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Eric Cormier

Publications and source records attributed to Eric Cormier.

13 recordsLinked to original sources
arXiv2026

Carrier-Envelope Phase Control of Orbital Angular Momentum in Solid-State High-Harmonic Generation

High-order harmonic generation (HHG) driven by optical vortices is a powerful route to produce structured light in different spectral regions. The nonlinear process transfers orbital angular momentum (OAM) from the driving field to the emitted harmonics according to the scaling law $l_q = q\times l$, a consequence of the rotational invariance and angular momentum conservation. Here, we show that, in the regime of few-cycle pulses, the topological charge (TC) of the harmonic radiation detected within a finite spectral window is no longer fixed by this scaling law alone, but is governed by the interplay between broken crystal inversion symmetry and carrier-envelope phase (CEP)-sensitive sub-cycle electron dynamics. By driving HHG in a ZnO crystal with few-cycle ($\approx 1.5$ cycles) vortex beams centered at 3.2~$\mu$m, we observed that the measured TC becomes strongly CEP-dependent, switching between adjacent integer values, but only when the inversion symmetry is broken and the harmonic emission is CEP-sensitive. The TC switching vanishes when either condition is removed. Numerical analysis reveals that the TC switching originates from a CEP-controlled redistribution of spectral weight among spectrally overlapping harmonic orders, which changes the dominant OAM channel within the detection window. These results identify the CEP as a degree of freedom for tailoring the topological structure of high-harmonic radiation, pointing toward waveform-controlled structured attosecond light sources.

physics.optics↗
arXiv2026

Measuring the dipole phase of Bloch-trajectory harmonics using a monolithic interferometer

Uncovering the dipole phase of gas-phase high harmonic generation was instrumental to understanding the recollision physics underlying attosecond pulse generation. Corresponding measurements in the condensed phase have not yet yielded a consistent picture. Here, we present a compact and inherently stable approach to high-harmonic interferometry in thin-film solids. We employ it to reveal the dipole phase of high-harmonic generation in polycrystalline ZnO, driven by broadband mid-IR laser pulses. We demonstrate that, under the conditions of our experiments, recollisions facilitated by Bloch oscillations represent the dominant contribution to high-harmonic generation just above the bandgap.

physics.optics↗
arXiv2026

Twisting harmonics: Transfer of orbital angular momentum in solid-state high-harmonic generation

Although solid-state platforms underpin modern electronics, little is known about how intense ultrashort light pulses carrying orbital angular momentum (OAM) interact with solids. This gap persists even though, for more conventional light-matter interactions, the complex underlying electron dynamics can often be confined to a single Brillouin zone and described well within the dipole approximation. Previous studies were restricted to nonlinear, perturbative regimes, largely because the generation of intense ultrashort vortex pulses, particularly in the mid-infrared spectral regime, has remained a long-standing challenge. Consequently, the role of structured light in driving nonlinear, non-perturbative processes in solids, and the associated transfer of angular momentum during these interactions, has not been systematically explored. Here, we investigate solid-state high-harmonic generation (HHG) driven by intense ultrashort structured light using a versatile experimental approach applicable to different materials and geometries. We demonstrate that the OAM of the driving field is coherently transferred to the emitted harmonics. In particular, we show that the OAM is conserved independently of the crystal symmetry, the range of electronic interactions, and the presence of strong spin-orbit coupling. These results establish OAM-resolved HHG as a robust framework for characterizing and controlling angular momentum transfer in solid-state HHG and open new avenues for structured-light-driven quantum technologies and topological materials investigations.

