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Eugene A. Demler

Publications and source records attributed to Eugene A. Demler.

At least 19 recordsLinked to original sources

Optical and magnetic signatures of drive-enhanced coherence in phase-disordered superconducting bilayers

Recent experiments demonstrating superconducting-like characteristics in materials above their equilibrium transition temperatures following strong sub-picosecond optical excitation have stimulated theoretical interest in phase-disordered superconductors subject to a periodically modulated superfluid stiffness. Previous analyses of the single-layer optical conductivity have shown that such a drive can enhance the low-frequency $1/ω$ response, even when the period-averaged stiffness remains unchanged. We extend these studies to bilayer systems, such as the YBa$_2$Cu$_3$O$_{6+x}$ (YBCO) cuprate, by considering drives with different symmetries. Specifically, we investigate a layer-symmetric drive, in which the two planes stiffen and soften simultaneously, and a layer-antisymmetric drive, in which one plane stiffens while the other softens. Both drives enhance correlations of the layer-averaged phase and generate comparable superconducting-like optical conductivities. Only the symmetric drive, however, strengthens relative-phase locking and the associated counterflow response to a magnetic field parallel to the planes. Thus, an enhanced $1/ω$ optical conductivity does not by itself imply enhanced magnetic screening. In view of applications to driven YBCO, where superconducting-like in-plane optics and transient diamagnetism have both been reported, our result provides a symmetry diagnostic: within a phase-synchronization mechanism, the experimentally active low-frequency stiffness modulation must contain a substantial layer-symmetric component.

cond-mat.supr-con

Flux-Floquet instability in fluctuating superconductors

In the past decade, photo-induced superconducting-like behaviors have been reported in a number of materials driven by intense pump fields. Of particular interest is the high-Tc cuprate YBCO, where such effect has been reported up to the so-called pseudogap temperature T*~300-400 K. In a recent experiment, a transient magnetic field which is proportional to and in the same direction of an applied field has been observed outside the sample, suggestive of flux exclusion due to the Meissner effect. In this paper, we present an alternative interpretation of these experiments based on a mechanism that we term the flux-Floquet instability of the sine-Gordon (SG) model. We take as our premise the model of preformed Cooper pairs in the pseudogap phase. Starting from the local superconducting order parameter in equilibrium, we introduce an extended SG model to describe the dynamics of the relative phase between the layers of a bilayer. We demonstrate that a combination of external magnetic field and strong terahertz drive used in experiments by Fava et al. results in a novel Floquet instability in the model. This instability leads to currents at the edges of the bilayer formed by defects or grain boundaries, with the current flowing in the opposite direction of the equilibrium screening current, producing a giant paramagnetic magnetization in the same direction as the applied field. We show how this scenario can fit most of the available data. To the extent that this model can account for the data, we conclude that the experiments have the important consequence of revealing the presence of local pairing in the pseudogap phase. More broadly our results reveal a new instability in the SG equation that is of fundamental interest, with potential applications such as providing a mechanism for generating large magnetic fields at ultrafast time scales in Josephson devices.

cond-mat.supr-con

Anomalous Eigenstates of a Doped Hole in the Ising Antiferromagnet

The problem of a mobile hole doped into an antiferromagnet Mott insulator is believed to underly the rich physics of several paradigmatic strongly correlated electron systems, ranging from heavy fermions to high-Tc superconductivity. Arguably the simplest incarnation of this problem corresponds to a doped Ising antiferromagnet, a problem widely considered essentially solved since almost 60 years by a popular yet approximate mapping to a single-particle problem on the Bethe lattice. Here we show that, despite its deceptive simplicity, the local spectrum of a single hole in a classical Ising-Néel state contains a series of anomalous, long-lived states that go beyond the well-known ladder-like spectrum with excited energies spaced as $J^{2/3} t^{1/3}$. The anomalous states we find through exact diagonalization and within the self-avoiding path approximation have excitation energies scaling approximately linear with $J$ and lead to a series of avoided crossings with the more pronounced ladder spectrum. By also computing different local, rotational spectra we explain the origin of the anomalous states as rooted in an approximate emergent local $C_3$ symmetry of the problem. From their direct spectral signatures we further conclude that these states lead to anomalously slow thermalization behavior -- hence representing a new type of quantum many-body scar state, potentially related to many-body scars predicted in lattice gauge theories.

