arXiv subjects

F. Riehle

Publications and source records attributed to F. Riehle.

At least 19 recordsLinked to original sources

arXiv2024

Ultrastable lasers: investigations of crystalline mirrors and closed cycle cooling at 124 K

We have investigated crystalline AlGaAs/GaAs optical coatings with three ultra-stable cavities operating at 4 K, 16 K, 124 K and 297 K. The response of the resonance frequencies of cavities to variations in optical power indicates effects beyond the photo-thermo-optic effect observed in dielectric coatings. These effects are strongly dependent on the intensity of the intracavity light at 1.5~\textmu m. When the rear side of the mirrors is illuminated with external light, we observe a prominent photo-modified birefringence for photon energies above the GaAs bandgap, which points to a possible mechanism relating our observations to the semiconductor properties of the coatings. Separately, we also present a low maintenance evolution of our 124 K silicon cavity system where the liquid nitrogen based cooling system is replaced with closed cycle cooling from a pulse-tube cryo-cooler.

physics.optics↗

arXiv2019

Optical clock intercomparison with $6\times 10^{-19}$ precision in one hour

Improvements in atom-light coherence are foundational to progress in quantum information science, quantum optics, and precision metrology. Optical atomic clocks require local oscillators with exceptional optical coherence due to the challenge of performing spectroscopy on their ultra-narrow linewidth clock transitions. Advances in laser stabilization have thus enabled rapid progress in clock precision. A new class of ultrastable lasers based on cryogenic silicon reference cavities has recently demonstrated the longest optical coherence times to date. In this work we utilize such a local oscillator, along with a state-of-the-art frequency comb for coherence transfer, with two Sr optical lattice clocks to achieve an unprecedented level of clock stability. Through an anti-synchronous comparison, the fractional instability of both clocks is assessed to be $4.8\times 10^{-17}/\sqrtτ$ for an averaging time $τ$ in seconds. Synchronous interrogation reveals a quantum projection noise dominated instability of $3.5(2)\times10^{-17}/\sqrtτ$, resulting in a precision of $5.8(3)\times 10^{-19}$ after a single hour of averaging. The ability to measure sub-$10^{-18}$ level frequency shifts in such short timescales will impact a wide range of applications for clocks in quantum sensing and fundamental physics. For example, this precision allows one to resolve the gravitational red shift from a 1 cm elevation change in only 20 minutes.

physics.atom-ph↗

arXiv2017

An ultrastable silicon cavity in a continuously operating closed-cycle cryostat at 4 K

We report on a laser locked to a silicon cavity operating continuously at 4 K with $1 \times 10^{-16}$ instability and a median linewidth of 17 mHz at 1542 nm. This is a ten-fold improvement in short-term instability, and a $10^4$ improvement in linewidth, over previous sub-10 K systems. Operating at low temperatures reduces the thermal noise floor, and thus is advantageous toward reaching an instability of $10^{-18}$, a long-sought goal of the optical clock community. The performance of this system demonstrates the technical readiness for the development of the next generation of ultrastable lasers that operate with ultranarrow linewidth and long-term stability without user intervention.

physics.optics↗

arXiv2017

1.5 $μ$m lasers with sub 10 mHz linewidth

We report on two ultrastable lasers each stabilized to independent silicon Fabry-Pérot cavities operated at 124 K. The fractional frequency instability of each laser is completely determined by the fundamental thermal Brownian noise of the mirror coatings with a flicker noise floor of $4 \times 10^{-17}$ for integration times between 0.8 s and a few tens of seconds. We rigorously treat the notorious divergencies encountered with the associated flicker frequency noise and derive methods to relate this noise to observable and practically relevant linewidths and coherence times. The individual laser linewidth obtained from the phase noise spectrum or the direct beat note between the two lasers can be as small as 5 mHz at 194 THz. From the measured phase evolution between the two laser fields we derive usable phase coherence times for different applications of 11 s and 60 s.

physics.ins-det↗

arXiv2016

Realization of a time-scale with an accurate optical lattice clock

Optical clocks are not only powerful tools for prime fundamental research, but are also deemed for the re-definition of the SI base unit second as they now surpass the performance of caesium atomic clocks in both accuracy and stability by more than an order of magnitude. However, an important obstacle in this transition has so far been the limited reliability of the optical clocks that made a continuous realization of a timescale impractical. In this paper, we demonstrate how this situation can be resolved and that a timescale based on an optical clock can be established that is superior to one based on even the best caesium fountain clocks. The paper also gives further proof of the international consistency of strontium lattice clocks on the $10^{-16}$ accuracy level, which is another prerequisite for a change in the definition of the second.

