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F. M. Marqués

Publications and source records attributed to F. M. Marqués.

At least 19 recordsLinked to original sources

The dipole strength distribution of $^8$He and decay characteristics

The weak binding and spatially extended neutron densities characteristic of drip-line nuclei give rise to a distinctive low-energy dipole response. The drip-line nucleus $^8$He is the most neutron-rich bound nucleus with a mass-to-charge ratio of $A/Z=4$. We measure the dipole response of $^8$He, including for the first time the four-neutron decay channel. A total dipole strength of $\sum B(E1)(E^*<15$~MeV$)=0.95(16)~e^2$fm$^2$ and a dipole polarizability of $α_D = 0.61(1)$~fm$^3$ are extracted from the differential Coulomb-excitation cross section and compared to state-of-the-art theoretical calculations employing coupled cluster and three-body approaches. We find that the dipole continuum is dominated, even at high excitation energies well above the $4n$ decay threshold, by two-neutron emission, pointing to a $^6$He$+2n$ structure of the excited dipole mode. No indication was found for a $4n$ final-state correlation, while pronounced $nn$ and $^6$He-$n$ final-state correlations are apparent.

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Direct observation of three-neutron emission from $^7$He$^*$ and the search for the trineutron

Three-neutron emission from $^7$He has been directly measured for the first time, following neutron knockout from a $^8$He beam at 156 MeV/nucleon. A resonance-like structure at $2.08(4)$ MeV above the $^4$He+$3n$ threshold [$E_x=2.68(4)$ MeV] with a width of $3.9(2)$ MeV was observed and deduced to arise predominately from the predicted $J^π=3/2^{-}_2$ level. The three-neutron invariant-mass spectrum was reconstructed and found to peak at around 1 MeV and could, through complete simulations incorporating neutron-neutron correlations, be very well described by the sequential decay of $^7$He$^*$ via the $2_1^+$ excited state of $^6$He. No evidence was found for any significant three-neutron correlations beyond those expected from well-established two-body interactions, including a trineutron resonance.

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Direct transfer to $^{46,48}$K as a survey of the $π(s_{1/2})$$-ν(sdpf)$ interaction

The collapse of the canonical $N=28$ magic number in nuclei with $Z<20$ has drawn significant interest as it relates to the emergence of an island of inversion centered on $^{42}$Si and $^{44}$S. In particular, interactions between the $πs_{1/2}$ orbital -- empty in $^{42}$Si and full in $^{44}$S -- and the neutron orbitals just above and below the $N=28$ gap are expected to be critical in this region, but remain relatively unexplored. In this paper, we expand upon the results of our previous study of the direct transfer reaction $^{47}$K(d,p$γ$)$^{48}$K [C.\,J.~Paxman \textit{et al.}, Phys. Rev. Lett. 134, 162504 (2025)] with the results of the complementary $^{47}$K(d,t$γ$)$^{46}$K reaction. Through this study, we present a comprehensive scan of the interaction between the critical $πs_{1/2}$ orbital and a broad range of neutron orbitals spanning nearly two full shells. We identify several discrepancies between the experimental results and state-of-the-art shell model calculations, which suggest a deficiency of the shell model to fully capture the complex proton configuration mixing in this region, highlighting a significant challenge for single-particle descriptions of the island of inversion.

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Unbound neutron $\nu0d_{3/2}$ strength in $^{17}$C and the N=16 shell gap

