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F. Sato

Publications and source records attributed to F. Sato.

16 recordsLinked to original sources
arXiv2026

Three-dimensional zigzag correlations in the van der Waals Kitaev magnet RuBr$_3$

Ruthenium trihalides Ru$X_3$ ($X$ = Cl, Br, I) provide a tunable platform for Kitaev magnetism in two-dimensional van der Waals materials. Despite their similar crystal structures and zigzag antiferromagnetic order, RuBr$_3$ exhibits a higher N\'eel temperature ($T_N$) than RuCl$_3$, suggesting their distinct proximity to the Kitaev quantum spin liquid phase. Using Ru $L_3$-edge resonant x-ray scattering, we show that, while the long-range zigzag order in RuBr$_3$ disappears at $T_N$, the zigzag correlations that persist well above $T_N$ show a pronounced spectral weight redistribution along the interlayer direction. These results suggest that the enhanced interlayer magnetic interactions driven by the extended Br 4$p$ orbitals stabilize three-dimensional zigzag correlations in RuBr$_3$.

cond-mat.str-el↗
arXiv2024

$J=1/2$ Pseudospins and $d$-$p$ Hybridization in the Kitaev Spin Liquid Candidates Ru$X_3$ ($X$ = Cl, Br, I)

The recent synthesis of ruthenium trihalides Ru$X_3$ ($X$ = Cl, Br, I) has enlarged the set of material candidates for Kitaev spin liquid. The realization of Kitaev model necessitates the formation of $J=1/2$ pseudospins in the octahedral crystal field. We use Ru $L_3$-edge resonant inelastic x-ray scattering to investigate the evolution of multiplet structures in Ru$X_3$. We identified quasi-elastic magnetic correlations and spin-orbit transitions to the $J=3/2$ states without discernible trigonal splitting, thereby validating the $J=1/2$ description of magnetism in the Ru$X_3$ family. Lineshape broadening in RuI$_3$ provides evidence for its bulk metallicity in the vicinity of a bandwidth-controlled metal-insulator transition. Our results highlight the pivotal role of halogen $p$ orbitals in controlling the electronic properties of Ru$X_3$.

cond-mat.str-el↗
arXiv2023

Magnetism in Kitaev Quantum Spin Liquid Candidate RuBr$_3$

The present studies show that long-range magnetic order takes place in RuBr$_3$ at $\approx$ 34 K. The observations of clear oscillations in the muon time spectra demonstrate the presence of well-defined internal fields at the muon sites. The magnetic ordering appears to be very robust and static suggesting a more conventional nature of magnetic ordering in the RuBr$_3$ system at zero field. Present investigations prove that in RuBr$_3$ the Kitaev interactions are likely to be weakened at zero field in comparison to the $\alpha$-RuCl$_3$ system. This proves that it is possible to tune the Kitaev interactions by replacing Cl with heavier halogen elements such as Br.

cond-mat.str-el↗
arXiv2020

Traps for pinning and scattering of antiferromagnetic skyrmions via magnetic properties engineering

Micromagnetic simulations have been performed to investigate the controllability of the skyrmion position in antiferromagnetic nanotracks with their magnetic properties modified spatially. In this study we have modeled magnetic defects as local variations on the material parameters, such as the exchange stiffness, saturation magnetization, perpendicular magnetocrystalline anisotropy and Dzyaloshinskii-Moriya constant. Thus, we have observed not only pinning (potential well) but also scattering (potential barrier) of antiferromagnetic skyrmions, when adjusting either a local increase or a local reduction for each material parameter. In order to control of the skyrmion motion it is very important to impose certain positions along the nanotrack where the skyrmion can stop. Magnetic defects incorporated intentionally in antiferromagnetic racetracks can be useful for such purpose. In order to provide guidelines for experimental studies, we vary both material parameters and size of the modified region. The found results show that the efficiency of skyrmion trap depends on a suitable combination of magnetic defect parameters. Furthermore, we discuss the reason why skyrmions are either attracted or repelled by a region magnetically modified.

physics.comp-ph↗
arXiv2019

Suppression of the skyrmion Hall effect in planar nanomagnets by the magnetic properties engineering: Skyrmion transport on nanotracks with magnetic strips

