arXiv subjects

Félix Desrochers

Publications and source records attributed to Félix Desrochers.

18 recordsLinked to original sources

arXiv2026

Energetics of fractional anomalous Hall crystals in rhombohedral graphene

Fractional anomalous Hall crystals (FAHCs) replicate the topological order of the fractional quantum Hall effect in the continuum without requiring any external magnetic field. They spontaneously break continuous translation symmetry like a Wigner crystal, but are distinguished by each unit cell holding a fixed fractional number of electrons. Until now, these states have been confined to theoretical speculation or engineered models, leaving open the question of whether they can plausibly emerge in actual physical systems. Here, we establish them as energetically competitive candidate states in a realistic material setting. We study rhombohedral pentalayer graphene (R5G) with variational wavefunctions that are exact zero modes of a recently proposed ideal model of R5G. We evaluate their energies using Monte Carlo, after reinstating realistic dispersion and screened Coulomb interactions. We find FAHCs to be energetically competitive with integer anomalous Hall crystals and Fermi liquids, and their stability follows a simple principle. Each crystal maps onto a parent quantum Hall liquid that fixes its interaction energy, while the kinetic energy favors crystal periods that match the finite-momentum minimum of R5G's Mexican-hat dispersion. A weak periodic potential can then selectively lower and pin the commensurate fractional crystals. This picture predicts how the integer and fractional quantum anomalous Hall stability windows evolve with twist angle and displacement field, which we compare to recent experiments. These results support a continuum-and-interactions-first route to fractional anomalous Hall states in rhombohedral graphene.

cond-mat.str-el↗

arXiv2026

Quantum Fisher Information as a Thermal Probe in Frustrated Magnets through Insights from Quantum Spin Ice

Quantum Fisher information (QFI) is a measure of multipartite entanglement accessible via inelastic neutron scattering. Here we demonstrate that QFI reveals thermal and dynamical properties of quantum spin ice (QSI), a three-dimensional quantum spin liquid with fractionalized excitations. By developing a multi-directed loop update quantum Monte Carlo algorithm, along with exact diagonalization and gauge mean-field theory, we compute the QFI for the pyrochlore lattice. The temperature and momentum dependence of QFI maps the phase diagram, distinguishing the ferromagnetic ordered phase, its critical region, the zero-flux QSI, and the $π$-flux QSI. QFI also captures two crossover scales: from trivial paramagnet to classical spin ice, then to QSI. We discuss the $π$-flux QSI in light of experiments on cerium-based pyrochlores. Our results suggest that QFI not only detects entanglement but also serves as a sensitive thermal and dynamical probe for frustrated quantum magnets.

cond-mat.str-el↗

arXiv2026

Elastic Response and Instabilities of Anomalous Hall Crystals

Anomalous Hall crystals (AHCs) are exotic phases of matter that simultaneously break continuous translation symmetry and exhibit the quantum anomalous Hall effect. AHCs have recently been proposed to explain the observation of an integer quantum anomalous Hall phase in a multilayer graphene system. Despite intense theoretical and experimental interest, little is known about the mechanical properties of AHCs. We study the elastic properties of AHCs first by using a continuum model with quadratic dispersion and uniform Berry curvature. We find using time-dependent Hartree-Fock that the stiffness of the AHC is an order of magnitude smaller than that of the WC, which we attribute to the finite Chern number of the AHC preventing exponential localization of the charge density. By modifying the dispersion relation to include a local minimum modeled after that of rhombohedral pentalayer graphene (R5G), we find that deformations away from the triangular lattice minimize the AHC's kinetic energy, which overwhelms the small stiffness and triggers a mechanical instability. Using a microscopic model of R5G, we observe a similar mechanical instability over an experimentally relevant parameter regime. We conclude that the topologically limited stiffness of AHCs makes them susceptible to mechanical instabilities, an important consideration when interpreting experiments in terms of AHCs.

