arXiv subjects

F. Parisi

Publications and source records attributed to F. Parisi.

At least 19 recordsLinked to original sources

arXiv2018

Maximum entropy approach to link prediction in bipartite networks

Within network analysis, the analytical maximum entropy framework has been very successful for different tasks as network reconstruction and filtering. In a recent paper, the same framework was used for link-prediction for monopartite networks: link probabilities for all unobserved links in a graph are provided and the most probable links are selected. Here we propose the extension of such an approach to bipartite graphs. We test our method on two real world networks with different topological characteristics. Our performances are compared to state-of-the-art methods, and the results show that our entropy-based approach has a good overall performance.

physics.soc-ph↗

arXiv2016

Avalanche-like metamagnetic transition in (LaNd)CaMnO manganites

We investigate the behavior of ultrasharp metamagnetic transitions in La(5/8-y)Nd(y)Ca(3/8)MnO(3) manganites. These compounds change from a low temperature ferromagnetic metallic state at low Nd doping to a charge-ordered antiferromagnetic insulator for high Nd content. At an intermediate doping a phase-separated state is established. At low temperatures (2 K), we observe an avalanche-like field-induced metamagnetic transition, when the entire compound changes abruptly from one phase to the other. We investigate the signatures of this ultrasharp transition using magnetization and specific heat measurements. We observe a first order transition in the specific heat associated with discontinuous jumps in the magnetization. A strong increase of the sample temperature is simultaneously observed. The results are interpret in terms of latent heat release from the field induced enhancement of the ferromagnetic fraction, triggering the avalanche process.

cond-mat.str-el↗

arXiv2016

Coupled magnetic and elastic properties in LaPr(CaSr)MnO manganites

We investigate a series of manganese oxides, the La0.225Pr0.4(Ca1-xSrx)0.375MnO3 system. The x = 0 sample is a prototype compound for the study of phase separation in manganites, where ferromagnetic and charge ordered antiferromagnetic phases coexist. Replacing Ca2+ by Sr2+ gradually turns the system into a homogeneous ferromagnet. Our results show that the material structure plays a major role in the observed magnetic properties. On cooling, at temperatures below 100 K, a strong contraction of the lattice is followed by an increase in the magnetization. This is observed both through thermal expansion and magnetostriction measurements, providing distinct evidence of magneto-elastic coupling in these phase separated compounds.

cond-mat.str-el↗

arXiv2014

Correlation between electrical and magnetic properties of phase separated manganites studied with a General Effective Medium model

We have performed electrical resistivity and DC magnetization measurements as a function of temperature, on polycrystalline samples of phase separated LaPrCaMnO. We have used the General Effective Medium Theory to obtain theoretical resistivity vs. temperature curves corresponding to different fixed ferromagnetic volume fraction values, assuming that the sample is a mixture of typical metallic like and insulating manganites. By comparing this data with our experimental resistivity curves we have obtained the relative ferromagnetic volume fraction of our sample as a function of temperature. This result matches with the corresponding magnetization data in excellent agreement, showing that a mixed phase scenario is the key element to explain both the magnetic and transport properties in the present compound.

cond-mat.mtrl-sci↗

arXiv2014

Numerical treatment of interfaces for second-order wave equations

In this article we develop a numerical scheme to deal with interfaces between touching numerical grids when solving the second-order wave equation. We show that it is possible to implement an interface scheme of "penalty" type for the second-order wave equation, similar to the ones used for first-order hyperbolic and parabolic equations, and the second-order scheme used by Mattsson et al (2008). These schemes, known as SAT schemes for finite difference approximations and penalties for spectral ones, and ours share similar properties but in our case one needs to pass at the interface a smaller amount of data than previously known schemes. This is important for multi-block parallelizations in several dimensions, for it implies that one obtains the same solution quality while sharing among different computational grids only a fraction of the data one would need for a comparable (in accuracy) SAT or Mattsson et al.'s scheme. The semi-discrete approximation used here preserves the norm and uses standard finite-difference operators satisfying summation by parts. For the time integrator we use a semi-implicit IMEX Runge-Kutta method. This is crucial, since the explicit Runge-Kutta method would be impractical given the severe restrictions that arise from the stiff parts of the equations.