Significant continuum strength has been observed to be populated in $^{17}$C produced in the d($^{16}$C,p) reaction at a beam energy of 17.2~MeV/nucleon. The strength appears at greater than $\sim$2~MeV above the single-neutron decay threshold and has been identified as arising from transfer into the neutron $0d_{3/2}$ orbital. Guided by shell model predictions the greater majority of the strength is associated with a 3/2$^+$ state at an excitation energy of 4.40$_{-0.14}^{+0.33}$ MeV and a much weaker 3/2$^+$ level at 5.60$_{-0.45}^{+1.35}$ MeV. The corresponding total widths were determined to be 3.45$_{-0.78}^{+1.82}$ and 1.6$_{-1.4}^{+4.6}$ MeV, respectively. From the backward angle proton differential cross sections and the branching ratios for neutron decay to the $^{16}$C(2$_{1}^{+}$) level, the corresponding spectroscopic factors to the ground state were deduced to be 0.47$\pm{10}$ and $<$0.09. Shell-model calculations employing the phenomenological SFO-tls interaction as well as Gamow Shell-Model calculations including continuum effects are in reasonable agreement with experiment, although the predicted strength lies at somewhat lower energy. The size of the N=16 shell gap ($\varepsilon_{ \nu0d_{3/2}}-\varepsilon _{ν1s_{1/2}}$) was estimated to be 5.08$_{-0.33}^{+0.43}$~MeV - some 1.3~MeV larger than found in the SFO-tls shell model calculation.

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Low-energy neutron cross-talk between organic scintillator detectors

A series of measurements have been performed with low-energy monoenergetic neutrons to characterise cross-talk between two organic scintillator detectors. Cross-talk time-of-flight spectra and probabilities were determined for neutron energies from 1.4 to 15.5 MeV and effective scattering angles ranging from $\sim$50° to $\sim$100°. Monte-Carlo simulations incorporating both the active and inactive materials making up the detectors showed reasonable agreement with the measurements. Whilst the time-of-flight spectra were very well reproduced, the cross-talk probabilities were only in approximate agreement with the measurements, with the most significant discrepancies ($\sim$40 %) occurring at the lowest energies. The neutron interaction processes producing cross-talk at the energies explored here are discussed in the light of these results.

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Probing exotic cross-shell interactions at N=28 with single-neutron transfer on 47K

We present the first measurement of the $^{47}$K($d,pγ$)$^{48}$K transfer reaction, performed in inverse kinematics using a reaccelerated beam of $^{47}$K. The level scheme of $^{48}$K has been greatly extended with nine new bound excited states identified and spectroscopic factors deduced. Detailed comparisons with SDPF-U and SDPF-MU shell-model calculations reveal a number of discrepancies with these results, and a preference for SDPF-MU is found. Intriguingly, an apparent systematic overestimation of spectroscopic factors and a poor reproduction of the energies for 1$^-$ states suggests that the mixing between the $πs^{\,\,\,1}_{1/2} d^{\,\,\,4}_{3/2}$ and $πs^{\,\,\,2}_{1/2} d^{\,\,\,3}_{3/2}$ proton configurations in $^{48}$K is not correctly described using current interactions, challenging our descriptions of light $N=28$ nuclei.

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Mass, spectroscopy and two-neutron decay of $^{16}$Be

The structure and decay of the most neutron-rich beryllium isotope, $^{16}$Be, has been investigated following proton knockout from a high-energy $^{17}$B beam. Two relatively narrow resonances were observed for the first time, with energies of $0.84(3)$ and $2.15(5)$ MeV above the two-neutron decay threshold and widths of $0.32(8)$ and $0.95(15)$ MeV respectively. These were assigned to be the ground ($J^π=0^+$) and first excited ($2^+$) state, with $E_x=1.31(6)$ MeV. The mass excess of $^{16}$Be was thus deduced to be $56.93(13)$ MeV, some $0.5$ MeV more bound than the only previous measurement. Both states were observed to decay by direct two-neutron emission. Calculations incorporating the evolution of the wavefunction during the decay as a genuine three-body process reproduced the principal characteristics of the neutron-neutron energy spectra for both levels, indicating that the ground state exhibits a strong spatially compact dineutron component, while the 2$^+$ level presents a far more diffuse neutron-neutron distribution.

