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F. A. Danevich

Publications and source records attributed to F. A. Danevich.

At least 73 records · Page 4Linked to original sources

Precise measurement of $2νββ$ decay of $^{100}$Mo with the CUPID-Mo detection technology

We report the measurement of the two-neutrino double-beta ($2νββ$) decay of $^{100}$Mo to the ground state of $^{100}$Ru using lithium molybdate (\crystal) scintillating bolometers. The detectors were developed for the CUPID-Mo program and operated at the EDELWEISS-III low background facility in the Modane underground laboratory. From a total exposure of $42.235$ kg$\times$d, the half-life of $^{100}$Mo is determined to be $T_{1/2}^{2ν}=[7.12^{+0.18}_{-0.14}\,\mathrm{(stat.)}\pm0.10\,\mathrm{(syst.)}]\times10^{18}$ years. This is the most accurate determination of the $2νββ$ half-life of $^{100}$Mo to date. We also confirm, with the statistical significance of $>3σ$, that the single-state dominance model of the $2νββ$ decay of $^{100}$Mo is favored over the high-state dominance model.

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First data from the CUPID-Mo neutrinoless double beta decay experiment

The CUPID-Mo experiment is searching for neutrinoless double beta decay in $^{100}$Mo, evaluating the technology of cryogenic scintillating Li$_{2}^{100}$MoO$_4$ detectors for CUPID (CUORE Upgrade with Particle ID). CUPID-Mo detectors feature background suppression using a dual-readout scheme with Li$_{2}$MoO$_4$ crystals complemented by Ge bolometers for light detection. The detection of both heat and scintillation light signals allows the efficient discrimination of $α$ from $γ$&$β$ events. In this proceedings, we discuss results from the first 2 months of data taking in spring 2019. In addition to an excellent bolometric performance of 6.7$\,$keV (FWHM) at 2615$\,$keV and an $α$ separation of better than 99.9\% for all detectors, we report on bulk radiopurity for Th and U. Finally, we interpret the accumulated physics data in terms of a limit of $T_{1/2}^{0ν}\,> 3\times10^{23}\,$yr for $^{100}$Mo and discuss the sensitivity of CUPID-Mo until the expected end of physics data taking in early 2020.

hep-ex↗

First search for $α$ decays of naturally occurring Hf nuclides with emission of $γ$ quanta

The first ever search for $α$ decays to the first excited state in Yb was performed for six isotopes of hafnium (174, 176, 177, 178, 179, 180) using a high purity Hf-sample of natural isotopic abundance with a mass of 179.8 g. For $^{179}$Hf, also $α$ decay to the ground state of $^{175}$Yb was searched for thanks to the $β$-instability of the daughter nuclide $^{175}$Yb. The measurements were conducted using an ultra low-background HPGe-detector system located 225 m underground. After 75 d of data taking no decays were detected but lower bounds for the half-lives of the decays were derived on the level of $\lim T_{1/2}\sim 10^{15}-10^{18}$~a. The decay with the shortest half-life based on theoretical calculation is the decay of $^{174}$Hf to the first $2^+$ 84.3~keV excited level of $^{170}$Yb. The experimental lower bound was found to be $T_{1/2}\geq 3.3\times 10^{15}$ a.

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First direct search for $2ε$ and $εβ^+$ decay of $^{144}$Sm and $2β^-$ decay of $^{154}$Sm

The first direct search for the double electron capture ($2ε$) and the electron capture with positron emission ($εβ^+$) in $^{144}$Sm to the ground state and to the excited levels of $^{144}$Nd was realized by measuring - over 1899 h - a 342 g sample of highly purified samarium oxide (Sm$_2$O$_3$) with the ultra-low background HP-Ge $γ$ spectrometer GeCris (465 cm$^3$) at the STELLA facility of the Gran Sasso National Laboratory (LNGS). No effect was observed and half-life limits were estimated at the level of $T_{1/2} \sim (0.1-1.3) \times 10^{20}$ yr (90% C.L.). Moreover, for the first time half-life limits of the double beta ($2β^-$) decay of $^{154}$Sm to several excited levels of $^{154}$Gd have been set; they are at the level of $T_{1/2} \sim (0.06-8) \times 10^{20}$ yr (90% C.L.).

