arXiv subjects

F. S. S. Rosa

Publications and source records attributed to F. S. S. Rosa.

At least 19 recordsLinked to original sources

arXiv2026

The Dance of the Sheared Eigenfunctions

In this work, we delve into the theory of sheared potentials in non-relativistic quantum mechanics. After defining what we mean by a family of sheared potentials, we consider these families in two particular but emblematic cases, the harmonic oscillator and the symmetric potential well proportional to $|x|$. In both cases, besides determining the spectra, we analyse the impact of the shearing process on the respective eigenfunctions. The latter analysis is typically left aside in the literature, but here we show that the sheared eigenfunctions yield insights that allow for a deeper understanding of the main features exhibited by the spectra. Finally, we make a few comments about the connection between the change in the spectra of a given sheared family and the necessary work that must be made by an external agent to implement such a change.

quant-ph↗

arXiv2023

Controlling electric and magnetic Purcell effects in phosphorene via strain engineering

We investigate the spontaneous emission lifetime of a quantum emitter near a substrate coated with phosphorene under the influence of uniaxial strain. We consider both electric dipole and magnetic dipole-mediated spontaneous transitions from the excited to the ground state. The modeling of phosphorene is performed by employing a tight-binding model that goes beyond the usual low-energy description. We demonstrate that both electric and magnetic decay rates can be strongly tuned by the application of uniform strain, ranging from a near-total suppression of the Purcell effect to a remarkable enhancement of more than 1300% due to the high flexibility associated with the puckered lattice structure of phosphorene. We also unveil the use of strain as a mechanism to tailor the most probable decay pathways of the emitted quanta. Our results show that uniaxially strained phosphorene is an efficient and versatile material platform for the active control of light-matter interactions thanks to its extraordinary optomechanical properties.

cond-mat.mes-hall↗

arXiv2021

Probing topological phase transitions via quantum reflection in the graphene family materials

We theoretically investigate the quantum reflection of different atoms by two-dimensional (2D) materials of the graphene family (silicene, germanene, and stanene), subjected to an external electric field and circularly polarized light. By using Lifshitz theory to compute the Casimir-Polder potential, which ensures that our predictions apply to all regimes of atom-2D surface distances, we demonstrate that the quantum reflection probability exhibits distinctive, unambiguous signatures of topological phase transitions that occur in 2D materials. We also show that the quantum reflection probability can be highly tunable by these external agents, depending on the atom-surface combination, reaching a variation of 40% for Rubidium in the presence of a stanene sheet. Our findings attest that not only dispersive forces play a crucial role in quantum reflection, but also that the topological phase transitions of the graphene family materials can be comprehensively and efficiently probed via atom-surface interactions at the nanoscale.

cond-mat.mes-hall↗

arXiv2021

Probing the screening of the Casimir interaction with optical tweezers

We measure the colloidal interaction between two silica microspheres in aqueous solution in the distance range from $0.2\,μ$m to $0.5\,μ$m with the help of optical tweezers. When employing a sample with a low salt concentration, the resulting interaction is dominated by the repulsive double-layer interaction which is fully characterized. The double-layer interaction is suppressed when adding $0.22\,$M of salt to our sample, thus leading to a purely attractive Casimir signal. When analyzing the experimental data for the potential energy and force, we find good agreement with theoretical results based on the scattering approach. At the distance range probed experimentally, the interaction arises mainly from the unscreened transverse magnetic contribution in the zero-frequency limit, with nonzero Matsubara frequencies providing a negligible contribution. In contrast, such unscreened contribution is not included by the standard theoretical model of the Casimir interaction in electrolyte solutions, in which the zero-frequency term is treated separately as an electrostatic fluctuational effect. As a consequence, the resulting attraction is too weak in this standard model, by approximately one order of magnitude, to explain the experimental data. Overall, our experimental results shed light on the nature of the thermal zero-frequency contribution and indicate that the Casimir attraction across polar liquids has a longer range than previously predicted.