physics.optics↗

arXiv2012

Providing 1E-16 short-term stability of a 1.5 μm laser to optical clocks

We report on transferring 1E-16-level fractional frequency stability of a "master laser" operated at 1.5 μm to a "slave laser" operated at 698 nm, using a femtosecond fiber comb as transfer oscillator. With the 698 nm laser, the 1S_0 - 3P_0 clock transition of 87Sr was resolved to a Fourier-limited line width of 1.5 Hz (before: 10 Hz). Potential noise sources contributed by the frequency comb are discussed in detail.

physics.optics↗

arXiv2012

A sub-40 mHz linewidth laser based on a silicon single-crystal optical cavity

State-of-the-art optical oscillators based on lasers frequency stabilized to high finesse optical cavities are limited by thermal noise that causes fluctuations of the cavity length. Thermal noise represents a fundamental limit to the stability of an optical interferometer and plays a key role in modern optical metrology. We demonstrate a novel design to reduce the thermal noise limit for optical cavities by an order of magnitude and present an experimental realization of this new cavity system, demonstrating the most stable oscillator of any kind to date. The cavity spacer and the mirror substrates are both constructed from single crystal silicon and operated at 124 K where the silicon thermal expansion coefficient is zero and the silicon mechanical loss is small. The cavity is supported in a vibration-insensitive configuration, which, together with the superior stiffness of silicon crystal, reduces the vibration related noise. With rigorous analysis of heterodyne beat signals among three independent stable lasers, the silicon system demonstrates a fractional frequency stability of 1E-16 at short time scales and supports a laser linewidth of <40 mHz at 1.5 μm, representing an optical quality factor of 4E15.

physics.optics↗

arXiv2011

The 87-Sr optical frequency standard at PTB

With 87-Sr atoms confined in a one dimensional optical lattice, the frequency of the optical clock transition 5s^2 ^1S_0 - 5s5p ^3P_0 has been determined to be 429 228 004 229 872.9(5) Hz. The transition frequency was measured with the help of a fs-frequency comb against one of PTB's H-masers whose frequency was measured simultaneously by the PTB Cs fountain clock CSF1. The Sr optical frequency standard contributes with a fractional uncertainty of 1.5 10^-16 to the total uncertainty. The agreement of the measured transition frequency with previous measurements at other institutes supports the status of this transition as secondary representation of the second with the currently smallest uncertainty.

physics.atom-ph↗

arXiv2011

Atomic clocks with suppressed blackbody radiation shift

We develop a nonstandard concept of atomic clocks where the blackbody radiation shift (BBRS) and its temperature fluctuations can be dramatically suppressed (by one to three orders of magnitude) independent of the environmental temperature. The suppression is based on the fact that in a system with two accessible clock transitions (with frequencies v1 and v2) which are exposed to the same thermal environment, there exists a "synthetic" frequency v_{syn} (v1-e12 v2) largely immune to the BBRS. As an example, it is shown that in the case of ion 171Yb+ it is possible to create a clock in which the BBRS can be suppressed to the fractional level of 10^{-18} in a broad interval near room temperature (300\pm 15 K). We also propose a realization of our method with the use of an optical frequency comb generator stabilized to both frequencies v1 and v2. Here the frequency v_{syn} is generated as one of the components of the comb spectrum and can be used as an atomic standard.

physics.atom-ph↗

arXiv2010

Hyper-Ramsey Spectroscopy of Optical Clock Transitions

We present non-standard optical Ramsey schemes that use pulses individually tailored in duration, phase, and frequency to cancel spurious frequency shifts related to the excitation itself. In particular, the field shifts and their uncertainties of Ramsey fringes can be radically suppressed (by 2-4 orders of magnitude) in comparison with the usual Ramsey method (using two equal pulses) as well as with single-pulse Rabi spectroscopy. Atom interferometers and optical clocks based on two-photon transitions, heavily forbidden transitions, or magnetically induced spectroscopy could significantly benefit from this method. In the latter case these frequency shifts can be suppressed considerably below a fractional level of 10^{-17}. Moreover, our approach opens the door for the high-precision optical clocks based on direct frequency comb spectroscopy.

physics.atom-ph↗

arXiv2009

Compensation of Field-Induced Frequency Shifts in Ramsey Spectroscopy of Optical Clock Transitions

We have extended Ramsey spectroscopy by stepping the probe frequency during the two Ramsey excitation pulses to compensate frequency shifts induced by the excitation itself. This makes precision Ramsey spectroscopy applicable even for transitions that have Stark and Zeeman shifts comparable to the spectroscopic resolution. The method enables a new way to evaluate and compensate key frequency shifts, which benefits in particular, optical clocks based on magnetic field-induced, spectroscopy, two-photon transitions, or heavily forbidden transitions.