cond-mat.str-el

Enhanced coherence in the periodically driven two-dimensional XY model

Strong optical drives have been shown to induce transient superconducting-like response in materials above their equilibrium $T_c$. Many of these materials already exhibit short-range superconducting correlations in equilibrium. This motivates the question: can external driving enhance coherence in systems with superconducting correlations but no long-range order? We explore this scenario in the two-dimensional XY model with a periodically modulated stiffness using overdamped Langevin dynamics. We find that, even though the modulation leaves the average coupling unchanged, the drive can markedly increase long-range, time-averaged correlations in systems well above the equilibrium Berezinskii-Kosterlitz-Thouless temperature. The outcome depends on the ratio of the drive frequency to the intrinsic relaxation rate: faster drives primarily heat the system, suppressing correlations and conductivity. For slower drives, the optical conductivity is modified so that the real part exhibits a prolonged effective Drude scattering time, while the imaginary part has a strengthened low-frequency $1/ω$ behavior. We map out these regimes across temperature, frequency, and amplitude, and rationalize them via simple analytics and vortex-thermalization arguments. Overall, we identify a generic nonequilibrium route to enhance coherence in XY-like systems, with potential relevance to experiments reporting light-induced superconductivity.

cond-mat.supr-con

Kondo impurity in an attractive Fermi-Hubbard bath: Equilibrium and dynamics

We investigate theoretically equilibrium and dynamical properties of a Kondo impurity coupled to either 1D or 2D superconductors, modeled by the attractive Fermi-Hubbard model. By employing a non-Gaussian variational approach, we go beyond the approximation of a constant superconducting (SC) gap. We show that dynamical properties of the system can be modified qualitatively, when space and time dependent renormalization of the SC gap and electron-impurity hybridization are included. For the ground state, we find the singlet-doublet phase transition and $π$-phase shifts of the SC order parameter. For dynamics, first we consider spin dynamics following an abrupt connection of the polarized impurity to the 2D bath. We find rapid relaxation of impurity polarization and directional emission of a magnetization pulse, which becomes damped as it propagates into the bulk. Then we analyze transport between two SC leads coupled through the impurity at finite bias voltage. Here we go beyond analysis of the steady state to investigate full-time dynamics following an abrupt application of the bias voltage. We uncover four distinct regimes in the transient dynamics and transport properties: (I) the AC Josephson effect regime; (II) dynamical competition between charge-density-wave (CDW) and SC orders with transient Kondo correlations; (III) the coexistence of AC and DC currents facilitated by partial Kondo screening and dynamical stabilization of the SC order; (IV) DC Kondo transport regime modified by the SC order. Regime II exhibits a dynamical transition from SC to CDW order that locally restores the U(1) symmetry. We argue that our findings for regime IV provide a theoretical explanation for the experimentally observed anomalous enhancement of DC conductance and suppression of the AC Josephson current. Finally, we discuss the potential experimental realization with ultracold atoms.

cond-mat.str-el

Hyperbolic Quantum Processor

Achieving strong coherent interaction between qubits separated by large distances holds the key to many important developments in quantum technology, including new designs of quantum computers, new platforms for quantum simulations and implementation of large scale quantum optical networks. However, the inherent mismatch between the spatial dimensions of a quantum emitter and the photon wavelength fundamentally limits the transmission of quantum entanglement over long distances. Here we demonstrate, that long-range qubit entanglement can be readily achieved when qubit interactions are mediated by optical polariton waves in a hyperbolic material, due to the phenomenon of the Hyperbolic Super-Resonance. We show that in this regime the resulting quantum gate fidelity that exceeds 99%, can be achieved with the use of qubits based on well known deep donors in silicon when their interactions are mediated by polariton fields in the substrate formed by a hyperbolic material (such as e.g. hexagonal boron nitride. At the physical level the proposed system is essentially a silicon-based optoelectronic chip, and it's readily accessible to the existing methods of semiconductor nanofabrication, leading to the integration densities of well over 10^8. qubits/cm^2, and therefore opening the way to scalable and fault-tolerant error correction in quantum computation. Furthermore, we demonstrate that, due to the optical time scales that define the duration of the gate operation in the proposed system, and sub-nanosecond time of the decoherence in deep donors in silicon at the liquid nitrogen temperatures, the proposed Hyperbolic Quantum Processor does not require dilution refrigeration and therefore offers a pathway to bring quantum computation to the realm of conventional engineering.

