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Euan Hendry

Publications and source records attributed to Euan Hendry.

17 recordsLinked to original sources

Real-time THz ptychography using an optically modulated aperture

Ptychography allows ordinary cameras to perform both quantitative phase and intensity imaging. However, the requirement for relative object to probe motion and high measurement count significantly limits imaging speed and application scope. In this work, we introduce optically modulated aperture ptychography, using a silicon photomodulator as a rapidly reconfigurable aperture, deployable across the microwave, millimeter wave and terahertz bands. We demonstrate experimentally at ~ 0.1 THz real-time ptychographic image capture, without moving parts. Furthermore, a reconfigurable aperture facilitates diverse and spatially multiplexed probes. We use a multiplexed known-probe reconstruction strategy that improves signal-to-noise ratio and increases the information content per measurement, enabling the capture of fluid dynamics at 16 fps. Our optical modulation approach enables high-throughput ptychographic imaging of dynamic samples, for applications such as non-destructive evaluation and in-vivo biomedical imaging.

physics.optics

A microwave super-resolution imaging approach towards breast cancer margin mapping

Accurate characterisation of margins in excised breast cancer tumours is critical to the success of surgical interventions. Yet margin status is typically confirmed post-operatively using histopathology. Here we present a microwave single pixel imaging technique designed for use in intraoperative margin assessment. By leveraging the photo-induced change in microwave transparency of a silicon modulator placed under the sample, we map the microwave reflectivity of tissue-mimicking phantoms with deeply sub-wavelength resolution, allowing hydration mapping across large areas (10 x 10 cm) at ~1 mm resolution. We evaluate the discriminatory capability of our method using gelatine-based tumour phantoms with water-content variations designed to mimic the contrast between malignant tissue and tumour margins in resected breast specimens. We demonstrate the capability to identify, locate and quantify inadequate margins up to the typically targeted minimum thickness of 2 mm. Furthermore, using numerical modelling, we show that our approach is expected to be resilient to patient-specific tissue differences. These results establish microwave single-pixel imaging as a promising route towards real-time intraoperative assessment of margins in excised breast tumours.

physics.optics

The 2024 Active Metamaterials Roadmap

Active metamaterials are engineered structures that possess novel properties that can be changed after the point of manufacture. Their novel properties arise predominantly from their physical structure, as opposed to their chemical composition and can be changed through means such as direct energy addition into wave paths, or physically changing/morphing the structure in response to both a user or environmental input. Active metamaterials are currently of wide interest to the physics community and encompass a range of sub-domains in applied physics (e.g. photonic, microwave, acoustic, mechanical, etc.). They possess the potential to provide solutions that are more suitable to specific applications, or which allow novel properties to be produced which cannot be achieved with passive metamaterials, such as time-varying or gain enhancement effects. They have the potential to help solve some of the important current and future problems faced by the advancement of modern society, such as achieving net-zero, sustainability, healthcare and equality goals. Despite their huge potential, the added complexity of their design and operation, compared to passive metamaterials creates challenges to the advancement of the field, particularly beyond theoretical and lab-based experiments. This roadmap brings together experts in all types of active metamaterials and across a wide range of areas of applied physics. The objective is to provide an overview of the current state of the art and the associated current/future challenges, with the hope that the required advances identified create a roadmap for the future advancement and application of this field.

physics.app-ph

Shrinking a gradient index lens antenna system with a spaceplate

The miniaturisation of optical systems is an ongoing challenge across the electromagnetic spectrum. While the thickness of optical elements themselves can be reduced using advances in metamaterials, it is the voids between these elements -- which are necessary parts of an optical system -- that occupy most of the volume. Recently, a novel optical element coined a `spaceplate' was proposed, that replaces a region of free space with a thinner optical element that emulates the free-space optical response function -- thus having the potential to substantially shrink the volume of optical systems. While there have been a few proof-of-principle demonstrations of spaceplates, they have not yet been deployed in a real-world optical system. In this work, we use a bespoke-designed spaceplate to reduce the length of a gradient index (GRIN) lens microwave antenna. Our antenna is designed to operate at 23.5 GHz, and the incorporation of a nonlocal metamaterial spaceplate enables the distance between the antenna feed and the GRIN lens to be reduced by almost a factor of two. We find the radiation patterns from a conventional and space-squeezed antenna are very similar, with a very low cross-polarisation, and only a minor increase in the side-lobe levels when introducing the spaceplate. Our work represents a first example of a spaceplate integrated into a functional optical system, highlighting the potential for this concept to reduce the physical size of optical systems in real-world applications.