quant-ph↗

arXiv2020

Tuning resonance energy transfer with magneto-optical properties of graphene

We investigate the resonance energy transfer (RET) rate between two quantum emitters near a suspended graphene sheet in vacuum under the influence of an external magnetic field. We perform the analysis for low and room temperatures and show that, due to the extraordinary magneto-optical response of graphene, it allows for an active control and tunability of the RET even in the case of room temperature. We also demonstrate that the RET rate is extremely sensitive to small variations of the applied magnetic field, and can be tuned up to a striking six orders of magnitude for quite realistic values of magnetic field. Moreover, we evidence the fundamental role played by the magnetoplasmon polaritons supported by the graphene monolayer as the dominant channel for the RET within a certain distance range. Our results suggest that magneto-optical media may take the manipulation of energy transfer between quantum emitters to a whole new level, and broaden even more its great spectrum of applications.

cond-mat.mes-hall↗

arXiv2020

Theory of optical tweezing of dielectric microspheres in chiral host media and its applications

We report for the first time the theory of optical tweezers of spherical dielectric particles embedded in a chiral medium. We develop a partial-wave (Mie) expansion to calculate the optical force acting on a dielectric microsphere illuminated by a circularly-polarized, highly focused laser beam. When choosing a polarization with the same handedness of the medium, the axial trap stability is improved, thus allowing for tweezing of high-refractive-index particles. When the particle is displaced off-axis by an external force, its equilibrium position is rotated around the optical axis by the mechanical effect of an optical torque. Both the optical torque and the angle of rotation are greatly enhanced in the presence of a chiral host medium when considering radii a few times larger than the wavelength. In this range, the angle of rotation depends strongly on the microsphere radius and the chirality parameter of the host medium, opening the way for a quantitative characterization of both parameters. Measurable angles are predicted even in the case of naturally occurring chiral solutes, allowing for a novel all-optical method to locally probe the chiral response at the nanoscale.

physics.optics↗

arXiv2020

Probing the optical chiral response of single nanoparticles with optical tweezers

We propose an enantioselective scheme to sort homogeneous chiral particles using optical tweezers. For a certain range of material parameters, we show that a highly focused circularly-polarized laser beam traps particles of a specific chirality selected by the handedness of the trapping beam. Furthermore, by applying a transverse Stokes drag force that displaces the trapped particle off-axis, we allow for the rotation of the particle center-of-mass around the trapping beam axis. The rotation angle is highly dependent on the handedness of the trapped particle and is easily measurable with standard video-microscopy techniques, allowing for an alternative mechanism for chiral resolution. Our platform not only allows for enantioselection of particles dispersed in solution but also paves the way to the characterization of the chiral parameter of individual, homogeneous chiral microspheres using optical tweezing.

physics.optics↗

arXiv2019

Enantioselective manipulation of chiral nanoparticles using optical tweezers

We put forward an enantioselective method for chiral nanoparticles using optical tweezers. We demonstrate that the optical trapping force in a typical, realistic optical tweezing setup with circularly-polarized trapping beams is sensitive to the chirality of core-shell nanoparticles, allowing for efficient enantioselection. It turns out that the handedness of the trapped particles can be selected by choosing the appropriate circular polarization of the trapping beam. The chirality of each individual trapped nanoparticle can be characterized by measuring the rotation of the equilibrium position under the effect of a transverse Stokes drag force. We show that the chirality of the shell gives rise to an additional twist, leading to a strong enhancement of the optical torque driving the rotation. Both methods are shown to be robust against variations of size and material parameters, demonstrating that they are particularly useful in (but not restricted to) several situations of practical interest in chiral plasmonics, where enantioselection and characterization of single chiral nanoparticles, each and every with its unique handedness and optical properties, are in order. In particular, our method could be employed to unveil the chiral response arising from disorder in individual plasmonic raspberries, synthesized by close-packing a large number of metallic nanospheres around a dielectric core.

