arXiv subjects

F. M. Peeters

Publications and source records attributed to F. M. Peeters.

At least 343 records · Page 19Linked to original sources

arXiv2008

Paramagnetic adsorbates on graphene: a charge transfer analysis

We introduce a modified version of the Hirshfeld charge analysis method and demonstrate its accurateness by calculating the charge transfer between the paramagnetic molecule NO2 and graphene. The charge transfer between paramagnetic molecules and a graphene layer as calculated with ab initio methods can crucially depend on the size of the supercell used in the calculation. This has important consequences for adsorption studies involving paramagnetic molecules such as NO2 physisorbed on graphene or on carbon nanotubes.

cond-mat.mtrl-sci↗

arXiv2008

Tuning of energy levels and optical properties of graphene quantum dots

We investigate theoretically the magnetic levels and optical properties of zigzag- and armchair-edged hexagonal graphene quantum dots (GQDs) utilizing the tight-binding method. A new bound edge state at zero energy appears for the zigzag GQDs in the absence of a magnetic field. The magnetic levels of GQDs exhibit a Hofstadter-butterfly spectrum and approach the Landau levels of two-dimensional graphene as the magnetic field increases. The optical properties are tuned by the size, the type of the edge, and the external magnetic field.

cond-mat.mes-hall↗

arXiv2008

Formation and Size-Dependence of Vortex Shells in Mesoscopic Superconducting Niobium Disks

Recent experiments [I.V. Grigorieva et al., Phys. Rev. Lett. 96, 077005 (2006)] on visualization of vortices using the Bitter decoration technique revealed vortex shells in mesoscopic superconducting Nb disks containing up to L=40 vortices. Some of the found configurations did not agree with those predicted theoretically. We show here that this discrepancy can be traced back to the larger disks with radii R ~ 1 to 2.5μm, i.e., R ~ 50-100ξ(0) used in the experiment, while in previous theoretical studies vortex states with vorticity L < 40 were analyzed for smaller disks with R ~ 5-20ξ(0). The present analysis is done for thin disks (mesoscopic regime) and for thick (macroscopic) disks where the London screening is taken into account. We found that the radius of the superconducting disk has a pronounced influence on the vortex configuration in contrast to, e.g., the case of parabolic confined charged particles. The missing vortex configurations and the region of their stability are found, which are in agreement with those observed in the experiment.

cond-mat.supr-con↗

arXiv2008

Dynamics of periodic anticrossings: Decoherence, pointer states and hysteresis curves

We consider a strongly driven two-level (spin) system, with a periodic external field that induces a sequence of avoided level crossings. The spin system interacts with a bosonic reservoir which leads to decoherence. A Markovian dynamical equation is introduced without relying on the rotating wave approximation in the system-external field interaction. We show that the time evolution of the two-level system is directed towards an incoherent sum of periodic Floquet states regardless of the initial state and even the type of the coupling to the environment. Analyzing the time scale of approaching these time-dependent pointer states, information can be deduced concerning the nature and strength of the system-environment coupling. The inversion as a function of the external field is usually multi-valued, and the form of these hysteresis curves is qualitatively different for low and high temperatures. For moderate temperatures we found that the series of Landau-Zener-Stückelberg-type transitions still can be used for state preparation, regardless of the decoherence rate. Possible applications include quantum information processing and molecular nanomagnets.

quant-ph↗

arXiv2007

Effect of the boundary condition on the vortex patterns in mesoscopic three-dimensional superconductors - disk and sphere

The vortex state of mesoscopic three-dimensional superconductors is determined using a minimization procedure of the Ginzburg-Landau free energy. We obtain the vortex pattern for a mesoscopic superconducting sphere and find that vortex lines are naturally bent and are closest to each other at the equatorial plane. For a superconducting disk with finite height, and under an applied magnetic field perpendicular to its major surface, we find that our method gives results consistent with previous calculations. The matching fields, the magnetization and $H_{c3}$, are obtained for models that differ according to their boundary properties. A change of the Ginzburg-Landau parameters near the surface can substantially enhance $H_{c3}$ as shown here.

cond-mat.supr-con↗

arXiv2007

Transverse magnetization and torque in asymmetrical mesoscopic superconductors

We show that asymmetrical mesoscopic superconductors bring new insight into vortex physics where we found the remarkable coexistence of long and short vortices. We study an asymmetrical mesoscopic sphere, that lacks one of its quadrants, and obtain its three-dimensional vortex patterns by solving the Ginzburg-Landau theory. We find that the vortex patterns are asymmetric whose effects are clearly visible and detectable in the transverse magnetization and torque.