physics.optics↗
arXiv2025

Sculpting ultrafast mid-infrared light for solid-state high harmonic generation

The ability to sculpt light in space, time, and polarization has revolutionized studies of light-matter interaction and enabled breakthroughs in optical communication, imaging, and ultrafast science. Among the many degrees of freedom of light, orbital angular momentum (OAM) further expands these capabilities by unlocking new regimes of control in information encoding, particle trapping and manipulation, and symmetry-driven selection rules. However, exploiting OAM to drive nonlinear, non-perturbative effects in solids remains challenging, especially in the mid-infrared (MIR) spectral regime-a key region for accessing these effects in ambient air, where spatial light modulators do not operate. Here, we circumvent this limitation by generating femtosecond, few-cycle MIR Bessel-Gauss vortex (BGV) and perfect optical vortices (POVs), using a robust, static spatial-shaping strategy. By utilizing these beams to drive nonlinear optical processes such as second-harmonic generation (SHG) and high-harmonic generation (HHG) in various solid-state materials, we show that the resulting harmonic beams faithfully inherit the structural characteristics of the drivers: the constant-intensity ring of the POVs is preserved across harmonic orders, while the BGV harmonic beams retain their intrinsic topological charge-dependent intensity profiles. Furthermore, by verifying the linear OAM up-scaling law, we confirm the conservation of OAM during SHG and HHG in solids. These results establish strong-field HHG in solids as a robust platform for synthesizing ultrafast structured harmonic light with controllable, high-value OAM.

physics.optics↗
arXiv2024

MIR laser CEP estimation using machine learning concepts in bulk high harmonic generation

Monitoring the carrier-envelope phase (CEP) is of paramount importance for experiments involving few cycle intense laser fields. Common measurement techniques include f-2f interferometry or stereo-ATI setups. These approaches are adequate, but are challenging to implement on demand, at different locations as additional metrology tools, in intense few cycle laser-matter interaction experiments, such as those prevalent in sophisticated user beamlines. In addition there are inherent difficulties for CEP measured at non-conventional laser wavelengths (like e.g. mid infrared) and measurements above 10 kHz laser repetition rates, on single shot basis. Here we demonstrate both by simulations and by experiments a machine learning (ML) driven method for CEP estimation in the mid infrared, which is readily generalizable for any laser wavelength and possibly up to MHz repetition rates. The concept relies on the observation of the spectrum of high harmonic generation (HHG) in bulk material and the use of ML techniques to estimate the CEP of the laser. Once the ML model is trained, the method provides a way for cheap and compact real-time CEP tagging. This technique can complement the otherwise sophisticated monitoring of CEP, and is able to capture the complex correlation between the CEP and the observable HHG spectra.

physics.optics↗
arXiv2024

Exploring Valence Electron Dynamics of Xenon through Laser-Induced Electron Diffraction

Strong-field ionization can induce electron motion in both the continuum and the valence shell of the parent ion. Here, we explore their interplay by studying laser-induced electron diffraction (LIED) patterns arising from interaction with the potentials of two-hole states of the xenon cation. The quantitative rescattering theory is used to calculate the corresponding photoelectron momentum distributions, providing evidence that the spin-orbit dynamics could be detected by LIED. We identify the contribution of these time-evolving hole states to the angular distribution of the rescattered electrons, particularly noting a distinct change along the backward scattering angles. We benchmark numerical results with experiments using ultrabroad and femtosecond laser pulses centered at \SI{3100}{nm}.

physics.atom-ph↗
arXiv2021

Energetic sub-2-cycle laser with 220 W average power

Few-cycle lasers are essential for many research areas such as attosecond physics that promises to address fundamental questions in science and technology. Therefore, further advancements are connected to significant progress in the underlying laser technology. Here, two-stage nonlinear compression of a 660 W femtosecond fiber laser system is utilized to achieve unprecedented average power levels of energetic ultrashort or even few-cycle laser pulses. In a first compression step 408 W, 320 uJ, 30fs pulses are achieved, which can be further compressed to 216 W, 170 uJ, 6.3 fs pulses in a second compression stage. This is the highest average power few-cycle laser system presented so far. It is expected to significantly advance the fields of high harmonic generation and attosecond science.

physics.optics↗
arXiv2019

Ab-initio calculations of laser-atom interactions reveal harmonics feedback during macroscopic propagation

We couple the full 3D ab initio quantum evolution of the light pulse polarization in interaction with an atom with a propagation model to simulate the propagation of ultrashort laser pulses over macroscopic dimensions, in the presence of self-generated harmonics up to order 11. We evidence a clear feedback of the generated harmonics on propagation, with an influence on the ionization probability as well as the yield of the harmonic generation itself.