physics.optics↗

arXiv2019

Resonance energy transfer at percolation transition

We compute the resonance energy transfer (RET) in a system composed of two quantum emitters near a host dielectric matrix in which metallic inclusions are inserted until the medium undergoes a dielectric-metal transition at percolation. We show that there is no peak in the RET rate at percolation, in contrast to what happens with the spontaneous emission rate of an emitter near the same critical medium. This result suggests that RET does not strongly correlate with the local density of states.

cond-mat.mes-hall↗

arXiv2019

An Integrodifferential Equation for Electromagnetic Fields in Linear Dispersive Media

We extend the usual derivation of the wave equation from Maxwell's equations in vacuum to the case of electromagnetic fields in dispersive homogeneous isotropic linear media. Usually, dispersive properties of materials are studied in Fourier space. However, it can be rewarding to consider these properties as causal functions of time. Due to temporal non locality, this procedure gives rise to an integrodifferential equation for the electromagnetic fields, which we also call a wave equation. We have not found this equation in the literature and we show in this paper why it can be useful.

physics.class-ph↗

arXiv2019

Scattering theory of the screened Casimir interaction in electrolytes

We apply the scattering approach to the Casimir interaction between two dielectric half-spaces separated by an electrolyte solution. We take the nonlocal electromagnetic response of the intervening medium into account, which results from the presence of movable ions in solution. In addition to the usual transverse modes, we consider longitudinal channels and their coupling by reflection at the surface of the local dielectric. The Casimir interaction energy is calculated from the matrix describing a round-trip of coupled transverse and longitudinal waves between the interacting surfaces. The nonzero-frequency contributions are approximately unaffected by the presence of ions. We find, at zero frequency, a contribution from longitudinal channels, which is screened over a distance of the order of the Debye length, alongside an unscreened term arising from transverse-magnetic modes. The latter defines the long-distance asymptotic limit for the interaction.

cond-mat.mes-hall↗

arXiv2018

Optimizing optical tweezing with directional scattering in composite microspheres

Trapping of microspheres with a single focused laser beam is usually limited to materials with relative refractive indexes slightly larger than one. We show that directional light scattering can be employed to optically trap high-index materials. For this purpose, we propose a material platform to achieve zero backward scattering (ZBS), also known as the first Kerker condition, in a composite media containing spherical inclusions of silica embedded in a SiC microsphere. By tuning the volume filling fraction of inclusions and the microsphere radius, stable trapping can be achieved, provided that ZBS is combined with the condition for destructive interference between the fields reflected at the external and internal interfaces of the microsphere when located at the focal point. We show that our proposal also holds even in the presence of a significant amount of spherical aberration, which is a common condition in most optical tweezers setups. In this case, achieving ZBS is essential for trapping high-index materials.

physics.optics↗

arXiv2017

Double-layer force suppression between charged microspheres

In this paper we propose a protocol to suppress double-layer forces between two microspheres immersed in a dielectric medium, being one microsphere metallic at a controlled potential ψM and the other a charged one either metallic or dielectric. The approach is valid for a wide range of distances between them. We show that, for a given distance between the two microspheres, the double-layer force can be totally suppressed by simply tuning ψM up to values dictated by the linearized Poisson-Boltzmann equation. Our key finding is that such values can be substantially different from the ones predicted by the commonly used proximity force approximation (PFA), also known as Derjaguin approximation, even in situations where the latter is expected to be accurate. The proposed procedure can be used to suppress the double-layer interaction in force spectroscopy experiments, thus paving the way for measurements of other surface interactions, such as Casimir dispersion forces.

physics.class-ph↗

arXiv2017

Characterizing critical exponents via Purcell effect

We investigate the role of phase transitions into the spontaneous emission rate of quantum emitters embedded in a critical medium. Using a Landau-Ginzburg approach, we find that, in the broken symmetry phase, the emission rate is reduced or even suppressed due to the photon mass generated by the Higgs mechanism. Moreover, we show that the spontaneous emission presents a remarkable dependence upon the critical exponents associated to a given phase transition, allowing for an optical determination of the universality class. Our findings not only demonstrate that the Purcell effect constitutes an efficient optical probe of distinct critical phenomena, but they also unveil that a more general connection between phase transitions and spontaneous emission exist, as previous experimental and numerical evidences suggest.

