SearcharxivSearch

arXiv subjects

Enze Lv

Publications and source records attributed to Enze Lv.

9 recordsLinked to original sources

$5/9-$Magnetization Plateau and Spin Supersolidity in YCu$_3$(OD)$_{7-x}$Br$_{2+x}$ under Magnetic Fields up to 120~T

We performed high-precision magnetization measurements up to 120~T on three compositions of the newly discovered kagome antiferromagnet YCu$_3$(OD)$_{7-x}$Br$_{2+x}$ (YCOB), revealing a previously unobserved 5/9 fractional magnetization plateau. All YCOB samples with different Br$^-$ concentrations exhibit nearly identical magnetization curves below 60~T, whereas the 5/9 plateau appears at markedly different fields in the ultrahigh-field regime. By modeling the experimental data using tensor-network calculations, we derive the effective spin Hamiltonians for the YCOB family with three spatially anisotropic Heisenberg couplings (the 3$J$-type model), which quantitatively reproduces the measured magnetization processes and captures the composition-dependent evolution of the 5/9 plateau. Furthermore, our theoretical analysis suggests the emergence of a spin supersolid phase in the field window between the 1/3 and 5/9 plateaus, which is sensitive to spin exchange parameters and accounts for the significant variation in the critical fields of the 5/9 plateau observed among different YCOB compositions.

cond-mat.str-el

Berezinskii-Kosterlitz-Thouless Quantum Supercriticality in XXZ Heisenberg Spin Chain

Quantum fluctuations can give rise to a singular quantum critical point (QCP) in the ground state, whose influence extends to finite temperatures, forming a quantum critical regime (QCR). Recently, it has been shown that in the quantum Ising model, the symmetry-breaking, longitudinal field can induce a quantum supercritical regime (QSR) emanating from the QCP, which hosts a universally enhanced quantum supercritical magnetocaloric effect (MCE). In this paper, we show that the QSR also emerges in the spin-1/2 XXZ model, in both the form of Ising and Berezinskii-Kosterlitz-Thouless (BKT) supercriticality. Using ground-state and finite-temperature tensor-network methods, we investigate quantum supercritical phenomena near a BKT QCP. We reveal a quantum supercritical crossover scaling $T \propto h^{2/3}$ and a Gr\"uneisen ratio scaling $\Gamma_h \propto T^{-3/2}$ for the BKT QCP, which differ from the corresponding Ising supercritical scalings. Nevertheless, we find that the scaling function $\phi_{\Gamma}(x)$ of the singular Gr\"uneisen ratio for both BKT and Ising cases can be approximately described by the same expression $\phi_{\Gamma}(x) \approx x/(1+x^2)$. Our work extends the study of quantum supercritical phenomena from the Ising to the XXZ Heisenberg model, thereby revealing the presence of BKT quantum supercriticality and broadening the scope of quantum supercritical physics.

cond-mat.str-el

Universally Diverging Gr\"uneisen Ratio of Holographic Quantum Criticality

Quantum criticality is a hallmark of strongly correlated electron systems, as seen in heavy-fermion materials and high-temperature superconductors. Holographic duality provides a powerful framework to investigate these systems by translating them into weakly coupled classical gravity living in one higher dimension. Here, we harness this approach to study a field-induced quantum critical point with dynamical exponent $z=3$ in Einstein-Maxwell-Chern-Simons theory. Our analysis of its thermodynamic properties reveals a new universality class. Notably, we identify a diverging Gr\"uneisen ratio with universal scaling $\sim T^{-2/3}$, a behavior that closely mirrors recent experiments on the heavy-fermion material CeRh$_6$Ge$_4$. These findings advance our understanding of metallic quantum criticality and highlight the potential of holographic duality as a tool for studying correlated quantum matters.

cond-mat.str-el

Ising Supercriticality and Universal Magnetocalorics in Spiral Antiferromagnet Nd$_3$BWO$_9$

