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Eric A. Wolf

Publications and source records attributed to Eric A. Wolf.

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Riemann Rarefaction Waves in a Strongly Interacting Fermi Gas

We investigate the expansion of a homogeneous, strongly interacting Fermi gas released into vacuum in a ``shock tube'' geometry. At unitarity, where the gas is scale invariant and nearly inviscid, we find that the resulting rarefaction wave dynamics are self-similar and in excellent agreement with Riemann's solution of the Euler equation for all temperatures probed. Probing interactions away from unitarity within the BEC-BCS crossover, we observe increasing deviations from the Riemann solution as viscosity increases. However, even on the BCS side, where the sound diffusivity is increased twenty-fold, self-similarity is still approximately preserved. This may reflect how 1D Navier-Stokes rarefaction flows approach Euler self-similar solutions at long times. Our work demonstrates the utility of strongly interacting Fermi gases for the study of nonlinear hydrodynamics in a highly controllable setting.

cond-mat.quant-gas

Geminate Exciton Fusion Fluorescence as a Probe of Triplet Exciton Transport after Singlet Fission

The geminate annihilation of two triplet excitons created by singlet exciton fission is affected by the dimensionality of transport as determined by typically anisotropic triplet exciton mobilities in organic molecular crystals. We analyze this process using a random-walk model where the time-dynamics of the geminate annihilation probability is determined by the average exciton hopping times along the crystallographic directions. The model is then applied to the geminate fluorescence dynamics in rubrene, where the main channel for triplet-triplet annihilation is via triplet fusion and subsequent photon emission, and we identify the transitions between transport in one, two, and three dimensions.

cond-mat.mtrl-sci

Quantum Beats of a Multiexciton State in Rubrene Single Crystals

We observe quantum beats in the nanosecond-scale photoluminescence decay of rubrene single crystals after photoexcitation with short laser pulses in a magnetic field of 0.1 to 0.3 T. The relative amplitude of the quantum beats is of the order of 5\%. Their frequency is $1.3$ GHz when the magnetic field is oriented parallel to the two-fold rotation axis of the rubrene molecules and decreases to $0.6$ GHz when the magnetic field is rotated to the crystal's molecular stacking direction. The amplitude of the quantum beats decays alongside the non-oscillatory photoluminescence background, which at low excitation densities has an exponential decay time of $ 4.0 \pm 0.2$~ns. We interpret this as the effective lifetime of a multiexciton state that originates from singlet-fission and can undergo geminate recombination back to the singlet state.

cond-mat.mtrl-sci