physics.optics↗
arXiv2018

Laser wakefield acceleration with high-power, few-cycle mid-IR lasers

The study of laser wakefield electron acceleration (LWFA) using mid-IR laser drivers is a promising path for future laser driven electronaccelerators, when compared to traditional near-IR laser drivers uperating at 0.8-1 {\mu}m central wavelength ({\lambda}laser), as the necessary vector potential a_0 for electron injection can be achieved with smaller laser powers due to the linear dependence on {\lambda}laser. In this work, we perform 2D PIC simulations on LWFA using few-cycle high power (5-15 TW) laser systems with {\lambda}laser ranging from 0.88-10 {\mu}m. Such few-cycle systems are currently under development, aiming at Gas High Harmonics Generation applications where the favourable {\lambda}laser^2 scaling extends the range of XUV photon energies. We keep a_0 and n_e/n_cr (n_e being the plasma density and n_cr being the critical density for each {\lambda}laser) as common denominators in outr simulations, allowing for comparisons between drivers of different {\lambda}laser, with respect to the accelerated electron beam energy, charge, and conversion efficiency. While the electron energies are mainly dominated by the plasma dynamics, the laser to electron beam energy conversion efficiency shows significant enhancement with longer wavelength laser drivers.

physics.plasm-ph↗
arXiv2014

Near infrared few-cycle pulses for high harmonic generation

We report on the development of tunable few-cycle pulses with central wavelengths from 1.6 um to 2 um. Theses pulses were used as a proof of principle for high harmonic generation in atomic and molecular targets. In order to generate such pulses we produced a filament in a 4 bar krypton cell. Spectral broadening by a factor of 2 to 3 of a 40 fs near infrared input pulse was achieved. The spectrally broadened output pulses were then compressed by fused silica plates down to the few-cycle regime close to the Fourier limit. The auto-correlation of these pulses revealed durations of about 3 cycles for all investigated central wavelengths. Pulses with a central wavelength of 1.7 um and up to 430 uJ energy per pulse were employed to generate high order harmonics in Xe, Ar and N2. Moving to near infrared few-cycle pulses opens the possibility to operate deeply in the non-perturbative regime with a Keldysh parameter smaller than 1. Hence, this source is suitable for the study of the non-adiabatic tunneling regime in most generating systems used for high order harmonic generation and attoscience.

physics.plasm-ph↗
arXiv2012

High-field quantum calculation reveals time-dependent negative Kerr contribution

The exact quantum time-dependent optical response of hydrogen under strong field near infrared excitation is investigated and compared to the perturbative model widely used for describing the effective atomic polarization induced by intense laser fields. By solving the full 3D time-dependent Schr\"{o}dinger equation, we exhibit a supplementary, quasi-instantaneous defocusing contribution missing in the weak-field model of polarization. We show that this effect is far from being negligible in particular when closures of ionization channels occur and stems from the interaction of electrons with their parent ions. It provides an interpretation to higher-order Kerr effect recently observed in various gases.

physics.optics↗
arXiv2002

Coulomb-Volkov approach of ionization by extreme ultraviolet laser pulses in the subfemtosecond regime

In conditions where the interaction betweeen an atom and a short high-frequency extreme ultraviolet laser pulse is a perturbation, we show that a simple theoretical approach, based on Coulomb-Volkov-type states, can make reliable predictions for ionization. To avoid any additional approximation, we consider here a standard case : the ionization of hydrogen atoms initially in their ground state. For any field parameter, we show that the method provides accurate energy spectra of ejected electrons, including many above threshold ionization peaks, as long as the two following conditions are simultaneously fulfilled : (i) the photon energy is greater than or equal to the ionization potential ; (ii) the ionization process is not saturated. Thus, ionization of atoms or molecules by the high order harmonic laser pulses which are generated at present may be addressed through this Coulomb-Volkov treatment.

physics.atom-ph↗