The celebrated analogy between the pressure-temperature phase diagram of a liquid-gas system and the field-temperature phase diagram of a ferromagnet has long been a cornerstone for understanding universality of phase transitions and critical phenomena. Here we extend this analogy to a highly frustrated antiferromagnet, the spiral Ising compound Nd$_3$BWO$_9$ with kagome layers. In its phase diagram, we identify a metamagnetic transition line with a critical endpoint (CEP) located at $\mu_0H_{\mathrm{c}} \simeq 1.04$ T and $T_{\mathrm{c}} \simeq 0.3$ K. Above the CEP, an Ising supercritical regime emerges with crossover lines that follow a universal scaling law, as evidenced by the specific heat, magnetic susceptibility, and magnetocaloric measurements. Remarkably, we observe highly sensitive magnetic cooling near the emergent CEP, characterized by a divergent magnetic Gr\"uneisen ratio $\Gamma_H \propto 1/t^{\beta+\gamma-1}$, with $\beta + \gamma \simeq 1.563$ the sum of critical exponents of the 3D Ising universality class and $t \equiv (T-T_{\rm c})/T_{\rm c}$ the reduced temperature. Adiabatic demagnetization from 2 K and 4 T reaches a minimum temperature of 195 mK, via a self-cascading process that combines supercritical and topological cooling. Our findings open a new avenue for studying supercritical phenomena and magnetic refrigeration with the frustrated rare-earth compounds RE$_3$BWO$_9$ and, more broadly, in Ising-anisotropic antiferromagnets such as spin ices.

cond-mat.str-el

Universal Scaling Functions of the Gr{\"u}neisen Ratio near Quantum Critical Points

The Gr\"uneisen ratio, defined as $\Gamma_g \equiv (1/T) (\partial T/\partial g)_S$, serves as a highly sensitive probe for detecting quantum critical points (QCPs) driven by an external feild $g$ and for characterizing the magnetocaloric effect (MCE). Near a QCP, the Gr\"uneisen ratio displays a universal divergence which is governed by a universality-class-dependent scaling function stemming from the scale invariance. In this work, we systematically investigate the universal scaling functions of Gr\"uneisen ratio in both one-dimensional (1D) and two-dimensional (2D) quantum spin systems, including the transverse-field Ising model, the spin-1/2 Heisenberg model, the quantum $q$-state Potts model ($q=3,4$) and the $J_1$-$J_2$ columnar dimer model. Our approach employs the thermal tensor-network method for infinite-size 1D systems and the stochastic series expansion quantum Monte Carlo (SSE QMC) simulations for 2D systems, enabling precise calculations of the Gr\"uneisen ratio near QCPs. Through data collapse analysis, we extract the corresponding scaling functions, which establish quantitative frameworks to interpret magnetocaloric experiments and guide the development of ultralow-temperature refrigeration.

cond-mat.str-el

Universal Magnetocaloric Effect near Quantum Critical Point of Magnon Bose-Einstein Condensation

Bose-Einstein condensation (BEC), a macroscopic quantum phenomenon arising from phase coherence and bosonic statistics, has been realized in quantum magnets. Here, we report the observation of a universal magnetocaloric effect (MCE) near a BEC quantum critical point (QCP) in copper sulfate crystal ($CuSO_4 \cdot 5H_2O$). By conducting magnetocaloric and nuclear magnetic resonance measurements, we uncover a field-driven BEC QCP, evidenced by the universal scaling law $T_c \propto (B_c - B)^{2/3}$ and the perfect data collapse of the magnetic Gr\"uneisen ratio. Thermal excitation triggers a dimensional crossover to a 1D quantum-critical regime, where the MCE scaling strictly matches the universality class of 1D Fermi gases. Notably, the quantum-critical MCE enables cooling down to 12.8 mK without helium-3, with very fast thermal relaxation rate that is critical for high cooling power. This work demonstrates the universal MCE in magnon BEC systems, using a common copper sulfate compound as a paradigmatic example, and paves the way for next-generation sub-Kelvin cooling.

