arXiv subjects

Eugene S. Polzik

Publications and source records attributed to Eugene S. Polzik.

At least 19 recordsLinked to original sources

arXiv2024

Optimal optomechanical cavity setups with highly reflecting membranes

Highly reflecting mechanically compliant membranes based on photonic-crystal patterns have recently gained increasing attention within cavity optomechanics due to their prospects of reaching high coupling rates in membrane-in-the-middle experiments. Here we present an analysis and comparison of four different setups in which highly reflecting membranes can be employed for cavity optomechanics, and discuss optimal choices w.r.t. the figures of merit cooperativity and efficiency-weighted cooperativity. The analysis encompasses three different types of membrane-in-the-middle setups (membrane-at-the-edge, membrane-in-the-actual-middle, and membrane-at-the-back), as well as the simple Fabry-Perot cavity. Interestingly, we identify and propose the membrane-at-the-back setup as an optimal choice in the limit of negligible membrane parasitic loss, which can reach enormous enhancements of optomechanical cooperativity, and if implemented with a low-loss membrane would pave the way to nonlinear optomechanics in the quantum regime.

physics.optics↗

arXiv2023

Roadmap on Nanoscale Magnetic Resonance Imaging

The field of nanoscale magnetic resonance imaging (NanoMRI) was started 30 years ago. It was motivated by the desire to image single molecules and molecular assemblies, such as proteins and virus particles, with near-atomic spatial resolution and on a length scale of 100 nm. Over the years, the NanoMRI field has also expanded to include the goal of useful high-resolution nuclear magnetic resonance (NMR) spectroscopy of molecules under ambient conditions, including samples up to the micron-scale. The realization of these goals requires the development of spin detection techniques that are many orders of magnitude more sensitive than conventional NMR and MRI, capable of detecting and controlling nanoscale ensembles of spins. Over the years, a number of different technical approaches to NanoMRI have emerged, each possessing a distinct set of capabilities for basic and applied areas of science. The goal of this roadmap article is to report the current state of the art in NanoMRI technologies, outline the areas where they are poised to have impact, identify the challenges that lie ahead, and propose methods to meet these challenges. This roadmap also shows how developments in NanoMRI techniques can lead to breakthroughs in emerging quantum science and technology applications.

cond-mat.mes-hall↗

arXiv2023

High-Field Optical Cesium Magnetometer for Magnetic Resonance Imaging

We present a novel high-field optical quantum magnetometer based on saturated absorption spectroscopy on the extreme angular-momentum states of the cesium D2 line. With key features including continuous readout, high sampling rate, and sensitivity and accuracy in the ppm-range, it represents a competitive alternative to conventional techniques for measuring magnetic fields of several teslas. The prototype has four small separate field probes, and all support electronics and optics are fitted into a single 19-inch rack to make it compact, mobile, and robust. The field probes are fiber coupled and made from non-metallic components, allowing them to be easily and safely positioned inside a 7 T MRI scanner. We demonstrate the capabilities of this magnetometer by measuring two different MRI sequences, and we show how it can be used to reveal imperfections in the gradient coil system, to highlight the potential applications in medical MRI. We propose the term EXAAQ (EXtreme Angular-momentum Absorption-spectroscopy Quantum) magnetometry, for this novel method.

physics.atom-ph↗

arXiv2023

Acoustic frequency atomic spin oscillator in the quantum regime

We experimentally demonstrate quantum behavior of a macroscopic atomic spin oscillator in the acoustic frequency range. Quantum back-action of the spin measurement, ponderomotive squeezing of light, and oscillator spring softening are observed at spin oscillation frequencies down to 6 kHz. Quantum noise sources characteristic of spin oscillators operating in the near-DC frequency range are identified and means for their mitigation are presented. These results constitute an important step towards quantum noise reduction and entanglement-enhanced sensing in the acoustic range using a negative-mass reference frame. In particular, the results are relevant for broadband noise reduction in gravitational wave detectors.

quant-ph↗

arXiv2023

Squeezed light from an oscillator measured at the rate of oscillation

Continuous measurements of the position of an oscillator become projective on position eigenstates when the measurements are made faster than the coherent evolution. We evidence an effect of this transition on a spin oscillator within an ensemble of $2\times10^{10}$ room-temperature atoms by observing correlations between the quadratures of the meter light field. These correlations squeeze the fluctuations of the light quadratures below the vacuum level. When the measurement is slower than the oscillation, we generate 11.5 dB and detect 8.5 dB of squeezing in a tunable band that is a fraction of the resonance frequency. When the measurement is as fast as the oscillation, we detect 4.7 dB of squeezing that spans more than one decade of frequencies below the resonance. Our results demonstrate a new regime of continuous quantum measurements on material oscillators, and set a new benchmark for the performance of a linear quantum sensor.