Micromagnetic simulations have been performed to investigate the suppression of the skyrmion Hall effect in nanotracks with their magnetic properties strategically modified. In particular, we study two categories of magnetically modified nanotracks. One of them, repulsive edges have been inserted in the nanotrack and, in the other, an attractive strip has been placed exactly on the longest axis of the nanotrack. Attractive and repulsive interactions can be generated from the engineering of magnetic properties. For instance, it is known that the skyrmion can be attracted to a region where the exchange stiffness constant is decreased. On the other hand, the skyrmion can be repelled from a region characterized by a local increase in the exchange stiffness constant. In order to provide a background for experimental studies, we vary not only the magnetic material parameters (exchange stiffness, perpendicular magnetocrystalline anisotropy and the Dzyaloshinskii-Moriya constant) but also the width of the region magnetically modified, containing either a local reduction or a local increase for each one of these magnetic properties. In the numerical simulations, the skyrmion motion was induced by a spin-polarized current and the found results indicate that it is possible to transport skyrmions around the longest axis of the nanotrack. In practice, the skyrmion Hall effect can be completely suppressed in magnetic nanotracks with strategically modified magnetic properties. Furthermore, we discuss in detail 6 ways to suppress the skyrmion Hall effect by the usage of nanotracks with repulsive edges and nanotracks with an attractive strip.

physics.comp-ph↗
arXiv2019

Investigation of domain wall pinning by square anti-notches and its applications in three terminals MRAM

In this work we perform investigations of the competition between domain-wall pinning and attraction by anti-notches and finite device borders. The conditions for optimal geometries, which can attain a stable domain-wall pinning, are presented. This allow us the proposition of a three-terminals device based on domain-wall pinning. We obtain, with very small pulses of current applied parallel to the nanotrack, a fast motion of the domain-wall between anti-notches. In addition to this, a swift stabilization of the pinned domain-wall is observed with a high percentage of orthogonal magnetization, enabling high magnetoresistive signal measurement. Thus, our proposed device is a promising magnetoresistive random access memories with good scalability, duration, and high speed information storage.

physics.app-ph↗
arXiv2018

Building traps for skyrmions by the incorporation of magnetic defects into nanomagnets: pinning and scattering traps by magnetic properties engineering

In this work we have used micromagnetic simulations to report four ways to build traps for magnetic skyrmions. Magnetic defects have been modeled as local variations in the material parameters, such as the exchange stiffness, saturation magnetization, magnetocrystalline anisotropy and Dzyaloshinskii-Moriya constant. We observe both pinning (potential well) and scattering (potential barrier) traps when tuning either a local increase or a local reduction for each one of these magnetic properties. It is found that the skyrmion-defect aspect ratio is a crucial parameter to build traps for skyrmions. In particular, the efficiency of the trap is compromised if the defect size is smaller than the skyrmion size, because they interact weakly. On the other hand, if the defect size is larger than the skyrmion diameter, the skyrmion-defect interaction becomes evident. Thus, the strength of the skyrmion-defect interaction can be tuned by the modification of the magnetic properties within a region with suitable size. Furthermore, the basic physics behind the mechanisms for pinning and for scattering is discussed. In particular, we discover that skyrmions move towards the magnetic region which tends to maximize its diameter; it enables the magnetic system to minimize its energy. Thus, we are able to explain why skyrmions are either attracted or repelled by a region with modified magnetic properties. Results here presented are of utmost significance for the development and realization of future spintronic devices, in which skyrmions will work as information carriers.

physics.comp-ph↗
arXiv2015

Surface Effects on the Mechanical Elongation of AuCu Nanowires: De-alloying and the Formation of Mixed Suspended Atomic Chains

We report here an atomistic study of the mechanical deformation of AuxCu(1-x) atomic-size wires (NWs) by means of high resolution transmission electron microscopy (HRTEM) experiments. Molecular dynamics simulations were also carried out in order to obtain deeper insights on the dynamical properties of stretched NWs. The mechanical properties are significantly dependent on the chemical composition that evolves in time at the junction; some structures exhibit a remarkable de-alloying behavior. Also, our results represent the first experimental realization of mixed linear atomic chains (LACs) among transition and noble metals; in particular, surface energies induce chemical gradients on NW surfaces that can be exploited to control the relative LAC compositions (different number of gold and copper atoms). The implications of these results for nanocatalysis and spin transport of one-atom-thick metal wires are addressed.

cond-mat.mtrl-sci↗
arXiv2011

Development and evaluation of 10-inch Photo-Multiplier Tubes for the Double Chooz experiment