cond-mat.str-el

Quantum Supercritical Regime with Universal Magnetocaloric Scaling in Ising Magnets

Quantum critical points ubiquitously emerge in strongly correlated systems, with their influence persisting at finite temperatures and external fields. A paradigmatic example is the quantum Ising magnet, where transverse field $g$ controlling quantum fluctuations can expand the quantum critical point into an extended quantum critical regime. In this work, we propose a distinct quantum supercritical regime originating also from the quantum critical point but controlled by the longitudinal field $h$ coupled to the order parameter. Through thermal tensor network simulations, we find the quantum supercritical regime is enclosed by the finite-temperature crossover boundaries $T \propto h^{{z\nu}/\Delta}$, where $z$, $\nu$ and $\Delta \equiv \beta+\gamma$ are critical exponents. We comprehend the supercritical scaling via thermal data collapse based on the derived scaling form. Amongst other intriguing phenomena in quantum supercritical regime, there exists an enhanced magnetocaloric effect characterized by a universally diverging magnetic Gr\"uneisen ratio $\Gamma_h \propto T^{-\Delta/{z\nu}}$, which indicates that a small symmetry-breaking field $h$ can generate dramatic temperature variation. We propose to observe the quantum supercritical regime in Ising-chain compound CoNb$_2$O$_6$ and related quantum materials, revealing a helium-3-free pathway to millikelvin cooling via the supercritical magnetocaloric effect.

cond-mat.str-el

Magnetocaloric Effect of Topological Excitations in Kitaev Magnets

Traditional magnetic sub-Kelvin cooling relies on the nearly free local moments in hydrate paramagnetic salts, whose utility is hampered by the dilute magnetic ions and low thermal conductivity. Here we propose to use instead fractional excitations inherent to quantum spin liquids (QSLs) as an alternative, which are sensitive to external fields and can induce a very distinctive magnetocaloric effect. With state-of-the-art tensor-network approach, we compute low-temperature properties of Kitaev honeycomb model. For the ferromagnetic case, strong demagnetization cooling effect is observed due to the nearly free $Z_2$ vortices via spin fractionalization, described by a paramagnetic equation of state with a renormalized Curie constant. For the antiferromagnetic Kitaev case, we uncover an intermediate-field gapless QSL phase with very large spin entropy, possibly due to the emergence of spinon Fermi surface. Potential realization of topological excitation cooling in Kitaev materials is also discussed, which may offer a promising pathway to circumvent existing limitations in the paramagnetic hydrates.

cond-mat.str-el

Quantum Supercritical Crossover with Dynamical Singularity

Bounded by crossover lines exhibiting universal scaling, the supercritical regime above the critical endpoint is characterized by strong fluctuations and intriguing phenomena. In this study, we extend this notable concept of supercritical crossover to the quantum critical endpoint (QCEP), by studying the prototypical mixed-field quantum Ising and Potts models through tensor network calculations and scaling analyses. We reveal the existence of quantum supercritical (QSC) crossover lines, determined by not only response functions but also quantum information quantities, near the QCEP. A supercritical scaling law, $h \sim (g - g_c)^{\Delta}$, is found, where $g$ ($h$) is the transverse (longitudinal) field, $g_c$ is the critical field, and $\Delta$ is the so-called gap exponent of the QCEP. Moreover, we demonstrate that the QSC crossover line acts as a boundary for the emergence of dynamical singularities in quench dynamics. This singularity manifests as a distinctive cusp with a critical exponent of 1/2, signaling a new dynamical universality class. We also propose utilizing Rydberg atom arrays as an experimental platform to observe these QSC crossovers and dynamical singularities. Our work establishes a theoretical framework for understanding the role of QCEP and associated supercritical crossovers in both equilibrium and non-equilibrium quantum many-body systems.

cond-mat.str-el