cond-mat.str-el↗

arXiv2026

Electric field control of a quantum spin liquid in weak Mott insulators

The triangular lattice Hubbard model at strong coupling, whose effective spin model contains both Heisenberg and ring exchange interactions, exhibits a rich phase diagram as the ratio of the hopping $t$ to onsite Coulomb repulsion $U$ is tuned. This includes a chiral spin liquid (CSL) phase. Nevertheless, this exotic phase remains challenging to realize experimentally because a given material has a fixed value of $t/U$ that can difficultly be tuned with external stimuli. One approach to address this problem is applying a DC electric field, which renormalizes the exchange interactions as electrons undergo virtual hopping processes; in addition to creating virtual doubly occupied sites, electrons must overcome electric potential energy differences. Performing a small $t/U$ expansion to fourth order, we derive the ring exchange model in the presence of an electric field and find that it not only introduces spatial anisotropy but also tends to enhance the ring exchange term compared to the dominant nearest-neighbor Heisenberg interaction. Thus, increasing the electric field serves as a way to increase the importance of the ring exchange at constant $t/U$. Through density matrix renormalization group calculations, we compute the ground state phase diagram of the ring exchange model for two different electric field directions. In both cases, we find that the electric field shifts the phase boundary of the CSL towards a smaller ratio of $t/U$. Therefore, the electric field can drive a magnetically ordered state into the CSL. This explicit demonstration opens the door to tuning other quantum spin systems into spin liquid phases via the application of an electric field.

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arXiv2026

Topological phonons in anomalous Hall crystals

Recent experiments on few-layer graphene structures have reported indirect signatures of anomalous Hall crystals (AHCs), but the need for a top gate to stabilize the phase precludes direct imaging of the emergent electronic lattice. This situation necessitates the investigation of alternative signatures of AHCs. The gapless phonons of the emergent electronic lattice provide a clear distinction from conventional quantum Hall states, but it may be difficult to disentangle these phonons from the plethora of other possible low-lying modes. Intriguingly, the quantum geometry of the underlying electronic ground state can imprint on the collective modes, possibly leading the phonons themselves to be topological. Were this the case, the resulting neutral chiral edge modes would provide a further signature of an AHC. Using time-dependent Hartree-Fock, we compute the spectra of collective modes of Wigner crystals (WCs) and AHCs arising in minimal models and study the topology of the phonons and low-lying excitons. Across the WC to AHC transition, we observe a series of band inversions among collective modes, producing topological phonons and excitons, and a sharp sign change in the phonon Chern number upon entering the AHC phase. We conclude by discussing the relevance of collective mode topology to experiments on candidate systems for AHCs.

cond-mat.mes-hall↗

arXiv2025

Quantum Spin Liquids in Pyrochlore Magnets With Non-Kramers Local Moments

Numerous experiments on pyrochlore oxides Pr$_2$(Zr, Sn, Hf, Ir)$_2$O$_7$ with non-Kramers Pr$^{3+}$ ions suggest that they support a quantum spin liquid (QSL) ground state, but the precise nature of the QSL remains unclear. Quantum spin ice with dominant dipolar Ising and smaller quadrupolar transverse exchange interactions is one such candidate, but a dominant inelastic neutron scattering signal suggests that such a picture may not be consistent with experimental results. The microscopic exchange couplings of these compounds are also not known, leaving room for many possible QSL states. In this work, we use Schwinger boson mean-field theory supplemented by a projective symmetry group classification to study possible $\mathbb{Z}_2$ QSLs in pyrochlore magnets with dipolar-quadrupolar non-Kramers local moments. We build a mean-field phase diagram and find four QSLs in the frustrated region of parameter space that are consistent with inelastic signals observed in neutron scattering data on Pr$_2$Zr$_2$O$_7$ and Pr$_2$Hf$_2$O$_7$. Among these, two robust QSLs occur in the regime with dominant transverse exchange rather than Ising exchange. We then compute the static and dynamic spin structure factors for these QSL candidates, which can be used to distinguish them in neutron scattering experiments.

