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F. Treussart

Publications and source records attributed to F. Treussart.

14 recordsLinked to original sources
arXiv2020

Single photon wavefront-splitting interference: An illustration of the light quantum in action

We present a new realization of the textbook experiment consisting in single-photon interference based on the pulsed, optically excited photoluminescence of a single colour centre in a diamond nanocrystal. Interferences are created by wavefront-splitting with a Fresnel's biprism and observed by registering the "single-photon clicks" with an intensified CCD camera. This imaging detector provides also a real-time movie of the build-up of the single-photon fringes. We perform a second experiment with two detectors sensitive to photons that follow either one or the other interference path. Evidence for single photon behaviour is then obtained from the absence of time coincidence between detections in these two paths.

quant-ph↗
arXiv2019

Probing plasmon-NV$^0$ coupling at the nanometer scale with photons and fast electrons

The local density of optical states governs an emitters lifetime and quantum yield through the Purcell effect. It can be modified by a surface plasmon electromagnetic field, but such a field has a spatial extension limited to a few hundreds of nanometers, which complicates the use of optical methods to spatially probe the emitter-plasmon coupling. Here we show that a combination of electron-based imaging, spectroscopies and photon-based correlation spectroscopy enables measurement of the Purcell effect with nanometer and nanosecond spatio-temporal resolutions. Due to the large variability of radiative lifetimes of emitters embedded in nanoparticles with inhomogeneous sizes we relied on a statistical approach to unambiguously probe the coupling between nitrogen-vacancy centers (NV^0) in nanodiamonds and surface plasmons in silver nanocubes. We quantified the Purcell effect by measuring the NV^0 excited state lifetimes in a large number of either isolated nanodiamonds or nanodiamond-nanocube dimers and demonstrated a statistically significant lifetime reduction for dimers.

cond-mat.mes-hall↗
arXiv2013

Quenching nitrogen-vacancy center photoluminescence with infrared pulsed laser

Diamond nanocrystals containing Nitrogen-Vacancy (NV) color centers have been used in recent years as fluorescent probes for near-field and cellular imaging. In this work we report that an infrared (IR) pulsed excitation beam can quench the photoluminescence of NV color center in a diamond nanocrystal (size < 50 nm) with an extinction ratio as high as ~90%. We attribute this effect to the heating of the nanocrystal consecutive to multi-photon absorption by the diamond matrix. This quenching is reversible: the photoluminescence intensity goes back to its original value when the IR laser beam is turned off, with a typical response time of hundred picoseconds, allowing for a fast control of NV color center photoluminescence. We used this effect to achieve sub-diffraction limited imaging of fluorescent diamond nanocrystals on a coverglass. For that, as in Ground State Depletion super-resolution technique, we combined the green excitation laser beam with the control IR depleting one after shaping its intensity profile in a doughnut form, so that the emission comes only from the sub-wavelength size central part.

physics.optics↗
arXiv2011

Study of the optimal conditions for NV- center formation in type 1b diamond, using photoluminescence and positron annihilation spectroscopies

We studied the parameters to optimize the production of negatively-charged nitrogen-vacancy color centers (NV-) in type~1b single crystal diamond using proton irradiation followed by thermal annealing under vacuum. Several samples were treated under different irradiation and annealing conditions and characterized by slow positron beam Doppler-broadening and photoluminescence (PL) spectroscopies. At high proton fluences another complex vacancy defect appears limiting the formation of NV-. Concentrations as high as 2.3 x 10^18 cm^-3 of NV- have been estimated from PL measurements. Furthermore, we inferred the trapping coefficient of positrons by NV-. This study brings insight into the production of a high concentration of NV- in diamond, which is of utmost importance in ultra-sensitive magnetometry and quantum hybrid systems applications.

cond-mat.mtrl-sci↗
arXiv2011

Diamond particles as nanoantennas for nitrogen-vacancy color centers

The photoluminescence of nitrogen-vacancy (NV) centers in diamond nanoparticles exhibits specific properties as compared to NV centers in bulk diamond. For instance large fluctuations of lifetime and brightness from particle to particle have been reported. It has also been observed that for nanocrystals much smaller than the mean luminescence wavelength, the particle size sets a lower threshold for resolution in Stimulated Emission Depletion (STED) microscopy. We show that all these features can be quantitatively understood by realizing that the absorption-emission of light by the NV center is mediated by the diamond nanoparticle which behaves as a dielectric nanoantenna.

physics.optics↗
arXiv2010

Surface-induced charge state conversion of nitrogen-vacancy defects in nanodiamonds