cond-mat.supr-con↗

arXiv2007

Threefold onset of vortex loops in superconductors with a magnetic core

A magnetic inclusion inside a superconductor gives rise to a fascinating complex of {\it vortex loops}. Our calculations, done in the framework of the Ginzburg-Landau theory, reveal that {\it loops always nucleate in triplets} around the magnetic core. In a mesoscopic superconducting sphere, the final superconducting state is characterized by those confined vortex loops and the ones that eventually spring to the surface of the sphere, evolving into {\it vortex pairs} piercing through the sample surface.

cond-mat.supr-con↗

arXiv2007

Exciton spectra in vertical stacks of triple and quadruple quantum dots in an electric field

We study an electron-hole pair in a stack of multiple quantum dots in the presence of an external electric field using the configuration interaction approach. We find that the bright energy levels can be grouped into families which are associated with the hole localized in a specific dot of the stack. The exciton energy levels undergo avoided crossings as function of the external electric field with different pattern for each family. We show that the variation of the depths of the dots along the stack can be deduced from the exciton spectrum. In the strong confinement limit the families are mixed by a weak electric field due to hole tunneling. This results in a characteristic multiple avoided crossing of energy levels belonging to different families with an accompanying modulation of the recombination probabilities and an appearance of a single particularly bright state. We discuss the modification of the spectrum when dots are added to the stack.

cond-mat.mes-hall↗

arXiv2007

Quasi-bound states of quantum dots in single and bilayer graphene

Dirac fermions interacting with a cylindrically symmetric quantum dot potential created in single and bilayer graphene are not confined but form quasi-bound states. The broadening of these quasi-bound states (i. e. the inverse of their lifetimes) decreases (increases) with the orbital momentum of the electron in the case of graphene (bilayer). Quasi-bound states with energy below (above) the barrier height are dominantly electron(hole)-like. A remarkable decrease of the energy level broadening is predicted for electron energies close to the barrier height, which are a consequence of the total internal reflection of the electronic wave at the dot edge.

cond-mat.mes-hall↗

arXiv2007

Adsorption of H2O, NH3, CO, NO2, and NO on graphene: A first-principles study

Motivated by the recent realization of graphene sensors to detect individual gas molecules, we investigate the adsorption of H2O, NH3, CO, NO2, and NO on a graphene substrate using first-principles calculations. The optimal adsorption position and orientation of these molecules on the graphene surface is determined and the adsorption energies are calculated. Molecular doping, i.e. charge transfer between the molecules and the graphene surface, is discussed in light of the density of states and the molecular orbitals of the adsorbates. The efficiency of doping of the different molecules is determined and the influence of their magnetic moment is discussed.

cond-mat.mtrl-sci↗

arXiv2007

Landau levels and oscillator strength in a biased bilayer of graphene

We obtain analytical expressions for the eigenstates and the Landau level spectrum of biased graphene bilayers in a magnetic field. The calculations are performed in the context of a four-band continuum model and generalize previous approximate results. Solutions are presented for the spectrum as a function of interlayer coupling, the potential difference between the layers and the magnetic field. The explicit expressions allow us to calculate the oscillator strength and the selection rules for electric dipole transitions between the Landau states. Some transitions are significantly shifted in energy relative to those in an unbiased bialyer and exhibit a very different magnetic field dependence.

cond-mat.mes-hall↗

arXiv2007

Hysteresis and re-entrant melting of a self-organized system of classical particles confined in a parabolic trap

A self-organized system composed of classical particles confined in a two-dimensional parabolic trap and interacting through a potential with a short-range attractive part and long-range repulsive part is studied as function of temperature. The influence of the competition between the short-range attractive part of the inter-particle potential and its long-range repulsive part on the melting temperature is studied. Different behaviors of the melting temperature are found depending on the screening length ($κ$) and the strength ($B$) of the attractive part of the inter-particle potential. A re-entrant behavior and a thermal induced phase transition is observed in a small region of ($κ,B$)-space. A structural hysteresis effect is observed as a function of temperature and physically understood as due to the presence of a potential barrier between different configurations of the system.

