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F. Radu

Publications and source records attributed to F. Radu.

At least 19 recordsLinked to original sources

Quasi-1D Spin Textures: From Chiral Soliton Lattice to Fan State

In most helimagnets, an applied magnetic field aligns the propagation direction of a helical spin texture with the field, resulting in a conical state and obscuring the unwinding process. Here, we access a complementary regime in the anisotropic chiral magnet Mn$_{1.4}$PtSn, where crystal symmetry constrains the propagation direction of the spin modulation. Using resonant elastic X-ray scattering in a vector magnet, we track the evolution of quasi-one-dimensional spin textures that propagate along a chiral crystallographic axis while the magnetic field is applied perpendicular to this direction. Together with micromagnetic simulations, our measurements reveal a transformation from the zero-field $\pi$-chiral soliton lattice into a fan-like state. In this state, the propagation direction remains transverse to the applied field, while the spins oscillate about the field direction. During magnetization, the modulation length decreases continuously with the field and approaches the field-polarized state. Simulations indicate that magnetostatic interactions in finite samples play a key role in stabilizing this behavior. Our results provide evidence for a fan-like regime in a chiral magnet and highlight how field orientation can be used to control one-dimensional spin textures.

cond-mat.mtrl-sci

Observation of distorted tilted conical phase at the surface of a bulk chiral magnet with resonant elastic x-ray scattering

We report on various magnetic configurations including spirals and skyrmions at the surface of the magnetic insulator Cu$_2$OSeO$_3$ at low temperatures with a magnetic field applied along <100> using resonant elastic X-ray scattering (REXS). We observe a well-ordered surface state referred to as a distorted tilted conical spiral (TC) phase over a wide range of magnetic fields. The distorted TC phase shows characteristic higher harmonic magnetic satellites in the REXS reciprocal space maps. Skyrmions emerge following static magnetic field cycling and appear to coexist with the distorted TC phase. Our results indicate that this phase represents a distinct and stable surface state that does not disappear with field cycling and persists until the field strength is increased sufficiently to create the field-polarized state.

cond-mat.str-el

Epitaxial monolayers of magnetic 2D semiconductor FeBr$_{2}$ grown on Au(111)

Magnetic two-dimensional (2D) semiconductors have attracted a lot of attention because modern preparation techniques are capable of providing single crystal films of these materials with precise control of thickness down to the single-layer limit. It opens up a way to study rich variety of electronic and magnetic phenomena with promising routes towards potential applications. We have investigated the initial stages of epitaxial growth of the magnetic van der Waals semiconductor FeBr\textsubscript{2} on a single-crystal Au(111) substrate by means of low-temperature scanning tunneling microscopy, low-energy electron diffraction, x-ray photoemission spectroscopy, low-energy electron emission microscopy and x-ray photoemission electron microscopy. Magnetic properties of the one- and two-layer thick films were measured via x-ray absorption spectroscopy/x-ray magnetic circular dichroism. Our findings show a striking difference in the magnetic behaviour of the single layer of FeBr\textsubscript{2} and its bulk counterpart, which can be attributed to the modifications in the crystal structure due to the interaction with the substrate.

cond-mat.mtrl-sci

Evidence of The Anomalous Fluctuating Magnetic State by Pressure Driven 4f Valence Change in EuNiGe$_3$

In rare-earth compounds with valence fluctuation, the proximity of the 4f level to the Fermi energy leads to instabilities of the charge configuration and the magnetic moment. Here, we provide direct experimental evidence for an induced magnetic polarization of the Eu$^{3+}$ atomic shell with J=0, due to intra-atomic exchange and spin-orbital coupling interactions with Eu$^{2+}$ atomic shell. By applying external pressure, a transition from antiferromagnetic to a fluctuating behavior in a EuNiGe$_3$ single crystals is probed. Magnetic polarization is observed for both valence states of Eu$^{2+}$ and Eu$^{3+}$ across the entire pressure range. The anomalous magnetism is discussed in terms of a homogeneous intermediate valence state where frustrated Dzyaloshinskii-Moriya couplings are enhanced by the onset of spin-orbital interaction and engender a chiral spin-liquid-like precursor.

