arXiv subjects

F. J. Garcia-Vidal

Publications and source records attributed to F. J. Garcia-Vidal.

At least 19 recordsLinked to original sources

arXiv2024

Fabry-Perot Resonance of Bilayer Metasurfaces

In this study, we constructed a Fabry-Perot cavity with nanostructured, thin resonant metasurfaces as meta-mirrors. We developed a temporal coupled-mode theory and provided an accurate generalization of Fabry-Perot resonance and analytically derived the transmission characteristics. The presence of metasurface mirrors introduces a substantial group delay, causing the field concentration to shift from the center of the Fabry-Perot cavity toward the metasurface region. This shift is accompanied by a significant increase in the quality factor of the FP resonance. In the frequency space, there are singular points where the quality factor increases exponentially. These singular points in meta-mirror cavities exist even when the cavity separations are smaller than the cavity length of the fundamental mode in the standard cavities. We discover two characteristic cavity separations, Lc and LQ, that differentiate the resonance in terms of lineshapes and the dominance of the quality factor. When L < Lc, there is strong evanescent interaction between the two metasurface mirrors, and the coupling of this interaction with the traditional resonance produces sharp Fano-shaped transmission peaks. When Lc < L< LQ, we have induced transparency peaks with lorentzian line-shapes and length-independent quality factors. This length-independence enables, the meta-mirror cavity to outperform the traditional cavities by achiveing high quality factor despite a shorter cavity length.

physics.optics↗

arXiv2024

Active Control of Polariton-Enabled Long-Range Energy Transfer

Optical control is achieved on the excited state energy transfer between spatially separated donor and acceptor molecules, both coupled to the same optical mode of a cavity. The energy transfer occurs through the formed hybrid polaritons and can be switched on and off by means of ultraviolet and visible light. The control mechanism relies on a photochromic component used as donor, whose absorption and emission properties can be varied reversibly through light irradiation, whereas in-cavity hybridization with acceptors through polariton states enables a 6-fold enhancement of acceptor/donor contribution to the emission intensity with respect to a reference multilayer. These results pave the way for synthesizing effective gating systems for the transport of energy by light, relevant for light-harvesting and light-emitting devices, and for photovoltaic cells.

physics.optics↗

arXiv2023

Spontaneous symmetry breaking in diffraction

The connection between symmetries and conservation laws is a cornerstone of physics. It underlies Bloch's theorem which explains wave phenomena in all linear periodic systems. Here we demonstrate that, in a nonlinear grating with memory, diffracted waves can spontaneously acquire momentum parallel to the lattice vector in quantities unconstrained by the grating period. In this breakdown of Bloch's theorem, which we also evidence in solutions to nonlinear Maxwell's equations, wave amplitudes no longer respect the discrete translation symmetry of the grating. Our findings reveal a rich phenomenology for waves in nonlinear periodic systems, and point to numerous opportunities for nonlinear lattices with broken symmetry in the context of imaging, sensing, and information processing in general.

physics.optics↗

arXiv2019

Single-atom control of the optoelectronic response in sub-nanometric cavities

By means of ab-initio time dependent density functional theory calculations carried out on an prototypical hybrid plasmonic device (two metallic nanoparticles bridged by a one-atom junction), we demonstrate the strong interplay between photoinduced excitation of localized surface plasmons and electron transport through the single atom. Such an interplay is remarkably sensitive to the atomic orbitals of the junction. Therefore, we show the possibility of a twofold tuning (plasmonic response and photoinduced current across the juntion) just by changing a single atom in the device.

physics.optics↗

arXiv2016

Non-reciprocal few-photon devices based on chiral waveguide-emitter couplings

We demonstrate the possibility of designing efficient, non reciprocal few-photon devices by exploiting the chiral coupling between two waveguide modes and a single quantum emitter. We show how this system can induce non-reciprocal photon transport at the single-photon level and act as an optical diode. Afterwards, we also show how the same system shows a transistor-like behaviour for a two-photon input. The efficiency in both cases is shown to be large for feasible experimental implementations. Our results illustrate the potential of chiral waveguide-emitter couplings for applications in quantum circuitry.

