, also called Förster resonances, which lead to an efficient energy transfer when the proper electric field is used. This electric field also enables resonances which do not respect the dipole-dipole selection rules under zero field. A few of these quasi-forbidden resonances have been observed but they are often overlooked. Here we show that in cold $^{133}$Cs atoms there is a large number of these resonances that display a significant transfer efficiency due to their strong interactions, even at low electric field. We also develop a graphical method enabling to find all possible resonances simultaneously. The resulting dramatic increase in the total number of addressable resonant energy transfers at different electric fields could have implications in the search for few-body interactions or macro-molecules built from Rydberg atoms.

physics.atom-ph↗

Four-level N-scheme crossover resonances in Rb saturation spectroscopy in magnetic fields

We perform saturated absorption spectroscopy on the D$\_2$ line for room temperature rubidium atoms immersed in magnetic fields within the 0.05-0.13 T range. At those medium-high field values the hyperfine structure in the excited state is broken by the Zeeman effect, while in the ground state hyperfine structure and Zeeman shifts are comparable. The observed spectra are composed by a large number of absorption lines. We identify them as saturated absorptions on two-level systems, on three-level systems in a V configuration and on four-level systems in a N or double-N configuration where two optical transitions not sharing a common level are coupled by spontaneous emission decays. We analyze the intensity of all those transitions within a unified simple theoretical model. We concentrate our attention on the double-N crossovers signals whose intensity is very large because of the symmetry in the branching ratios of the four levels. We point out that these structures, present in all alkali atoms at medium-high magnetic fields, have interesting properties for electromagnetically induced transparency and slow light applications.

physics.atom-ph↗

Three-level superadiabatic quantum driving

The superadiabatic quantum driving, producing a perfect adiabatic transfer on a given Hamitonian by introducing an additional Hamiltonian, is theoretically analysed for transfers within a three-level system. Our starting point is the stimulated Raman adiabatic passage, realized through different schemes of laser pulses. We determine the superadiabatic correction for each scheme. The fidelity, robustness and transfer time of all the superadiabatic transfer schemes are discussed. We derive that all superadiabatic corrections are based on a $π$- (or near-$π$)-area pulse coupling between the initial and final states. The benefits in the protocol robustness overcome the difficulties associated to the actual implementation of the three-level superadiabatic transfer.

quant-ph↗

Continued fraction analysis of dressed systems: application to periodically driven optical lattices

Radio-frequency quantum engineering of spins is based on the dressing by a non resonant electromagnetic field. Radio-frequency dressing occurs also for the motion of particles, electrons or ultracold atoms, within a periodic spatial potential. The dressing, producing a renormalisation and also a freeze of the system energy, is described by different approaches, dressed atom, magnetic resonance semiclassical treatment, continued fraction solution of the Schrödinger equation. A comparison between those solutions points out that the semiclassical treatment, to be denoted as the $S$-solution, represents the most convenient tool to evaluate the tunneling renormalization of ultracold atoms.

physics.atom-ph↗