We present a study of the charge state conversion of single nitrogen-vacancy (NV) defects hosted in nanodiamonds (NDs). We first show that the proportion of negatively-charged NV$^{-}$ defects, with respect to its neutral counterpart NV$^{0}$, decreases with the size of the ND. We then propose a simple model based on a layer of electron traps located at the ND surface which is in good agreement with the recorded statistics. By using thermal oxidation to remove the shell of amorphous carbon around the NDs, we demonstrate a significant increase of the proportion of NV$^{-}$ defects in 10-nm NDs. These results are invaluable for further understanding, control and use of the unique properties of negatively-charged NV defects in diamond

cond-mat.mtrl-sci↗
arXiv2010

Grafting fluorescent nanodiamonds onto optical tips

We recently (Optics Express 17, 19969 (2009)) introduced an all-optical method for grafting onto the apex of an optical tip a single 20 nm nanodiamond with single color-center occupancy and used the resulting single-photon tip in scanning near-field imaging at room temperature, thereby achieving a genuine scanning single-photon microscopy working in ambient conditions. A variant of this method is described that allows for attaching several nanodiamonds onto the tip apex, releasing them all at once and finally recapturing them one by one by the scanning tip. This underlines the flexibility and powerfulness of our method and its variant that could be used in applications where a fixed number of selected optically active nano-objects requires positioning, or repositioning, at well defined locations with nanometer accuracy.

cond-mat.mes-hall↗
arXiv2009

Near-field optical microscopy with a nanodiamond-based single photon tip

We introduce a point-like scanning single-photon source that operates at room temperature and offers an exceptional photostability (no blinking, no bleaching). This is obtained by grafting in a controlled way a diamond nanocrystal (size around 20 nm) with single nitrogen-vacancy color-center occupancy at the apex of an optical probe. As an application, we image metallic nanostructures in the near-field, thereby achieving a near-field scanning single-photon microscopy working at room temperature on the long term. Our work may be of importance to various emerging fields of nanoscience where an accurate positioning of a quantum emitter is required such as for example quantum plasmonics.

physics.optics↗
arXiv2009

High nitrogen-vacancy density diamonds for magnetometry applications

Nitrogen-vacancy (NV) centers in millimeter-scale diamond samples were produced by irradiation and subsequent annealing under varied conditions. The optical and spin relaxation properties of these samples were characterized using confocal microscopy, visible and infrared absorption, and optically detected magnetic resonance. The sample with the highest NV- concentration, approximately 16 ppm = 2.8 x 10^{18} cm^{-3}, was prepared with no observable traces of neutrally-charged vacancy defects. The effective transverse spin relaxation time for this sample was T2* = 118(48) ns, predominately limited by residual paramagnetic nitrogen which was determined to have a concentration of 52(7) ppm. Under ideal conditions, the shot-noise limited sensitivity is projected to be ~150 fT/\sqrt{Hz} for a 100 micron-scale magnetometer based on this sample. Other samples with NV- concentrations from .007 to 12 ppm and effective relaxation times ranging from 27 to 291 ns were prepared and characterized.

cond-mat.mtrl-sci↗
arXiv2009

Illustration of quantum complementarity using single photons interfering on a grating

A recent experiment performed by S. S. Afshar et al. has been interpreted as a violation of Bohr's complementarity principle between interference visibility and which-path information in a two-path interferometer. We have reproduced this experiment, using true single-photon pulses propagating in a two-path wavefront- splitting interferometer realized with a Fresnel's biprism, and followed by a grating with adjustable transmitting slits. The measured values of interference visibility V and which-path information, characterized by the distinguishability parameter D, are found to obey the complementarity relation V^2+D^2=<1. This result demonstrates that the experiment can be perfectly explained by the Copenhagen interpretation of quantum mechanics.

quant-ph↗
arXiv2005

Single-photon emission in the near infrared from diamond colour centre

Optically active colour centres based on Nickel-Nitrogen impurities are observed in natural diamond under continuous-wave excitation. The spectral analysis shows that the single emitters have a narrow-band emission in the near infrared, around 780 nm, which is almost entirely concentrated in the zero phonon line even at room temperature. The colour centre excited-state lifetime is as short as 2 ns, and the photoluminescence is linear polarized. These striking features pave the way to the realization of a triggered single photon source based on this colour centre emission well suited for open-air single-photon Quantum Key Distribution operating in day-light conditions.

cond-mat.other↗
arXiv2005

Photoluminescence of single colour defects in 50 nm diamond nanocrystals

We used optical confocal microscopy to study optical properties of diamond 50 nm nanocrystals first irradiated with an electron beam, then dispersed as a colloidal solution and finally deposited on a silica slide. At room temperature, under CW laser excitation at a wavelength of 514.5 nm we observed perfectly photostable single Nitrogen-Vacancy (NV) colour defects embedded in the nanocrystals. From the zero-phonon line around 575 nm in the spectrum of emitted light, we infer a neutral NV0 type of defect. Such nanoparticle with intrinsic fluorescence are highly promising for applications in biology where long-term emitting fluorescent bio-compatible nanoprobes are still missing.

cond-mat.mtrl-sci↗
arXiv2002

Direct Measurement of the Photon Statistics of a Triggered Single Photon Source

We studied intensity fluctuations of a single photon source relying on the pulsed excitation of the fluorescence of a single molecule at room temperature. We directly measured the Mandel parameter Q(T) over 4 orders of magnitude of observation timescale T, by recording every photocount. On timescale of a few excitation periods, subpoissonian statistics is clearly observed and the probablility of two-photons events is 10 times smaller than Poissonian pulses. On longer times, blinking in the fluorescence, due to the molecular triplet state, produces an excess of noise.

quant-ph↗