arXiv subjects

F. Gunsing

Publications and source records attributed to F. Gunsing.

At least 37 records · Page 2Linked to original sources

arXiv2021

Calibration of nuclear recoils at the 100 eV scale using neutron capture

The development of low-threshold detectors for the study of coherent elastic neutrino-nucleus scattering and for the search for light dark matter necessitates methods of low-energy calibration. We suggest this can be provided by the nuclear recoils resulting from the $γ$ emission following thermal neutron capture. In particular, several MeV-scale single-$γ$ transitions induce well-defined nuclear recoil peaks in the 100 eV range. Using the FIFRELIN code, complete schemes of $γ$-cascades for various isotopes can be predicted with high accuracy to determine the continuous background of nuclear recoils below the calibration peaks. We present a comprehensive experimental concept for the calibration of CaWO$_4$ and Ge cryogenic detectors at a research reactor. For CaWO$_4$ the simulations show that two nuclear recoil peaks at 112.5 eV and 160.3 eV should be visible above background simply in the spectrum of the cryogenic detector. Then we discuss how the additional tagging for the associated $γ$ increases the sensitivity of the method and extends its application to a wider energy range and to Ge cryogenic detectors.

physics.ins-det↗

arXiv2020

Imaging neutron capture cross sections: i-TED proof-of-concept and future prospects based on Machine-Learning techniques

i-TED is an innovative detection system which exploits Compton imaging techniques to achieve a superior signal-to-background ratio in ($n,γ$) cross-section measurements using time-of-flight technique. This work presents the first experimental validation of the i-TED apparatus for high-resolution time-of-flight experiments and demonstrates for the first time the concept proposed for background rejection. To this aim both $^{197}$Au($n,γ$) and $^{56}$Fe($n, γ$) reactions were measured at CERN n\_TOF using an i-TED demonstrator based on only three position-sensitive detectors. Two \cds detectors were also used to benchmark the performance of i-TED. The i-TED prototype built for this study shows a factor of $\sim$3 higher detection sensitivity than state-of-the-art \cds detectors in the $\sim$10~keV neutron energy range of astrophysical interest. This paper explores also the perspectives of further enhancement in performance attainable with the final i-TED array consisting of twenty position-sensitive detectors and new analysis methodologies based on Machine-Learning techniques.

physics.ins-det↗

arXiv2019

Review and new concepts for neutron-capture measurements of astrophysical interest

The idea of slow-neutron capture nucleosynthesis formulated in 1957 triggered a tremendous experimental effort in different laboratories worldwide to measure the relevant nuclear physics input quantities, namely ($n,γ$) cross sections over the stellar temperature range (from few eV up to several hundred keV) for most of the isotopes involved from Fe up to Bi. A brief historical review focused on total energy detectors will be presented to illustrate how, advances in instrumentation have led, over the years, to the assessment and discovery of many new aspects of $s$-process nucleosynthesis and to the progressive refinement of theoretical models of stellar evolution. A summary will be presented on current efforts to develop new detection concepts, such as the Total-Energy Detector with $γ$-ray imaging capability (i-TED). The latter is based on the simultaneous combination of Compton imaging with neutron time-of-flight (TOF) techniques, in order to achieve a superior level of sensitivity and selectivity in the measurement of stellar neutron capture rates.

physics.ins-det↗

arXiv2019

Unrecognized Sources of Uncertainties (USU) in Experimental Nuclear Data

Evaluated nuclear data uncertainties are often perceived as unrealistic, most often because they are thought to be too small. The impact of this issue in applied nuclear science has been discussed widely in recent years. Commonly suggested causes are: poor estimates of specific error components, neglect of uncertainty correlations, and overlooked known error sources. However, instances have been reported where very careful, objective assessments of all known error sources have been made with realistic error magnitudes and correlations provided, yet the resulting evaluated uncertainties still appear to be inconsistent with observed scatter of predicted mean values. These discrepancies might be attributed to significant unrecognized sources of uncertainty (USU) that limit the accuracy to which these physical quantities can be determined. The objective of our work has been to develop procedures for revealing and including USU estimates in nuclear data evaluations involving experimental input data. We conclude that the presence of USU may be revealed, and estimates of magnitudes made, through quantitative analyses. This paper identifies several specific clues that can be explored by evaluators in identifying the existence of USU. It then describes numerical procedures to generate quantitative estimates of USU magnitudes. Key requirements for these procedures to be viable are that sufficient numbers of data points be available, for statistical reasons, and that additional supporting information about the measurements be provided by the experimenters. Realistic examples are described to illustrate these procedures and demonstrate their outcomes as well as limitations. Our work strongly supports the view that USU is an important issue in nuclear data evaluation, with significant consequences for applications, and that this topic warrants further investigation by the nuclear science community.