physics.app-ph

Terahertz imaging through emissivity control

Adoption of terahertz technologies is hindered by the lack of cost-effective THz sources. Here we demonstrate a fundamentally new way to generate and control THz radiation, via spatio-temporal emissivity modulation. By patterning the optical photoexcitation of a surface-passivated silicon wafer, we locally control the free-electron density, and thereby pattern the wafer's emissivity in the THz part of the electromagnetic spectrum. We show how this unconventional source of controllable THz radiation enables a new form of incoherent computational THz imaging. We use it to image various concealed objects, demonstrating this scheme has the penetrating capability of state-of-the-art THz imaging approaches, without the requirement of femto-second pulsed laser sources. Furthermore, the incoherent nature of thermal radiation also ensures the obtained images are free of interference artifacts. Our spatio-temporal emissivity control paves the way towards a new family of long-wavelength structured illumination, imaging and spectroscopy systems.

physics.optics

High-harmonic generation enhancement with graphene heterostructures

We investigate high-harmonic generation in graphene heterostructures consisting of metallic nanoribbons separated from a graphene sheet by either a few-nanometer layer of aluminum oxide or an atomic monolayer of hexagonal boron nitride. The nanoribbons amplify the near-field at the graphene layer relative to the externally applied pumping, thus allowing us to observe third- and fifth-harmonic generation in the carbon monolayer at modest pump powers in the mid-infrared. We study the dependence of the nonlinear signals on the ribbon width and spacer thickness, as well as pump power and polarization, and demonstrate enhancement factors relative to bare graphene reaching 1600 and 4100 for third- and fifth-harmonic generation, respectively. Our work supports the use of graphene heterostructures to selectively enhance specific nonlinear processes of interest, an essential capability for the design of nanoscale nonlinear devices.

cond-mat.mes-hall

Space-squeezing optics in the microwave spectral region

Optical systems often consist largely of empty space, as diffraction effects that occur through free-space propagation can be crucial to their function. Contracting these voids offers a path to the miniaturisation of a wide range of optical devices. Recently, a new optical element - coined a 'spaceplate' - has been proposed, that is capable of emulating the effects of diffraction over a specified propagation distance using a thinner non-local metamaterial [Nat. Commun. 12, 3512 (2021)]. The compression factor of such an element is given by the ratio of the length of free-space that is replaced to the thickness of the spaceplate itself. In this work we test a prototype spaceplate in the microwave spectral region (20-23\,GHz) - the first such demonstration designed to operate in ambient air. Our device consists of a Fabry-Pérot cavity formed from two reflective metasurfaces, with a compression factor that can be tuned by varying the size of perforations within each layer. Using a pair of directive horn antennas, we measure a space compression factor of up to approx. 6 over an NA of 0.34 and fractional bandwidth of 6%. We also investigate the fundamental trade-offs that exist between the compression factor, transmission efficiency, numerical aperture (NA) and bandwidth of this single resonator spaceplate design, and highlight that it can reach arbitrarily high compression factors by restricting its NA and bandwidth.

physics.optics

Spatiotemporal refraction of light in an epsilon-near-zero ITO layer

When light travels through a medium in which the refractive index is rapidly changing with time, the light will undergo a shift in its frequency. Large frequency shifting effects have recently been reported for transparent conductive oxides. These observations have been interpreted as emerging from temporal changes to the propagation phase in a bulk medium resulting from temporal variations in the refractive index, an effect referred to as temporal refraction. Here, we show that the frequency shift in an epsilon-near-zero (ENZ) layer made of indium tin oxide (ITO) originates not only from this bulk response, but includes a significant effect resulting from temporal changes to the spatial boundary conditions. This boundary effect can lead to a dominant opposing shift to the bulk effect for certain angles. Hence, this process gives rise to a frequency shift that can be tailored through the angle of incidence, decoupling the amplitude and phase modulation.