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The $0\nu2β$-decay CROSS experiment: preliminary results and prospects

Neutrinoless double-beta decay is a key process in particle physics. Its experimental investigation is the only viable method that can establish the Majorana nature of neutrinos, providing at the same time a sensitive inclusive test of lepton number violation. CROSS (Cryogenic Rare-event Observatory with Surface Sensitivity) aims at developing and testing a new bolometric technology to be applied to future large-scale experiments searching for neutrinoless double-beta decay of the promising nuclei $^{100}$Mo and $^{130}$Te. The limiting factor in large-scale bolometric searches for this rare process is the background induced by surface radioactive contamination, as shown by the results of the CUORE experiment. The basic concept of CROSS consists of rejecting this challenging background component by pulse-shape discrimination, assisted by a proper coating of the faces of the crystal containing the isotope of interest and serving as energy absorber of the bolometric detector. In this paper, we demonstrate that ultra-pure superconductive Al films deposited on the crystal surfaces act successfully as pulse-shape modifiers, both with fast and slow phonon sensors. Rejection factors higher than 99.9% of $α$ surface radioactivity have been demonstrated in a series of prototypes based on crystals of Li$_2$MoO$_4$ and TeO$_2$. We have also shown that point-like energy depositions can be identified up to a distance of $\sim 1$ mm from the coated surface. The present program envisions an intermediate experiment to be installed underground in the Canfranc laboratory (Spain) in a CROSS-dedicated facility. This experiment, comprising $\sim 3\times 10^{25}$ nuclei of $^{100}$Mo, will be a general test of the CROSS technology as well as a worldwide competitive search for neutrinoless double-beta decay, with sensitivity to the effective Majorana mass down to 70 meV in the most favorable conditions.

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The CUPID-Mo experiment for neutrinoless double-beta decay: performance and prospects

CUPID-Mo is a bolometric experiment to search for neutrinoless double-beta decay ($0νββ$) of $^{100}$Mo. In this article, we detail the CUPID-Mo detector concept, assembly, installation in the underground laboratory in Modane in 2018, and provide results from the first datasets. The demonstrator consists of an array of 20 scintillating bolometers comprised of $^{100}$Mo-enriched 0.2 kg Li$_2$MoO$_4$ crystals. The detectors are complemented by 20 thin cryogenic Ge bolometers acting as light detectors to distinguish $α$ from $γ$/$β$ events by the detection of both heat and scintillation light signals. We observe good detector uniformity, facilitating the operation of a large detector array as well as excellent energy resolution of 5.3 keV (6.5 keV) FWHM at 2615 keV, in calibration (physics) data. Based on the observed energy resolutions and light yields a separation of $α$ particles at much better than 99.9\% with equally high acceptance for $γ$/$β$ events is expected for events in the region of interest for $^{100}$Mo $0νββ$. We present limits on the crystals' radiopurity ($\leq$3 $μ$Bq/kg of $^{226}$Ra and $\leq$2 $μ$Bq/kg of $^{232}$Th). Based on these initial results we also discuss a sensitivity study for the science reach of the CUPID-Mo experiment, in particular, the ability to set the most stringent half-life limit on the $^{100}$Mo $0νββ$ decay after half a year of livetime. The achieved results show that CUPID-Mo is a successful demonstrator of the technology - developed in the framework of the LUMINEU project - selected for the CUPID experiment, a proposed follow-up of CUORE, the currently running first tonne-scale cryogenic $0νββ$ experiment.

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Experimental searches for rare alpha and beta decays

The current status of the experimental searches for rare alpha and beta decays is reviewed. Several interesting observations of alpha and beta decays, previously unseen due to their large half-lives ($10^{15} - 10^{20}$ yr), have been achieved during the last years thanks to the improvements in the experimental techniques and to the underground locations of experiments that allows to suppress backgrounds. In particular, the list includes first observations of alpha decays of $^{151}$Eu, $^{180}$W (both to the ground state of the daughter nuclei), $^{190}$Pt (to excited state of the daughter nucleus), $^{209}$Bi (to the ground and excited states of the daughter nucleus). The isotope $^{209}$Bi has the longest known half-life of $T_{1/2} \approx 10^{19}$ yr relatively to alpha decay. The beta decay of $^{115}$In to the first excited state of $^{115}$Sn (E$_{exc} = 497.334$ keV), recently observed for the first time, has the $Q_β$ value of only $(147 \pm 10)$ eV, which is the lowest $Q_β$ value known to-date. Searches and investigations of other rare alpha and beta decays ($^{48}$Ca, $^{50}$V, $^{96}$Zr, $^{113}$Cd, $^{123}$Te, $^{178m2}$Hf, $^{180m}$Ta and others) are also discussed.

