arXiv subjects

Eun-Sang Choi

Publications and source records attributed to Eun-Sang Choi.

9 recordsLinked to original sources

arXiv2025

Phase Diagram and Spectroscopic Signatures of a Supersolid in Quantum Ising Magnet K$_2$Co(SeO$_3$)$_2$

A supersolid is a quantum-entangled state of matter exhibiting the dual characteristics of superfluidity and solidity. Theory predicts that hard-core bosons with repulsive interactions on a triangular lattice can form supersolid phases at half filling and near complete filling. Leveraging an exact mapping between bosons and spin-$\frac{1}{2}$ degrees of freedom, we investigate these phases in the spin-$\frac{1}{2}$ triangular-lattice antiferromagnet \K212 with exchange constants $J_z = 2.96(2)$~meV and $J_{\perp} = 0.21(3)$~meV. At zero field, neutron diffraction reveals the gradual development for $T<15$~K of quasi-two-dimensional $\sqrt{3}\times\sqrt{3}$ magnetic order with $Z_3$ translational symmetry breaking (solidity) albeit with 44(5)% reduced amplitude at $T=0.3$~K indicating strong quantum fluctuations. These are apparent in equidistant bands of continuum neutron scattering for $\hslashω_n\approx n\times J_z$, where $n=0,1,2,3$. The lowest energy ($n=0$) $\bf Q$-dependent continuum has a lower resonant edge and includes a quasi-elastic component at K $(\frac{1}{3}\frac{1}{3})$ consistent with broken $U(1)$ spin rotational symmetry (boson superfluidity). Competing instabilities are apparent in soft albeit finite-energy modes at M $(\frac{1}{2}0)$ and at $\frac{1}{2}$K $(\frac{1}{6}\frac{1}{6})$. For $\bf c$-axis-oriented magnetic fields $17~{\rm T} <μ_0 H< 21~{\rm T}$ that almost saturate the magnetization, corresponding to nearly filling the lattice with bosons, we find a new phase consistent with a second supersolid. These phases are separated by a pronounced 1/3 magnetization plateau that supports coherent spin waves, from which we determine the spin Hamiltonian.

cond-mat.str-el↗

arXiv2025

Flux Jumps up to 17 T in ReBCO Tape Stack Cables and their Suppression with Increased Intertape Spacing

The magnetization of ReBCO tape stacks and tape stack cables in high magnetic fields (up to 30 T) are not commonly reported. Here we report magnetization measurements of tape stack cables in magnetic fields up to 30 T at 4.2 K. We observed that flux jumps, commonly relegated to low field regimes for single tapes, persisted up to 17 T in tape stacks, an effect which could have substantial technological relevance for high field applications including fusion devices or accelerator magnets. On the other hand, with the use of small spacers, we could suppress flux jump behavior, in some cases eliminating jumps entirely. Our findings provide critical insights for the optimization of designs for ReBCO cables for high-field applications, including fusion magnets and particle accelerators.

cond-mat.supr-con↗

arXiv2023

Interplay between local moment and itinerant magnetism in the layered metallic antiferromagnet TaFe$_{1.14}$Te$_3$

Two-dimensional (2D) antiferromagnets have garnered considerable interest for the next generation of functional spintronics. However, many available bulk materials from which 2D antiferromagnets are isolated are limited by their sensitivity to air, low ordering temperatures, and insulating transport properties. TaFe$_{1+y}$Te$_3$ offers unique opportunities to address these challenges with increased air stability, metallic transport properties, and robust antiferromagnetic order. Here, we synthesize TaFe$_{1+y}$Te$_3$ ($y$ = 0.14), identify its structural, magnetic, and electronic properties, and elucidate the relationships between them. Axial-dependent high-field magnetization measurements on TaFe$_{1.14}$Te$_3$ reveal saturation magnetic fields ranging between 27-30 T with a saturation magnetic moment of 2.05-2.12 $μ_B$. Magnetotransport measurements confirm TaFe$_{1.14}$Te$_3$ is metallic with strong coupling between magnetic order and electronic transport. Angle-resolved photoemission spectroscopy measurements across the magnetic transition uncover a complex interplay between itinerant electrons and local magnetic moments that drives the magnetic transition. We further demonstrate the ability to isolate few-layer sheets of TaFe$_{1.14}$Te$_3$ through mechanical exfoliation, establishing TaFe$_{1.14}$Te$_3$ as a potential platform for 2D spintronics based on metallic layered antiferromagnets.

cond-mat.mtrl-sci↗

arXiv2021

A magnetic Weyl semimetallic phase in thin films of Eu$_2$Ir$_2$O$_7$

The interplay between electronic interactions and strong spin-orbit coupling is expected to create a plethora of fascinating correlated topological states of quantum matter. Of particular interest are magnetic Weyl semimetals originally proposed in the pyrochlore iridates, which are only expected to reveal their topological nature in thin film form. To date, however, direct experimental demonstrations of these exotic phases remain elusive, due to the lack of usable single crystals and the insufficient quality of available films. Here, we report on the discovery of the long-sought magnetic Weyl semi-metallic phase in (111)-oriented Eu$_2$Ir$_2$O$_7$ high-quality epitaxial thin films. The topological magnetic state shows an intrinsic anomalous Hall effect with colossal coercivity but vanishing net magnetization, which emerges below the onset of a peculiar magnetic phase with all-in-all-out antiferromagnetic ordering. The observed anomalous Hall conductivity arises from the non-zero Berry curvature emanated by Weyl node pairs near the Fermi level that act as sources and sinks of Berry flux, activated by broken cubic crystal symmetry at the top and bottom terminations of the thin film.