physics.data-an↗

arXiv2019

Measurement of the 235U(n,f) cross section relative to the 6Li(n,t) and 10B(n,alpha) standards from thermal to 170 keV neutron energy range at n_TOF

The 235U(n,f) cross section was measured in a wide energy range at n_TOF relative to 6Li(n,t) and 10B(n,alpha), with high resolution and in a wide energy range, with a setup based on a stack of six samples and six silicon detectors placed in the neutron beam. This allowed us to make a direct comparison of the reaction yields under the same experimental conditions, and taking into account the forward/backward emission asymmetry. A hint of an anomaly in the 10÷30 keV neutron energy range had been previously observed in other experiments, indicating a cross section systematically lower by several percent relative to major evaluations. The present results indicate that the evaluated cross section in the 9÷18 keV neutron energy range is indeed overestimated, both in the recent updates of ENDF/B-VIII.0 and of the IAEA reference data. Furthermore, these new high-resolution data confirm the existence of resonance-like structures in the keV neutron energy region. The new, high accuracy results here reported may lead to a reduction of the uncertainty in the 1÷100 keV neutron energy region. Finally, the present data provide additional confidence on the recently re-evaluated cross section integral between 7.8 and 11 eV.

nucl-ex↗

arXiv2018

The $^{7}$Be($\boldsymbol{n,p}$)$^{7}$Li reaction and the Cosmological Lithium Problem: measurement of the cross section in a wide energy range at n_TOF (CERN)

We report on the measurement of the $^{7}$Be($n, p$)$^{7}$Li cross section from thermal to approximately 325 keV neutron energy, performed in the high-flux experimental area (EAR2) of the n\_TOF facility at CERN. This reaction plays a key role in the lithium yield of the Big Bang Nucleosynthesis (BBN) for standard cosmology. The only two previous time-of-flight measurements performed on this reaction did not cover the energy window of interest for BBN, and showed a large discrepancy between each other. The measurement was performed with a Si-telescope, and a high-purity sample produced by implantation of a $^{7}$Be ion beam at the ISOLDE facility at CERN. While a significantly higher cross section is found at low-energy, relative to current evaluations, in the region of BBN interest the present results are consistent with the values inferred from the time-reversal $^{7}$Li($p, n$)$^{7}$Be reaction, thus yielding only a relatively minor improvement on the so-called Cosmological Lithium Problem (CLiP). The relevance of these results on the near-threshold neutron production in the p+$^{7}$Li reaction is also discussed.

nucl-ex↗

arXiv2018

Cross section measurements of $^{155,157}$Gd(n,$γ$) induced by thermal and epithermal neutrons

Neutron capture measurements on $^{155}$Gd and $^{157}$Gd were performed using the time-of-flight technique at the n\_TOF facility at CERN. Four samples in form of self-sustaining metallic discs isotopically enriched in $^{155}$Gd and $^{157}$Gd were used. The measurements were carried out at the experimental area (EAR1) at 185 m from the neutron source, with an array of 4 C$_6$D$_6$ liquid scintillation detectors. The capture cross sections of $^{155}$Gd and $^{157}$Gd at neutron kinetic energy of 0.0253 eV have been estimated to be 62.2(2.2) kb and 239.8(9.3) kb, respectively, thus up to 6\% different relative to the ones reported in the nuclear data libraries. A resonance shape analysis has been performed in the resolved resonance region up to 180 eV and 300 eV, respectively, in average resonance parameters have been found in good agreement with evaluations. Above these energies the observed resonance-like structures in the cross section have been tentatively characterised in terms of resonance energy and area up to 1 keV.

nucl-ex↗

arXiv2017

Experimental setup and procedure for the measurement of the 7Be(n,p)7Li reaction at n_TOF

Following the completion of the second neutron beam line and the related experimental area (EAR2) at the n_TOF spallation neutron source at CERN, several experiments were planned and performed. The high instantaneous neutron flux available in EAR2 allows to investigate neutron indiced reactions with charged particles in the exit channel even employing targets made out of small amounts of short-lived radioactive isotopes. After the successful measurement of the 7Be(n,α)α cross section, the 7Be(n,p)7Li reaction was studied in order to provide still missing cross section data of relevance for Big Bang Nucleosynthesis (BBN), in an attempt to find a solution to the cosmological Lithium abundance problem. This paper describes the experimental setup employed in such a measurement and its characterization.

physics.ins-det↗

arXiv2016

Neutron capture cross section measurement of 238U at the n TOF CERN facility with C6D6 scintillation detectors in the energy region from 1 eV to 700 keV

