arXiv subjects

Eric B. Norrgard

Publications and source records attributed to Eric B. Norrgard.

17 recordsLinked to original sources

arXiv2026

Development of a Quantum Blackbody Thermometer toward Primary On-orbit Thermometry

We present a roadmap to a deployable, intrinsically calibrated thermometer with long-term accuracy of 30 mK, exceeding existing on-orbit resistance-based thermometers. Our quantum blackbody thermometer is based on measuring fluorescence ratios of optically excited rubidium atoms in microfabricated vapor cells. The key advantage of the quantum blackbody thermometer is that long-term stability of the fluorescence ratios is guaranteed by the immutable physical properties (transition strengths) of the rubidium atom. This should be compared against resistance-based thermometers, such as platinum resistance thermometers, which may be calibrated with exceptional accuracy but are susceptible to temporal drift and shifts due to improper handling.

physics.atom-ph↗

arXiv2025

Atomic and molecular systems for radiation thermometry

Atoms and simple molecules are excellent candidates for new standards and sensors because they are both all identical and their properties are determined by the immutable laws of quantum physics. Here, we introduce the concept of building a standard and sensor of radiative temperature using atoms and molecules. Such standards are based on precise measurement of the rate at which blackbody radiation (BBR) either excites or stimulates emission for a given atomic transition. We summarize the recent results of two experiments while detailing the rate equation models required for their interpretation. The cold atom thermometer (CAT) uses a gas of laser cooled $^{85}$Rb Rydberg atoms to probe the BBR spectrum near 130~GHz. This primary, {\it i.e.}, not traceable to a measurement of like kind, temperature measurement currently has a total uncertainty of approximately 1~\%, with clear paths toward improvement. The compact blackbody radiation atomic sensor (CoBRAS) uses a vapour of $^{85}$Rb and monitors fluorescence from states that are either populated by BBR or populated by spontaneous emission to measure the blackbody spectrum near 24.5~THz. The CoBRAS has an excellent relative precision of $u(T)\approx 0.13$~K, with a clear path toward implementing a primary

physics.atom-ph↗

arXiv2025

Population-resolved measurement of an avoided crossing of light-dressed states

A two-level system coupled by a coherent field is a ubiquitous system in atomic and molecular physics. In the rotating wave approximation, the light-dressed states are well described by a simple 2x2 Hamiltonian which can be easily solved analytically and is thus used in quantum mechanics education and as a basis for intuition for more complicated systems. The solution to the Hamiltonian is an avoided crossing between the light-dressed ground and excited states. In experiments, the avoided crossing is probed spectroscopically, meaning only the energies, or eigenvalues of the Hamiltonian, are measured. Here, we present a measurement of the avoided crossing which also resolves population, thus indicating the amplitude coefficients of the eigenvectors of the Hamiltonian. We perform the measurement in Rydberg states of cold rubidium atoms, resolving the energies spectroscopically with our pump lasers and the populations of each state using selective field ionization.

physics.atom-ph↗

arXiv2024

Compact Blackbody Radiation Atomic Sensor: Measuring Temperature using Optically Excited Atoms in Vapor Cells

We demonstrate a blackbody radiation thermometer based on optically excited rubidium atoms in a vapor cell. The temperature measurement is fast, with statistical uncertainty as low as 0.1% in one second. We resolve temperature with a precision of 0.04% in the range 308 K to 344 K when averaging for several seconds. Additionally, we describe an extension to this measurement scheme where the device operates as a self-calibrated, or primary, thermometer. We make progress toward realizing a primary thermometer by demonstrating a temperature-dependent self-consistent calibration scheme, with temperature accuracy of order 1% limited by the uncertainty in atomic transition dipole matrix elements.

physics.atom-ph↗

arXiv2024

Primary quantum thermometry of mm-wave blackbody radiation via induced state transfer in Rydberg states of cold atoms