cond-mat.str-el

Chiral surface spin textures in Cu$_2$OSeO$_3$ unveiled by soft x-ray scattering in specular reflection geometry

Resonant elastic soft x-ray magnetic scattering (XRMS) is a powerful tool to explore long-periodic spin textures in single crystals. However, due to the limited momentum transfer range imposed by long wavelengths of photons in the soft x-ray region, Bragg diffraction is restricted to crystals with the large lattice parameters. Alternatively, small angle x-ray scattering has been involved in the soft energy x-ray range which, however, brings in difficulties with the sample preparation that involves focused ion beam milling to thin down the crystal to below a few hundred nm thickness. We show how to circumvent these restrictions by using XRMS in specular reflection from a sub-nanometer smooth crystal surface. The method allows observing diffraction peaks from the helical and conical spin modulations at the surface of a Cu$_2$OSeO$_3$ single crystal and probing their corresponding chirality as contributions to the dichroic scattered intensity. The results suggest a promising way to carry out XRMS studies on plethora of noncentrosymmetric systems hitherto unexplored with soft x-rays due to the absence of the commensurate Bragg peaks in the available momentum transfer range.

cond-mat.mtrl-sci

Laser induced ultrafast Gd 4f spin dynamics in Co100-xGdx alloys by means of time-resolved XMCD

We have studied the laser induced ultrafast quenching of Gd 4f magnetic order in ferrimagnetic Co100-xGdx alloys to highlight the role of the inter-atomic exchange coupling. We have taken advantage of the ultrashort soft X-ray pulses deliver by the femtoslicing beamline at the BESSY II synchrotron radiation source at the Helmholtz-Zentrum Berlin to perform element- and time-resolved X-ray Magnetic Circular Dichroism spectroscopy.Our results show that the laser induced quenching of Gd 4f magnetic order occurs on very different time-scales for the Co72Gd28, the Co77Gd23 and the Co79Gd21 alloys. Most of the magnetic moment losses occur within the first picosecond (ps) while the electron distribution is strongly out of equilibrium. After the equilibration of the electrons and lattice temperatures (t > 1 ps), the magnetic losses occur on slower rates that depend on the alloy composition: increasing the Co composition speeds up the demagnetization of Gd 4f sublattice. The strength of the inter-atomic exchange coupling which depends on composition, determines the efficiency of the angular momentum flow from the Gd 4f spin towards the lattice. Our results are in qualitative agreements with the predictions of the microscopic three temperatures model for ferrimagnetic alloys.

cond-mat.mtrl-sci

Search for enhanced magnetism at the interface between Bi$_2$Se$_3$ and EuSe

Enhanced magnetism has recently been reported for the topological-insulator/ferromagnet interface Bi$_2$Se$_3$/EuS with Curie temperatures claimed to be raised above room temperature from the bulk EuS value of 16 K. Here we investigate the analogous interface Bi$_2$Se$_3$/EuSe. EuSe is a low-temperature layered ferrimagnet that is particularly sensitive to external perturbations. We find that superconducting quantum interference device (SQUID) magnetometry of Bi$_2$Se$_3$/EuSe heterostructures reveals precisely the magnetic phase diagram known from EuSe, including the ferrimagnetic phase below 5 K, without any apparent changes from the bulk behavior. Choosing a temperature of 10 K to search for magnetic enhancement, we determine an upper limit for a possible magnetic coercive field of 3 mT. Using interface sensitive x-ray absorption spectroscopy we verify the magnetic divalent configuration of the Eu at the interface without contamination by Eu3+, and by x-ray magnetic circular dichroism (XMCD) we confirm at the interface the magnetic hysteresis obtained by SQUID. XMCD data obtained at 10 K in a magnetic field of 6 T indicate a magnetic spin moment of mz,spin = 7 $\mu$B/Eu$^{2+}$, in good agreement with the SQUID data and the expected theoretical moment of Eu2+. Subsequent XMCD measurements in zero field show, however, that sizable remanent magnetization is absent at the interface for temperatures down to about 10 K.