The aim of this work is to provide a precise and accurate measurement of the 238U(n,g) reaction cross section in the energy region from 1 eV to 700 keV. This reaction is of fundamental importance for the design calculations of nuclear reactors, governing the behaviour of the reactor core. In particular, fast reactors, which are experiencing a growing interest for their ability to burn radioactive waste, operate in the high energy region of the neutron spectrum. In this energy region most recent evaluations disagree due to inconsistencies in the existing measurements of up to 15%. In addition, the assessment of nuclear data uncertainty performed for innovative reactor systems shows that the uncertainty in the radiative capture cross-section of 238U should be further reduced to 1-3% in the energy region from 20 eV to 25 keV. To this purpose, addressed by the Nuclear Energy Agency as a priority nuclear data need, complementary experiments, one at the GELINA and two at the n_TOF facility, were proposed and carried out within the 7th Framework Project ANDES of the European Commission. The results of one of these 238U(n,g) measurements performed at the n_TOF CERN facility are presented in this work. The gamma-ray cascade following the radiative neutron capture has been detected exploiting a setup of two C6D6 liquid scintillators. Resonance parameters obtained from this work are on average in excellent agreement with the ones reported in evaluated libraries. In the unresolved resonance region, this work yields a cross section in agreement with evaluated libraries up to 80 keV, while for higher energies our results are significantly higher.

nucl-ex↗

arXiv2016

Study of the 238U(d,p) surrogate reaction via the simultaneous measurement of gamma-decay and fission probabilities

We investigated the 238U(d,p) reaction as a surrogate for the n + 238U reaction. For this purpose we measured for the first time the gamma-decay and fission probabilities of 239U* simultaneously and compared them to the corresponding neutron-induced data. We present the details of the procedure to infer the decay probabilities, as well as a thorough uncertainty analysis, including parameter correlations. Calculations based on the continuum-discretized coupled-channels and distorted-wave Born approximations were used to correct our data from detected protons originating from elastic and inelastic deuteron breakup. In the region where the fission and gamma-decay probabilities compete, the corrected fission probability is in agreement with neutron-induced data, whereas the gamma-decay probability is much higher than the neutron-induced data. The performed statistical-model calculations are not able to explain these results.

nucl-ex↗

arXiv2016

An improved method for estimating the neutron background in measurements of neutron capture reactions

The relation between the neutron background in neutron capture measurements and the neutron sensitivity related to the experimental setup is examined. It is pointed out that a proper estimate of the neutron background may only be obtained by means of dedicated simulations taking into account the full framework of the neutron-induced reactions and their complete temporal evolution. No other presently available method seems to provide reliable results, in particular under the capture resonances. An improved neutron background estimation technique is proposed, the main improvement regarding the treatment of the neutron sensitivity, taking into account the temporal evolution of the neutron-induced reactions. The technique is complemented by an advanced data analysis procedure based on relativistic kinematics of neutron scattering. The analysis procedure allows for the calculation of the neutron background in capture measurements, without requiring the time-consuming simulations to be adapted to each particular sample. A suggestion is made on how to improve the neutron background estimates if neutron background simulations are not available.

nucl-ex↗

arXiv2016

Integral measurement of the $^{12}$C(n,p)$^{12}$B reaction up to 10 GeV

The integral measurement of the $^{12}$C(n,p)$^{12}$B reaction was performed at the neutron time of flight facility n_TOF at CERN. The total number of $^{12}$B nuclei produced per neutron pulse of the n_TOF beam was determined using the activation technique in combination with a time of flight technique. The cross section is integrated over the n_TOF neutron energy spectrum from reaction threshold at 13.6 MeV to 10 GeV. Having been measured up to 1 GeV on basis of the $^{235}$U(n,f) reaction, the neutron energy spectrum above 200 MeV has been reevaluated due to the recent extension of the cross section reference for this particular reaction, which is otherwise considered a standard up to 200 MeV. The results from the dedicated GEANT4 simulations have been used to evaluate the neutron flux from 1 GeV up to 10 GeV. The experimental results related to the $^{12}$C(n,p)$^{12}$B reaction are compared with the evaluated cross sections from major libraries and with the predictions of different GEANT4 models, which mostly underestimate the $^{12}$B production. On the contrary, a good reproduction of the integral cross section derived from measurements is obtained with TALYS-1.6 calculations, with optimized parameters.

nucl-ex↗

arXiv2016

Experimental setup and procedure for the measurement of the 7Be(n,α)α reaction at n_TOF

