arXiv subjects

F. W. Foss Jr.

Publications and source records attributed to F. W. Foss Jr..

4 recordsLinked to original sources

arXiv2020

Radio Frequency and DC High Voltage Breakdown of High Pressure Helium, Argon, and Xenon

Motivated by the possibility of guiding daughter ions from double beta decay events to single-ion sensors for barium tagging, the NEXT collaboration is developing a program of R&D to test radio frequency (RF) carpets for ion transport in high pressure xenon gas. This would require carpet functionality in regimes at higher pressures than have been previously reported, implying correspondingly larger electrode voltages than in existing systems. This mode of operation appears plausible for contemporary RF-carpet geometries due to the higher predicted breakdown strength of high pressure xenon relative to low pressure helium, the working medium in most existing RF carpet devices. In this paper we present the first measurements of the high voltage dielectric strength of xenon gas at high pressure and at the relevant RF frequencies for ion transport (in the 10 MHz range), as well as new DC and RF measurements of the dielectric strengths of high pressure argon and helium gases at small gap sizes. We find breakdown voltages that are compatible with stable RF carpet operation given the gas, pressure, voltage, materials and geometry of interest.

physics.ins-det↗

arXiv2019

Barium Chemosensors with Dry-Phase Fluorescence for Neutrinoless Double Beta Decay

The nature of the neutrino is one of the major open questions in experimental nuclear and particle physics. The most sensitive known method to establish the Majorana nature of the neutrino is detection of the ultra-rare process of neutrinoless double beta decay. However, identification of one or a handful of decay events within a large mass of candidate isotope, without obfuscation by backgrounds is a formidable experimental challenge. One hypothetical method for achieving ultra-low-background neutrinoless double beta decay sensitivity is the detection of single $^{136}$Ba ions produced in the decay of $^{136}$Xe (`barium tagging'). To implement such a method, a single-ion-sensitive barium detector must be developed and demonstrated in bulk liquid or dry gaseous xenon. This paper reports on the development of two families of dry-phase barium chemosensor molecules for use in high pressure xenon gas detectors, synthesized specifically for this purpose. One particularly promising candidate, an anthracene substituted aza-18-crown-6 ether, is shown to respond in the dry phase with almost no intrinsic background from the unchelated state, and to be amenable to barium sensing through fluorescence microscopy. This interdisciplinary advance, paired with earlier work demonstrating sensitivity to single barium ions in solution, opens a new path toward single ion detection in high pressure xenon gas.

physics.ins-det↗

arXiv2019

Barium Tagging with Selective, Dry-Functional, Single Molecule Sensitive On-Off Fluorophores for the NEXT Experiment

In the search for neutrinoless double beta decay, understanding and reducing backgrounds is crucial for success. An advance that could drive backgrounds to negligible levels would be the ability to efficiently detect the barium daughter in $^{136}$Xe to $^{136}$Ba double beta decay, since no conventional radioactive process can produce barium ions or atoms in xenon at significant rates. In xenon gas, the barium daughter most likely survives as a dication. An approach under development by the NEXT collaboration involves transporting this ion from the active medium onto a coated transparent plane supporting a barium-sensitive fluorescent dye, monitored via fluorescence microscopy. Upon exposure to a barium dication, the dye will begin fluorescing, which, when correlated with the detection of a double electron signal at the anode, would confirm double beta decay.Our results have shown that a single barium ion can be resolved via Single Molecule Fluorescent Imaging (SMFI). The next challenge is a realization of this technique within in a large volume of xenon gas. Significant advances have recently been made: custom barium-tagging molecules that fluoresce strongly in the dry state when exposed to barium have been demonstrated, and devices constructed that can observe fluorescence via in-vacuum or in-gas Total Internal Reflection Fluorescence Microscopy. We present the status of this technique and the outlook for barium tagging with On-Off switchable fluorophores, including new results with a Ba$^{2+}$-selective dye that functions under our desired conditions in the visible region and with single ion sensitivity.

physics.ins-det↗

arXiv2019

Progress toward Barium Tagging in High Pressure Xenon Gas with Single Molecule Fluorescence Imaging

We present an update on the development of techniques to adapt Single Molecule Fluorescent Imaging for the tagging of individual barium ions in high pressure xenon gas detectors, with the goal of realizing a background-free neutrinoless double beta decay technology. Previously reported progress is reviewed, including the recent demonstration of single barium dication sensitivity using SMFI. We then describe two important advances: 1) the development of a new class of custom barium sensing fluorescent dyes, which exhibit a significantly stronger response to barium than commercial calcium sensing compounds in aqueous solution; 2) the first demonstration of a dry-phase chemosensor for barium ions. This proceeding documents work presented at the 9th Symposium on Large TPCs for Rare Event Detection in Paris, France.

physics.ins-det↗