quant-ph↗

arXiv2023

Entanglement-enhanced magnetic induction tomography

Magnetic induction tomography (MIT) is a sensing protocol, exploring conductive objects via their response to radio-frequency magnetic fields. MIT is used in nondestructive testing ranging from geophysics to medical applications. Atomic magnetometers, employed as MIT sensors, allow for significant improvement of the MIT sensitivity and for exploring its quantum limits. Here we report entanglement-enhanced MIT with an atomic magnetometer used as the sensing element. We generate an entangled and spin squeezed state of atoms of the sensor by stroboscopic quantum non-demolition measurement. We then utilize this spin state to demonstrate the improvement of one-dimensional MIT sensitivity beyond the standard quantum limit.

quant-ph↗

arXiv2022

Phononically shielded photonic-crystal mirror membranes for cavity quantum optomechanics

We present a highly reflective, sub-wavelength-thick membrane resonator featuring high mechanical quality factor and discuss its applicability for cavity optomechanics. The $88.5~\text{nm}$ thin stoichiometric silicon-nitride membrane, designed and fabricated to combine 2D-photonic and phononic crystal patterns, reaches reflectivities up to $99.89~\%$ and a mechanical quality factor of $2.9 \times 10^7$ at room temperature. We construct a Fabry-Perot-type optical cavity, with the membrane forming one terminating mirror. The optical beam shape in cavity transmission shows a stark deviation from a simple Gaussian mode-shape, consistent with theoretical predictions. We demonstrate optomechanical sideband cooling to mK-mode temperatures, starting from room temperature. At higher intracavity powers we observe an optomechanically induced optical bistability. The demonstrated device has potential to reach high cooperativities at low light levels desirable for e.g. optomechanical sensing and squeezing applications or fundamental studies in cavity quantum optomechanics, and meets the requirements for cooling to the quantum ground state of mechanical motion from room temperature.

physics.optics↗

arXiv2022

Small animal biomagnetism applications

The functioning of the human brain, nervous system and heart is based on the conduction of electrical signals. These electrical signals also create magnetic fields which extend outside the human body. Highly sensitive magnetometers, such as superconducting quantum interference device magnetometers or optically pumped magnetometers, placed outside the human body can detect these biomagnetic fields and provide non-invasive measurements of e.g. brain activity, nerve impulses, and cardiac activity. Animal models are used widely in medical research, including for disease diagnostics and for drugs testing. We review the topic of biomagnetic recordings on animal models using optically pumped magnetometers, and present our experiments on detecting nerve impulses in the frog sciatic nerve and the heart beat in an isolated guinea pig heart.

physics.med-ph↗

arXiv2022

Precision Measurement of the Excited State Landé g-factor and Diamagnetic Shift of the Cesium D$_{2}$ Line

We have performed saturated absorption spectroscopy on the cesium D$_{2}$ line in 3 T and 7 T magnetic fields. By means of sideband spectroscopy on the extreme angular momentum states we have measured the linear magnetic frequency shift of the transition to be $γ_1 = 13.994\:301(11)$ GHz/T. This corresponds to an optical magnetic field measurement of better than 1 ppm accuracy. From this value we can calculate the fine structure Landé g-factor $g_J\left(6^2P_{3/2}\right) = 1.334\:087\:49(52)$. This is consistent with the previous best measurement, and improves the accuracy by more than two orders of magnitude. We have also measured, for the first time ever, the quadratic diamagnetic shift as $γ_2 = 0.4644(35)\:\mathrm{MHz/T^2}$. Our work opens up the field of accurate high field optical magnetometry using atomic cesium. These high accuracy measurements also allow for testing of advanced atomic structure models, as our results are incompatible with the Russel-Saunders coupling value, and the hydrogen-constant-core-model value, by 31 and 7 standard deviations respectively.

physics.atom-ph↗

arXiv2022

Trajectories without quantum uncertainties in composite systems with disparate energy spectra

It is well established that measurement-induced quantum back action (QBA) can be eliminated in composite systems by engineering so-called quantum-mechanics-free subspaces (QMFSs) of commuting variables, leading to a trajectory of a quantum system without quantum uncertainties. This situation can be realized in a composite system that includes a negative-mass subsystem, which can be implemented by, e.g., a polarized spin ensemble or a two-tone-driven optomechanical system. The realization of a trajectory without quantum uncertainties implies entanglement between the subsystems, and allows for measurements of motion, fields and forces with, in principle, unlimited precision. To date, these principles have been developed theoretically and demonstrated experimentally for a number of composite systems. However, the utility of the concept has been limited by the dominating requirement of close proximity of the resonance frequencies of the system of interest and the negative-mass reference system, and by the need to embed the subsystems in a narrowband cavity, which could be problematic while at the same time achieving good overcoupling. Here we propose a general approach which overcomes these limitations by employing periodic modulation of the driving fields (e.g., two-tone driving) in combination with coherent or measurement-based anti-noise paths. This approach makes it possible to engineer a QMFS of two systems with vastly different spectra and with arbitrary signs of their masses, while dispensing with the need to embed the subsystems in a sideband-resolving cavity. We discuss the advantages of this novel approach for applications such as QBA evasion in gravitational wave detection, force sensing, and entanglement generation between disparate systems.