physics.comp-ph↗

arXiv2011

Decoupling electrocaloric effect from Joule heating in a solid state cooling device

We report a heat dynamics analysis of the electrocaloric effect (ECE) in commercial multilayer capacitors based on BaTiO3 dielectric, a promising candidate for applications as a solid state cooling device. Direct measurements of the time evolution of the sample's temperature changes under different applied voltages allow us to decouple the contributions from Joule heating and from the ECE. Heat balance equations were used to model the thermal coupling between different parts of the system. Fingerprints of Joule heating and the ECE could be resolved at different time scales. We argue that Joule heating and the thermal coupling of the device to the environment must be carefully taken in to account in future developments of refrigeration technologies employing the ECE.

cond-mat.mtrl-sci↗

arXiv2010

Magnetocaloric effect in manganites: metamagnetic transitions for magnetic refrigeration

We present a study of the magnetocaloric effect in La5/8-yPryCa3/8MnO3 (y=0.3) and Pr0.5Ca0.09Sr0.41MnO3 manganites. The low temperature state of both ystems is the result of a competition between the antiferromagnetic and ferromagnetic phases. The samples display magnetocaloric effect evidenced in an adiabatic temperature change during a metamagnetic transition from an antiferromagnetic to a ferromagnetic phase . As additional features, La5/8-yPryCa3/8MnO3 exhibits phase separation characterized by the coexistence of antiferromagnetic and ferromagnetic phases and Pr0.5Ca0.09Sr0.41MnO3 displays inverse magnetocaloric effect in which temperature decreases while applying an external magnetic field. In both cases, a significant part of the magnetocaloric effect appears from non-reversible processes. As the traditional thermodynamic description of the effect usually deals with reversible transitions, we developed an alternative way to calculate the adiabatic temperature change in terms of the change of the relative ferromagnetic fraction induced by magnetic field. To evaluate our model, we performed direct measurement of the sample's adiabatic temperature change by means of a differential thermal analysis. An excellent agreement has been obtained between experimental and calculated data. These results show that metamagnetic transition in manganites play an important role in the study of magnetic refrigeration.

cond-mat.str-el↗

arXiv2008

Equilibrium tuned by a magnetic field in phase separated manganite

We present magnetic and transport measurements on La5/8-yPryCa3/8MnO3 with y = 0.3, a manganite compound exhibiting intrinsic multiphase coexistence of sub-micrometric ferromagnetic and antiferromagnetic charge ordered regions. Time relaxation effects between 60 and 120K, and the obtained magnetic and resistive viscosities, unveils the dynamic nature of the phase separated state. An experimental procedure based on the derivative of the time relaxation after the application and removal of a magnetic field enables the determination of the otherwise unreachable equilibrium state of the phase separated system. With this procedure the equilibrium phase fraction for zero field as a function of temperature is obtained. The presented results allow a correlation between the distance of the system to the equilibrium state and its relaxation behavior.

cond-mat.str-el↗

arXiv2007

Spatial motion of the magnetic avalanches associated to the CO-AFM to CD-FM transition in La$_{0.225}$Pr$\_{0.40}$Ca$\_{0.375}$MnO$\_{3}$ manganite

Very fast magnetic avalanches in (La, Pr)-based manganites are the signature of a phase transition from an insulating blocked charge-ordered (CO-AFM) state to a charge delocalized ferromagnetic (CD-FM) state. We report here the experimental observation that this transition does not occur neither simultaneously nor randomly in the whole sample but there is instead a spatial propagation with a velocity of the order of tens of m/s. Our results show that avalanches are originated in the inside of the sample, move to the outside and occur at values of the applied magnetic field that depend on the CD-FM fraction in the sample. Moreover, a change in the gradient of the magnetic field along the sample shifts the point where the avalanches are ignited.