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Validation of the $^{10}\mathrm{Be}$ Ground-State Molecular Structure Using $^{10}\mathrm{Be}(p,pα)^{6}\mathrm{He}$ Triple Differential Reaction Cross-Section Measurements

The cluster structure of the neutron-rich isotope $^{10}$Be has been probed via the $(p,pα)$ reaction at 150 MeV/nucleon in inverse kinematics and in quasifree conditions. The populated states of $^{6}$He residues were investigated through missing mass spectroscopy. The triple differential cross-section for the ground-state transition was extracted for quasifree angle pairs ($θ_{p}$, $θ_α$) and compared to distorted-wave impulse approximation reaction calculations performed in a microscopic framework using successively the Tohsaki-Horiuchi-Schuck-Röpke product wave-function and the wave-function deduced from Antisymmetrized Molecular Dynamics calculations. The remarkable agreement between calculated and measured cross-sections in both shape and magnitude validates the molecular structure description of the $^{10}$Be ground-state, configured as an $α$-$α$ core with two valence neutrons occupying $π$-type molecular orbitals.

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Silicon tracker array for RIB experiments at SAMURAI

This work describes a silicon tracker system developed for experiments with proton-rich radioactive ion beams at the SAMURAI superconducting spectrometer of RIBF at RIKEN. The system is designed for accurate angular reconstruction and atomic number identification of relativistic heavy ions and protons which are simultaneously produced in reactions motivated by studies of proton capture reactions of interest for nuclear astrophysics. The technical characteristics of the tracking array are described in detail as are its performance in two pilot experiments. The physics justification for such a system is also presented.

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Searching for universality of dineutron correlation at the surface of Borromean nuclei

The dineutron correlation is systematically studied in three different Borromean nuclei near the neutron dripline, 11Li, 14Be and 17B, via the (p, pn) knockout reaction measured at the RIBF facility in RIKEN. For the three nuclei, the correlation angle between the valence neutrons is found to be largest in the same range of intrinsic momenta, which can be associated to the nuclear surface. This result reinforces the prediction that the formation of the dineutron is universal in environments with low neutron density, such as the surface of neutron-rich Borromean nuclei.

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Intruder configurations in $^{29}$Ne at the transition into the island of inversion: Detailed structure study of $^{28}$Ne

Detailed $γ$-ray spectroscopy of the exotic neon isotope $^{28}$Ne has been performed for the first time using the one-neutron removal reaction from $^{29}$Ne on a liquid hydrogen target at 240~MeV/nucleon. Based on an analysis of parallel momentum distributions, a level scheme with spin-parity assignments has been constructed for $^{28}$Ne and the negative-parity states are identified for the first time. The measured partial cross sections and momentum distributions reveal a significant intruder $p$-wave strength providing evidence of the breakdown of the $N=20$ and $N=28$ shell gaps. Only a weak, possible $f$-wave strength was observed to bound final states. Large-scale shell-model calculations with different effective interactions do not reproduce the large $p$-wave and small $f$-wave strength observed experimentally, indicating an ongoing challenge for a complete theoretical description of the transition into the island of inversion along the Ne isotopic chain.

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Cross-shell states in $^{15}$C: a test for p-sd interactions

The low-lying structure of $^{15}$C has been investigated via the neutron-removal $^{16}$C$(d,t)$ reaction. Along with bound neutron sd-shell hole states, unbound p-shell hole states have been firmly confirmed. The excitation energies and the deduced spectroscopic factors of the cross-shell states are an important measure of the $[(p)^{-1}(sd)^{2}]$ neutron configurations in $^{15}$C. Our results show a very good agreement with shell-model calculations using the SFO-tls interaction for $^{15}$C. However, a modification of the $p$-$sd$ and $sd$-$sd$ monopole terms was applied in order to reproduce the $N=9$ isotone $^{17}$O. In addition, the excitation energies and spectroscopic factors have been compared to the first calculations of $^{15}$C with the $ab~ initio$ self-consistent Green's function method employing the NNLO$_{sat}$ interaction. The results show the sensitivity to the size of the $N=8$ shell gap and highlight the need of going beyond the current truncation scheme in the theory.