cond-mat.str-el

Magnetization relaxation and search for the magnetic gap in bulk-insulating V-doped (Bi, Sb)$_2$Te$_3$

V-doped (Bi,Sb)$_2$Te$_3$ has a ten times higher magnetic coercivity than its Cr-doped counterpart and therefore is believed to be a superior system for the quantum anomalous Hall effect (QAHE). The QAHE requires the opening of a magnetic band gap at the Dirac point. We do not find this gap by angle-resolved photoelectron spectroscopy down to 1 K. By x-ray magnetic circular dichroism (XMCD) we directly probe the magnetism at the V site and in zerofield. Hysteresis curves of the XMCD signal show a strong dependence of the coercivity on the ramping velocity of the magnetic field. The XMCD signal decays on a time scale of minutes which we conclude contributes to the absence of a detectable magnetic gap at the Dirac point.

cond-mat.mtrl-sci

Observation of compact ferrimagnetic skyrmions in DyCo$_3$ film

Owing to the experimental discovery of magnetic skyrmions stabilized by the Dzyaloshinskii-Moriya and/or dipolar interactions in thin films, there is a recent upsurge of interest in magnetic skyrmions with antiferromagnetic spins in order to overcome the fundamental limitations inherent with skyrmions in ferromagnetic materials. Here, we report on the observation of compact ferrimagnetic skyrmions for the class of amorphous alloys consisting of 4f rare-earth and 3d transition-metal elements with perpendicular magnetic anisotropy, using a DyCo$_3$ film, that are identified by combining x-ray magnetic scattering, scanning transmission x-ray microscopy, and Hall transport technique. These skyrmions, with antiparallel aligned Dy and Co magnetic moments and a characteristic core radius of about 40~nm, are formed during the nucleation and annihilation of the magnetic maze-like domain pattern exhibiting a topological Hall effect contribution. Our findings provide a promising route for fundamental research in the field of ferrimagnetic/antiferromagnetic spintronics towards practical applications.

cond-mat.mtrl-sci

Charge transfer induced interfacial ferromagnetism in La$_{0.7}$Sr$_{0.3}$MnO$_3$/NdNiO$_3$

Charge transfer induced interfacial ferromagnetism and its impact on the exchange bias effect in La$_{0.7}$Sr$_{0.3}$MnO$_3$/NdNiO$_3$ correlated oxide heterostructures were investigated by soft x-ray absorption and x-ray magnetic circular dichroism spectra in a temperature range from 10 to 300 K. Besides the antiferromagnetic Ni$_3^+$ cations which are naturally part of the NdNiO$_3$ layer, Ni$_2^+$ ions are formed at the interface due to a charge transfer mechanism involving the Mn element of the adjacent layer. They exhibit a ferromagnetic behavior due to the exchange coupling to the Mn$_4^+$ ions in the La$_{0.7}$Sr$_{0.3}$MnO$_3$ layer. This can be seen as detrimental to the strength of the unidirectional anisotropy since a significant part of the interface does not contribute to the pinning of the ferromagnetic layer. By analyzing the line shape changes of the x-ray absorption at the Ni L$_{2,3}$ edges, the metal-insulator transition of the NdNiO$_3$ layer is resolved in an element specific manner. This phase transition is initiated at about 120 K, way above the paramagnetic to antiferromagnetic transition of NdNiO$_3$ layer which measured to be 50 K. Exchange bias and enhanced coercive fields were observed after field cooling the sample through the Neel temperature of the NdNiO$_3$ layer. Different from La$_{0.7}$Sr$_{0.3}$MnO$_3$/LaNiO$_3$, the exchange bias observed in La$_{0.7}$Sr$_{0.3}$MnO$_3$/NdNiO$_3$ is due to the antiferromagnetism of NdNiO$_3$ and the frustration at the interface. These results suggest that reducing the interfacial orbital hybridization may be used as a tunable parameter for the strength of the exchange bias effect in all-oxide heterostructures which exhibit a charge transfer mechanism.

