arXiv subjects

F. Dubin

Publications and source records attributed to F. Dubin.

At least 19 recordsLinked to original sources

arXiv2025

Supersolid crystals of dipolar excitons in a lattice

In condensed-matter physics, long-range correlations introduce quantum states of matter that challenge intuition. For instance, supersolids combine symmetry-breaking crystalline structure, i.e. density order, and frictionless superfluid flow. Envisioned over fifty years ago, supersolids have proven to only exist under very stringent conditions, with experimental evidence limited to few observations. Many-body phases with supersolid properties in fact reduce to a few recent observations for weakly interacting Bose gases. Here, we demonstrate a new framework to realize supersolid crystals in the strong interaction regime, by confining dipolar bosons in a lattice with long-range hopping. We study dipolar excitons that genuinely realize this lattice model. At fractional lattice fillings - 1/4, 1/3 and 1/2 - we report mesoscopic quantum solids, across over 100 sites, spontaneously breaking translational symmetry. At the same time, we show that off-diagonal long-range order is induced by long-range hopping, such that exciton solids are superfluids. State-of-the-art numerical methods quantitatively confirm that supersolidity builds up in the ground-state of the lattice Hamiltonian. Our studies of strongly-correlated supersolid crystals open new frontiers for exploration in condensed matter physics.

cond-mat.quant-gas↗

arXiv2025

Probing moire excitons in MoSe2/WSe2 heterobilayers by combined micro-photoluminescence and lateral force microscopy

We study interlayer excitons in MoSe2/WSe2 heterobilayers, by combining lateral force microscopy and micro-photoluminescence spectroscopy. This allows us to correlate the spatial profile of the moir\'e superlattice with the distribution of optically active states accessible to interlayer excitons. In heterostructures where a few degrees twist angle is imposed between the MoSe and WSe crystallographic axes, we show that a continuous moir\'e lattice is realized across areas close to the optical diffraction limit. In such regions, the photoluminescence reduces to a few narrow-band lines only, energetically distributed consistently with the geometry of the moir\'e lattice. This correlation reveals that interlayer excitons explore a controlled periodic confinement, paving the way towards implementations of Bose-Hubbard models.

cond-mat.mes-hall↗

arXiv2022

Extended Bose-Hubbard model with dipolar excitons

The Hubbard model constitutes one of the most celebrated theoretical frameworks of condensed-matter physics. It describes strongly correlated phases of interacting quantum particles confined in lattice potentials. For bosons, the Hubbard Hamiltonian has been deeply scrutinised for short-range on-site interactions. However, accessing longer-range couplings has remained elusive experimentally. This marks the frontier towards the extended Bose-Hubbard Hamiltonian that allows insulating ordered phases at fractional lattice fillings. Here we implement this Hamiltonian by confining semiconductor dipolar excitons in an artificial two-dimensional square lattice. Strong dipolar repulsions between nearest neighbouring lattice sites then stabilise an insulating state at half filling. This characteristic feature of the extended Bose-Hubbard model exhibits signatures theoretically expected for a checkerboard spatial order. Our work thus highlights that dipolar excitons enable controlled implementations of boson-like arrays with strong off-site interactions, in lattices with programmable geometries and over 100 sites.

cond-mat.str-el↗

arXiv2020

Observation of Algebraic Time Order for Two-Dimensional Dipolar Excitons

Emergence of algebraic quasi-long-range order is a key feature of superfluid phase transitions at two dimensions. For this reduced dimensionality interactions prevent Bose-Einstein condensation with true long range order, at any finite temperature. Here, we report the occurence of algebraic order in a strongly interacting quantum liquid formed by dipolar excitons confined in a bilayer semiconductor heterostructure. We observe a transition from exponential to algebraic decay of the excitons temporal coherence, accompanied by a universal scaling behaviour of the equation of state. Our results provide strong evidence for a Berezinskii-Kosterlitz-Thouless (BKT) transition in a multi-component boson-like system governed by strong dipolar interactions.

cond-mat.quant-gas↗

arXiv2014

Effects of fermion exchanges on the polarization of exciton condensates

Exchange processes are responsible for the stability of elementary boson condensates with respect to their possible fragmentation. This remains true for composite bosons when single fermion exchanges are included but spin degrees of freedom are ignored. We here show that their inclusion can produce a "spin-fragmentation" of a condensate of dark excitons, i.e., an unpolarized condensate with equal amount of dark excitons with spins (+2) and (-2). Quite surprisingly, for spatially indirect excitons of semiconductor bilayers, we predict that the condensate polarization can switch from unpolarized to fully polarized, depending on the distance between the layers confining electrons and holes. Remarkably, the threshold distance associated to this switching lies in the regime where experiments are nowadays carried out.