quant-ph↗

arXiv2016

Uncoupled dark states can inherit polaritonic properties

When a collection of quantum emitters interacts with an electromagnetic field, the whole system can enter into the collective strong coupling regime in which hybrid light-matter states, i.e., polaritons can be created. Only a small portion of excitations in the emitters are coupled to the light field, and there are many dark states that, in principle, retain their pure excitonic nature. Here we theoretically demonstrate that these dark states can have a delocalized character, which is inherent to polaritons, despite the fact that they do not have a photonic component. This unexpected behavior only appears when the electromagnetic field displays a discrete spectrum. In this case, when the main loss mechanism in the hybrid system stems from the radiative losses of the light field, dark states are even more efficient than polaritons in transferring excitations across the structure.

cond-mat.mes-hall↗

arXiv2015

Nonequilibrium plasmon emission drives ultrafast carrier relaxation dynamics in photoexcited graphene

The fast decay of carrier inversion in photoexcited graphene has been attributed to optical phonon emission and Auger recombination. Plasmon emission provides another pathway that, as we show here, drives the carrier relaxation dynamics on ultrafast timescales. In studying the nonequilibrium relaxation dynamics we find that plasmon emission effectively converts inversion into hot carriers, whose energy is then extracted by optical phonon emission. This mechanism not only explains the observed fs-lifetime of inversion but also offers the prospect for atomically thin ultrafast plasmon emitters.

cond-mat.mes-hall↗

arXiv2014

Ab-initio nanoplasmonics: The impact of atomic structure

We present an ab-initio study of the hybridization of localized surface plasmons in a metal nanoparticle dimer. The atomic structure, which is often neglected in theoretical studies of quantum nanoplasmonics, has a strong impact on the optical absorption properties when sub-nanometric gaps between the nanoparticles are considered. We demonstrate that this influences the hybridization of optical resonances of the dimer, and leads to significantly smaller electric field enhancements as compared to the standard jellium model. In addition we show that the corrugation of the metal surface at a microscopic scale becomes as important as other well-known quantum corrections to the plasmonic response, implying that the atomic structure has to be taken into account to obtain quantitative predictions for realistic nanoplasmonic devices.

physics.optics↗

arXiv2014

Generation, manipulation, and detection of two-qubit entanglement in waveguide QED

We study the possibility of using guided photons to generate, control, and measure the entanglement of two qubits that is mediated by a one-dimensional waveguide. We show how entanglement can be generated both with single photon and with two-photon wavepackets. The introduction of a second photon allows for a manipulation of the entanglement between the qubits, and phenomena such as sudden death and revival of entanglement appear. Finally, we propose a procedure for entanglement detection via the scattering output of a single-photon over a qubit state.

quant-ph↗

arXiv2014

Plasmonic Brownian ratchet

Here we present a Brownian ratchet based on plasmonic interactions. By periodically turning on and off a laser beam that illuminates a periodic array of plasmonic nanostructures with broken spatial symmetry, the random thermal motion of a subwavelength dielectric bead is rectified into one direction. By means of the Molecular Dynamics technique we show a statistical directed drift in particle flow.

cond-mat.mes-hall↗

arXiv2014

Reversible dynamics of single quantum emitters near metal-dielectric interfaces

Here we present a systematic study of the dynamics of a single quantum emitter near a flat metal-dielectric interface. We identify the key elements that determine the onset of reversibility in these systems by using a formalism suited for absorbing media and through an exact integration of the dynamics. Moreover, when the quantum emitter separation from the surface is small, we are able to describe the dynamics within a pseudomode description that yields analytical understanding and allows more powerful calculations.

cond-mat.mes-hall↗

arXiv2013

Non-Markovian effects in waveguide-mediated entanglement

We study the generation and evolution of entanglement between two qubits coupled through one-dimensional waveguide modes. By using a complete quantum electrodynamical formalism we go beyond the Markovian approximation. The diagonalization of the hamiltonian is carried out, and a set of quasi-localized eigenstates is found. We show that when the qubit-waveguide coupling is increased, the Markov approximation is not anymore valid, and the generation of entanglement is worsened.