cond-mat.mtrl-sci

Polarized neutron channeling in weakly magnetic films

We describe a new sensitive method for the investigation of weakly magnetic films placed inside a tri-layer planar waveguide. Polarized neutrons tunnel into the waveguide through the surface, channel along the layers and are emitted from the end face as a narrow and slightly divergent microbeam. Polarization analysis permits to detect very small magnetization in the order of a few 10 Gauss. The magnetic film containing the rare-earth element Tb was investigated using both fixed wavelength and time-of-flight polarized neutron reflectometers. The experimental results are presented and discussed.

cond-mat.mtrl-sci

Divergence of neutron microbeams from planar waveguides

Neutron planar waveguides are focusing devices generating a narrow neutron beam of submicron width. Such a neutron microbeam can be used for the investigation of local microstructures with high spatial resolution. The essential parameter of the microbeam is its angular width. The main contribution to the microbeam angular divergence is Fraunhofer diffraction on a narrow slit. We review and discuss various ways to characterize the angular divergence of the neutron microbeam using time-of-flight and fixed wavelength reflectometers.

cond-mat.mtrl-sci

Magnetic-field-induced incommensurate to collinear spin order transition in NiBr$_{2}$

The triangular spin lattice of NiBr$_{2}$ is a canonical example of a frustrated helimagnet that shows a temperature-driven phase transition from a collinear commensurate antiferromagnetic structure to an incommensurate spin helix on cooling. Employing neutron diffraction, bulk magnetization, and magnetic susceptibility measurements, we have studied the f\hspace*{.5pt}ield-induced magnetic states of the NiBr$_{2}$ single crystal. Experimental f\hspace*{.5pt}indings enable us to recapitalize the driving forces of the spin spiral ordering in the triangular spin-lattice systems, in general. Neutron diffraction data conf\hspace*{.5pt}irms, at low temperature below T$_{{\rm m}}$ = 22.8(1) K, the presence of diffraction satellites characteristic of an incommensurate magnetic state, which are symmetrically arranged around main magnetic reflections that evolve just below T$_{{\rm N}}$ = 44.0(1) K. Interestingly, a f\hspace*{.5pt}ield-induced transition from the incommensurate to commensurate spin phase has been demonstrated that enforces spin helix to restore the high temperature compensated antiferromagnetic structure. This spin reorientation can be described as a spin-flop transition in the (\hbox{$a$--$b$}) basal plane of a triangular spin lattice system. These f\hspace*{.5pt}indings offer a new pathway to control the spin helix in incommensurate phases that are currently considered having high technical implications in the next-generation data storage devices.

cond-mat.mtrl-sci

Neutron channeling in a nonmagnetic planar waveguide

We investigate neutron propagation in a middle layer of a planar waveguide which is a tri-layer thin film. A narrow divergent microbeam emitted from the end face of the film is registered. The neutron channeling length is experimentally measured as a function of the guiding channel width. Experimental results are compared with calculations.

physics.app-ph

Experimental determination of exchange constants in antiferromagnetic Mn$_2$Au

Mn$_2$Au is an important antiferromagnetic (AF) material for spintronics applications. Due to its very high N\'eel temperature of about 1500 K, some of the basic properties are difficult to explore, such as the AF susceptibility and the exchange constants. Experimental determination of these properties is further complicated in thin films by unavoidable presence of uncompensated and quasiloose spins on antisites and at interfaces. Using x-ray magnetic circular dichroism (XMCD), we have measured the spin and orbital contribution to the susceptibility in the direction perpendicular to the in-plane magnetic moments of a Mn$_2$Au(001) film and in fields up to 8 T. By performing these measurements at a low temperature of 7 K and at room temperature, we were able to separate the loose spin contribution from the susceptibility of AF coupled spins. The value of the AF exchange constant obtained with this method for a 10 nm thick Mn$_2$Au(001) film equals to (24 $\pm$ 5) meV.