cond-mat.str-el↗

arXiv2019

Giant thermal magnetoconductivity in CrCl$_3$ and a general model for spin-phonon scattering

Insulating quantum magnets lie at the forefront both of fundamental research into quantum matter and of technological exploitation in the increasingly applied field of spintronics. In this context, the magnetic thermal transport is a particularly sensitive probe of the elementary spin and exotic topological excitations in unconventional magnetic insulators. However, magnetic contributions to heat conduction are invariably intertwined with lattice contributions, and thus the issue of spin-phonon coupling in determining the spin and thermal transport properties becomes more important with emergent topological magnetic system. Here we report the observation of an anomalously strong enhancement of the thermal conductivity, occurring at all relevant temperatures, in the layered honeycomb material CrCl$_3$ in the presence of an applied magnetic field. Away from the magnetically ordered phase at low temperatures and small fields, there is no coherent spin contribution to the heat conduction, and hence the effect must be caused by a strong suppression of the phonon thermal conductivity due to magnetic fluctuations, which are in turn suppressed by the field. We build an empirical model for the thermal conductivity of CrCl$_3$ within a formalism assuming an independently determined number of spin-flip processes and an efficiency of the phonon scattering events they mediate. By extracting the intrinsic phonon thermal conductivity we obtain a quantitative description at all fields and temperatures and demonstrate that the scattering efficiency is entirely independent of the field. In this way we use CrCl$_3$ as a model system to understand the interactions between spin and phonon excitations in the context of thermal transport. We anticipate that the completely general framework we introduce will have broad implications for the interpretation of transport phenomena in magnetic quantum materials.

cond-mat.str-el↗

arXiv2019

Anomalous peak effect in iron-based superconductors Ba$_{1-x}$K$_x$Fe$_2$As$_2$ ($x \approx$ 0.69 and 0.76) for magnetic-field directions close to the $ab$ plane and its possible relation to the spin paramagnetic effect

We report magnetic torque measurements on iron-pnictide superconductors Ba$_{1-x}$K$_x$Fe$_2$As$_2$ ($x \approx$ 0.69 and 0.76) up to an applied field of $B_a$ = 45 T. The peak effect is observed in torque-vs-field curves below the irreversibility field. It is enhanced and becomes asymmetric as the field is tilted from the $c$ axis. For field directions close to the $ab$ plane, increasing- and decreasing-field curves peak at markedly different fields, and exhibit a sharp jump, suggestive of a first-order phase transition, on the high- and the low-field side of the peak, respectively. Complicated history dependence of the torque is observed in the peak-effect region. We construct and discuss the temperature ($T$)--applied-magnetic-field ($B_a$) phase diagram. Since the upper critical field for the $ab$-plane direction is comparable to the Pauli limit, we also consider possible influence of the spin paramagnetic effect on the anomalous peak effect.

cond-mat.supr-con↗

arXiv2016

Fermi surface reconstruction in FeSe under high pressure

We report Shubnikov-de Haas (SdH) oscillation measurements on FeSe under high pressure up to $P$ = 16.1 kbar. We find a sudden change in SdH oscillations at the onset of the pressure-induced antiferromagnetism at $P$ $\sim$ 8 kbar. We argue that this change can be attributed to a reconstruction of the Fermi surface by the antiferromagnetic order. The negative d$T_c$/d$P$ observed in a range between $P$ $\sim$ 8 and 12 kbar may be explained by the reduction in the density of states due to the reconstruction. The ratio of the transition temperature to the effective Fermi energy remains high under high pressure: $k_BT_c/E_F$ $\sim$ 0.1 even at $P$ = 16.1 kbar.

cond-mat.supr-con↗

arXiv2014

Anomalous Fermi surface in FeSe seen by Shubnikov-de Haas oscillation measurements

We have observed Shubnikov-de Haas oscillations in FeSe. The Fermi surface deviates significantly from predictions of band-structure calculations and most likely consists of one electron and one hole thin cylinder. The carrier density is in the order of 0.01 carriers/ Fe, an order-of-magnitude smaller than predicted. Effective Fermi energies as small as 3.6 meV are estimated. These findings call for elaborate theoretical investigations incorporating both electronic correlations and orbital ordering.

cond-mat.supr-con↗

arXiv2012

Large and homogeneous mass enhancement in the rattling-induced superconductor KOs$_2$O$_6$

We have determined the Fermi surface in KOs$_2$O$_6$ ($T_c$ = 9.6 K and $B_{c2} \sim$ 32 T) via de Haas-van Alphen (dHvA) oscillation measurements and a band structure calculation. We find effective masses up to 26(1) $m_e$ ($m_e$ is the free electron mass), which are unusually heavy for compounds where the mass enhancement is mostly due to electron-phonon interactions. Orbit-resolved mass enhancement parameters $λ_{dHvA}$ are large but fairly homogeneous, concentrated in the range 5 -- 8. We discuss origins of the large homogeneous mass enhancement in terms of rattling motion of the K ions.

cond-mat.supr-con↗