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First search for 2$\varepsilon$ and $\varepsilonβ^+$ processes in $^{168}$Yb

The double-electron capture and the electron capture with positron emission in $^{168}$Yb have been investigated for the first time at the STELLA facility of the Gran Sasso underground laboratory (Italy) measuring 371 g of highly purified ytterbium oxide placed on the end-cap of a 465 cm$^3$ ultra-low-background high purity Germanium detector (HPGe). No gamma associated to double beta processes in $^{168}$Yb have been observed after 2074 h of data taking. This has allowed setting the half-life limits on the level of $\lim T_{1/2}\sim$ $10^{14}-10^{18}$ yr at 90\% C.L. Particularly, a lower half-life limit on a possible resonant neutrinoless double-electron capture in $^{168}$Yb to the $(2)^-$ 1403.7 keV excited state of $^{168}$Er is set as $T_{1/2}\geq1.9\times 10^{18}$ yr at 90\% C.L. Half-life limits $T_{1/2}^{2ν(0ν)}\geq 4.5(4.3)\times10^{16}$ yr were set on the $2ν(0ν)2β^-$ decay of $^{176}$Yb to the $2^+$ 84.3 keV first excited level of $^{176}$Hf.

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First Results from the AMoRE-Pilot neutrinoless double beta decay experiment

The Advanced Molybdenum-based Rare process Experiment (AMoRE) aims to search for neutrinoless double beta decay (0$νββ$) of $^{100}$Mo with $\sim$100 kg of $^{100}$Mo-enriched molybdenum embedded in cryogenic detectors with a dual heat and light readout. At the current, pilot stage of the AMoRE project we employ six calcium molybdate crystals with a total mass of 1.9 kg, produced from $^{48}$Ca-depleted calcium and $^{100}$Mo-enriched molybdenum ($^{48\textrm{depl}}$Ca$^{100}$MoO$_4$). The simultaneous detection of heat(phonon) and scintillation (photon) signals is realized with high resolution metallic magnetic calorimeter sensors that operate at milli-Kelvin temperatures. This stage of the project is carried out in the Yangyang underground laboratory at a depth of 700 m. We report first results from the AMoRE-Pilot $0νββ$ search with a 111 kg$\cdot$d live exposure of $^{48\textrm{depl}}$Ca$^{100}$MoO$_4$ crystals. No evidence for $0νββ$ decay of $^{100}$Mo is found, and a upper limit is set for the half-life of 0$νββ$ of $^{100}$Mo of $T^{0ν}_{1/2} > 9.5\times10^{22}$ y at 90% C.L.. This limit corresponds to an effective Majorana neutrino mass limit in the range $\langle m_{ββ}\rangle\le(1.2-2.1)$ eV.

hep-ex↗

Half-life measurements of $^{212}$Po with thorium-loaded liquid scintillator

Precise measurement of half-life of $^{212}$Po (one of the daughter nuclides in radioactive chain of $^{232}$Th) was realized by means of liquid scintillator based on toluene doped by complex of thorium and trioctylphosphine oxide with concentration of Th $\sim0.1$ mass %. Fast photomultiplier tube and high frequency oscilloscope were used to acquire the scintillation signals waveforms. The algorithms were developed to find pairs of $^{212}$Bi beta-decays and subsequent $^{212}$Po alpha-decays, to calculate time differences between the events in the pair, and to build $^{212}$Bi beta-decay and $^{212}$Po alpha-decay energy spectra. Preliminary the $^{212}$Po half-life is $T_{1/2} = (294.8 \pm 1.9)$ ns. The experiment is in progress aiming at reduction of the statistical and systematic uncertainties.