quant-ph↗

arXiv2021

Cavity-enhanced sum-frequency generation of blue light with near-unity conversion efficiency

We report on double-resonant highly efficient sum-frequency generation in the blue range. The system consists of a 10-mm-long periodically poled KTP crystal placed in a double-resonant bow-tie cavity and pumped by a fiber laser at 1064.5 nm and a Ti:sapphire laser at 849.2 nm. An optical power of 375 mW at 472.4 nm in a TEM$_{00}$ mode was generated with pump powers of 250 mW at 849.2 nm and 200 mW at 1064.5 nm coupled into the double-resonant ring resonator with 88$\%$ mode-matching. The resulting internal conversion efficiency of 95($\pm 3$)$\%$ of the photons mode-matched to the cavity constitutes, to the best of our knowledge, the highest overall achieved quantum conversion efficiency using continuous-wave pumping. Very high conversion efficiency is rendered possible due to very low intracavity loss on the level of 0.3$\%$ and high nonlinear conversion coefficient up to 0.045(0.015) W$^{-1}$. Power stability measurements performed over one hour show a stability of 0.8$\%$. The generated blue light can be tuned within 5 nm around the center wavelength of 472.4 nm, limited by the phase-matching of our nonlinear crystal. This can however be expanded to cover the entire blue spectrum (420 nm to 510 nm) by proper choice of nonlinear crystals and pump lasers. Our experimental results agree very well with analytical and numerical simulations taking into account cavity impedance matching and depletion of the pump fields.

physics.optics↗

arXiv2021

Carrier-mediated optomechanical forces in semiconductor nanomembranes with coupled quantum wells

In the majority of optomechanical experiments, the interaction between light and mechanical motion is mediated by radiation pressure, which arises from momentum transfer of reflecting photons. This is an inherently weak interaction, and optically generated carriers in semiconductors have been predicted to be the mediator of different and potentially much stronger forces. Here we demonstrate optomechanical forces induced by electron-hole pairs in coupled quantum wells embedded into a free-free nanomembrane. We identify contributions from the deformation-potential and piezoelectric coupling and observe optically driven motion about three orders of magnitude larger than expected from radiation pressure. The amplitude and phase of the driven oscillations are controlled by an applied electric field, which tunes the carrier lifetime to match the mechanical period. Our work opens perspectives for not only enhancing the optomechanical interaction in a range of experiments, but also for interfacing mechanical objects with complex macroscopic quantum objects, such as excitonic condensates.

cond-mat.mes-hall↗

arXiv2021

High-frequency broadband laser phase noise cancellation using a delay line

Laser phase noise remains a limiting factor in many experimental settings, including metrology, time-keeping, as well as quantum optics. Hitherto this issue was addressed at low frequencies, ranging from well below 1 Hz to maximally 100 kHz. However, a wide range of experiments, such as, e.g., those involving nanomechanical membrane resonators, are highly sensitive to noise at higher frequencies in the range of 100 kHz to 10 MHz, such as nanomechanical membrane resonators. Here we employ a fiber-loop delay line interferometer optimized to cancel laser phase noise at frequencies around 1.5 MHz. We achieve noise reduction in 300 kHz-wide bands with a peak reduction of more than 10 dB at desired frequencies, reaching phase noise of less than -160 dB (rad$^2$/Hz) with a Ti:Al$_2$O$_3$ laser. These results provide a convenient noise reduction technique to achieve deep ground-state cooling of mechanical motion.

physics.optics↗

arXiv2021

Calibration of Spin-Light Coupling by Coherently Induced Faraday Rotation

Calibrating the strength of the light-matter interaction is an important experimental task in quantum information and quantum state engineering protocols. The strength of the off-resonant light-matter interaction in multi-atom spin oscillators can be characterized by the coupling rate $Γ_\text{S}$. Here we utilize the Coherently Induced Faraday Rotation (CIFAR) signal for determining the coupling rate. The method is suited for both continuous and pulsed readout of the spin oscillator, relying only on applying a known polarization modulation to the probe laser beam and detecting a known optical polarization component. Importantly, the method does not require changes to the optical and magnetic fields performing the state preparation and probing. The CIFAR signal is also independent of the probe beam photo-detection quantum efficiency, and allows direct extraction of other parameters of the interaction, such as the tensor coupling $ζ_\text{S}$, and the damping rate $γ_\text{S}$. We verify this method in the continuous wave regime, probing a strongly coupled spin oscillator prepared in a warm cesium atomic vapour.