quant-ph

Metastable Photo-Induced Superconductivity far above $T_{\textrm{c}}$

Inspired by the striking discovery of metastable superconductivity in $\mathrm{K}_3\mathrm{C}_{60}$ at 100K, far above $T_{\textrm{c}}=20K$, we discuss possible mechanisms for long-lived, photo-induced superconductivity. Starting from a model of optically-driven Raman phonons coupled to inter-band electronic transitions, we develop a microscopic mechanism for photo-controlling the pairing interaction. Leveraging this mechanism, we first investigate long-lived superconductivity arising from the thermodynamic metastable trapping of the driven phonon. We then propose an alternative route, where the superconducting gap created by an optical drive leads to a dynamical bottleneck in the equilibration of quasi-particles. We conclude by discussing implications of both scenarios for experiments that can be used to discriminate between them. Our work provides falsifiable explanations for the nanosecond-scale photo-induced superconductivity found in $\mathrm{K}_3\mathrm{C}_{60}$, while simultaneously offering a theoretical basis for exploring metastable superconductivity in other quantum materials.

cond-mat.supr-con

Quantum noise spectroscopy of dynamical critical phenomena

The transition between distinct phases of matter is characterized by the nature of fluctuations near the critical point. We demonstrate that noise spectroscopy can not only diagnose the presence of a phase transition, but can also determine fundamental properties of its criticality. In particular, by analyzing a scaling collapse of the decoherence profile, one can directly extract the critical exponents of the transition and identify its universality class. Our approach naturally captures the presence of conservation laws and distinguishes between classical and quantum phase transitions. In the context of quantum magnetism, our proposal complements existing techniques and provides a novel toolset optimized for interrogating two-dimensional magnetic materials.

quant-ph

Theory of resonantly enhanced photo-induced superconductivity

Optical driving of materials has emerged as a versatile tool to control their properties, with photo-induced superconductivity being among the most fascinating examples. In this work, we show that light or lattice vibrations coupled to an electronic interband transition naturally give rise to electron-electron attraction that may be enhanced when the underlying boson is driven into a non-thermal state. We find this phenomenon to be resonantly amplified when tuning the boson's frequency close to the energy difference between the two electronic bands. This result offers a simple microscopic mechanism for photo-induced superconductivity and provides a recipe for designing new platforms in which light-induced superconductivity can be realized. We propose a concrete setup consisting of a graphene-hBN-SrTiO$_3$ heterostructure, for which we estimate a superconducting $T_{\rm c}$ that may be achieved upon driving the system.

cond-mat.supr-con

Time-domain anyon interferometry in Kitaev honeycomb spin liquids and beyond

Motivated by recent experiments on the Kitaev honeycomb magnet $α\text{-RuCl}_3$, we introduce time-domain probes of the edge and quasiparticle content of non-Abelian spin liquids. Our scheme exploits ancillary quantum spins that communicate via time-dependent tunneling of energy into and out of the spin liquid's chiral Majorana edge state. We show that the ancillary-spin dynamics reveals the edge-state velocity and, in suitable geometries, detects individual non-Abelian anyons and emergent fermions via a time-domain counterpart of quantum-Hall anyon interferometry. We anticipate applications to a wide variety of topological phases in solid-state and cold-atoms settings.

cond-mat.str-el

Resonantly enhanced polariton wave mixing and Floquet parametric instability

We introduce a new theoretical approach for analyzing pump and probe experiments in non-linear acousto-optic systems. In our approach, the effect of coherently pumped polaritons is modeled as providing time-periodic modulation of the system parameters. Within this framework, propagation of the probe pulse is described by the Floquet version of Maxwell's equations and leads to such phenomena as frequency mixing and resonant parametric production of polariton pairs. We analyze light reflection from a slab of insulating material with a strongly excited phonon-polariton mode and obtain analytic expressions for the frequency-dependent reflection coefficient for the probe pulse. Our results are in agreement with recent experiments by Cartella et al. which demonstrated light amplification in resonantly excited SiC insulator. We show that, beyond a critical pumping strength, such systems should exhibit Floquet parametric instability, which corresponds to resonant scattering of the pump polaritons into pairs of finite momentum polaritons. We find that the parametric instability should be achievable in SiC using current experimental techniques and discuss its signatures, including the non-analytic frequency dependence of the reflection coefficient and the probe pulse afterglow. We discuss possible applications of the parametric instability phenomenon and suggest that similar types of instabilities can be present in other photoexcited non-linear systems.