The goal of Double Chooz experiment is a precise measurement of the last unknown mixing angle theta_13 using two identical detectors placed at far and near sites from Chooz reactor cores. The detector is optimized for reactor-neutrino detection using specially developed 10-inch PMTs. We developed two types of measurement systems and evaluated 400 PMTs before the installation. Those PMTs fulfill our requirements, and a half of those have been installed to the far detector in 2009. The character and performance data of the PMTs are stored in a database and will be referenced in analysis and MC simulation.

physics.ins-det↗
arXiv2007

Molecular Recognition Effects in the Surface Diffusion of Large Organic Molecules: The Case of Violet Lander

Violet Lander (VL) (C108H104) is a large organic molecule that when deposited on Cu (110) exhibited lock-and-key like behavior (Otero et al., Nature Mater. 3, 779 (2004)). In this work we report on a detailed fully atomistic molecular dynamics study of this phenomenon. Our results show that it has its physical basis in the interplay of the molecular hydrogens and the Cu(110) atomic spacing, which is a direct consequence of an accidental commensurability between molecule and surface dimensions. This knowledge could be used to engineer new molecules capable of displaying lock-and-key behavior with new potential applications in nanotechology.

cond-mat.mtrl-sci↗
arXiv2006

On the Formation of Copper Linear Atomic Suspended Chains

We report high resolution transmission electron microscopy and classical molecular dynamics simulation results of mechanically stretching copper nanowires conducting to linear atomic suspended chains (LACs) formation. In contrast with some previous experimental and theoretical work in literature that stated that the formation of LACs for copper should not exist our results showed the existence of LAC for the [111], [110], and [100] crystallographic directions, being thus the sequence of most probable occurence.

cond-mat.mtrl-sci↗
arXiv2006

Nanowires and Suspended Atom Chains from Metal alloys

We present a study of the elongation and rupture of gold-silver alloy nanowires. Atomistic details of the evolution were derived from time-resolved atomic resolution transmission electron microscopy and molecular dynamics simulations. The results show the occurrence of gold enrichment at the nanojunction region, leading to a gold-like structural behavior even for alloys with minor gold content. Our observations have also revealed the formation of mixed (Au and Ag) linear atomic chains.

cond-mat.mtrl-sci↗
arXiv2004

Structure and magnetism in nanocrystalline Ca(La)B$_6$ films

Nanocrystalline films of La-doped CaB$_6$ have been fabricated by using a rf-magnetron sputtering. Lattice expansion of up to 6% with respect to the bulk value was observed along the direction perpendicular to the film plane, which arises from the trapping of Ar gas into the film. Large ferromagnetic moment of 3 ~ 4 Bohr magneton per La has been observed in some La-doped films only when the lattice expansion rate is larger than 2.5%.

cond-mat.mtrl-sci↗
arXiv1998

A Large-scale CO Imaging of the Galactic Center. II. Dynamical Properties of Molecular Clouds

The data from the Nobeyama Radio Observatory 45 m telescope Galactic Center CO survey have been analyzed to generate a compilation of molecular clouds with intense CO emission in this region. Clouds are identified in an automated manner throughout the main part of the survey data for all CO emission peaks exceeding 10 K ($T_R^*$). Correlations between the size, velocity dispersion, virial mass, and the CO luminosity, for the molecular clouds in the Galactic center were shown. We diagnosed gravitational stabilities of identified clouds assuming that the disk clouds are nearly at the onset of gravitational instability. Most of the clouds and cloud complexes in the Galactic center are gravitationally stable, while some clouds with intense CO emission are gravitationally unstable.

astro-ph↗
arXiv1998

A High Velocity Cloud near the Center of the Galaxy

We report the detection of a peculiar molecular cloud, CO 0.02-0.02, lying about 5' Galactic-east from the center of the Galaxy. (12)CO images taken with NRO 45 m telescope showed that it is relatively compact (about 3x4 pc^2) as well as having a very large velocity width (DV>=100 km s(-1)). The cloud has a virial mass about one order of magnitude larger than the LTE mass, 9E4 M(solar), indicating the cloud is apparently gravitationally unbound. New observations with the JCMT 15 m and the NRO 45 m telescope show that CO 0.02-0.02 is very bright in the CO J=3-2, and in the HCN and HCO+ J=1-0 lines. It appears that the environment may have an unusually high density and temperature, which may be related to the very broad CO line-width. We propose that CO 0.02-0.02 may have been accelerated, heated and compressed in a series of supernovae shocks which have occurred within the last (3-5)E4$ years.

astro-ph↗