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F. Husstedt

Publications and source records attributed to F. Husstedt.

4 recordsLinked to original sources

Superconductivity in epitaxial PtSb(0001) thin films

We report superconductivity in epitaxial PtSb(0001) thin films grown on SrF2(111). Electrical transport measurements reveal a superconducting transition at $T_{\mathrm c}=1.72$ K. The field-induced broadening of the transition and the presence of finite upper critical fields are consistent with type-II superconductivity. We determine the resistively defined upper critical fields for magnetic fields applied perpendicular and parallel to the film plane and parameterize their temperature dependence using an anisotropic Ginzburg-Landau approach. For the thickest film ($d=50$ nm), this yields coherence lengths of $\xi_{ab}\approx 55$ nm and $\xi_c\approx 14$ nm. Current-voltage characteristics show sizeable critical currents, with a critical current density reaching $J_{\mathrm c}\approx 6e4$ A/cm$^2$ at 0.5 K. These results establish epitaxial PtSb as a superconducting thin-film platform compatible with lattice-matched heterostructures in the NiAs-type materials family.

cond-mat.supr-con

Acoustic signatures of the field-induced electronic-topological transitions in YbNi$_4$P$_2$

We investigated the magnetoelastic properties of an YbNi$_4$P$_2$ single crystal at low temperatures under magnetic fields directed along the crystallographic [001] axis. We report a series of strong anomalies in the sound velocity, which is consistent with the cascade of electronic-topological transitions reported previously for this compound. In particular, we identify the vanishing of a small orbit on the Fermi surface, associated with a quantum-oscillation frequency of 34 T. Furthermore, the different transitions are better resolved with acoustic modes of particular symmetry. Using a microscopic model adapted to the strongly correlated electronic structure of YbNi$_4$P$_2$, we describe our results by inspecting realistic electron-phonon couplings in reciprocal space for each acoustic mode. This shows how the $k$ selectivity of ultrasound experiments allows to investigate Fermi-surface reconstructions in strongly correlated electronic systems.

cond-mat.str-el

$\mathbb{Z}_2$ Vortex Crystal Candidate in the Triangular $S=1/2$ Quantum Antiferromagnet

The prospect of merging the paradigms of geometric frustration on a triangular lattice and bond anisotropies in the strong spin-orbit coupling limit holds tremendous promise in the ongoing hunt for exotic quantum materials. Here we identify a new candidate system to realize such physics, the organic quantum antiferromagnet (CD$_3$ND$_3$)$_2$NaRuCl$_6$. We report a combination of thermodynamic, magneto-elastic and neutron scattering experiments on single-crystals to determine the phase diagram in axial magnetic fields $\mathbf{H \parallel c}$ and propose a minimal model Hamiltonian. (CD$_3$ND$_3$)$_2$NaRuCl$_6$ displays an ideal triangular arrangement of Ru$^{3+}$ ions adopting the spin-orbital entangled $j_{\rm eff} = 1/2$ state. It hosts residual magnetic order below $T_{\rm N} = 0.23$ K and a highly unusual $H-T$ phase diagram including three different incommensurate states. Spin-waves in the high-field polarized regime are well described by a Heisenberg-like triangular lattice Hamiltonian with a potential sub-leading bond dependent anisotropy term $J_{\pm\pm}$. We discuss possible candidate magnetic structures in the various observed phases and propose two mechanisms that could explain the field-dependent incommensurability, requiring either a small ferromagnetic Kitaev term or a tiny magneto-elastic $J-J'$ isosceles distortion driven by pseudospin-lattice coupling. We argue that the multi-$\mathbf{q}$ ground state in zero magnetic field is a prime candidate for hosting the $\mathbb{Z}_2$ vortex crystal proposed on the triangular Heisenberg-Kitaev model. (CD$_3$ND$_3$)$_2$NaRuCl$_6$ is the first member in an extended family of quantum triangular lattice magnets, providing a new playground to study the interplay of geometric frustration and spin-orbit effects.

cond-mat.str-el

Excitation Spectrum and Spin Hamiltonian of the Frustrated Quantum Ising Magnet Pr$_3$BWO$_9$

We present a thorough experimental investigation on single crystals of the rare-earth based frustrated quantum antiferromagnet Pr$_3$BWO$_9$, a purported spin-liquid candidate on the breathing kagome lattice. This material possesses a disordered ground state with an unusual excitation spectrum involving a coexistence of sharp spin-waves and broad continuum excitations. Nevertheless, we show through a combination of thermodynamic, magnetometric and spectroscopic probes with detailed theoretical modeling that it should be understood in a completely different framework. The crystal field splits the lowest quasi-doublet states into two singlets moderately coupled through frustrated superexchange, resulting in a simple effective Hamiltonian of an Ising model in a transverse magnetic field. While our neutron spectroscopy data do point to significant correlations within the kagome planes, the dominant interactions are out-of-plane, forming frustrated triangular spin-tubes through two competing ferro-antiferromagnetic bonds. The resulting ground state is a simple quantum paramagnet, but with significant modifications to both thermodynamic and dynamic properties due to small perturbations to the transverse field Ising model in the form of hyperfine enhanced nuclear moments and weak structural disorder.

cond-mat.str-el