cond-mat.other↗

arXiv2005

Thermodynamic modeling of phase separation in manganites

We present a phenomenological model based on the thermodynamics of the phase separated state of manganites, accounting for its static and dynamic properties. Through calorimetric measurements on La$_{0.225}$Pr$_{0.40}$Ca$ _{0.375}$MnO$_{3}$ the low temperature free energies of the coexisting ferromagnetic and charge ordered phases are evaluated. The phase separated state is modeled by free energy densities uniformly spread over the sample volume. The calculations contemplate the out of equilibrium features of the coexisting phase regime, to allow a comparison between magnetic measurements and the predictions of the model. A phase diagram including the static and dynamic properties of the system is constructed, showing the existence of blocked and unblocked regimes which are characteristics of the phase separated state in manganites.

cond-mat.mtrl-sci↗

arXiv2005

Dynamic phase separation in La(5/8-y)Pr(y)Ca(3/8)MnO(3)

Detailed magnetization measurements in La_{5/8-y}Pr_{y}Ca_{3/8} MnO_{3}, including magnetic relaxation properties, demonstrate the dynamic nature of the phase separated state in manganites. The difference between the field-cooled-cooling and zero-field-cooled magnetization curves signals the existence in the latter of blocked metastable states separated by high energy barriers. Results of the magnetic viscosity show that the system becomes unblocked in a certain temperature window, where large relaxation rates are observed. We propose a simple phenomenological model in which the system evolves through a hierarchy of energy barriers, which separates the coexisting phases. The calculated magnetization curves using this model reproduce all the qualitative features of the experimental data. The overall results allowed us to construct an H-T phase diagram, where frozen and dynamical phase separation regions are clearly distinguished.

cond-mat.str-el↗

arXiv2004

Magnetoresistive memory in phase separated La$_{0.5}$Ca$_{0.5}$MnO$_{3}$

We have studied a non volatile memory effect in the mixed valent compound La$_{0.5}$Ca$_{0.5}$MnO$_{3}$ induced by magnetic field (H). In a previous work [R.S. Freitas et al., Phys. Rev. B 65 (2002) 104403], it has been shown that the response of this system upon application of H strongly depends on the temperature range, related to three well differentiated regimes of phase separation occurring below 220 K. In this work we compare memory capabilities of the compound, determined following two different experimental procedures for applying H, namely zero field cooling and field cooling the sample. These results are analyzed and discussed within the scenario of phase separation.

cond-mat.mtrl-sci↗

arXiv2004

Abrupt field-induced transition triggered by magnetocaloric effect in phase-separated manganites

The occurrence at low temperatures of an ultrasharp field-induced transition in phase separated manganites is analyzed. Experimental results show that magnetization and specific heat step-like transitions below 5 K are correlated with an abrupt change of the sample temperature, which happens at a certain critical field. This temperature rise, a magnetocaloric effect, is interpreted as produced by the released energy at the transition point, and is the key to understand the existence of the abrupt field-induced transition. A qualitative analysis of the results suggests the existence of a critical growing rate of the ferromagnetic phase, beyond which an avalanche effect is triggered.

cond-mat.mtrl-sci↗

arXiv2003

Low temperature irreversibility induced by thermal cycles on two prototypical phase separated manganites

We have studied the effect of irreversibility induced by repeated thermal cycles on the electric transport and magnetization of polycrystalline samples of La0.5Ca0.5MnO3 and La0.325Pr0.3Ca0.375MnO3. An increase of the resistivity and a decrease of the magnetization at different temperature ranges after cycling is obtained in the temperature range between 300 K and 30 K. Both compounds are known to exhibit intrinsic submicrometric coexistence of phases and undergo a sequence of phase transitions related to structural changes. Changes induced by thermal cycling can be partially inhibited by applying magnetic field and hydrostatic pressure. Our results suggest that the growth and coexistence of phases with different structures gives rise to microstructural tracks and strain accommodation, producing the observed irreversibility. Irrespective of the actual ground state of each compound, the effect of thermal cycling is towards an increase of the amount of the insulating phase in both compounds.

