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F. J. García de Abajo

Publications and source records attributed to F. J. García de Abajo.

13 recordsLinked to original sources

Unity-order coupling between free electrons and multiphoton waveguided Fock states

Electron beams enable highly localized near-field excitation of waveguided optical modes, yet their coupling is typically limited by short interaction times along straight-line trajectories with fixed impact parameters. Here, we theoretically demonstrate that electrostatic steering overcomes this limitation by introducing a tunable turning point in grazing electron trajectories, thus controlling the minimum electron--waveguide separation and producing strong coupling to waveguided modes. Specifically, we consider a biased rectangular silicon waveguide, where a repulsive static field deflects a grazing electron. In this configuration, the electron turning point governs both the coupling strength and the modal selectivity, which can be dynamically tuned through the electron incidence angle and the applied bias. In addition, the aloof electron--waveguide interaction suppresses lossy high-energy channels (e.g., above the silicon band gap) while preserving substantial excitation of the targeted waveguided modes. Using a practical biasing configuration and 100~keV electrons, we predict an average yield exceeding ten photons per electron, with voltage-tunable control of the interaction. Our results establish electrostatic steering as a practical route for engineering and enhancing free-electron coupling to waveguided photonic modes.

cond-mat.mes-hall↗

Ultrafast Transverse Modulation of Free Electrons by Interaction with Shaped Optical Fields

Spatio-temporal shaping of electron beams is a bold frontier in electron microscopy, enabling new routes toward spatial-resolution enhancement, selective probing, low-dose imaging and faster data acquisition. Over the last decade, shaping methods evolved from passive phase plates to low-speed electrostatic and magnetostatic displays. Recently, higher shaping speed and flexibility have become feasible by the advent of ultrafast electron microscopy, embodying a swift change of paradigm that relies on using light to control free electrons. Here, we experimentally demonstrate that arbitrary transverse modulation of electron beams is possible without the need for designing and fabricating complicated electron-optics elements or material nanostructures, but rather resorting to shaping light beams reflected from a planar thin film. We demonstrate arbitrary transverse modulation of electron wavepackets via inelastic interaction with a shaped ultrafast light field controlled by an external spatial light modulator (SLM). We illustrate this method by generating Hermite-Gaussian (HG) electron beams with HG10 and HG01 symmetry and discuss their possible use in enhancing the imaging contrast of microscopic features. Relative to current schemes, our approach adopting an external SLM dramatically widens the range of patterns that can be imprinted on the electron wave function and makes electron shaping a much easier task to perform.

physics.optics↗

Ultrafast Generation and Control of an Electron Vortex Beam via Chiral Plasmonic Near Fields

Vortex-carrying matter waves, such as chiral electron beams, are of significant interest in both applied and fundamental science. Continuous wave electron vortex beams are commonly prepared via passive phase masks imprinting a transverse phase modulation on the electron's wave function. Here, we show that femtosecond chiral plasmonic near fields enable the generation and dynamic control on the ultrafast timescale of an electron vortex beam. The vortex structure of the resulting electron wavepacket is probed in both real and reciprocal space using ultrafast transmission electron microscopy. This method offers a high degree of scalability to small length scales and a highly efficient manipulation of the electron vorticity with attosecond precision. Besides the direct implications in the investigation of nanoscale ultrafast processes in which chirality plays a major role, we further discuss the perspectives of using this technique to shape the wave function of charged composite particles, such as protons, and how it can be used to probe their internal structure.

quant-ph↗

Ultrafast holography enabled by quantum interference of ultrashort electrons

Holography relies on the interference between a known reference and a signal of interest to reconstruct both the amplitude and phase of that signal. Commonly performed with photons and electrons, it finds numerous applications in imaging, cryptography and arts. With electrons, the extension of holography to the ultrafast time domain remains a challenge, although it would yield the highest possible combined spatio-temporal resolution. Here, we show that holograms of local electromagnetic fields can be obtained with combined attosecond/nanometer resolution in an ultrafast transmission electron microscope (UEM). Unlike conventional holography, where the signal and the reference are spatially separated and then recombined to interfere, in our method we use electromagnetic fields to split an electron wave function in a quantum coherent superposition of different energy states. In the image plane, spatial modulation of the electron-energy distribution reflects the phase relation between reference and signal fields, which we map via energy-filtered UEM. Beyond imaging applications, this approach allows implementing optically-controlled and spatially-resolved quantum measurements in parallel, providing an efficient and versatile tool for the exploration of electron quantum optics.

cond-mat.mes-hall↗

meV resolution in laser-assisted energy-filtered transmission electron microscopy

The electronic, optical, and magnetic properties of quantum solids are determined by their low-energy (< 100 meV) many-body excitations. Dynamical characterization and manipulation of such excitations relies on tools that combine nm-spatial, fs-temporal, and meV-spectral resolution. Currently, phonons and collective plasmon resonances can be imaged in nanostructures with sub-nm and 10s meV space/energy resolution using state-of-the-art energy-filtered transmission electron microscopy (TEM), but only under static conditions, while fs-resolved measurements are common but lack spatial or energy resolution. Here, we demonstrate a new method of spectrally resolved photon-induced near-field electron microscopy (SRPINEM) that allows us to obtain nm-fs-resolved maps of nanoparticle plasmons with an energy resolution determined by the laser linewidth (20 meV in this work), and not limited by electron beam and spectrometer energy spreading. This technique can be extended to any optically-accessible low-energy mode, thus pushing TEM to a previously inaccessible spectral domain with an unprecedented combination of space, energy and temporal resolution.