Rydberg states of alkali atoms are highly sensitive to electromagnetic radiation in the GHz-to-THz regime because their transitions have large electric dipole moments. Consequently, environmental blackbody radiation (BBR) can couple Rydberg states together at $μ$s timescales. Here, we track the BBR-induced transfer of a prepared Rydberg state to its neighbors and use the evolution of these state populations to characterize the BBR field at the relevant wavelengths, primarily at 130 GHz. We use selective field ionization readout of Rydberg states with principal quantum number $n\sim30$ in $^{85}$Rb and substantiate our ionization signal with a theoretical model. With this detection method, we measure the associated blackbody-radiation-induced time dynamics of these states, reproduce the results with a simple semi-classical population transfer model, and demonstrate that this measurement is temperature sensitive with a statistical sensitivity to the fractional temperature uncertainty of 0.09 Hz$^{-1/2}$, corresponding to 26 K$\cdot$Hz$^{-1/2}$ at room temperature. This represents a calibration-free SI-traceable temperature measurement, for which we calculate a systematic fractional temperature uncertainty of 0.006, corresponding to 2 K at room temperature when used as a primary temperature standard.

physics.atom-ph↗

arXiv2024

Revisiting collisional broadening of $^{85}$Rb Rydberg levels: conclusions for vapor cell manufacture

Electrometry based on electromagnetically induced transparency (EIT) in alkali Rydberg vapor cells may suffer reduced sensitivity due to spurious line broadening effects, caused by surface charges, contaminant gases, or other manufacturing defects. In order to draw conclusions about the deleterious effects of potential contaminant gases inside Rydberg electrometry vapor cells, we revisit collisional broadening and shifts of both the D$_2$ line and Rydberg levels of rubidium. Specifically, we measure the broadening and shifts of the $5{\rm S}_{1/2}\rightarrow 5{\rm P}_{3/2}$ (i.e., the D$_2$ line) and $5{\rm S}_{1/2}\rightarrow 5{\rm P}_{3/2}\rightarrow (25{\rm D},27{\rm S},30{\rm D},32{\rm S},35{\rm D},37{\rm S})$ transitions of $^{85}$Rb due to He, Ne, N$_2$ and Ar. By combining these measurements with observations of velocity changing collisions in the sub-Doppler spectrum of the D$_2$ line, we conclude the following: (1) that contaminant gases are most likely not the cause of irregular line shapes or shifts of Rydberg transitions due to the high pressures required, and (2) the sub-Doppler spectrum of the D$_2$ line, through its accompanying loss of contrast at high pressures, can validate that a vapor cell is sufficiently free of contaminant gas for EIT electrometry. We use the theory of Omont, J. Phys. France 38, 1343 (1977), to extend our results to a wide variety of possible contaminant gases and further derive scaling laws applicable to all gases.

physics.atom-ph↗

arXiv2024

Spectroscopy of laser cooling transitions in MgF

We measure the complete set of transition frequencies necessary to laser cool and trap MgF molecules. Specifically, we report the frequency of multiple low $J$ transitions of the $X^2Σ^+(v^{\prime\prime}=0,1) \rightarrow A^2Π_{1/2}(v^\prime=0)$, $X^2Σ^+(v^{\prime\prime}=1,2) \rightarrow A^2Π_{1/2}(v^\prime=1)$, and $X^2Σ^+(v^{\prime\prime}=1) \rightarrow B^2Σ^+(v^{\prime}=0)$ bands of MgF. The measured $X^2Σ^+(v^{\prime\prime}=1)\rightarrow B^2Σ^+(v^\prime=0)$ spectrum allowed the spin-rotation and hyperfine parameters of the $B^2Σ^+(v=0)$ state of MgF to be determined. Furthermore, we demonstrate optical cycling in MgF by pumping molecules into the $X^2Σ^+(v=1,2)$ states. Optical pumping enhances the spectroscopic signals of transitions originating in the $N^{\prime\prime}=1$ level of the $X^2Σ^+(v^{\prime\prime}=1,2)$ states.

physics.atom-ph↗

arXiv2024

Investigation of fluorescence versus transmission readout for three-photon Rydberg excitation used in electrometry

We present a three-photon based fluorescence readout method where the strength of the fluorescence scales with the strength of the radio-frequency (RF) field being applied. We compare this method to conventional three-photon electromagnetically-induced transparency (EIT) and electromagnetically-induced absorption (EIA). Our demonstrated EIA/EIT sensitivity in the collinear three-photon Cesium system is the best reported to date at roughly 30 uVm^{-1}Hz^{-1/2}. The fluorescence is nearly 4 fold better in sensitivity compared to EIA/EIT readout.