cond-mat.soft↗

arXiv2007

Rearrangement of the vortex lattice due to instabilities of vortex flow

With increasing applied current we show that the moving vortex lattice changes its structure from a triangular one to a set of parallel vortex rows in a pinning free superconductor. This effect originates from the change of the shape of the vortex core due to non-equilibrium effects (similar to the mechanism of vortex motion instability in the Larkin-Ovchinnikov theory). The moving vortex creates a deficit of quasiparticles in front of its motion and an excess of quasiparticles behind the core of the moving vortex. This results in the appearance of a wake (region with suppressed order parameter) behind the vortex which attracts other vortices resulting in an effective direction-dependent interaction between vortices. When the vortex velocity $v$ reaches the critical value $v_c$ quasi-phase slip lines (lines with fast vortex motion) appear which may coexist with slowly moving vortices between such lines. Our results are found within the framework of the time-dependent Ginzburg-Landau equations and are strictly valid when the coherence length $ξ(T)$ is larger or comparable with the decay length $L_{in}$ of the non-equilibrium quasiparticle distribution function. We qualitatively explain experiments on the instability of vortex flow at low magnetic fields when the distance between vortices $a \gg L_{in} \gg ξ(T)$. We speculate that a similar instability of the vortex lattice should exist for $v>v_c$ even when $a<L_{in}$.

cond-mat.supr-con↗

arXiv2007

Optical properties of (In,Ga)As capped InAs quantum dots grown on [11k] substrates

Using three-dimensional k.p calculation including strain and piezoelectricity, we showed that the size of the quantum dot (QD) in the growth direction determines the influence of the (In,Ga)As capping layer on the optical properties of [11k] grown InAs QDs, where k=1,2,3. For flat dots, increase of In concentration in the capping layer leads to a decrease of the transition energy, as is the case of [001] grown QDs, whereas for large dots an increase of the In concentration in the capping layer is followed by an increase of the transition energy up to a critical concentration of In, after which the optical transition energy starts to decrease.

cond-mat.mtrl-sci↗

arXiv2007

A three-dimensional model for artificial atoms and molecules: Influence of substrate orientation and magnetic field dependence

A full three-dimensional model for the calculation of the electronic structure of semiconductor quantum dots (QD) and molecules (QDM) grown on high index surfaces and/or in the presence of an external magnetic field is presented. The strain distribution of the dots is calculated using continuum elasticity and singe-particle states are extracted from the nonsymmetrized eight-band k.p theory. The model properly takes into account the effects of different substrate orientation by rotation of the coordinate system in the way that one coordinate coincides with the growth direction, whereas the effects of a tilted external magnetic field are taken into account throught the Zeeman effect and employing a gauge invariant scheme based on Wilson's formulation of lattice gauge theory. We point out the role of piezoelectricity for InAs/GaAs QDs grown on [11k], where k = 1,2,3,4,5,7,9 and for QDMs containing eight InAs/GaAs QDs grown on [11l], where l = 1,2,3. We predict the variation of the transition energies of the QDM as a function of substrate orientation and interdot distances in the molecule. We address the magnetic field direction dependent variation of the electronic properties of QD and QDM.

cond-mat.mtrl-sci↗

arXiv2007

Tunable quantum dots in bilayer graphene

We demonstrate theoretically that quantum dots in bilayers of graphene can be realized. A position-dependent doping breaks the equivalence between the upper and lower layer and lifts the degeneracy of the positive and negative momentum states of the dot. Numerical results show the simultaneous presence of electron and hole confined states for certain doping profiles and a remarkable angular momentum dependence of the quantum dot spectrum which is in sharp contrast with that for conventional semiconductor quantum dots. We predict that the optical spectrum will consist of a series of non-equidistant peaks.

cond-mat.mes-hall↗

arXiv2007

Graphene-based resonant-tunneling strucures

Resonant electronic transmission through graphene-based double barriers (wells) is studied as a function of the incident wave vector, the widths and heights (depths) of the barriers (wells), and the separation between them. Resonant features in the transmission result from resonant electron states in the wells or hole states in the barriers and strongly influence the ballistic conductance of the structures.

cond-mat.mes-hall↗

arXiv2007

Symmetric and asymmetric states in mesoscopic superconducting wire in voltage driven regime

The response of a mesoscopic homogeneous superconducting wire, connected with bulk normal metal reservoirs, is theoretically investigated as function of the applied voltage. The finite relaxation length of the nonequilibrium quasiparticle distribution function $\bar{L_E}$ is included where we assumed that our wire is in the dirty limit. We found that {\it both} symmetric and asymmetric states can exist which are characterized by a stationary symmetric and asymmetric distribution of the order parameter with respect to the center of the wire. Current voltage characteristics of the wire with length $L>\bar{L_E}$ being in the symmetric state show a pronounced S-behavior. The asymmetric state may exist only for voltages larger than some critical value and coexist with the symmetric state in a finite voltage interval. For wires with $L \sim \bar{L_E}$ the asymmetric state survives up to higher values of the voltage than the symmetric one and may exist both in the voltage and the current driven regimes. We propose an experiment to observe reversible switching between those stationary symmetric and asymmetric states.

cond-mat.supr-con↗