physics.optics

Higgs-mediated optical amplification in a non-equilibrium superconductor

The quest for new functionalities in quantum materials has recently been extended to non-equilibrium states, which are interesting both because they exhibit new physical phenomena and because of their potential for high-speed device applications. Notable advances have been made in the creation of metastable phases and in Floquet engineering under external periodic driving. In the context of non-equilibrium superconductivity, examples have included the generation of transient superconductivity above the thermodynamic transition temperature, the excitation of coherent Higgs mode oscillations, and the optical control of the interlayer phase in cuprates. Here, we propose theoretically a novel non-equilibrium phenomenon, through which a prompt quench from a metal to a transient superconducting state could induce large oscillations of the order parameter amplitude. We argue that this oscillating mode could act as a source of parametric amplification of the incident radiation. We report experimental results on optically driven K$_3$C$_{60}$ that are consistent with these predictions. The effect is found to disappear when the onset of the excitation becomes slower than the Higgs mode period, consistent with the theory proposed here. These results open new possibilities for the use of collective modes in many-body systems to induce non-linear optical effects.

cond-mat.supr-con

Probing and dressing magnetic impurities in a superconductor

We propose a method to probe and control the interactions between an ensemble of magnetic impurities in a superconductor via microwave radiation. Our method relies upon the presence of sub-gap Yu-Shiba-Rusinov (YSR) states associated with the impurities. Depending on the sign of the detuning, radiation generates either a ferro- or antiferromagnetic contribution to the exchange interaction. This contribution can bias the statistics of the random exchange constants stemming from the RKKY interaction. Moreover, by measuring the microwave response at the YSR resonance, one gains information about the magnetic order of the impurities. To this end, we estimate the absorption coefficient as well as the achievable strength of the microwave-induced YSR-interactions using off-resonant radiation. The ability to utilize microwave fields to both probe and control impurity spins in a superconducting host may open new paths to studying metallic spin glasses.

cond-mat.mes-hall

Dicke time crystals in driven-dissipative quantum many-body systems

The Dicke model -- a paradigmatic example of superradiance in quantum optics -- describes an ensemble of atoms which are collectively coupled to a leaky cavity mode. As a result of the cooperative nature of these interactions, the system's dynamics are captured by the behavior of a single mean-field, collective spin. In this mean-field limit, it has recently been shown that the interplay between photon losses and periodic driving of light-matter coupling can lead to time-crystalline-like behavior of the collective spin. In this work, we investigate whether such a Dicke time crystal is stable to perturbations that explicitly break the mean-field solvability of the conventional Dicke model. In particular, we consider the addition of short-range interactions between atoms, which breaks the collective coupling and leads to complex many-body dynamics. In this context, the interplay between periodic driving, dissipation and interactions yields a rich set of dynamical responses including long-lived and metastable Dicke time crystals, where losses can cool down the many-body heating resulting from the continuous pump of energy from the periodic drive. Specifically, when the additional short-range interactions are ferromagnetic, we observe time crystalline behavior at non-perturbative values of the coupling strength, suggesting the possible existence of stable dynamical order in a driven-dissipative quantum many-body system. These findings illustrate the rich nature of novel dynamical responses with many-body character in quantum optics platforms.

cond-mat.quant-gas

Exploring the Kondo model in and out of equilibrium with alkaline-earth atoms

We propose a scheme to realize the Kondo model with tunable anisotropy using alkaline-earth atoms in an optical lattice. The new feature of our setup is Floquet engineering of interactions using time-dependent Zeeman shifts, that can be realized either using state-dependent optical Stark shifts or magnetic fields. The properties of the resulting Kondo model strongly depend on the anisotropy of the ferromagnetic interactions. In particular, easy-plane couplings give rise to Kondo singlet formation even though microscopic interactions are all ferromagnetic. We discuss both equilibrium and dynamical properties of the system that can be measured with ultracold atoms, including the impurity spin susceptibility, the impurity spin relaxation rate, as well as the equilibrium and dynamical spin correlations between the impurity and the ferromagnetic bath atoms. We analyze the non-equilibrium time evolution of the system using a variational non-Gaussian approach, which allows us to explore coherent dynamics over both short and long timescales, as set by the bandwidth and the Kondo singlet formation, respectively. In the quench-type experiments, when the Kondo interaction is suddenly switched on, we find that real-time dynamics shows crossovers reminiscent of poor man's renormalization group flow used to describe equilibrium systems. For bare easy-plane ferromagnetic couplings, this allows us to follow the formation of the Kondo screening cloud as the dynamics crosses over from ferromagnetic to antiferromagnetic behavior. On the other side of the phase diagram, our scheme makes it possible to measure quantum corrections to the well-known Korringa law describing the temperature dependence of the impurity spin relaxation rate. Theoretical results discussed in our paper can be measured using currently available experimental techniques.