quant-ph↗

arXiv2023

Simulations of a frequency-chirped magneto-optical trap of MgF

We simulate the capture process of MgF molecules into a frequency-chirped molecular MOT. Our calculations show that by chirping the frequency, the MOT capture velocity is increased by about of factor of 4 to 80 m/s, allowing for direct loading from a two-stage cryogenic buffer gas beam source. Moreover, we simulate the effect of this frequency chirp for molecules already present in the MOT. We find that the MOT should be stable with little to no molecule loss. The chirped MOT should thus allow loading of multiple molecule pulses to increase the number of trapped molecules

physics.atom-ph↗

arXiv2021

Electromagnetically induced transparency based Rydberg-atom sensor for quantum voltage measurements

We investigate the Stark shift in Rydberg rubidium atoms through electromagnetically induced transparency for the measurement of direct current (dc) and 60~Hz alternating current (ac) voltages. This technique has direct applications to atom-based measurements of dc and ac voltage and the calibration of voltage instrumentation. We present experimental results for different atomic states that allow for dc and ac voltage measurements ranging from 0~V to 12~V. A Rydberg atom-based voltage standard could become an alternative calibration method with more favorable size, weight, power consumption, and cost compared to the more precise Josephson voltage standard. In this study, we also demonstrate how the voltage measurements can be utilized to determine the atomic polarizability for the Rydberg states. The Rydberg atom-based voltage measurement technology would become a complimentary method for dissemination of the voltage scale directly to the end user.

physics.atom-ph↗

arXiv2021

Quantum Blackbody Thermometry

Blackbody radiation (BBR) sources are calculable radiation sources that are frequently used in radiometry, temperature dissemination, and remote sensing. Despite their ubiquity, blackbody sources and radiometers have a plethora of systematics. We envision a new, primary route to measuring blackbody radiation using ensembles of polarizable quantum systems, such as Rydberg atoms and diatomic molecules. Quantum measurements with these exquisite electric field sensors could enable active feedback, improved design, and, ultimately, lower radiometric and thermal uncertainties of blackbody standards. A portable, calibration-free Rydberg-atom physics package could also complement a variety of classical radiation detector and thermometers. The successful merger of quantum and blackbody-based measurements provides a new, fundamental paradigm for blackbody physics.

physics.atom-ph↗

arXiv2020

Measurement of the molecular dipole moment and the hyperfine and $Λ$-doublet splittings of the $B^3Π_1$ state of thallium fluoride

We report high-precision measurements on the thallium fluoride $\tilde{J} = 1$ hyperfine manifold of the $B^3Π_1$ ($ν= 0$) state. This state is of special interest because it is central to an optical cycling scheme that is envisioned to play an important role in enhancing the sensitivity of the CeNTREX nuclear Schiff-moment experiment presently under construction. The measurements are made by monitoring the fluorescence induced by narrow-band laser excitation of a cryogenic molecular beam. We use a multipass arrangement of the laser beam to enhance fluorescence. When viewed with a camera, we can spatially resolve images from adjacent passes that approach the molecules from opposing directions. These images yield a sensitive visual method to identify the central frequency of a transition. Coupling these line-center determinations with frequency calibration from an acousto-optic modulator has allowed a more precise determination of the $\tilde{J} = 1$ manifold of hyperfine level splittings. We observe Stark shifts of the $\tilde{J} = 1$ levels and infer a permanent electric dipole moment of 2.28(7) D and $Λ$-doublet splittings for the $F_1' = 1/2$ and $F_1' = 3/2$ manifolds of 14.4(9) MHz and 17.4(11) MHz, respectively.

