arXiv subjects

F. Michelini

Publications and source records attributed to F. Michelini.

5 recordsLinked to original sources

arXiv2017

Dynamical photo-induced electronic properties of molecular junctions

Nanoscale molecular-electronic devices and machines are emerging as promising functional elements, naturally flexible and efficient, for next generation technologies. A deeper understanding of carrier dynamics in molecular junctions is expected to benefit many fields of nanoelectronics and power-devices. We determine time-resolved charge current flowing at donor- acceptor interface in molecular junctions connected to metallic electrodes by means of quantum transport simulations. The current is induced by the interaction of the donor with a Gaussian-shape femtosecond laser pulse. Effects of the molecular internal coupling, metal- molecule tunneling and light-donor coupling on photocurrent are discussed. We then examine the junction working through the time-resolved donor density of states. Non-equilibrium reorganization of hybridized molecular orbitals through the light-donor interaction gives rise to two phenomena: the dynamical Rabi shift and the appearance of Floquet-like states. Such insights into the dynamical photoelectronic structure of molecules are of strong interest for ultrafast spectroscopy, and open avenues toward the possibility of analyzing and controlling the internal properties of quantum nanodevices with pump-push photocurrent spectroscopy.

cond-mat.mes-hall↗

arXiv2017

Getting information from the mixed electrical-heat noise

We give a classification of the different types of noise in a quantum dot, for variable temperature, voltage and frequency. It allows us first to show which kind of information can be extracted from the electrical noise, such as the ac-conductance or the Fano factor. And next, to classify the mixed electrical-heat noise, and to identify in which regimes information on the Seebeck coefficient, on the thermoelectric figure of merit, or on the thermoelectric efficiency can be obtained.

cond-mat.mes-hall↗

arXiv2016

Heat-charge mixed noise and thermoelectric efficiency fluctuations

The close relationship between the noise and the thermoelectric conversion is studied in a quantum dot using a quantum approach based on the non-equilibrium Green function technique. We show that both the figure of merit and the efficiency can be written in term of noise and we highlight the central role played by the correlator between the charge current and the heat current that we call the mixed noise. After giving the expression of this quantity as an integral over energy, we calculate it, first in the linear response regime, next in the limit of small transmission through the barriers (Schottky regime) and finally in the intermediate regime. We discuss the notion of efficiency fluctuations and we also see here that the mixed noise comes into play.

cond-mat.mes-hall↗

arXiv2007

Broadening processes in GaAs delta-doped quantum wire superlattices

We use both Quantum Hall and Shubnikov de Haas experiments at high magnetic field and low temperature to analyse broadening processes of Landau levels in a delta-doped 2D quantum well superlattice and a 1D quantum wire superlattice generated from the first one by controlled dislocation slips. We deduce first the origin of the broadening from the damping factor in the Shubnikov de Haas curves in various configurations of the magnetic field and the measured current for both kinds of superlattice. Then, we write a general formula for the resistivity in the Quantum Hall effect introducing a dephasing factor we link to the process of localization.

cond-mat.mes-hall↗

arXiv2007

Non-orthogonal Theory of Polarons and Application to Pyramidal Quantum Dots

We present a general theory for semiconductor polarons in the framework of the Froehlich interaction between electrons and phonons. The latter is investigated using non-commuting phonon creation/annihilation operators associated with a natural set of non-orthogonal modes. This setting proves effective for mathematical simplification and physical interpretation and reveals a nested coupling structure of the Froehlich interaction. The theory is non-perturbative and well adapted for strong electron-phonon coupling, such as found in quantum dot (QD) structures. For those particular structures we introduce a minimal model that allows the computation and qualitative prediction of the spectrum and geometry of polarons. The model uses a generic non-orthogonal polaron basis, baptized the "natural basis". Accidental and symmetry-related electronic degeneracies are studied in detail and are shown to generate unentangled zero-shift polarons, which we consistently eliminate. As a practical example, these developments are applied to realistic pyramidal GaAs QDs. The energy spectrum and the 3D-geometry of polarons are computed and analyzed, and prove that realistic pyramidal QDs clearly fall in the regime of strong coupling. Further investigation reveals an unexpected substructure of "weakly coupled strong coupling regimes", a concept originating from overlap considerations. Using Bennett's entanglement measure, we finally propose a heuristic quantification of the coupling strength in QDs.

cond-mat.other↗