quant-ph↗

arXiv2013

Theory of the strong coupling between quantum emitters and propagating surface plasmons

Here we present the theoretical foundation of the strong coupling phenomenon between quantum emitters and propagating surface plasmons observed in two-dimensional metal surfaces. For that purpose, we develop an ab-initio quantum framework that accounts for the coherent coupling be- tween emitters and surface plasmons and incorporates the presence of dissipation and dephasing. For both a single emitter and a disordered ensemble of emitters, our formalism is able to reveal the key physical mechanisms that explain the reported phenomenology and also to determine the physical parameters that optimize the strong coupling.

cond-mat.mes-hall↗

arXiv2012

Graphene supports the propagation of subwavelength optical solitons

We study theoretically nonlinear propagation of light in a graphene monolayer. We show that the large intrinsic nonlinearity of graphene at optical frequencies enables the formation of quasi one-dimensional self-guided beams (spatial solitons) featuring subwavelength widths at moderate electric-field peak intensities. We also demonstrate a novel class of nonlinear self-confined modes resulting from the hybridization of surface plasmon polaritons with graphene optical solitons.

physics.optics↗

arXiv2012

Analytical expressions for the Electromagnetic Dyadic Green's Function in Graphene and thin layers

An analytical general analysis of the electromagnetic Dyadic Green's Function for two-dimensional sheet (or a very thin film) is presented, with an emphasis on on the case of graphene. A modified steepest descent treatment of the fields from a point dipole given in the form of Sommerfeld integrals is performed. We sequentially derive the expressions for both out-of-plane and in-plane fields of both polarizations. It is shown that the analytical approximation provided is very precise in a wide range of distances from a point source, down to a deep subwavelength region (1/100 of wavelength). We separate the contribution from the pole, the branch point and discuss their interference. The asymptotic expressions for the fields are composed of the plasmon, Norton wave and the components corresponding to free space.

cond-mat.mes-hall↗

arXiv2011

Surface plasmon enhanced absorption and suppressed transmission in periodic arrays of graphene ribbons

Resonance diffraction in the periodic array of graphene micro-ribbons is theoretically studied following a recent experiment [L. Ju et al, Nature Nanotech. 6, 630 (2011)]. Systematic studies over a wide range of parameters are presented. It is shown that a much richer resonant picture would be observable for higher relaxation times of charge carriers: more resonances appear and transmission can be totally suppressed. The comparison with the absorption cross-section of a single ribbon shows that the resonant features of the periodic array are associated with leaky plasmonic modes. The longest-wavelength resonance provides the highest visibility of the transmission dip and has the strongest spectral shift and broadening with respect to the single-ribbon resonance, due to collective effects.

cond-mat.mes-hall↗

arXiv2011

Edge and waveguide THz surface plasmon modes in graphene micro-ribbons

Surface plasmon modes supported by graphene ribbon waveguides are studied and classified. The properties of both modes with the field concentration within the ribbon area (waveguiding modes) and on the edges (edge modes) are discussed. The waveguide and edge modes are shown to be separated from each other by a gap in wavenumbers. The even-parity hybridized edge mode results to be the fundamental electromagnetic mode of the ribbon, possessing also the lowest losses. All the plasmonic modes in the ribbons have an optimum frequency, at which the absorption losses are minimum, due to competition between the plasmon confinement and the frequency dependence of absorption in graphene.

cond-mat.other↗

arXiv2011

Exploring qubit-qubit entanglement mediated by one-dimensional plasmonic nanowaveguides

We exploit the qubit-qubit coupling induced by plasmon-polariton modes in a one-dimensional nanowaveguide to obtain various two-qubit entanglement situations. Firstly, we observe three phenomena occurring when preparing the initial state of the system and leaving it freely relax: spontaneous formation of entanglement, sudden birth and revival. Then, we show that plugging a laser to each of the qubit, the system arrives to an steady state which, depending on their inter-qubit distance, can also be entangled. For this situation, we also characterize the quantum state of the system showing the entanglement-purity- diagram typical for two-qubit systems.

cond-mat.mtrl-sci↗