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F. Schlawin

Publications and source records attributed to F. Schlawin.

6 recordsLinked to original sources

Magnetization of electronic ground states in frustrated superstable graphs

Geometric frustration lies at the heart of many unconventional quantum phases in strongly interacting electron systems. Here, we analytically determine the ground state magnetization of the half-filled Hubbard model on frustrated geometries where superstable states -- eigenstates which are robust against frustration -- are manifest. Our results apply to a broad class of lattices, including those where altermagnetic and superconducting states are known to emerge. Furthermore, they provide evidence for phase transitions involving a geometric rearrangement of magnetic correlations in the thermodynamic limit.

cond-mat.str-el

Lieb's Theorem and Maximum Entropy Condensates

Coherent driving has established itself as a powerful tool for guiding a many-body quantum system into a desirable, coherent non-equilibrium state. A thermodynamically large system will, however, almost always saturate to a featureless infinite temperature state under continuous driving and so the optical manipulation of many-body systems is considered feasible only if a transient, prethermal regime exists, where heating is suppressed. Here we show that, counterintuitively, in a broad class of lattices Floquet heating can actually be an advantageous effect. Specifically, we prove that the maximum entropy steady states which form upon driving the ground state of the Hubbard model on unbalanced bi-partite lattices possess uniform off-diagonal long-range order which remains finite even in the thermodynamic limit. This creation of a `hot' condensate can occur on \textit{any} driven unbalanced lattice and provides an understanding of how heating can, at the macroscopic level, expose and alter the order in a quantum system. We discuss implications for recent experiments observing emergent superconductivity in photoexcited materials.

cond-mat.str-el

Dynamical order and superconductivity in a frustrated many-body system

In triangular lattice structures, spatial anisotropy and frustration can lead to rich equilibrium phase diagrams with regions containing complex, highly entangled states of matter. In this work we study the driven two-rung triangular Hubbard model and evolve these states out of equilibrium, observing how the interplay between the driving and the initial state unexpectedly shuts down the particle-hole excitation pathway. This restriction, which symmetry arguments fail to predict, dictates the transient dynamics of the system, causing the available particle-hole degrees of freedom to manifest uniform long-range order. We discuss implications of our results for a recent experiment on photo-induced superconductivity in ${\rm κ- (BEDT-TTF)_{2}Cu[N(CN)_{2}]Br}$ molecules.

cond-mat.str-el

Evidence for metastable photo-induced superconductivity in K$_3$C$_{60}$

Far and mid infrared optical pulses have been shown to induce non-equilibrium unconventional orders in complex materials, including photo-induced ferroelectricity in quantum paraelectrics, magnetic polarization in antiferromagnets and transient superconducting correlations in the normal state of cuprates and organic conductors. In the case of non-equilibrium superconductivity, femtosecond drives have generally resulted in electronic properties that disappear immediately after excitation, evidencing a state that lacks intrinsic rigidity. Here, we make use of a new optical device to drive metallic K$_3$C$_{60}$ with mid-infrared pulses of tunable duration, ranging between one picosecond and one nanosecond. The same superconducting-like optical properties observed over short time windows for femtosecond excitation are shown here to become metastable under sustained optical driving, with lifetimes in excess of ten nanoseconds. Direct electrical probing becomes possible at these timescales, yielding a vanishingly small resistance. Such a colossal positive photo-conductivity is highly unusual for a metal and, when taken together with the transient optical conductivities, it is rather suggestive of metastable light-induced superconductivity.

cond-mat.supr-con

Photo-molecular high temperature superconductivity

Superconductivity in organic conductors is often tuned by the application of chemical or external pressure. With this type of tuning, orbital overlaps and electronic bandwidths are manipulated, whilst the properties of the molecular building blocks remain virtually unperturbed.Here, we show that the excitation of local molecular vibrations in the charge-transfer salt $κ-(BEDT-TTF)_2Cu[N(CN)_2]Br$ induces a colossal increase in carrier mobility and the opening of a superconducting-like optical gap. Both features track the density of quasi-particles of the equilibrium metal, and can be achieved up to a characteristic coherence temperature $T^* \approxeq 50 K$, far higher than the equilibrium transition temperature $T_C = 12.5 K$. Notably, the large optical gap achieved by photo-excitation is not observed in the equilibrium superconductor, pointing to a light induced state that is different from that obtained by cooling. First-principle calculations and model Hamiltonian dynamics predict a transient state with long-range pairing correlations, providing a possible physical scenario for photo-molecular superconductivity.

cond-mat.supr-con

Nonlinear Spectroscopy of Controllable Many-Body Quantum Systems

We establish a novel approach to probing spatially resolved multi-time correlation functions of interacting many-body systems, with scalable experimental overhead. Specifically, designing nonlinear measurement protocols for multidimensional spectra in a chain of trapped ions with single-site addressability enables us, e.g., to distinguish coherent from incoherent transport processes, to quantify potential anharmonicities, and to identify decoherence-free subspaces.

quant-ph