cond-mat.mtrl-sci↗

arXiv2002

Persistent magnetoresistive memory in phase separated manganites

We have studied magnetic and transport properties on different manganese oxide based compounds exhibiting phase separation: polycrystalline La5/8-yPryCa3/8MnO3 (y=0.3) and La1/2Ca1/2Mn1-zFezO3 (z = 0.05), and single crystals of La5/8-yPryCa3/8MnO3 (y=0.35). Time dependent effects indicate that the fractions of the coexisting phases are dynamically changing in a definite temperature range. We found that in this range the ferromagnetic fraction f can be easily tuned by application of low magnetic fields (< 1 T). The effect is persistent after the field is turned off, thus the field remains imprinted in the actual value of f and can be recovered through transport measurements. This effect is due both to the existence of a true phase separated equilibrium state with definite equilibrium fraction f0, and to the slow growth dynamics. The fact that the same global features were found on different compounds and in polycrystalline and single crystalline samples, suggests that the effect is a general feature of some phase separated media.

cond-mat.mtrl-sci↗

arXiv2002

Non-volatile magnetoresistive memory in phase separated La$_{0.325}$Pr$_{0.300}$Ca$_{0.375}$MnO$_3$

We have measured magnetic and transport response on the polycrystalline La$_{5/8-y}$Pr$_y$Ca$_{3/8}$MnO$_3$ ($y=0.30$, average grain size 2 microns) compound. In the temperature range where ferromagnetic metallic and insulating regions coexist we observed a persistent memory of low magnetic fields ($<$ 1 T) which is determined by the actual amount of the ferromagnetic phase. The possibility to manipulate this fraction with relatively small external perturbations is related to the phase separated nature of these manganese oxide based compounds. The colossal magnetoresistance figures obtained (about 80%) are determined by the fraction enlargement mechanism. Self-shielding of the memory to external fields is found under certain described circumstances. We show that this non-volatile memory has multilevel capability associated with different applied low magnetic field values.

cond-mat.str-el↗

arXiv2002

Novel dynamical effects and persistent memory in phase separated manganites

The time dependent response of the magnetic and transport properties of Fe-doped phase separated (PS) manganite La$_{0.5}$Ca$_{0.5}$MnO$_{3}$ is reported. The nontrivial coexistence of ferromagnetic (FM) and non FM regions induces a slow dynamics which leads to time relaxation and cooling rate dependence within the PS regime. This dynamics influences drastically on physical properties. On one hand, metallic like behavior, assumed to be a fingerprint of percolation, can be also observed before the FM phase percolates as a result of dynamical contributions. On the other one, two novel effects for the manganites are reported, namely the rejuvenation of the resistivity after ageing, and a persistent memory of low magnetic fields ($<$ 1 T), imprinted in the amount of the FM phase. As a distinctive fact, this memory can be recovered through transport measurements.

cond-mat.str-el↗

arXiv2001

Correlation between magnetic and transport properties of phase separated La$_{0.5}$Ca$_{0.5}$MnO$_{3}$

The effect of low magnetic fields on the magnetic and electrical transport properties of polycrystalline samples of the phase separated compound La$_{0.5}$Ca$_{0.5}$MnO$_{3}$ is studied. The results are interpreted in the framework of the field induced ferromagnetic fraction enlargement mechanism. A fraction expansion coefficient af, which relates the ferromagnetic fraction f with the applied field H, was obtained. A phenomenological model to understand the enlargement mechanism is worked out.

cond-mat.mtrl-sci↗