cond-mat.str-el↗

arXiv2025

Fermi Surface Bosonization for Non-Fermi Liquids

Understanding non-Fermi liquids in dimensions higher than one remains one of the most formidable challenges in modern condensed matter physics. These systems, characterized by an abundance of gapless degrees of freedom and the absence of well-defined quasiparticles, defy conventional analytical frameworks. Inspired by recent work [Delacretaz, Du, Mehta, and Son, Physical Review Research, 4, 033131 (2022)], we present a procedure for bosonizing Fermi surfaces that does not rely on the existence of sharp excitation and is thus directly applicable to non-Fermi liquids. Our method involves parameterizing the generalized fermionic distribution function through a bosonic field that describes frequency-dependent local variations of the chemical potential in momentum space. We propose an effective action that produces the collisionless quantum Boltzmann equation as its equation of motion and can be used for any dimension and Fermi surface of interest. Even at the quadratic order, this action reproduces non-trivial results obtainable only through involved analysis with alternative means. By offering an alternative method directly applicable to studying the low-energy physics of Fermi and non-Fermi liquids, our work potentially stands as an important building block in advancing the comprehension of strange metals and associated phenomena.

cond-mat.str-el↗

arXiv2025

Electronic Crystal Phases in the Presence of Non-Uniform Berry Curvature and Tunable Berry Flux: The $λ_N$-Jellium model

Recent experiments on multilayer graphene systems have rekindled interest in electronic crystal phases in two dimensions -- but now for phases enriched by non-trivial quantum geometry. In this work, we introduce a simple continuum model with tunable Berry curvature distribution and total flux, enabling systematic study of crystallization in geometrically nontrivial bands. In the noninteracting limit, the addition of a C6-symmetric periodic potential yields a rich phase diagram, for which we provide several analytical insights. Notably, we derive a general formula for the Chern number in the weak-potential regime that is broadly applicable to single-band projected models. Removing the periodic potential and treating Coulomb interactions self-consistently at the Hartree-Fock level, the resulting phase diagrams host a variety of crystalline states, including anomalous Hall crystals, halo Wigner crystals in which localized electrons spontaneously acquire orbital angular momentum leading to depleted electron occupation at the zone center, and a novel halo anomalous Hall crystal that combines these properties with a finite Chern number. We identify why these phases are energetically favorable through analytical and energetic considerations. Our results provide insight into the interplay between crystallization and band geometry, while also offering a simple toy model amenable to numerical methods beyond mean-field.

cond-mat.str-el↗

arXiv2024

Fractional matter coupled to the emergent gauge field in a quantum spin ice

Electronic spins can form long-range entangled phases of condensed matter named quantum spin liquids. Their existence is conceptualized in models of two- or three-dimensional frustrated magnets that evade symmetry-breaking order down to zero temperature. Quantum spin ice (QSI) is a theoretically well-established example described by an emergent quantum electrodynamics, with excitations behaving like photon and matter quasiparticles. The latter are fractionally charged and equivalent to the `spinons' emerging from coherent phases of singlets in one dimension, where clear experimental proofs of fractionalization exist. However, in frustrated magnets it remains difficult to establish consensual evidence for quantum spin liquid ground states and their fractional excitations. Here, we use backscattering neutron spectroscopy to achieve extremely high resolution of the time-dependent magnetic response of the candidate QSI material Ce$_2$Sn$_2$O$_7$. We find a gapped spectrum featuring a threshold and peaks that match theories for pair production and propagation of fractional matter excitations (spinons) strongly coupled to a background gauge field. The multiple peaks are a specific signature of the $π$-flux phase of QSI, providing spectroscopic evidence for fractionalization in a three-dimensional quantum spin liquid.