cond-mat.quant-gas↗

arXiv2013

Optical signatures of a fully dark exciton condensate

We propose optical means to reveal the presence of a dark exciton condensate that does not yield any photoluminescence at all. We show that (i) the dark exciton density can be obtained from the blueshift of the excitonic absorption line induced by dark excitons; (ii) the polarization of the dark condensate can be deduced from the blueshift dependence on probe photon polarization and also from Faraday effect, linearly polarized dark excitons leaving unaffected the polarization plane of an unabsorbed photon beam. These effects result from carrier exchanges between dark and bright excitons.

cond-mat.quant-gas↗

arXiv2012

Observation of macroscopic coherence in self-organized dipolar excitons

We report experiments showing that spatially indirect excitons confined in a wide single quantum well can exhibit macroscopic spatial coherence. Extended coherence is spontaneously established in the regime where indirect excitons form a distinctive ring shaped pattern fragmented into microscopic beads. These contain a large concentration of indirect excitons at sub-Kelvin temperatures, the excitons spatial coherence being the greatest in the vicinity of the fragments.

cond-mat.mes-hall↗

arXiv2012

A quantum detector for photon entanglement

We use a single trapped 40Ca+ ion as a resonant, polarization-sensitive absorber to detect and characterize the entanglement of tunable narrowband photon pairs from a spontaneous parametric down-conversion source. Single-photon absorption is marked by a quantum jump in the ion and heralded by coincident detection of the partner photon. For three polarization basis settings of absorption and detection of the herald, we find maximum coincidences always for orthogonal polarizations. The polarization entanglement is further evidenced by tomographic reconstruction of the biphoton quantum state.

quant-ph↗

arXiv2012

On-demand confinement of semiconductor excitons by all-optical control

In condensed-matter physics, remarkable advances have been made with atomic systems by establishing a thorough control over cooling and trapping techniques. In semiconductors, this method may also provide a deterministic approach to reach the long standing goal of harnessing collective quantum phenomena with exciton gases. While long-lived excitons are simply cooled to very low temperatures using cryogenic apparatus, engineering confining potentials has been a challenging task. This degree of control was only achieved recently with devices realized by highly demanding nano-fabrication processes. Here, we demonstrate an alternative to this technology and show how a proper optical excitation allows to manipulate in-situ the exciton transport. Our approach is based on the optically controlled injection and spatial patterning of charges trapped in a field-effect device. Thus, electric field gradients are created and implement microscopic traps or anti-traps for the excitons dipole. Accordingly, any confinement geometry can be realized by shaping the spatial profile of a laser excitation. Hence, we succeed in trapping exciton gases in a density range where quantum correlations are predicted at our very low bath temperature.

cond-mat.mes-hall↗

arXiv2012

Non-linear dynamics and inner-ring photoluminescence pattern of indirect excitons

We study the photoluminescence dynamics of ultra-cold indirect excitons optically created in a double quantum well heterostructure. Above a threshold laser excitation, our experiments reveal the apparition of the so-called inner photoluminescence ring. It is characterized by a ring shaped photoluminescence which suddenly collapses once the laser excitation is terminated. We show that the spectrally resolved dynamics is in agreement with an excitonic origin for the inner-ring which is formed due to a local heating of indirect excitons by the laser excitation. To confirm this interpretation and exclude the ionization of indirect excitons, we evaluate the excitonic density that is extracted from the energy of the photoluminescence emission. It is shown that optically injected carriers play a crucial role in that context as these are trapped in our field-effect device and then vary the electrostatic potential controlling the confinement of indirect excitons. This disruptive effect blurs the estimation of the exciton concentration. However, it suppressed by smoothing the electrostatic environment of the double quantum well by placing the latter behind a super-lattice. In this improved geometry, we then estimate that the exciton density remains one order of magnitude smaller than the critical density for the ionization of indirect excitons (or Mott transition) in the regime where the inner-ring is formed.

