arXiv subjects

F. Oručević

Publications and source records attributed to F. Oručević.

4 recordsLinked to original sources

arXiv2025

Quantum magnetic imaging of current density in lithium-ion batteries

The projected rapid growth of battery cell production over the next decade demands advanced diagnostic tools for quality control, ageing prediction, and recycling. Most existing techniques lack the spatial and temporal resolution required to capture internal electrochemical processes non-invasively. Here, we present magnetic imaging of current densities in battery cells, a sensitive quantum-magnetometry method that uses optically pumped magnetometers (OPMs) to perform real-time imaging of internal dynamics in open-circuit configuration. We demonstrate this approach for monitoring relaxation processes in 6000 mA h lithium-ion cells following pulsed discharges across a range of pulse durations and currents as well as states of charge. The measurement results are benchmarked against superconducting-quantum-interference-device (SQUID) magnetometry and validated with three-dimensional finite element simulations. Equivalent circuit models are employed to interpret the relaxation profiles, revealing spatially resolved features and transient magnetic-field signatures that are inaccessible with complementary non-invasive techniques such as electrochemical impedance spectroscopy (EIS). This work establishes OPM-based magnetic imaging of battery current density as a powerful diagnostic tool with potential impact on cell development, manufacturing quality assurance, and second-life assessment.

quant-ph↗

arXiv2023

Quantum gas-enabled direct mapping of active current density in percolating networks of nanowires

Electrically percolating nanowire networks are amongst the most promising candidates for next-generation transparent electrodes. Scientific interest in these materials stems from their intrinsic current distribution heterogeneity, leading to phenomena like percolating pathway re-routing and localized self-heating, which can cause irreversible damage. Without an experimental technique to resolve the current distribution, and an underpinning nonlinear percolation model, one relies on empirical rules and safety factors to engineer these materials. We introduce Bose-Einstein microscopy to address the long-standing problem of imaging active current flow in 2D materials. We report on improvement of the performance of this technique, whereby observation of dynamic redistribution of current pathways becomes feasible. We show how this, combined with existing thermal imaging methods, eliminates the need for assumptions between electrical and thermal properties. This will enable testing and modelling individual junction behaviour and hotspot formation. Investigating both reversible and irreversible mechanisms will contribute to the advancement of devices with improved performance and reliability.

physics.app-ph↗

arXiv2019

Additively manufactured ultra-high vacuum chamber below $10^{-10}$ mbar

Metal-based additive manufacturing (AM) represents a paradigm change in engineering and production methods across multiple industries and sectors. AM methods enable mass reduction and performance optimisation well beyond that achievable via conventional manufacturing, thereby impacting significantly on aerospace and space technologies. Technologies relying on high and ultra-high vacuum (UHV), such as x-ray photo-electron spectroscopy, photo-sensors, cameras and cryostats, could also benefit greatly from AM. Despite recent advances in AM processing of metals, additively manufactured UHV chambers have so far not been achieved. Reducing the mass of UHV equipment is particularly critical for the development of portable cold atom systems, which are expected to underpin the next generation of sensing and timekeeping technologies and to allow novel space-based sensors for fundamental research. We demonstrate here an additively manufactured UHV chamber reaching a pressure below $10^{-10}$ mbar, enabling a cloud of cold $^{85}$Rb atoms to be trapped - the starting point for many precision timekeeping and sensing devices. The chamber is manufactured from aluminium alloy AlSi10Mg by laser powder bed fusion and has a mass of less than a third of a commercially-available equivalent. Outgassing analysis based on mass spectrometry was performed and it was demonstrated that even without active pumping the system remains in the $10^{-9}$ mbar regime for up to 48 hours.

quant-ph↗

arXiv2017

3D-printed components for quantum devices

Recent advances in the preparation, control and measurement of atomic gases have led to new insights into the quantum world and unprecedented metrological sensitivities, e.g. in measuring gravitational forces and magnetic fields. The full potential of applying such capabilities to areas as diverse as biomedical imaging, non-invasive underground mapping, and GPS-free navigation can only be realised with the scalable production of efficient, robust and portable devices. Here we introduce additive manufacturing as a production technique of quantum device components with unrivalled design freedom, providing a step change in efficiency, compactness and facilitating systems integration. As a demonstrator we present a compact ultracold atom source using less than ten milliwatts power to produce large samples of cold rubidium gases in an ultrahigh vacuum environment. This disruptive technology opens the door to drastically improved integrated structures, which will further reduce power consumption, size and assembly complexity in scalable series manufacture of bespoke quantum devices.

quant-ph↗