cond-mat.quant-gas

Bose polarons in ultracold atoms in one dimension: beyond the Fröhlich paradigm

Mobile impurity atoms immersed in Bose-Einstein condensates provide a new platform for exploring Bose polarons. Recent experimental advances in the field of ultracold atoms make it possible to realize such systems with highly tunable microscopic parameters and to explore equilibrium and dynamical properties of polarons using a rich toolbox of atomic physics. In this paper we present a detailed theoretical analysis of Bose polarons in one dimensional systems of ultracold atoms. By combining a non-perturbative renormalization group approach with numerically exact diffusion Monte Carlo calculations we obtain not only detailed numerical results over a broad range of parameters but also qualitative understanding of different regimes of the system. We find that an accurate description of Bose polarons requires the inclusion of two-phonon scattering terms which go beyond the commonly used Fröhlich model. Furthermore we show that when the Bose gas is in the strongly interacting regime, one needs to include interactions between the phonon modes. We use several theoretical approaches to calculate the polaron energy and its effective mass. The former can be measured using radio-frequency spectroscopy and the latter can be studied experimentally using impurity oscillations in a harmonic trapping potential. We compare our theoretical results for the effective mass to the experiments by Catani et al. [PRA 85, 023623 (2012)]. In the weak-to-intermediate coupling regimes we obtain excellent quantitative agreement between theory and experiment, without any free fitting parameter. We supplement our analysis by full dynamical simulations of polaron oscillations in a shallow trapping potential. We also use our renormalization group approach to analyze the full phase diagram and identify regions that support repulsive and attractive polarons, as well as multi-particle bound states.

cond-mat.quant-gas

Strong coupling Bose polarons in a BEC

We use a non-perturbative renormalization group approach to develop a unified picture of the Bose polaron problem, where a mobile impurity is strongly interacting with a surrounding Bose-Einstein condensate (BEC). A detailed theoretical analysis of the phase diagram is presented and the polaron-to-molecule transition is discussed. For attractive polarons we argue that a description in terms of an effective Fröhlich Hamiltonian with renormalized parameters is possible. Its strong coupling regime is realized close to a Feshbach resonance, where we predict a sharp increase of the effective mass. Already for weaker interactions, before the polaron mass diverges, we predict a transition to a regime where states exist below the polaron energy and the attractive polaron is no longer the ground state. On the repulsive side of the Feshbach resonance we recover the repulsive polaron, which has a finite lifetime because it can decay into low-lying molecular states. We show for the entire range of couplings that the polaron energy has logarithmic corrections in comparison with predictions by the mean-field approach. We demonstrate that they are a consequence of the polaronic mass renormalization which is due to quantum fluctuations of correlated phonons in the polaron cloud.

cond-mat.quant-gas

Quantum correlations at infinite temperature: the dynamical Nagaoka effect

Do quantum correlations play a role in high temperature dynamics of many-body systems? A common expectation is that thermal fluctuations lead to fast decoherence and make dynamics classical. In this paper, we provide a striking example of a single particle created in a featureless, infinite temperature spin bath which not only exhibits non-classical dynamics but also induces strong long-lived correlations between the surrounding spins. We study the non-equilibrium dynamics of a hole created in a fermionic or bosonic Mott insulator in the atomic limit, which corresponds to a degenerate spin system. In the absence of interactions, the spin correlations arise purely from quantum interference, and the correlations are both antiferromagnetic and ferromagnetic, in striking contrast to the equilibrium Nagaoka effect. These results are relevant for several condensed matter spin systems, and should be observable using state of the art bosonic or fermionic quantum gas microscopes.

cond-mat.quant-gas