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Final results of the Aurora experiment to study 2$β$ decay of $^{116}$Cd with enriched $^{116}$CdWO$_4$ crystal scintillators

The double-beta decay of $^{116}$Cd has been investigated with the help of radiopure enriched $^{116}$CdWO$_4$ crystal scintillators (mass of 1.162 kg) at the Gran Sasso underground laboratory. The half-life of $^{116}$Cd relatively to the $2\nu2β$ decay to the ground state of $^{116}$Sn was measured with the highest up-to-date accuracy as $T_{1/2}=(2.63^{+0.11}_{-0.12})\times10^{19}$ yr. A new improved limit on the 0$ν$2$β$ decay of $^{116}$Cd to the ground state of $^{116}$Sn was set as $T_{1/2}\geq 2.2 \times 10^{23}$ yr at 90\% C.L., which is the most stringent known restriction for this isotope. It corresponds to the effective Majorana neutrino mass limit in the range $\langle m_ν\rangle\le(1.0-1.7)$ eV, depending on the nuclear matrix elements used in the estimations. New improved half-life limits for the 0$ν$2$β$ decay with majoron(s) emission, Lorentz-violating $2\nu2β$ decay and $2β$ transitions to excited states of $^{116}$Sn were set at the level of $T_{1/2}\geq 10^{20}-10^{22}$ yr. New limits for the hypothetical lepton-number violating parameters (right-handed currents admixtures in weak interaction, the effective majoron-neutrino coupling constants, R-parity violating parameter, Lorentz-violating parameter, heavy neutrino mass) were set.

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Double beta decay of $^{150}$Nd to the first excited $0^+$ level of $^{150}$Sm: preliminary results

The double beta decay of $^{150}$Nd to the first excited 0$^+$ level of $^{150}$Sm ($E_{exc}$ = 740.5 keV) has been investigated with the help of the ultra-low-background setup consisting of four HP Ge (high-purity germanium) detectors (${\approx}$ 225 cm$^3$ volume each one) at the Gran Sasso underground laboratory of INFN (Italy). A highly purified 2.381-kg sample of neodymium oxide (Nd$_2$O$_3$) was used as a source of $γ$ quanta expected in the decays. Gamma quanta with energies 334.0 keV and 406.5 keV emitted after deexcitation of the $0_1^+$ 740.5 keV level of $^{150}$Sm are observed in the coincidence spectra accumulated over 16375 h. The half-life relatively to the two neutrino double beta decay $^{150}$Nd $\rightarrow$ $^{150}$Sm(0$_1^+$) is measured as $T_{1/2} = [4.7_{-1.9}^{+4.1}\text{(stat)} {\pm} 0.5\text{(syst)}] {\times} 10^{19} y$, in agreement with results of previous experiments.

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First search for $2\varepsilon$ and $\varepsilonβ^+$ decay of $^{162}$Er and new limit on $2β^{-}$ decay of $^{170}$Er to the first excited level of $^{170}$Yb

The first search for double electron capture ($2\varepsilon$) and electron capture with positron emission ($\varepsilonβ^+$) of $^{162}$Er to the ground state and to several excited levels of $^{162}$Dy was realized with 326 g of highly purified erbium oxide. The sample was measured over 1934 h by the ultra-low background HP Ge $γ$ spectrometer GeCris (465 cm$^3$) at the Gran Sasso underground laboratory. No effect was observed, the half-life limits were estimated at the level of $\lim T_{1/2}\sim 10^{15}-10^{18}$ yr. A possible resonant $0νKL_1$ capture in $^{162}$Er to the $2^+$ 1782.7 keV excited state of $^{162}$Dy is restricted as $T_{1/2}\geq5.0\times 10^{17}$ yr at 90% C.L. A new improved half-life limit $T_{1/2}\geq4.1\times 10^{17}$ yr was set on the $2β^-$ decay of $^{170}$Er to the $2^+$ 84.3 keV first excited state of $^{170}$Yb.

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A multi-isotope $0\nu2β$ bolometric experiment

There are valuable arguments to perform neutrinoless double beta ($0\nu2β$) decay experiments with several nuclei: the uncertainty of nuclear-matrix-ele\-ment calculations; the possibility to test these calculations by using the ratio of the measured lifetimes; the unpredictability of possible breakthroughs in the detection technique; the difficulty to foresee background in $0\nu2β$ decay searches; the limited amount of isotopically enriched materials. We propose therefore approaches to estimate the Majorana neutrino mass by combining experimental data collected with different $0\nu2β$ decay candidates. In particular, we apply our methods to a next-generation experiment based on scintillating and Cherenkov-radiation bolometers. Current results indicate that this technology can effectively study up to four different isotopes simultaneously ($^{82}$Se, $^{100}$Mo, $^{116}$Cd and $^{130}$Te), embedded in detectors which share the same concepts and environment. We show that the combined information on the Majorana neutrino mass extracted from a multi-candidate bolometric experiment is competitive with that achievable with a single isotope, once that the cryogenic experimental volume is fixed. The remarkable conceptual and technical advantages of a multi-isotope investigation are discussed. This approach can be naturally applied to the proposed CUPID project, follow-up of the CUORE experiment that is currently taking data in the Gran Sasso underground laboratory.