physics.optics

Total internal reflection based super-resolution imaging for sub-IR frequencies

For measurements designed to accurately determine layer thickness, there is a natural trade-off between sensitivity to optical thickness and lateral resolution due to the angular ray distribution required for a focused beam. We demonstrate a near-field imaging approach that enables both sub-wavelength lateral resolution and optical thickness sensitivity. We illuminate a sample in a total internal reflection geometry, with a photo-activated spatial modulator in the near-field, which allows optical thickness images to be computationally reconstructed in a few seconds. We demonstrate our approach at 140 GHz (wavelength 2.15 mm), where images are normally severely limited in spatial resolution, and demonstrate mapping of optical thickness variation in inhomogeneous biological tissues.

physics.app-ph

Approximations used in the analysis of signals in pump-probe spectroscopy

In pump-probe spectroscopy, one often needs to analyse the transmission or reflection of electromagnetic waves through optically pumped media. Here, it is common practice to approximate the analysis in order to extract non-equilibrium values for the optical constants of the media. Concentrating on optical pump-THz probe spectroscopy, and using the transfer matrix approach, we present a general method for evaluating the applicability of the most common approximations. Somewhat surprisingly, we find that these approximations are truly valid only in extreme cases where the optical thickness of the sample is several orders of magnitude smaller or larger than the probe wavelength.

physics.optics

Impact of pump wavelength on terahertz emission of a cavity-enhanced spintronic trilayer

We systematically study the pump-wavelength dependence of terahertz pulse generation in thin-film spintronic THz emitters composed of a ferromagnetic Fe layer between adjacent nonmagnetic W and Pt layers. We find that the efficiency of THz generation is essentially at for excitation by 150 fs pulses with center wavelengths ranging from 900 to 1500 nm, demonstrating that the spin current does not depend strongly on the pump photon energy. We show that the inclusion of dielectric overlayers of TiO2 and SiO2, designed for a particular excitation wavelength, can enhance the terahertz emission by a factor of of up to two in field.

physics.optics

Sign inversion in the terahertz photoconductivity of single-walled carbon nanotube films

In recent years, there have been conflicting reports regarding the ultrafast photoconductive response of films of single walled carbon nanotubes (CNTs), which apparently exhibit photoconductivities that can differ even in sign. Here, we observe explicitly that the THz photoconductivity of CNT films is a highly variable quantity which correlates with the length of the CNTs, while the chirality distribution has little influence. Moreover, by comparing the photo-induced change in THz conductivity with heat-induced changes, we show that both occur primarily due to heat-generated modification of the Drude electron relaxation rate, resulting in a broadening of the plasmonic resonance present in finite-length metallic and doped semiconducting CNTs. This clarifies the nature of the photo-response of CNT films and demonstrates the need to carefully consider the geometry of the CNTs, specifically the length, when considering them for application in optoelectronic devices.

cond-mat.mes-hall

Influence of nanotube length and density on the plasmonic terahertz response of single-walled carbon nanotubes

We measure the conductivity spectra of thin films comprising bundled single-walled carbon nanotubes (CNTs) of different average lengths in the frequency range 0.3-1000 THz and temperature interval 10-530 K. The observed temperature-induced changes in the terahertz conductivity spectra are shown to depend strongly on the average CNT length, with a conductivity around 1 THz that increases/decreases as the temperature increases for short/long tubes. This behaviour originates from the temperature dependence of the electron scattering rate, which we obtain from Drude fits of the measured conductivity in the range 0.3-2 THz for 10 $μ$m length CNTs. This increasing scattering rate with temperature results in a subsequent broadening of the observed THz conductivity peak at higher temperatures and a shift to lower frequencies for increasing CNT length. Finally, we show that the change in conductivity with temperature depends not only on tube length, but also varies with tube density. We record the effective conductivities of composite films comprising mixtures of WS$_2$ nanotubes and CNTs vs CNT density for frequencies in the range 0.3-1 THz, finding that the conductivity increases/decreases for low/high density films as the temperature increases. This effect arises due to the density dependence of the effective length of conducting pathways in the composite films, which again leads to a shift and temperature dependent broadening of the THz conductivity peak.