physics.optics↗

arXiv2009

Collisional losses, decoherence, and frequency shifts in optical lattice clocks with bosons

We have quantified collisional losses, decoherence and the collision shift in a one-dimensional optical lattice clock with bosonic 88Sr. The lattice clock is referenced to the highly forbidden transition 1S0 - 3P0 at 698 nm, which becomes weakly allowed due to state mixing in a homogeneous magnetic field. We were able to quantify three decoherence coefficients, which are due to dephasing collisions, inelastic collisions between atoms in the upper and lower clock state, and atoms in the upper clock state only. Based on the measured coefficients, we determine the operation parameters at which a 1D-lattice clock with 88Sr shows no degradation due to collisions on the relative accuracy level of 10-16.

physics.atom-ph↗

arXiv2008

Interrogation laser for a strontium lattice clock

We report on the setup and characterization of a 698 nm master-slave diode laser system to probe the 1S0-3P0 clock transition of strontium atoms confined in a one-dimensional optical lattice. A linewidth in the order of around 100 Hz of the laser system has been measured with respect to an ultrastable 657 nm diode laser with 1 Hz linewidth using a femtosecond fiber comb as transfer oscillator. The laser has been used to measure the magnetically induced 1S0-3P0 clock transition in 88Sr where a linewidth of 165 Hz has been observed. The transfer oscillator method provides a virtual beat signal between the two diode lasers that has been used to phase lock the 698 nm laser to the 1 Hz linewidth laser at 657 nm, transferring its stability to the 698 nm laser system.

physics.optics↗

arXiv2006

Optical Clocks in Space

The performance of optical clocks has strongly progressed in recent years, and accuracies and instabilities of 1 part in 10^18 are expected in the near future. The operation of optical clocks in space provides new scientific and technological opportunities. In particular, an earth-orbiting satellite containing an ensemble of optical clocks would allow a precision measurement of the gravitational redshift, navigation with improved precision, mapping of the earth's gravitational potential by relativistic geodesy, and comparisons between ground clocks.

gr-qc↗

arXiv2004

The optical calcium frequency standards of PTB and NIST

We describe the current status of the Ca optical frequency standards with laser-cooled neutral atoms realized in two different laboratories for the purpose of developing a possible future optical atomic clock. Frequency measurements performed at the Physikalisch-Technische Bundesanstalt (PTB) and the National Institute of Standards and Technology (NIST) make the frequency of the clock transition of 40Ca one of the best known optical frequencies (relative uncertainty 1.2e-14) and the measurements of this frequency in both laboratories agree to well within their respective uncertainties. Prospects for improvement by orders of magnitude in the relative uncertainty of the standard look feasible.

physics.atom-ph↗

arXiv2002

Photoassociation spectroscopy of cold calcium atoms

Photoassociation spectroscopy experiments on 40Ca atoms close to the dissociation limit 4s4s 1S0 - 4s4p 1P1 are presented. The vibronic spectrum was measured for detunings of the photoassociation laser ranging from 0.6 GHz to 68 GHz with respect to the atomic resonance. In contrast to previous measurements the rotational splitting of the vibrational lines was fully resolved. Full quantum mechanical numerical simulations of the photoassociation spectrum were performed which allowed us to put constraints on the possible range of the calcium scattering length to between 50 a_0 and 300 a_0.

physics.atom-ph↗

arXiv2002

An Optical Clock with Ultracold Neutral Atoms

We demonstrate how to realize an optical clock with neutral atoms that is competitive to the currently best single ion optical clocks in accuracy and superior in stability. Using ultracold atoms in a Ca optical frequency standard we show how to reduce the relative uncertainty to below 1E-15. We observed atom interferences for stabilization of the laser to the clock transition with a visibility of 0.36, which is 70 % of the ultimate limit achievable with atoms at rest. A novel scheme was applied to detect these atom interferences with the prospect to reach the quantum projection noise limit at an exceptional low instability of 4E-17 in 1 s.

physics.atom-ph↗

arXiv2001

Doppler cooling and trapping on forbidden transitions

Ultracold atoms at temperatures close to the recoil limit have been achieved by extending Doppler cooling to forbidden transitions. A cloud of ^40Ca atoms has been cooled and trapped to a temperature as low as 6 μK by operating a magneto-optical trap on the spin-forbidden intercombination transition. Quenching the long-lived excited state with an additional laser enhanced the scattering rate by a factor of 15, while a high selectivity in velocity was preserved. With this method more than 10% of pre-cooled atoms from a standard magneto-optical trap have been transferred to the ultracold trap. Monte-Carlo simulations of the cooling process are in good agreement with the experiments.

physics.atom-ph↗