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Radioactive contamination of scintillators

Low counting experiments (search for double $β$ decay and dark matter particles, measurements of neutrino fluxes from different sources, search for hypothetical nuclear and subnuclear processes, low background $α$, $β$, $γ$ spectrometry) require extremely low background of a detector. Scintillators are widely used to search for rare events both as conventional scintillation detectors and as cryogenic scintillating bolometers. Radioactive contamination of a scintillation material plays a key role to reach low level of background. Origin and nature of radioactive contamination of scintillators, experimental methods and results are reviewed. A programme to develop radiopure crystal scintillators for low counting experiments is discussed briefly.

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Growth and characterization of a Li2Mg2(MoO4)3 scintillating bolometer

Lithium magnesium molybdate (Li$_2$Mg$_2$(MoO$_4$)$_3$) crystals were grown by the low-thermal-gradient Czochralski method. Luminescence properties of the material (emission spectra, thermally stimulated luminescence, dependence of intensity on temperature, phosphorescence) have been studied under X-Ray excitation in the temperature interval from 8 K to 400 K, while at the same being operated as a scintillating bolometer at 20 mK for the first time. We demonstrated that Li$_2$Mg$_2$(MoO$_4)_3$ crystals are a potentially promising detector material to search for neutrinoless double beta decay of $^{100}$Mo.

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Investigation of 2$β$ Decay of $^{116}$Cd with the Help of Enriched $^{116}$CdWO$_4$ Crystal Scintillators

Double beta decay of $^{116}$Cd has been investigated with the help of radiopure enriched $^{116}$CdWO$_4$ crystal scintillators in the experiment Aurora. The half-life of $^{116}$Cd relatively to the 2$ν$2$β$ decay of $^{116}$Cd to the ground level of $^{116}$Sn is measured with the highest up-to-date accuracy as $T_{1/2}$ = [2.69 $\pm$ 0.02 (stat.) $\pm$ 0.14 (syst.)] $\times$ 10$^{19}$ yr. A new improved limit on the 0$ν$2$β$ decay of $^{116}$Cd to the ground state of $^{116}$Sn is set as $T_{1/2}\geq 2.4 \times 10^{23}$ yr at 90\% C.L., that corresponds to the effective Majorana neutrino mass limit in the range $\langle$$m_ν$$\rangle$ $\le$ $(1.1-1.6)$ eV, depending on the nuclear matrix elements used in the estimations. New improved limits on other $2β$ processes in $^{116}$Cd (decays with majoron emission, transitions to excited levels of $^{116}$Sn) were set at the level of $T_{1/2}\geq 10^{21}-10^{22}$ yr.

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Development of $^{100}$Mo-containing scintillating bolometers for a high-sensitivity neutrinoless double-beta decay search

This paper reports on the development of a technology involving $^{100}$Mo-enriched scintillating bolometers, compatible with the goals of CUPID, a proposed next-generation bolometric experiment to search for neutrinoless double-beta decay. Large mass ($\sim$1~kg), high optical quality, radiopure $^{100}$Mo-containing zinc and lithium molybdate crystals have been produced and used to develop high performance single detector modules based on 0.2--0.4~kg scintillating bolometers. In particular, the energy resolution of the lithium molybdate detectors near the $Q$-value of the double-beta transition of $^{100}$Mo (3034~keV) is 4--6~keV FWHM. The rejection of the $α$-induced dominant background above 2.6~MeV is better than 8$σ$. Less than 10~$μ$Bq/kg activity of $^{232}$Th ($^{228}$Th) and $^{226}$Ra in the crystals is ensured by boule recrystallization. The potential of $^{100}$Mo-enriched scintillating bolometers to perform high sensitivity double-beta decay searches has been demonstrated with only 10~kg$\times$d exposure: the two neutrino double-beta decay half-life of $^{100}$Mo has been measured with the up-to-date highest accuracy as $T_{1/2}$ = [6.90 $\pm$ 0.15(stat.) $\pm$ 0.37(syst.)] $\times$ 10$^{18}$~yr. Both crystallization and detector technologies favor lithium molybdate, which has been selected for the ongoing construction of the CUPID-0/Mo demonstrator, containing several kg of $^{100}$Mo.

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