quant-ph↗

arXiv2016

Purcell effect at metal-insulator transitions

We investigate the spontaneous emission rate of a two-level quantum emitter next to a composite medium made of randomly distributed metallic inclusions embedded in a dielectric host matrix. In the near-field, the Purcell factor can be enhanced by two-orders of magnitude relative to the case of an homogeneous metallic medium, and reaches its maximum precisely at the insulator-metal transition. By unveiling the role of the decay pathways on the emitter's lifetime, we demonstrate that, close to the percolation threshold, the radiation emission process is dictated by electromagnetic absorption in the heterogeneous medium. We show that our findings are robust against change in material properties, shape of inclusions, and apply for different effective medium theories as well as for a wide range of transition frequencies.

cond-mat.mes-hall↗

arXiv2015

Probing the Casimir force with optical tweezers

We propose to use optical tweezers to probe the Casimir interaction between microspheres inside a liquid medium for geometric aspect ratios far beyond the validity of the widely employed proximity force approximation. This setup has the potential for revealing unprecedented features associated to the non-trivial role of the spherical curvatures. For a proof of concept, we measure femtonewton double layer forces between polystyrene microspheres at distances above $400$ nm by employing very soft optical tweezers, with stiffness of the order of fractions of a fN/nm. As a future application, we propose to tune the Casimir interaction between a metallic and a polystyrene microsphere in saline solution from attraction to repulsion by varying the salt concentration. With those materials, the screened Casimir interaction may have a larger magnitude than the unscreened one. This line of investigation has the potential for bringing together different fields including classical and quantum optics, statistical physics and colloid science, while paving the way for novel quantitative applications of optical tweezers in cell and molecular biology.

physics.optics↗

arXiv2015

Active magneto-optical control of spontaneous emission in graphene

We investigate the spontaneous emission rate of a two-level quantum emitter near a graphene-coated substrate under the influence of an external magnetic field or strain induced pseudo-magnetic field. We demonstrate that the application of the magnetic field can substantially increase or decrease the decay rate. We show that a suppression as large as 99$\%$ in the Purcell factor is achieved even for moderate magnetic fields. The emitter's lifetime is a discontinuous function of $|{\bf B}|$, which is a direct consequence of the occurrence of discrete Landau levels in graphene. We demonstrate that, in the near-field regime, the magnetic field enables an unprecedented control of the decay pathways into which the photon/polariton can be emitted. Our findings strongly suggest that a magnetic field could act as an efficient agent for on-demand, active control of light-matter interactions in graphene at the quantum level.

cond-mat.mes-hall↗

arXiv2015

The influence of a surface in the non-retarded interaction between two atoms

In this work we obtain analytical expressions for the non-additivity effects in the dispersive interaction between two atoms and perfectly conducting surface of arbitrary shape in the non-retarded regime. We show that this three bodies quantum-mechanical problem can be solved by mapping it into a two-bodies electrostatic one. We apply the general formulas developed in this paper in several examples. Firstly we re-derive the London interaction as a particular case of our formalism. Then we treat two atoms in the presence of a plane, re-obtained the result displayed in the literature. After we add some new examples. A particularly interesting one is two atoms inside a plate capacitor, a situation where non-additivity is very manifest since the plates lead to the exponentially suppression of the interaction of the atoms, provided the atoms are separated by a distance of the order of the distance between the plates or greater. Our results holds even in the presence of other atoms inside the plate capacitor. As a last example we deal with two atoms in the presence of a sphere, both grounded and isolated. We show that for realistic experimental parameters the non-additivity may be relevant for the force in each atom.

quant-ph↗