cond-mat.str-el↗

arXiv2024

Magnetic Field Response of Dipolar-Octupolar Quantum Spin Ice

Dipolar-octupolar (DO) pyrochlore systems Ce$_2$(Zr,Sn,Hf)$_2$O$_7$ have garnered much attention as recent investigations suggest that they may stabilize a novel quantum spin ice (QSI), a quantum spin liquid (QSL) with an emergent $U(1)$ gauge field. In particular, the experimentally estimated microscopic exchange parameters place Ce$_2$Zr$_2$O$_7$ in the $π$-flux QSI regime, and recent neutron scattering experiments have corroborated some key theoretical predictions. On the other hand, to make a definitive conclusion, more multifaceted experimental signatures are desirable. In this regard, recent neutron scattering investigation of the magnetic field dependence of the spin correlations in Ce$_2$Zr$_2$O$_7$ may provide valuable information. However, there have not been any comprehensive theoretical studies for comparison. In this work, we provide such information using gauge mean-field theory (GMFT), allowing for theoretical investigation beyond the perturbative regime. In particular, we construct the phase diagrams for the [110], [111], and [001] field directions. Furthermore, we demonstrate the distinctive evolution of the equal-time and dynamical spin structure factors as a function of the magnetic field for each field direction. These predictions will help future experiments confirm the true nature of the DO-QSI.

cond-mat.str-el↗

arXiv2024

Emergent photons and fractionalized excitations in a quantum spin liquid

A quantum spin liquid (QSL) arises from a highly entangled superposition of many degenerate classical ground states in a frustrated magnet, and is characterized by emergent gauge fields and deconfined fractionalized excitations (spinons). Because such a novel phase of matter is relevant to high-transition-temperature superconductivity and quantum computation, the microscopic understanding of QSL states is a long-sought goal in condensed matter physics. The 3D pyrochlore lattice of corner-sharing tetrahedra can host a QSL with U(1) gauge fields called quantum spin ice (QSI), which is a quantum (with effective $S=1/2$) analog of the classical (with large effective moment) spin ice. A key difference between QSI and classical spin ice is the predicted presence of the linearly dispersing collective excitations near zero energy, dubbed the "photons", arising from emergent quantum electrodynamics, in addition to the spinons at higher energies. Recently, 3D pyrochlore systems Ce2M2O7 (M = Sn, Zr, Hf) have been suggested as effective $S=1/2$ QSI candidates, but there has been no evidence of quasielastic magnetic scattering signals from photons, a key signature for a QSI. Here, we use polarized neutron scattering experiments on single crystals of Ce2Zr2O7 to conclusively demonstrate the presence of magnetic excitations near zero energy at 50 mK in addition to signatures of spinons at higher energies. By comparing the energy (E), wave vector (Q), and polarization dependence of the magnetic excitations with theoretical calculations, we conclude that Ce2Zr2O7 is the first example of a dipolar-octupolar $π$ flux QSI with dominant dipolar Ising interactions, therefore identifying a microscopic Hamiltonian responsible for a QSL.

cond-mat.str-el↗

arXiv2024

Quantum Fluctuations Suppress the Critical Fields in BaCo$_2$(AsO$_4$)$_2$

Early efforts to realize exotic quantum ground states in frustrated magnets focused on frustration arising from the lattice geometry alone. Attention has shifted to bond-dependent anisotropic interactions, as well as further-neighbor interactions, on non-geometrically-frustrated lattices due to their greater versatility. The honeycomb magnet BaCo$_2$(AsO$_4$)$_2$ recently emerged as a candidate host for both bond-dependent (e.g. Kitaev) and third-neighbor ($J_3$) interactions, and has become a model experimental system due to its relatively low levels of disorder. Understanding the relative importance of different exchange interactions holds the key to achieving novel ground states, such as quantum spin liquids. Here, we use the magnetotropic susceptibility to map out the intermediate and high-field phase diagram of BaCo$_2$(AsO$_4$)$_2$ as a function of the out-of-plane magnetic field direction at $T = 1.6$ K. We show that the experimental data are qualitatively consistent with classical Monte Carlo results of the XXZ-$J_1$-$J_3$ model with small Kitaev and off-diagonal exchange couplings included. However, the calculated critical fields are systematically larger than the experimental values. Infinite-DMRG computations on the quantum model reveal that quantum corrections from a nearby ferromagnetic state are likely responsible for the suppressed critical fields. Together, our experiment and theory analyses demonstrate that, while quantum fluctuations play an important role in determining the phase diagram, most of the physics of BaCo$_2$(AsO$_4$)$_2$ can be understood in terms of the classical dynamics of long-range ordered states, leaving little room for the possibility of a quantum spin liquid.