cond-mat.mes-hall↗

Electrical Control of Optical Emitter Relaxation Pathways enabled by Graphene

Controlling the energy flow processes and the associated energy relaxation rates of a light emitter is of high fundamental interest, and has many applications in the fields of quantum optics, photovoltaics, photodetection, biosensing and light emission. While advanced dielectric and metallic systems have been developed to tailor the interaction between an emitter and its environment, active control of the energy flow has remained challenging. Here, we demonstrate in-situ electrical control of the relaxation pathways of excited erbium ions, which emit light at the technologically relevant telecommunication wavelength of 1.5 $μ$m. By placing the erbium at a few nanometres distance from graphene, we modify the relaxation rate by more than a factor of three, and control whether the emitter decays into either electron-hole pairs, emitted photons or graphene near-infrared plasmons, confined to $<$15 nm to the sheet. These capabilities to dictate optical energy transfer processes through electrical control of the local density of optical states constitute a new paradigm for active (quantum) photonics.

cond-mat.mes-hall↗

Single-photon nonlinear optics with graphene plasmons

We show that it is possible to realize significant nonlinear optical interactions at the few photon level in graphene nanostructures. Our approach takes advantage of the electric field enhancement associated with the strong confinement of graphene plasmons and the large intrinsic nonlinearity of graphene. Such a system could provide a powerful platform for quantum nonlinear optical control of light. As an example, we consider an integrated optical device that exploits this large nonlinearity to realize a single photon switch.

cond-mat.mes-hall↗

Extraordinary absorption of sound in porous lamella-crystals

We present the design of a structured material supporting complete absorption of sound with a broadband response and functional for any direction of incident radiation. The structure which is fabricated out of porous lamellas is arranged into a low-density crystal and backed by a reflecting support. Experimental measurements show that strong all-angle sound absorption with almost zero reflectance takes place for a frequency range exceeding two octaves. We demonstrate that lowering the crystal filling fraction increases the wave interaction time and is responsible for the enhancement of intrinsic material dissipation, making the system more absorptive with less material.

cond-mat.mtrl-sci↗

Vacuum friction in rotating particles

We study the frictional torque acting on particles rotating in empty space. At zero temperature, vacuum friction transforms mechanical energy into light emission and produces particle heating. However, particle cooling relative to the environment occurs at finite temperatures and low rotation velocities. Radiation emission is boosted and its spectrum significantly departed from a hot-body emission profile as the velocity increases. Stopping times ranging from hours to billions of years are predicted for materials, particle sizes, and temperatures accessible to experiment. Implications for the behavior of cosmic dust are discussed.

quant-ph↗

Robust plasmon waveguides in strongly-interacting nanowire arrays

Arrays of parallel metallic nanowires are shown to provide a tunable, robust, and versatile platform for plasmon interconnects, including high-curvature turns with minimum signal loss. The proposed guiding mechanism relies on gap plasmons existing in the region between adjacent nanowires of dimers and multi-wire arrays. We focus on square and circular silver nanowires in silica, for which excellent agreement between both boundary element method and multiple multipolar expansion calculations is obtained. Our work provides the tools for designing plasmon-based interconnects and achieving high degree of integration with minimum cross talk between adjacent plasmon guides.

cond-mat.other↗

Optically tunable surfaces with trapped particles in microcavities

We introduce optically tunable surfaces based upon metallic gold nanoparticles trapped in open, water-filled gold cavities. The optical properties of the surfaces change dramatically with the presence and location of the particles inside the cavities. The precise position of the particles is shown to be controllable through optical forces exerted by external illumination, thus leading to all-optical tunability, whereby the optical response of the surfaces is tuned through externally applied light. We discuss the performance of the cavity-particle complex in detail and provide theoretical support for its application as a novel concept of large-scale optically tunable system.

cond-mat.mtrl-sci↗

Surface plasmon polariton modes in a single-crystal Au nanoresonator fabricated using focused-ion-beam milling

We use focused-ion-beam milling of a single-crystal Au surface to fabricate a 590-nm-long linear ridge that acts as a surface plasmon nanoresonator. Cathodoluminescence imaging spectroscopy is then used to excite and image surface plasmons on the ridge. Principal component analysis reveals distinct plasmonic modes, which proves confinement of surface-plasmon oscillations to the ridge. Boundary-element-method calculations confirm that a linear ridge is able to support highly-localized surface-plasmon modes (mode diameter < 100 nm). The results demonstrate that focused-ion-beam milling can be used in rapid prototyping of nanoscale single-crystal plasmonic components.

physics.optics↗

The role of electromagnetic trapped modes in extraordinary transmission in nanostructured materials

We assert that the physics underlying the extraordinary light transmission (reflection) in nanostructured materials can be understood from rather general principles based on the formal scattering theory developed in quantum mechanics. The Maxwell equations in passive (dispersive and absorptive) linear media are written in the form of the Schrödinger equation to which the quantum mechanical resonant scattering theory (the Lippmann-Schwinger formalism) is applied. It is demonstrated that the existence of long-lived quasistationary eigenstates of the effective Hamiltonian for the Maxwell theory naturally explains the extraordinary transmission properties observed in various nanostructured materials. Such states correspond to quasistationary electromagnetic modes trapped in the scattering structure. Our general approach is also illustrated with an example of the zero-order transmission of the TE-polarized light through a metal-dielectric grating structure. Here a direct on-the-grid solution of the time-dependent Maxwell equations demonstrates the significance of resonances (or trapped modes) for extraordinary light transmissio

physics.comp-ph↗