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Border of the Island of Inversion: Unbound states in $^{29}$Ne

The nucleus $^{29}$Ne is situated at the border of the island of inversion. Despite significant efforts, no bound low-lying intruder $f_{7/2}$-state, which would place $^{29}$Ne firmly inside the island of inversion, has yet been observed. Here, the first investigation of unbound states of $^{29}$Ne is reported. The states were populated in $^{30}\mathrm{Ne}(p,pn)$ and $^{30}\mathrm{Na}(p,2p)$ reactions at a beam energy of around $230$ MeV/nucleon, and analyzed in terms of their resonance properties, partial cross sections and momentum distributions. The momentum distributions are compared to calculations using the eikonal, direct reaction model, allowing $\ell$-assignments for the observed states. The lowest-lying resonance at an excitation energy of 1.48(4) MeV shows clear signs of a significant $\ell$=3-component, giving first evidence for $f_{7/2}$ single particle strength in $^{29}$Ne. The excitation energies and strengths of the observed states are compared to shell-model calculations using the sdpf-u-mix interaction

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19B isotope as a 17B-n-n three-body cluster close to unitary limit

We describe 19B in terms of a 17B-n-n three-body system, where the two-body subsystems 17B-n and n-n are unbound (virtual) states close to the unitary limit. The energy of 19B ground state is well reproduced and two low-lying resonances are predicted. Their eventual link with the Efimov physics is discussed. This model can be extended to describe the recently discovered resonant states in 20,21B.

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Low-lying single-particle structure of 17C and the N = 14 sub-shell closure

The first investigation of the single-particle structure of the bound states of 17C, via the d(16C, p) transfer reaction, has been undertaken. The measured angular distributions confirm the spin-parity assignments of 1/2+ and 5/2+ for the excited states located at 217 and 335 keV, respectively. The spectroscopic factors deduced for these states exhibit a marked single-particle character, in agreement with shell model and particle-core model calculations, and combined with their near degeneracy in energy provide clear evidence for the absence of the N = 14 sub-shell closure. The very small spectroscopic factor found for the 3/2+ ground state is consistent with theoretical predictions and indicates that the ν1d3/2 strength is carried by unbound states. With a dominant l = 0 valence neutron configuration and a very low separation energy, the 1/2+ excited state is a one-neutron halo candidate.

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Surface localization of the dineutron in $^{11}$Li

The formation of a dineutron in the nucleus $^{11}$Li is found to be localized to the surface region. The experiment measured the intrinsic momentum of the struck neutron in $^{11}$Li via the $(p,pn)$ knockout reaction at 246 MeV/nucleon. The correlation angle between the two neutrons is, for the first time, measured as a function of the intrinsic neutron momentum. A comparison with reaction calculations reveals the localization of the dineutron at $r\sim3.6$ fm. The results also support the density dependence of dineutron formation as deduced from Hartree-Fock-Bogoliubov calculations for nuclear matter.

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Study of multi-neutron emission in the $β$-decay of $^{11}$Li

The kinematics of two-neutron emission following the $β$-decay of $^{11}$Li was investigated for the first time by detecting the two neutrons in coincidence and by measuring their angle and energy. An array of liquid-scintillator neutron detectors was used to reject cosmic-ray and $γ$-ray backgrounds by pulse-shape discrimination. Cross-talk events in which two detectors are fired by a single neutron were rejected using a filter tested on the $β$-1n emitter $^9$Li. A large cross-talk rejection rate is obtained ($> 95 \%$) over most of the energy range of interest. Application to $^{11}$Li data leads to a significant number of events interpreted as $β$-2n decay. A discrete neutron line at $\approx$ 2 MeV indicates sequential two-neutron emission, possibly from the unbound state at 10.6 MeV excitation energy in $^{11}$Be.

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Study of multi-neutron systems with SAMURAI spectrometer

The tetraneutron has been drawing the attention of the nuclear physics community for decades, but a firm conclusion on its existence and properties is still far from being reached despite many experimental and theoretical efforts. New measurements have recently been performed at RIBF with the SAMURAI spectrometer by applying complementary reaction probes, which will help to pin down the properties of this four-neutron system.

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