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Eric Wahlberg

Publications and source records attributed to Eric Wahlberg.

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Boosting superconductivity in ultrathin YBa$_2$Cu$_3$O$_{7-\delta}$ films via nanofaceted substrates

In cuprate high-temperature superconductors the doping level is fixed during synthesis, hence the charge carrier density per CuO$_2$ plane cannot be easily tuned by conventional gating, unlike in 2D materials. Strain engineering has recently emerged as a powerful tuning knob for manipulating the properties of cuprates, in particular charge and spin orders, and their delicate interplay with superconductivity. In thin films, additional tunability can be introduced by the substrate surface morphology, particularly nanofacets formed by substrate surface reconstruction. Here we show a remarkable enhancement of the superconducting onset temperature $T_{\mathrm{c}}^{\mathrm{on}}$ and the upper critical magnetic field $H_{c,2}$ in nanometer-thin YBa$_2$Cu$_3$O$_{7-\delta}$ films grown on a substrate with a nanofaceted surface. We theoretically show that the enhancement is driven by electronic nematicity and unidirectional charge density waves, where both elements are captured by an additional effective potential at the interface between the film and the uniquely textured substrate. Our findings show a new paradigm in which substrate engineering can effectively enhance the superconducting properties of cuprates. This approach opens an exciting frontier in the design and optimization of high-performance superconducting materials.

cond-mat.supr-con

Engineering underdoped CuO$_2$ nanoribbons in nm-thick $a$-axis YBa$_2$Cu$_3$O$_{7-δ}$ films

In underdoped cuprate high $T_{\mathrm{c}}$ superconductors, various local orders and symmetry breaking states, in addition to superconductivity, reside in the CuO$_2$ planes. The confinement of the CuO$_2$ planes can therefore play a fundamental role in modifying the hierarchy between the various orders and their intertwining with superconductivity. Here we present the growth of $a$-axis oriented YBa$_2$Cu$_3$O$_{7-δ}$ films, spanning the whole underdoped side of the phase diagram. In these samples, the CuO$_2$ planes are confined by the film thickness, effectively forming unit-cell-thick nanoribbons. The unidirectional confinement at the nanoscale enhances the in-plane anisotropy of the films. By X-ray diffraction and resistance vs temperature measurements, we have discovered the suppression of the orthorhombic-to-tetragonal transition at low dopings, and a very high anisotropy of the normal state resistance in the $b$-$c$ plane, the latter being connected to a weak coupling between adjacent CuO$_2$ nanoribbons. These findings show that the samples we have grown represent a novel system, different from the bulk, where future experiments can possibly shed light on the rich and mysterious physics occurring within the CuO$_2$ planes.

cond-mat.supr-con

Mapping the phase diagram of a YBa$_2$Cu$_3$O$_{7-δ}$ nanowire through electromigration

We use electromigration (EM) to tune the oxygen content of YBa$_2$Cu$_3$O$_{7-δ}$ (YBCO) nanowi\-res. During EM, the dopant oxygen atoms in the nanowire are moved under the combined effect of electrostatic force and Joule heating. The EM current can be tuned to either deplete or replenish nanowires with oxygen, allowing fine tuning of its hole doping level. Electrical transport measurements and Kelvin probe microscopy corroborate good homogeneity of the doping level along the electromigrated nanowires. Thus, EM provides an effective method to study transport properties of YBCO in a wide doping range at the nanoscale in one and the same device.

cond-mat.supr-con