cond-mat.str-el↗

arXiv2024

Spectroscopic signatures of fractionalization in octupolar quantum spin ice

Recent investigations on the dipolar-octupolar compounds Ce$_2$Zr$_2$O$_7$ and Ce$_2$Sn$_2$O$_7$ suggest that they may stabilize so-called $π$-flux octupolar quantum spin ice ($π$-O-QSI), a novel three-dimensional quantum spin liquid hosting emergent photons. Confirmation of such an exotic phase would require the prediction of a distinctive signature and its subsequent experimental observation. So far, however, theoretical predictions for any such sharp smoking-gun signatures are lacking. In this Letter, we thoroughly investigate O-QSI using an extension of gauge mean-field theory. This framework produces a phase diagram consistent with previous studies and an energy-integrated neutron scattering signal with intensity-modulated rod motifs, as reported in experiments and numerical studies. We predict that the dynamical spin structure factor of $π$-O-QSI is characterized by a broad continuum with three distinctive peaks as a consequence of the two mostly flat spinon bands. These three peaks should be measurable by high-resolution inelastic neutron scattering. Such spectroscopic signatures would be clear evidence for the realization of $π$-flux quantum spin ice.

cond-mat.str-el↗

arXiv2024

Finite Temperature Dynamics in 0-Flux and $π$-Flux Quantum Spin Ice: Self-Consistent Exclusive Boson Approach

Quantum spin ice (QSI) is an emblematic three-dimensional $U(1)$ quantum spin liquid (QSL) on the pyrochlore lattice that hosts gapless photon-like modes and spinon excitations. Despite its notable status and the current rise of strong material candidates Ce$_2$(Zr, Sn, Hf)$_2$O$_7$, there are still only a few analytical approaches to model the low-energy behavior of QSI. These analytical methods are essential to gain insight into the physical interpretation of measurements. We here introduce the self-consistent exclusive boson representation (SCEBR) to model emergent spinon excitations in QSI. By treating the presence of other emergent charges in an average way, the SCEBR extends the range of validity of the exclusive boson representation previously introduced by Hao, Day, and Gingras [Hao, Day, and Gingras, Physical Review B, 90, 214430 (2014)] to numerous cases of physical relevance. We extensively benchmark the approach and provide detailed analytical expressions for the spinon dispersion, the Bogoliubov transformation that diagonalizes the system, and the dynamical spin structure factor for 0- and $π$-flux QSI. Finite temperature properties are further investigated to highlight essential differences between the thermodynamic behavior of the 0- and $π$-flux phases. We notably show that the SCEBR predicts a reduction of the spinon bandwidth with increasing temperature, consistent with previous quantum Monte-Carlo results, through suppression of spinon hopping by thermal occupation. The SCEBR thus provides a powerful analytical tool to interpret experiments on current and future candidate material that has several advantages over other widely used methods.

cond-mat.str-el↗

arXiv2023

A pseudofermion functional renormalization group study of dipolar-octupolar pyrochlore magnets

Motivated by recent experiments on Ce$_2$Zr$_2$O$_7$ that reveal a dynamic, liquid-like ground state, we study the nearest neighbor XYZ Hamiltonian of dipolar-octupolar pyrochlore magnets with the pseudofermion functional renormalization group (PFFRG), which is numerically implemented by the SpinParser software. Taking the interaction between the octupolar components to be dominant and antiferromagnetic, we map out the phase diagram demarcating the quantum disordered and magnetically ordered states. We identify four distinct phases, namely the $0$-flux and $π$-flux quantum spin ices, and the all-in-all-out magnetic orders along the local $z$ and $x$ axes. We further use the static two-spin correlations output by the PFFRG algorithm to compute the polarized neutron scattering cross-sections, which are able to capture several qualitative features observed experimentally, in the materially relevant parameter regime that stabilizes the $π$-flux quantum spin ice. Our results provide support for a quantum spin liquid ground state in Ce$_2$Zr$_2$O$_7$.