cond-mat.mtrl-sci

The complete micromagnetic characterization of asymmetrically sandwiched ferromagnetic films

The magnetic properties of ferromagnetic thin films down to the nanoscale are ruled by the exchange stiffness, anisotropies and the effects of magnetic fields. As surfaces break inversion symmetry, an additional effective chiral exchange is omnipresent in any magnetic nanostructure. These so-called Dzyaloshinskii-Moriya interactions (DMI) affect all inhomogeneous magnetic states either subtly or spectacularly. E.g., DMIs cause a chirality selection of the rotation sense and can fix the local rotation axis for the magnetization in domain walls (DW). But, they can stabilize also entirely different twisted magnetic structures. The chiral skyrmions a two-dimensional particle-like topological soliton is the ultimately smallest of these objects, which currently is targetted as a possible information carrier in novel spintronic devices. Observation and quantification of the chiral exchange effects provide for the salient point in understanding magnetic properties in ultrathin films and other nanostructures. An easy and reliable method to determine the DMI constant as materials parameter of asymmetric thin films is the crucial problem. Here, we put forth an experimental approach for the determination of the complete set of the micromagnetic parameters. Quasi-static Kerr microcopy observations of DW creep motion and equilibrium sizes of circular magnetic objects in combination with standard magnetometry are used to derive a consistent set of these materials parameters in polycrystalline ultrathin film systems, namely CrOx/Co/Pt stacks. The quantified micromagnetic model for these films identifies the circular magnetic objects, as seen by the optical microscopy, as ordinary bubble domains with homochiral walls. From micromagnetic calculations, the chiral skyrmions stabilized by the DMI in these films are shown to have diameters in the range 40-200nm, too small to be observed by optical microscopy.

cond-mat.mtrl-sci

Terahertz spin currents and inverse spin Hall effect in thin-film heterostructures containing complex magnetic compounds

Terahertz emission spectroscopy of ultrathin multilayers of magnetic and heavy metals has recently attracted much interest. This method not only provides fundamental insights into photoinduced spin transport and spin-orbit interaction at highest frequencies but has also paved the way to applications such as efficient and ultrabroadband emitters of terahertz electromagnetic radiation. So far, predominantly standard ferromagnetic materials have been exploited. Here, by introducing a suitable figure of merit, we systematically compare the strength of terahertz emission from X/Pt bilayers with X being a complex ferro-, ferri- and antiferromagnetic metal, that is, dysprosium cobalt (DyCo$_5$), gadolinium iron (Gd$_{24}$Fe$_{76}$), Magnetite (Fe$_3$O$_4$) and iron rhodium (FeRh). We find that the performance in terms of spin-current generation not only depends on the spin polarization of the magnet's conduction electrons but also on the specific interface conditions, thereby suggesting terahertz emission spectroscopy to be a highly surface-sensitive technique. In general, our results are relevant for all applications that rely on the optical generation of ultrafast spin currents in spintronic metallic multilayers.

cond-mat.mtrl-sci

Application of Zeeman spatial beam-splitting in polarized neutron reflectometry

Neutron Zeeman spatial beam-splitting is considered at reflection from magnetically noncollinear films. Two applications of Zeeman beam-splitting phenomenon in polarized neutron reflectometry are discussed. One is the construction of polarizing devices with high polarizing efficiency. Another one is the investigations of magnetically noncollinear films with low spin-flip probability. Experimental results are presented for illustration.

cond-mat.mtrl-sci