quant-ph↗

arXiv2020

Room-temperature single-photon source with near-millisecond built-in memory

Non-classical photon sources are a crucial resource for distributed quantum networks. Photons generated from matter systems with memory capability are particularly promising, as they can be integrated into a network where each source is used on-demand. Among all kinds of solid state and atomic quantum memories, room-temperature atomic vapours are especially attractive due to their robustness and potential scalability. To-date room-temperature photon sources have been limited either in their memory time or the purity of the photonic state. Here we demonstrate a single-photon source based on room-temperature memory. Following heralded loading of the memory, a single photon is retrieved from it after a variable storage time. The single-photon character of the retrieved field is validated by the strong suppression of the two-photon component with antibunching as low as $g^{(2)}_{\text{RR|W=1}} = 0.20 \pm 0.07$. Non-classical correlations between the heralding and the retrieved photons are maintained for up to $τ_{\text{NC}}^{\mathcal R} = (0.68\pm 0.08)$ ms, more than two orders of magnitude longer than previously demonstrated with other room-temperature systems. Correlations sufficient for violating Bell inequalities exist for up to $τ_{\text{BI}} = (0.15 \pm 0.03)$ ms.

quant-ph↗

arXiv2020

Measurement and simulation of atomic motion in nanoscale optical trapping potentials

Atoms trapped in the evanescent field around a nanofiber experience strong coupling to the light guided in the fiber mode. However, due to the intrinsically strong positional dependence of the coupling, thermal motion of the ensemble limits the use of nanofiber trapped atoms for some quantum tasks. We investigate the thermal dynamics of such an ensemble by using short light pulses to make a spatially inhomogeneous population transfer between atomic states. As we monitor the wave packet of atoms created by this scheme, we find a damped oscillatory behavior which we attribute to sloshing and dispersion of the atoms. Oscillation frequencies range around 100 kHz, and motional dephasing between atoms happens on a timescale of 10 $μ$s. Comparison to Monte Carlo simulations of an ensemble of 1000 classical particles yields reasonable agreement for simulated ensemble temperatures between 25 $μ$K and 40 $μ$K.

physics.atom-ph↗

arXiv2020

Phonon counting thermometry of an ultracoherent membrane resonator near its motional ground state

Generation of non-Gaussian quantum states of macroscopic mechanical objects is key to a number of challenges in quantum information science, ranging from fundamental tests of decoherence to quantum communication and sensing. Heralded generation of single-phonon states of mechanical motion is an attractive way towards this goal, as it is, in principle, not limited by the object size. Here we demonstrate a technique which allows for generation and detection of a quantum state of motion by phonon counting measurements near the ground state of a 1.5 MHz micromechanical oscillator. We detect scattered photons from a membrane-in-the-middle optomechanical system using an ultra-narrowband optical filter, and perform Raman-ratio thermometry and second-order intensity interferometry near the motional ground state ($\bar{n}=0.23\pm0.02$ phonons). With an effective mass in the nanogram range, our system lends itself for studies of long-lived non-Gaussian motional states with some of the heaviest objects to date.

quant-ph↗

arXiv2020

Entanglement between Distant Macroscopic Mechanical and Spin Systems

Entanglement is a vital property of multipartite quantum systems, characterised by the inseparability of quantum states of objects regardless of their spatial separation. Generation of entanglement between increasingly macroscopic and disparate systems is an ongoing effort in quantum science which enables hybrid quantum networks, quantum-enhanced sensing, and probing the fundamental limits of quantum theory. The disparity of hybrid systems and the vulnerability of quantum correlations have thus far hampered the generation of macroscopic hybrid entanglement. Here we demonstrate, for the first time, generation of an entangled state between the motion of a macroscopic mechanical oscillator and a collective atomic spin oscillator, as witnessed by an Einstein-Podolsky-Rosen variance below the separability limit, $0.83 \pm 0.02<1$. The mechanical oscillator is a millimeter-size dielectric membrane and the spin oscillator is an ensemble of $10^9$ atoms in a magnetic field. Light propagating through the two spatially separated systems generates entanglement due to the collective spin playing the role of an effective negative-mass reference frame and providing, under ideal circumstances, a backaction-free subspace; in the experiment, quantum backaction is suppressed by 4.6 dB. Our results pave the road towards measurement of motion beyond the standard quantum limits of sensitivity with applications in force, acceleration,and gravitational wave detection, as well as towards teleportation-based protocols in hybrid quantum networks.

quant-ph↗