The newly built second experimental area EAR2 of the n_TOF spallation neutron source at CERN allows to perform (n, charged particles) experiments on short-lived highly radioactive targets. This paper describes a detection apparatus and the experimental procedure for the determination of the cross-section of the 7Be(n,α) reaction, which represents one of the focal points toward the solution of the cosmological Lithium abundance problem, and whose only measurement, at thermal energy, dates back to 1963. The apparently unsurmountable experimental difficulties stemming from the huge 7Be γ-activity, along with the lack of a suitable neutron beam facility, had so far prevented further measurements. The detection system is subject to considerable radiation damage, but is capable of disentangling the rare reaction signals from the very high background. This newly developed setup could likely be useful also to study other challenging reactions requiring the detectors to be installed directly in the neutron beam.

physics.ins-det↗

arXiv2016

Pulse processing routines for neutron time-of-flight data

A pulse shape analysis framework is described, which was developed for n_TOF-Phase3, the third phase in the operation of the n_TOF facility at CERN. The most notable feature of this new framework is the adoption of generic pulse shape analysis routines, characterized by a minimal number of explicit assumptions about the nature of pulses. The aim of these routines is to be applicable to a wide variety of detectors, thus facilitating the introduction of the new detectors or types of detectors into the analysis framework. The operational details of the routines are suited to the specific requirements of particular detectors by adjusting the set of external input parameters. Pulse recognition, baseline calculation and the pulse shape fitting procedure are described. Special emphasis is put on their computational efficiency, since the most basic implementations of these conceptually simple methods are often computationally inefficient.

physics.ins-det↗

arXiv2015

Experimental level densities of atomic nuclei

It is almost 80 years since Hans Bethe described the level density as a non-interacting gas of protons and neutrons. In all these years, experimental data were interpreted within this picture of a fermionic gas. However, the renewed interest of measuring level density using various techniques calls for a revision of this description. In particular, the wealth of nuclear level densities measured with the Oslo method favors the constant-temperature level density over the Fermi-gas picture. From the basis of experimental data, we demonstrate that nuclei exhibit a constant-temperature level density behavior for all mass regions and at least up to the neutron threshold.

nucl-ex↗

arXiv2014

Measurement and analysis of the Am-243 neutron capture cross section at the n_TOF facility at CERN

Background:The design of new nuclear reactors and transmutation devices requires to reduce the present neutron cross section uncertainties of minor actinides. Purpose: Reduce the $^{243}$Am(n,$γ$) cross section uncertainty. Method: The $^{243}$Am(n,$γ$) cross section has been measured at the n_TOF facility at CERN with a BaF$_{2}$ Total Absorption Calorimeter, in the energy range between 0.7 eV and 2.5 keV. Results: The $^{243}$Am(n,$γ$) cross section has been successfully measured in the mentioned energy range. The resolved resonance region has been extended from 250 eV up to 400 eV. In the unresolved resonance region our results are compatible with one of the two incompatible capture data sets available below 2.5 keV. The data available in EXFOR and in the literature has been used to perform a simple analysis above 2.5 keV. Conclusions: The results of this measurement contribute to reduce the $^{243}$Am(n,$γ$) cross section uncertainty and suggest that this cross section is underestimated up to 25% in the neutron energy range between 50 eV and a few keV in the present evaluated data libraries.

nucl-ex↗

arXiv2014

High accuracy determination of the $^{238}$U/$^{235}$U fission cross section ratio up to $\sim$1 GeV at n_TOF (CERN)

The $^{238}$U to $^{235}$U fission cross section ratio has been determined at n_TOF up to $\sim$1 GeV, with two different detection systems, in different geometrical configurations. A total of four datasets have been collected and compared. They are all consistent to each other within the relative systematic uncertainty of 3-4%. The data collected at n_TOF have been suitably combined to yield a unique fission cross section ratio as a function of the neutron energy. The result confirms current evaluations up to 200 MeV. A good agreement is also observed with theoretical calculations based on the INCL++/Gemini++ combination up to the highest measured energy. The n_TOF results may help solving a long-standing discrepancy between the two most important experimental dataset available so far above 20 MeV, while extending the neutron energy range for the first time up to $\sim$1 GeV.

nucl-ex↗

arXiv2014

Measurement of the $^{12}$C($n,p$)$^{12}$B cross section at n_TOF (CERN) by in-beam activation analysis

The integral cross section of the $^{12}$C($n,p$)$^{12}$B reaction has been determined for the first time in the neutron energy range from threshold to several GeV at the n_TOF facility at CERN. The measurement relies on the activation technique, with the $β$-decay of $^{12}$B measured over a period of four half-lives within the same neutron bunch in which the reaction occurs. The results indicate that model predictions, used in a variety of applications, are mostly inadequate. The value of the integral cross section reported here can be used as a benchmark for verifying or tuning model calculations.

nucl-ex↗