physics.atom-ph↗

arXiv2020

Nuclear spin-dependent parity-violating effects in light polyatomic molecules

Measurements of nuclear spin-dependent parity-violating (NSD-PV) effects provide an excellent opportunity to test nuclear models and to search for physics beyond the Standard Model. Molecules possess closely-spaced states with opposite parity which may be easily tuned to degeneracy to greatly enhance the observed parity-violating effects. A high-sensitivity measurement of NSD-PV effects using light triatomic molecules is in preparation [E. B. Norrgard, et al., Commun. Phys. 2, 77 (2019)]. Importantly, by comparing these measurements in light nuclei with prior and ongoing measurements in heavier systems, the contribution to NSD-PV from $Z^0$-boson exchange between the electrons and the nuclei may be separated from the contribution of the nuclear anapole moment. Furthermore, light triatomic molecules offer the possibility to search for new particles, such as the postulated $Z^{\prime}$ boson. In this work, we detail a sensitive measurement scheme and present high-accuracy molecular and nuclear calculations needed for interpretation of NSD-PV experiments on triatomic molecules composed of light elements Be, Mg, N, and C. The ab initio nuclear structure calculations, performed within the No-Core Shell Model (NCSM) provide a reliable prediction of the magnitude of different contributions to the NSD-PV effects in the four nuclei. These results differ significantly from the predictions of the standard single-particle model and highlight the importance of including many-body effects in such calculations. In order to extract the NSD-PV contributions from measurements, a parity-violating interaction parameter $W_{\text{PV}}$, which depends on molecular structure, needs to be known with high accuracy. We have calculated these parameters for the triatomic molecules of interest using the relativistic coupled-cluster approach.

physics.atom-ph↗

arXiv2018

Nuclear-Spin Dependent Parity Violation in Optically Trapped Polyatomic Molecules

We investigate using optically trapped linear polyatomic molecules as probes of nuclear spin-dependent parity violation. The presence of closely spaced, opposite-parity $\ell$-doublets is a general feature of such molecules, allowing parity-violation-sensitive pairs of levels to be brought to degeneracy in magnetic fields typically 100 times smaller than in diatomics. Assuming laser cooling and trapping of polyatomics at the current state-of-the-art for diatomics, we expect to measure nuclear spin-dependent parity-violating matrix elements $iW$ with 70 times better sensitivity than the current best measurements. Our scheme should allow for 10 \% measurements of $iW$ in nuclei as light as Be or as heavy as Yb, with averaging times on order the of 10 days and 1 second, respectively.

physics.atom-ph↗

arXiv2018

A 3D-printed alkali metal dispenser

We demonstrate and characterize a source of Li atoms made from direct metal laser sintered titanium. The source's outgassing rate is measured to be $5 \,(2)\cdot 10^{-7}$\,$\rm{Pa}~ \rm{L}~ \rm{s}^{-1}$ at a temperature $T=330\,^\circ$C, which optimizes the number of atoms loaded into a magneto-optical trap. The source loads $\approx 10^7$ $^7$Li atoms in the trap in $\approx 1$\,s. The loaded source weighs 700\,mg and is suitable for a number of deployable sensors based on cold atoms.

physics.ins-det↗

arXiv2017

Hyperfine Structure of the $B^3Π_1$ State and Predictions of Optical Cycling Behavior in the $X\rightarrow B$ transition of TlF

The rotational and hyperfine spectrum of the $X^1Σ^+ \rightarrow B^3Π_1$ transition in TlF molecules was measured using laser-induced fluorescence from both a thermal and a cryogenic molecular beam. Rotational and hyperfine constants for the $B$ state are obtained. The large magnetic hyperfine interaction of the Tl nuclear spin leads to significant mixing of the lowest $B$ state rotational levels. Updated, more precise measurements of the $B\rightarrow X$ vibrational branching fractions are also presented. The combined rovibrational branching fractions allow for the prediction of the number of photons that can be scattered in a given TlF optical cycling scheme.

physics.atom-ph↗

arXiv2016

In-vacuum scattered light reduction with cupric oxide surfaces for sensitive fluorescence detection

We demonstrate a simple and easy method for producing low-reflectivity surfaces that are ultra-high vacuum compatible, may be baked to high temperatures, and are easily applied even on complex surface geometries. Black cupric oxide (CuO) surfaces are chemically grown in minutes on any copper surface, allowing for low-cost, rapid prototyping and production. The reflective properties are measured to be comparable to commercially available products for creating optically black surfaces. We describe a vacuum apparatus which uses multiple blackened copper surfaces for sensitive, low-background detection of molecules using laser-induced fluorescence.

physics.ins-det↗