cond-mat.mes-hall

A platform for time-resolved scanning Kerr microscopy in the near-field

Time-resolved scanning Kerr microscopy (TRSKM) is a powerful technique for the investigation of picosecond magnetization dynamics at sub-micron length scales by means of the magneto-optical Kerr effect (MOKE). The spatial resolution of conventional (focused) Kerr microscopy using a microscope objective lens is determined by the optical diffraction limit so that the nanoscale character of the magnetization dynamics is lost. Here we present a platform to overcome this limitation by means of a near-field TRSKM that incorporates an atomic force microscope (AFM) with optical access to a metallic AFM probe with a nanoscale aperture at its tip. We demonstrate the near-field capability of the instrument through the comparison of time-resolved polar Kerr images of magnetization dynamics within a microscale NiFe rectangle acquired using both near-field and focused TRSKM techniques at a wavelength of 800 nm. The flux-closure domain state of the in-plane equilibrium magnetization provided the maximum possible dynamic polar Kerr contrast across the central domain wall, and enabled an assessment of the magneto-optical spatial resolution of each technique. Line profiles extracted from the Kerr images demonstrate that the near-field spatial resolution was enhanced with respect to that of the focused Kerr images. Furthermore, the near-field polar Kerr signal (~1 mdeg) was more than half that of the focused Kerr signal, despite the potential loss of probe light due to internal reflections within the AFM tip. We have confirmed the near-field operation by exploring the influence of the tip-sample separation, and have determined the spatial resolution to be ~550 nm for an aperture with a sub-wavelength diameter of 400 nm. The spatial resolution of the near-field TRSKM was in good agreement with finite element modelling of the aperture...

cond-mat.mtrl-sci

Subwavelength THz imaging of graphene photoconductivity

Using a spatially structured, optical pump pulse with a THz probe pulse, we are able to determine spatial variations of the ultrafast THz photoconductivity with sub-wavelength resolution (75 $μm \approx λ/5$ at 0.8 THz) in a planar graphene sample. We compare our results to Raman spectroscopy and correlate the existence of the spatial inhomogeneities between the two measurements. We find a strong correlation with inhomogeneity in electron density. This demonstrates the importance of eliminating inhomogeneities in doping density during CVD growth and fabrication for photoconductive devices.

physics.optics

The Roles of Substrate vs Nonlocal Optical Nonlinearities in the Excitation of Surface Plasmons in Graphene

It has recently been demonstrated that difference frequency mixing (DFM) can generate surface plasmons in graphene [1]. Here, we present detailed calculations comparing the contributions to this effect from substrate and from graphene nonlinearities. Our calculations show that the substrate (quartz) nonlinearity gives rise to a surface plasmon intensity that is around twelve orders of magnitude smaller than that arising from the intrinsic graphene response. This surprisingly efficient intrinsic process, given the centrosymmetric structure of graphene, arises almost entirely due to non-local contributions to the second order optical nonlinearity of graphene.

physics.optics

All-Optical Generation of Surface Plasmons in Graphene

Here we present an all-optical plasmon coupling scheme, utilising the intrinsic nonlinear optical response of graphene. We demonstrate coupling of free-space, visible light pulses to the surface plasmons in a planar, un-patterned graphene sheet by using nonlinear wave mixing to match both the wavevector and energy of the surface wave. By carefully controlling the phase-matching conditions, we show that one can excite surface plasmons with a defined wavevector and direction across a large frequency range, with an estimated photon efficiency in our experiments approaching $10^{-5}$.

physics.optics