cond-mat.str-el↗

arXiv2023

Symmetry fractionalization in the gauge mean-field theory of quantum spin ice

Symmetry fractionalization is a ubiquitous feature of topologically ordered states that can be used to classify different symmetry-enriched topological phases and reveal some of their unique experimental signatures. Despite its vast popularity, there is currently no available framework to study symmetry fractionalization of quantum spin ice (QSI) -- a $U(1)$ quantum spin liquid (QSL) on the pyrochlore lattice supporting emergent photons -- within the most widely used theoretical framework to describe it, gauge mean-field theory (GMFT). In this work, we provide an extension of GMFT that allows for the classification of space-time symmetry fractionalization. The construction classifies all GMFT Ansätze that yield physical wavefunctions invariant under given symmetries and a specific low-energy gauge structure. As an application of the framework, we first show that the only two Ansätze with emergent $U(1)$ gauge fields that respect all space-group symmetries are the well-known 0- and $π$-flux states. We then showcase how the framework may describe QSLs beyond the currently known ones by classifying chiral $U(1)$ QSI. We find two new states described by $π/2$- and $3π/2$-fluxes of the emergent gauge field threading the hexagonal plaquettes of the pyrochlore lattice. We finally discuss how the different ways translation symmetries fractionalize for all these states lead to unique experimentally relevant signatures and compute their respective inelastic neutron scattering cross-section to illustrate the argument.

cond-mat.str-el↗

arXiv2022

Geometrical frustration versus Kitaev interactions in BaCo$_2$(AsO$_4$)$_2$

Recently, Co-based honeycomb magnets have been proposed as promising candidate materials to host the Kitaev spin liquid state. One of the front-runners is BaCo$_2$(AsO$_4$)$_2$ (BCAO), where it was suggested that the exchange processes between Co$^{2+}$ ions via the surrounding edge-sharing oxygen octahedra could give rise to bond-dependent Kitaev interactions. In this work, we present and analyze comprehensive inelastic neutron scattering studies of BCAO with fields in the honeycomb plane. Combining the constraints from the magnon excitations in the high-field polarized state and the inelastic spin structure factor measured in zero magnetic field, we examine two leading theoretical models: the Kitaev-type \JKG model and the \XXZ model. We show that the existing experimental data can be consistently accounted for by the \XXZ model but not by the \JKG model, and we discuss the implications of these results for the realization of a spin liquid phase in BCAO and more generally for the realization of the Kitaev model in cobaltates.

cond-mat.str-el↗

arXiv2021

Competing $U(1)$ and $\mathbb{Z}_2$ dipolar-octupolar quantum spin liquids on the pyrochlore lattice: application to Ce$_2$Zr$_2$O$_7$

Recent experiments on the dipolar-octupolar pyrochlore compound Ce$_2$Zr$_2$O$_7$ indicate that it may realize a three-dimensional quantum spin liquid (QSL). In particular, the analyses of available data suggest that the system is in a region of parameter space, where the so-called $π$-flux $U(1)$ octupolar quantum spin ice (QSI) with an emergent photon could be realized. On the other hand, because the system is far from the perturbative classical spin ice regime, it is unclear whether the quantum ground state is primarily a coherent superposition of 2-in-2-out configurations as in the canonical QSI phases. In this work, we explore other possible competing quantum spin liquid states beyond QSI using the Schwinger boson parton construction of the dipolar-octupolar pseudospin-1/2 model. After classifying all symmetric $U(1)$ and $\mathbb{Z}_2$ QSLs using the projective symmetry group (PSG), we construct a mean-field phase diagram that possesses a number of important features observed in an earlier exact diagonalization study. In the experimentally relevant frustrated region of the phase diagram, we find two closely competing gapped $\mathbb{Z}_2$ QSLs with a narrow spinon dispersion. The equal-time and dynamical spin structure factors of these states show key features similar to what was reported in neutron scattering experiments. Hence, these QSLs are closely competing ground states in addition to the $π$-flux $U(1)$ QSI, and they should be taken into account on equal footing for the interpretation of experiments on Ce$_2$Zr$_2$O$_7$.

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