cond-mat.mes-hall↗

arXiv2010

Quantum magnetism and counterflow supersolidity of up-down bosonic dipoles

We study a gas of dipolar Bosons confined in a two-dimensional optical lattice. Dipoles are considered to point freely in both up and down directions perpendicular to the lattice plane. This results in a nearest neighbor repulsive (attractive) interaction for aligned (anti-aligned) dipoles. We find regions of parameters where the ground state of the system exhibits insulating phases with ferromagnetic or anti-ferromagnetic ordering, as well as with rational values of the average magnetization. Evidence for the existence of a novel counterflow supersolid quantum phase is also presented.

cond-mat.other↗

arXiv2009

Polarization-correlated photon pairs from a single ion

In the fluorescence light of a single atom, the probability for emission of a photon with certain polarization depends on the polarization of the photon emitted immediately before it. Here correlations of such kind are investigated with a single trapped calcium ion by means of second order correlation functions. A theoretical model is developed and fitted to the experimental data, which show 91% probability for the emission of polarization-correlated photon pairs within 24 ns.

quant-ph↗

arXiv2009

Bandwidth-tunable single photon source in an ion trap quantum network

We report a tunable single-photon source based on a single trapped ion. Employing spontaneous Raman scattering and in-vacuum optics with large numerical aperture, single photons are efficiently created with controlled temporal shape and coherence time. These can be varied between 70 ns and 1.6 $μ$s, as characterized by operating two sources simultaneously in two remote ion traps which reveals mutual and individual coherence through two-photon interference.

quant-ph↗

arXiv2009

Resonant interaction of a single atom with single photons from a down-conversion source

We observe the interaction of a single trapped calcium ion with single photons produced by a narrow-band, resonant down-conversion source [A. Haase et al., Opt. Lett. 34, 55 (2009)], employing a quantum jump scheme. Using the temperature dependence of the down-conversion spectrum and the tunability of the narrow source, absorption of the down-conversion photons is quantitatively characterized.

quant-ph↗

arXiv2009

Role of Fermion Exchanges in Statistical Signatures of Composite Bosons

We study statistical signatures of composite bosons made of two fermions using a new many-body approach. Extending number-states to composite bosons, two-particle correlations as well as the dispersion of the probability distribution are analyzed. We show that the particle composite nature reduces the anti-bunching effect predicted for elementary bosons. Furthermore, the probability distribution exhibits a dispersion which is greater for composite bosons than for elementary bosons. This dispersion corresponds to the one of sub-Poissonian processes, as for a quantum state, but, unlike its elementary boson counterpart, it is not minimum. In general, our work shows that it is necessary to take into account the Pauli exclusion principle which takes place between fermionic components of composite bosons - along the line here used - to possibly extract statistical properties in a precise way.

quant-ph↗

arXiv2008

Raman spectroscopy of a single ion coupled to a high-finesse cavity

We describe an ion-based cavity-QED system in which the internal dynamics of an atom is coupled to the modes of an optical cavity by vacuum-stimulated Raman transitions. We observe Raman spectra for different excitation polarizations and find quantitative agreement with theoretical simulations. Residual motion of the ion introduces motional sidebands in the Raman spectrum and leads to ion delocalization. The system offers prospects for cavity-assisted resolved-sideband ground-state cooling and coherent manipulation of ions and photons.

quant-ph↗

arXiv2008

Quantum interference from remotely trapped ions

We observe quantum interference of photons emitted by two continuously laser-excited single ions, independently trapped in distinct vacuum vessels. High contrast two-photon interference is observed in two experiments with different ion species, calcium and barium. Our experimental findings are quantitatively reproduced by Bloch equation calculations. In particular, we show that the coherence of the individual resonance fluorescence light field is determined from the observed interference.

quant-ph↗

arXiv2006

The exciton many-body theory extended to arbitrary composite bosons

We have recently constructed a many-body theory for composite excitons, in which the possible carrier exchanges between $N$ excitons can be treated exactly through a set of dimensionless ``Pauli scatterings'' between two excitons. Many-body effects with excitons turn out to be rather simple because excitons are the exact one-electron-hole-pair eigenstates of the semiconductor Hamiltonian, thus forming a complete orthogonal set for one-pair states. It can however be of interest to extend this new many-body theory to more complicated composite bosons, \emph{i. e.}, ``cobosons'', which are not necessarily the one-pair eigenstates of the system Hamiltonian, nor even orthogonal. The purpose of this paper is to derive the ``Pauli scatterings'' and the ``interaction scatterings'' of these cobosons formally, \emph{i. e.}, just in terms of their wave functions and the interaction potentials which exist between the fermions from which they are constructed. We also explain how to derive many-body effects in this very general system of composite bosons.

cond-mat.mes-hall↗